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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Design of Quasi-Integral Experiments at the Flexible Neutron Source at the University of Tennessee

Nuclear reaction data libraries make use of experimental data that are differential in reaction and neutron energy for evaluation and data that are integral in reaction and energy for validation. In many cases, integral measurements can provide lower experimental uncertainties than differential measurements, but the impact of individual reactions and energies cannot generally be determined from the single experimental observable. “Quasi-integral” or “quasi-differential” measurements, which are integral in one characteristic (energy or reaction) and differential in the other, can often provide a middle ground of lower experimental uncertainties combined with some ability to unpack the impact of individual reactions or energies. Furthermore, the Flexible Neutron Source (FNS) at the University of Tennessee, Knoxville, is a new experimental facility that can perform integral and quasi-integral measurements by removing components of the integral configuration to determine the impact of specific reactions. Possible flux-averaged cross-section measurements, flux perturbation measurements, and neutron downscattering measurements are simulated here to show the value of the FNS to evaluation and validation of nuclear data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Investigation of Benchmark $k$ eff Sensitivity and Uncertainty for 239 Pu fission in Specific Energy Ranges

Nuclear data at intermediate energies (from 1 to 100s of keV) are evaluated based on scarce differential data and theory unable to capture physics’ expected structure. There is also a lack of integral data. This is a known deficiency and is challenging to address. Calculated effective multiplication factor, k eff , values for intermediate energy experiments are ~25× further from experiment than for fast energies and are often well outside the experimental uncertainties. The goal of the PARADIGM (PARallel Approach of Differential and InteGral Measurements) project is to significantly re duce the uncertainties of intermediate energy nuclear data for 239 Pu. To this end, PARADIGM simultaneously optimizes experiments at both the Los Alamos Neutron Science Center (LANSCE) and National Criticality Experiments Research Center (NCERC). The combined set of data will inform new intermediate-energy nuclear data. By execution of differential and integral experiments, establishment of new theory, and undertaking nuclear data evaluation in parallel, the timeline to deliver improved nuclear data to users will be reduced significantly that is to three years. For the PARADIGM project, it was decided to optimize an integral experiment for two neutron energy ranges, within the full intermediate energy range. The low energy range goes from 1 to 30 keV, while the higher energy range goes from 30 to 600 keV. This work focuses on nuclear data sensitivities and uncertainties for 239 Pu fission for existing experiments in the International Criticality Safety Benchmark Evaluation Project (ICSBEP). When designing new experiments, it is important to understand what benchmarks currently exist. For a more traditional experiment design (in which a specific application model(s) exists), comparisons would be made between the application model(s) and existing benchmarks. For PARADIGM, there is no specific application model, but instead the specific nuclear data reaction and energy ranges of interest can be explored for existing benchmarks.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

ENDF/B-VIII.1: Photonuclear Sublibrary

The photonuclear sublibrary aims to describe nuclear reactions between incident gamma particles and different nuclei. For ENDF/B-VIII.1, we adopted around 200 evaluations from the IAEA Coordinated Research Project (CRP) on photonuclear data while, for a few select mission-critical materials, evaluations from ENDF/B-VIII.0 were maintained. Additionally, many fixes to many files were implemented. Finally, ENDF/B-VIII.1 includes a new photonuclear file, 242 Pu, which was adopted from JENDL-5.0.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Learning nuclear cross sections across the chart of nuclides with graph neural networks

We explore the use of deep learning techniques to learn how nuclear cross sections change as we add or remove protons and neutrons. As a proof of principle, we focus on the neutron-induced reactions in the fast energy regime. Our approach follows a two-stage learning framework. First, we apply representation learning to encode cross section data into a latent space using either variational autoencoders (VAEs) or implicit neural representations (INRs). Then, we train graph neural networks (GNNs) on the resulting embeddings to predict missing values across the nuclear chart by leveraging the topological structure of neighboring isotopes. We demonstrate accurate cross section predictions within a 9 × 9 block of missing nuclei. We also find that the optimal GNN training strategy depends on the type of latent representation used, with VAE embeddings performing best under end-to-end optimization in the original space, while INR embeddings achieve better results when the GNN is trained only in the latent space. Furthermore, using clustering algorithms, we map groups of latent vectors into regions of the nuclear chart and show that VAEs and INRs can discover some of the neutron magic numbers. These findings suggest that deep-learning models based on the representation encoding of cross sections combined with graph neural networks hold significant potential in augmenting nuclear theory models, e.g., by providing reliable estimates of covariances of cross sections, including cross-material covariances.

Machine learning↗
DOE OSTI2025

Parameterizations of electron scattering form factors for elastic scattering and electroexcitation of nuclear states in 27 Al and 40 Ca

Here, we report on empirical parameterizations of longitudinal ($\mathscr{R}$ L ) and transverse ($\mathscr{R}$ T ) nuclear elec- tromagnetic form factors for elastic scattering and the excitations of nuclear states in 27 Al and 40 Ca. The parameterizations are needed for the calculations of radiative corrections in measurements of electron scattering cross sections on 27 Al and 40 Ca in the quasi-elastic, resonance and inelastic con- tinuum regions, provide the contribution of nuclear excitations in investigations of the Coulomb Sum Rule, and test theoretical model predictions for excitation of nuclear states in electron and neutrino interactions on nuclear targets at low energies.

elastic scattering reactions↗
DOE OSTI2024

Summary of light-element evaluation work: nuclear data uncertainty quantification

Hale & Paris (T-2) have evaluated the 15 N system to provide nuclear cross section and covariance information for nuclear data uncertainty quantification. This memo gives a brief discussion of the R-matrix method used to generate this nuclear scattering and reaction data in the ENDF-6 format.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Not-quite-transcendental Functions for Logarithmic Interpolation of Tabulated Data

From tabulated nuclear and degenerate equations of state to photon and neutrino opacities and nuclear reaction rates, tabulated data is ubiquitous in computational astrophysics. The dynamic range that must be covered by these tables typically spans many orders of magnitude. Here we present a novel strategy for accurately and performantly interpolating tabulated data that spans these large dynamic ranges. We demonstrate the efficacy of this strategy in tabulated lookups for nuclear and terrestrial equations of state. We show that this strategy is a faster drop-in replacement for linear interpolation of logarithmic grids.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2026

Enabling event-by-event precision in γ-ray cascades for neutron-induced reactions

Neutron-induced γ-ray spectra provide key inputs for modern active interrogation applications. A precise modeling of the nuclear reaction and subsequent emission of γ rays is challenging and often impossible due to limitations on evaluated data file formats and nuclear transport simulation codes. We present a framework that addresses these challenges by combining experimental data and reaction-model calculation outputs into an extended candidate version of the Generalized Nuclear Data Structure (GNDS) file, the successor format for the legacy Evaluated Nuclear Data File (ENDF-6). This proposed GNDS hierarchical format contains all the necessary ingredients for inline γ-ray cascade reproduction with event-by-event precision, including continuum–continuum and continuum–discrete transitions following neutron-capture and inelastic neutron scattering reactions. Cascade-event generation based on our approach demonstrates improved energy conservation on an event-by-event basis and permits the use of γ-γ coincidences in applications. This work offers, for the first time, a method to generate neutron-capture and inelastic neutron-scattering γ-ray cascades where energy conservation, correlations, and experimental primaries are fully accounted for.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Artificial-intelligence-assisted analysis of 28 Si * → 7⁢𝛼 breakup data

Mid-weight 𝛼-conjugate nuclei are predicted to possess exotic toroid like resonances with high angular momenta. The search for these states in 28 Si* is the main point of two published experimental investigations of the peripheral 28 Si + 12 C reaction by Cao and collaborators and by Hannaman and collaborators. In this work, we develop a novel artificial intelligence (AI) based machine learning method utilizing the Gaussian Mixture Model (GMM) to analyze available experimental and theoretical data. Here, we additionally study the reaction with the Hybrid 𝛼-Cluster (H⁡𝛼⁢C) model. In all the examined data, our results suggest the presence of underlying structure which is close to that predicted for toroidal states.

Breakup reactions↗
DOE OSTI2026

Nuclear Structure and Decay Data for A=220 Isobars

Here, this work presents a comprehensive and critical evaluation of experimental nuclear spectroscopic data from reactions and decays for all 11 known nuclides with mass number A=220 (Pb, Bi, Po, At, Rn, Fr, Ra, Ac, Th, Pa, and Np). Recommended values are produced for level energies, spins and parities, half-lives, and radiation properties including energies, branching ratios, and multipolarities of γ rays, as well as characteristics of β and α radiation decays, based on all available experimental data. This work supersedes previous A=220 evaluations: 2011Br05, 1997Ar04, 1986Ma45, 1976El04.

Chen, J. [Michigan State University, East Lansing,↗
DOE OSTI2026

Measurement of the 252 Cf ⁢(sf) prompt fission neutron spectrum utilizing 12 C ⁡(𝑛, 𝑛) and 9 Be ⁢(𝑛, 𝑛) neutron scattering reference measurements

The 252 Cf spontaneous fission (sf), prompt fission neutron spectrum (PFNS) is a fundamental quantity for nuclear physics measurements of neutron-emitting reactions. This energy distribution of neutrons emitted from fission has been considered a neutron data standard for decades and has been utilized as a reference for neutron detection efficiency, validation of Monte Carlo simulations, benchmarking of dosimetry standards, and more. A significant portion of the global collection of nuclear data on neutron-induced reactions is correlated with the 252 Cf ⁢(sf) PFNS. Despite the reliance on this quantity by the nuclear physics community, the historical collection of 252 Cf PFNS measurements display systematic disagreements that are not understood or easily explained. These experimental discrepancies could potentially bias the 252 Cf PFNS Standard evaluation. On top of this, these past experiments frequently employed correlated experimental measurement or analysis methods. The artificial intelligence (AI)/machine learning (ML)-informed californium chi-nuclear data experiment (AIACHNE) project was formed to (a) investigate these discrepancies utilizing AI/ML methods to identify outlying regions of literature data, assign these regions to features of the experiment itself, and perform an improved evaluation of the 252 Cf PFNS and (b) perform a new experimental measurement of this quantity designed to improve upon the existing literature database. Here, in this work, we report on the AIACHNE 252 Cf PFNS experiment utilizing a new analysis method uncorrelated with all previous measurements: neutron efficiency determinations based on elastic neutron scattering on 12 C and 9 Be . This new method provides an independent test of the existing literature data and evaluation of the 252 Cf ⁢(sf) PFNS. The method is described with detailed covariance quantification procedures, as well as a direct discussion of the sources of uncertainty described as requirements in the “Templates” series of papers. The 252 Cf ⁢(sf) PFNS reported in this work agrees well with the overall shape of the existing standard PFNS evaluation as well as many literature measurements, thus verifying the current evaluation utilizing new techniques. However, the results suggest that there are deficiencies in the angle-differential 12 C and 9 Be ⁢(𝑛, 𝑛) evaluated nuclear data, which produce unphysical structures in the reported result. While these structures are relatively minor, they become obvious because of the high statistical precision of the data and the expected smooth continuity of the 252 Cf ⁢(sf) PFNS.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Nuclear Structure and Decay Data for A=35 Isobars

Here, this work presents a comprehensive and critical evaluation of experimental nuclear spectroscopic data from reactions and decays for all 11 known nuclides with mass number 35 (Ne, Na, Mg, Al, Si, P, S, Cl, Ar, K, Ca). Recommended values are produced for level energies, spins and parities, half-lives, and radiation properties including energies, branching ratios, and multipolarities of γ rays, as well as characteristics of β radiation decays, based on a rigorous assessment of all available experimental data. Discrepancies among existing results are carefully addressed. This work supersedes earlier full evaluations of A=35 published by 2011Ch48, 1990En08 (also 1998En04 update) and 1978En02.

Sun, Lijie [Michigan State University, East Lansin↗
DOE OSTI2025

Measurement of the 28 Si ⁢(𝑛,𝑛′⁢𝛾) cross section with 𝑛, 𝛾, and correlated 𝑛−𝛾 angular distributions

Silicon has become an unavoidable element in the circuitry central to everyday life. In turn, the interactions of silicon isotopes with neutrons for nuclear physics applications, among other motivations, have become increasingly important to understand. The dominant isotope of silicon, 28 Si, is thus of primary interest for enhanced understanding for neutron transport calculations and related investigations. Unfortunately, the existing measurement database for neutron scattering reactions on 28 Si is minimal, and nuclear data evaluations on this topic have not been updated for decades. This article details new measurements of the 28 Si ⁢(𝑛,𝑛′⁢𝛾) reaction utilizing multiple analysis methods available within the correlated gamma neutron array for scattering (CoGNAC). Specifically, high-precision near-threshold results and high-incident-energy results were obtained using the 𝛾-only and correlated 𝑛−𝛾 techniques. First-ever measurements of the correlated 𝑛−𝛾 angular distribution for particles emitted following population of the first excited state in 28 Si were obtained as well, which provide unique insight into theoretical descriptions of the inelastic neutron scattering reaction mechanism itself and detailed guidance for nuclear reaction models. The results agree well with literature data where they exist, and substantially expand on the current database for neutron reactions on 28 Si .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Microjet printing of metal salt or oxide targets for nuclear reaction studies on radionuclides

Radioactive targets for direct measurements of neutron-induced reactions are required to improve evaluated cross-section data and, ultimately, the fidelity of neutron reaction network simulations. Electrodeposition and molecular plating are the current state-of-the-art radioactive target production techniques, but not all metals can be electrodeposited or molecular plated with high yields. Alternative techniques can be expensive or may produce targets that are unsatisfactory in terms of thickness, yield, or purity. Microjet printing is a new, rather inexpensive technique that utilizes equipment with a small footprint and has the potential to produce thin, highly radioactive targets with good uniformity and minimal impurities from the target fabrication process. This study involved optimizing the process of producing microjet printed targets to allow for the fabrication of a stable vanadium(V) oxide (V 2 O 5 ) target that was compared with an analogous electrodeposition V 2 O 5 target manufactured via the application of a vanadium chemical conversion coating on aluminum (Al) foil. Finally, the results from these studies suggest microjet printing could be used to produce relatively uniform target layers with adequate film thicknesses (< 15 μm). V 2 O 5 microjet printed targets, when compared with chemical conversion coating V 2 O 5 targets, appeared to be qualitatively less uniform and quantitatively larger in thickness (11.7(27) μm vs. 5.3(18) μm). However, the conversion coating target contained more impurities and the Al backing had a higher background contribution to measurements of neutron-induced reactions as opposed to targets produced via microjet printing. Overall, the results from this study suggest microjet printing has the capability to be an excellent alternative target production technique to the electrodeposition and molecular plating methods.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

Forward modeling approach to nuclear reaction cross sections: Applications in neutron inelastic scattering

The development of nuclear reaction models for the production of evaluated nuclear data has traditionally been performed by comparing measured cross sections with predictions from reaction model codes whose physical input parameters are adjusted to obtain the best agreement between measured and modeled results. To more directly probe reaction model inputs, this work introduces a forward modeling approach to experimental reaction cross-section determination, where the most important physical input parameters to reaction model calculations are obtained via 𝜒 2 minimization between measured and calculated observables. This was demonstrated using data collected by the Gamma Energy Neutron Energy Spectrometer for Inelastic Scattering (GENESIS) at the 88-inch cyclotron at Lawrence Berkeley National Laboratory, a detection array consisting of organic liquid scintillators and high-purity germanium (HPGe) detectors. Using a broad-spectrum neutron beam and a 99.98%-enriched 56 Fe target, GENESIS was used to perform a simultaneous measurement of 56 Fe 𝛾-ray production cross sections and secondary neutron energy and angle distributions. The results of the forward modeling approach to the determination of energy-differential 𝛾-ray production cross sections for the yrast 4 + → 2 + and 6 + → 4 + transitions, as well as eight other off-yrast transitions, were compared against those obtained using conventional techniques, and the results are in good agreement. In addition to discrete 𝛾-ray yield total scattered neutron energy-angular distributions as a function of incident neutron energy were also obtained using forward modeling and found to agree with evaluated data, with the exception of elastic scattering at small angles. The fitted reaction model parameters obtained through forward modeling were also used to calculate the cross section for the unobserved (𝑛, 2⁢𝑛) reaction; excellent agreement with the current evaluation was obtained, providing a validation of the predictive capabilities of the forward model approach. This work bridges the gap between nuclear data experiment and evaluation by providing a new means for extracting inelastic neutron-scattering cross sections and neutron-induced 𝛾-ray production data while directly probing reaction model physics.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

R -matrix analysis of n + nat Cl reactions up to 1.2 MeV

The R -matrix analysis of neutron-induced reactions for two stable chlorine isotopes ( 35 Cl and 37 Cl) was performed in the energy range of thermal up to 1.2 MeV. Starting from the repository of the ENDF/B-VIII.0 library and following recent measurement series, this work represents a significant improvement, particularly in the evaluation of the ( n , p ) reaction channel. The evaluation methodology used the R -matrix code SAMMY to generate a set of Reich–Moore resonance parameters for both stable chlorine isotopes. Consistent with recently measured 35 Cl( n , p ) data, the presented evaluation features a dramatic increase in the magnitude of the ( n , p ) reaction channel over the ENDF/B-VIII.1 nuclear data library and previous ENDF/B libraries.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Measurement of the branching ratio of 16 N , 15 C , 12 B , and 13 B isotopes through the nuclear muon capture reaction in the Super-Kamiokande detector

The Super-Kamiokande detector has measured solar neutrinos for more than 25 years. The sensitivity for solar neutrino measurement is limited by the uncertainties of energy scale and background modeling. Decays of unstable isotopes with relatively long half-lives through nuclear muon capture, such as 16 N, 15 C, 12 B, and 13 B, are detected as background events for solar neutrino observations. Here, in this study, we developed a method to form a pair of stopping muon and decay candidate events and evaluated the production rates of such unstable isotopes. We then measured their branching ratios considering both their production rates and the estimated number of nuclear muon capture processes as Br⁡( 16 N) = (9.0 ± 0.1)%, Br⁡( 15 C) = (0.6 ± 0.1)%, Br⁡( 12 B) = (0.98 ± 0.18)%, Br⁡( 13 B) = (0.14 ± 0.12)%, respectively. The result for 16 N has world-leading precision at present and the results for 15 C, 12 B, and 13 B are the first branching ratio measurements for those isotopes.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗