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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

A workflow to assess the efficacy of brine extraction for managing injection-induced seismicity potential using data from a CO 2 injection site near Decatur, Illinois

Injection of CO 2 for storage in a geologic formation increases pore pressure and alters in situ stresses. Depending on the orientation of any existing fault and fracture planes, such as critically stressed planes, this stress alteration will modify normal stresses acting on planes and could result in frictional sliding and release stored energy in the form of seismicity. Brine extraction (BE) is a technique that can be applied prior to, or during, CO 2 injection to reduce pore pressure for increasing storage capacity and, potentially, for reducing the likelihood of frictional sliding. Here a workflow is described to assess the efficacy of BE for mitigating frictional sliding (i.e., seismicity) during injection and entails: site characterization, stress calculations and failure assessment, static and dynamic modeling, and BE operational planning. Site characterization describes the stress field used to calculate the Coulomb Failure Function (CFF) that constrains allowable pore pressure changes and injection rates in the numerical simulation of CO 2 injection scenarios. The inclusion of BE in the workflow allows for determination of the potential need for pressure reduction, and evaluation of the effectiveness of this operation. Example application of the workflow using an injection field dataset near Decatur, IL, provides insight on fracture planes and stresses at the site, formation properties and the impact of variable CO 2 injection-rate targets on whether BE plans are required. The study workflow indicates that BE could enhance CO 2 injection rate by 39% and correspondingly reduce the potential for injection-induced seismicity as indicated by a reduction in CFF.

58 GEOSCIENCES↗
DOE OSTI2025

Plasma modification through boron particulate injection in the full tungsten environment of WEST

Recent experiments have confirmed the compatibility of extended boron particulate injections with high performance plasma discharges in the full tungsten (W) environment of WEST. Utilizing an impurity powder dropper (IPD) equipped with boron (B) powders a series of extended experimental programs providing controlled injections have quantified plasma response to varying levels of injection rate and total injection quantity. Calibration of injection quantities confirmed through post-situ testing of the IPD and cross-correlated with both high-speed camera illumination and spectroscopic measurement have allowed for the first time a fine scale determination of the effects of powder introduction on plasma performance. Plasma enhancement, consistent with turbulence reduction through profile modification, has been observed with sustained increases in the stored energy (WMHD), by 18%, electron temperature (T e ) by 35%, and neutron rate (N n ) by up to 200%, all of which scale positively with increasing powder injection rates. These injections have also resulted in both prompt and extended reductions in native impurity content, decreases in post injection radiated power, and strong decreases in divertor deuterium signatures signifying a reduction in recycling suggesting enhanced boron layer formation which provides a reduction of source terms and leads to enhanced gettering of main ion and impurity sources.

Lunsford, R. [Princeton Plasma Physics Laboratory ↗
DOE OSTI2024

Cyclic Injection Leads to Larger and More Frequent Induced Earthquakes under Volume-Controlled Conditions

As carbon storage technologies advance globally, methods to understand and mitigate induced earthquakes become increasingly important. Although the physical processes that relate increased subsurface pore pressure changes to induced earthquakes have long been known, reliable methods to forecast and control induced seismic sequences remain elusive. Suggested reservoir engineering scenarios for mitigating induced earthquakes typically involve modulation of the injection rate. Some operators have implemented periodic shutdowns (i.e., effective cycling of injection rates) to allow reservoir pressures to equilibrate (e.g., Paradox Valley) or shut-in wells after the occurrence of an event of concern (e.g., Basel, Switzerland). Other proposed scenarios include altering injection rates, actively managing pressures through coproduction of fluids, and preinjection brine extraction. Here, in this work, we use 3D physics-based earthquake simulations to understand the effects of different injection scenarios on induced earthquake rates, maximum event magnitudes, and postinjection seismicity. For comparability, the modeled injection considers the same cumulative volume over the project’s operational life but varies the schedule and rates of fluid injected. Simulation results show that cyclic injection leads to more frequent and larger events than constant injection. Furthermore, with intermittent injection scenario, a significant number of events are shown to occur during pauses in injection, and the seismicity rate remains elevated for longer into the postinjection phase compared to the constant injection scenario.

58 GEOSCIENCES↗
DOE OSTI2021

Hydraulic Modeling of Induced and Propagated Fractures: Analysis of Flow and Pressure Data From Hydromechanical Experiments in the COSC-1 Deep Borehole in Crystalline Rock Near Åre, Sweden

To characterize the coupled hydromechanical behavior of rock fractures, the step-rate injection method for fracture in-situ properties (SIMFIP) was conducted with a specialized downhole probe developed by Guglielmi et.al. In June 2019, a field campaign was carried out near Åre, Sweden, where the SIMFIP probe was applied in the Collisional Orogeny in the Scandinavian Caledonides-1 scientific borehole to understand the dynamics of injection-induced fracture initiation, fracture opening, and shearing due to water injection-withdrawal in a borehole interval isolated by two packers. Three intervals were investigated at ~500 m depth: (a) an unfractured section (intact rock), (b) a section with non-conductive fractures, and (c) a section with hydraulically conductive fractures. Pressure, injection flow rate, and borehole wall displacement were simultaneously measured during the tests. In the present study, the geometry of the induced fracture and deformation of existing fractures at different time stages of the tests are determined based on a hydrologic model by using the measured pressure and flow data during each time stage of the experiment. A numerical model for the fluid flow within the fracture and the packed-off borehole interval is implemented within COMSOL Multiphysics. By matching model simulations with observed data for all three sections, estimates of the induced and propagated fractures' radius and aperture at successive time stages have been obtained in each case. We could also determine the non-linear relationship between fracture aperture and pressure for values above fracture opening pressures. The model results provide insights for the understanding of pressure-induced fracture initiation and propagation in crystalline rock.

58 GEOSCIENCES↗
NASA NTRS1990

The influence of Oort clouds on the mass and chemical balance of the interstellar medium

The contribution of stellar encounters and interstellar erosion to comet cloud mass injection to the ISM is calculated. It is shown that evaporative mass loss from passing stars and SNe results in an average Galactic mass injection rate of up to 10 to the -5th solar mass/yr if such clouds are frequent around solar-type stars. Cometary erosion by interstellar grains produces an injection rate of 10 to the -5th to 10 to the -4th solar mass/yr. An injection rate of 2 x 10 to the -5th solar mass/yr is calculated. Each of these rates could be increased by a factor of about 15 if the comet clouds contain a significant amount of smaller debris. It is concluded that the total mass injection rate of material to the ISM by comet clouds is small compared to other ISM mass injection sources. Comet cloud mass loss to the ISM could be responsible for a sizeable fraction of the metal and dust abundances of the ISM if Oort clouds are common.

Stern, S. Alan↗
DOE OSTI2023

Effect of initial water saturation on the performance of fracturing fluids with and without polyallylamine under simulated EGS conditions

Objectives/Scope: StimuFrac (US Patents 9,873,828 B2 and 9,447,315 B2), a CO 2 - reactive polymer aqueous solution [polyallylamine (PAA) 1wt% in water] combined with CO 2 , can be used as a potentially less water-intensive fracturing fluid for enhanced geothermal systems (EGS). Our previous results show that in hot dry rock (HDR), PAA/CO 2 fracturing fluids outperformed other fluids such as water, CO 2 , and CO 2 /water in generating large fractures with less fluid consumed. The objective of this work is to investigate the effect of initial water saturation on the performance of StimuFrac by conducting hydraulic fracturing tests with ½ foot cubic rock samples held under representative EGS stress/temperature conditions and by using cyclic injection strategies (under constant injection rate). The resulting fracture hydraulic conductivities, breakdown pressures, and volumes of fluids required are compared. Methods/Procedures/Process: To simulate geothermal reservoir conditions, in all tests, the rock sample was held under triaxial confinement and at 200 °C, and different volumes of water were initially injected into the rock sample before any fracturing processes were initiated. For the single-cycle PAA (or water) alternating CO 2 (PAG or WAG) injection fracturing experiments, one complete cycle consisted of two steps: (1) injecting a PAA slug (or water slug) followed by (2) injecting CO 2 to initiate and propagate the fracture. For experiments involving multiple injection cycles, the CO 2 injection pressure is increased until it peaks and begins to decline (indicating fracture initiation at this moment), and then continued being injected for another 30 seconds to propagate the fracture. Then, these two-step cycles [injection of PAA (or water) followed by CO 2 injection (up to 2-4 mL/min)] are repeated. Applications/Significance/Novelty: The results of this study suggest that water saturation significantly affects the fracturing fluid transmission into the rock pore space, thus affecting the fracture initiation and propagation. In this study, fracturing tests via a single injection cycle or multiple injection cycles were performed. Splitting the rock samples in half after testing reveals that fracture propagation is significantly limited under high water saturation conditions (three-day initial water injection) compared to stimulation experiments performed in hot dry rock. The fractures propagate less than 1/3 of the distance from the wellbore to the outer rock surface, and in some cases, no fracture is generated. This may be caused by leak-off dominating the fracturing process and the fluid injection rate is insufficient to overcome leak-off, even under high injection rate conditions. Additionally, CO 2 could be leaking off into the wellbore annulus and this may be making it more difficult to generate sufficiently high-pressure gradients away from the near-wellbore region. Under low water saturation conditions (dry rock or after 1-day initial water injection), PAA/CO 2 consistently generated significantly larger fractures compared with the other fluids. CO 2 generated large fractures only in the hot dry rock and only when using high injection rates, though data variability is high.

58 GEOSCIENCES↗
DOE OSTI2023

Laboratory investigation of hydraulic fracturing in granitic rocks using active and passive seismic monitoring

SUMMARY Knowledge of the fracturing processes can be important for the optimization of pressurized fluid injection operations in the deep underground rock mass. Active and passive seismic monitoring techniques have been used in the field for tracking or mapping the propagating hydraulic fracture. Although both these monitoring techniques provide valuable information about the generated fracture network, it is difficult for either technique to comprehensibly identify the different processes associated with hydraulic fracturing. The combined active and passive monitoring has the potential for better characterization of the complex hydraulic fracturing phenomena. In this study, laboratory hydraulic fracturing experiments with combined active and passive seismic monitoring were conducted on true triaxially loaded Barre granite cubes with different fluid injection rates. The seismic inelastic fracturing was detected by 16 passive acoustic emission sensors, where 3678 and 2370 seismic source events were detected for the high and low injection rate experiments, respectively. For active monitoring, strong variations in the attributes of signals were observed which were transmitted through four source–receiver pairs, placed both perpendicular and parallel to the generated hydraulic fracture. Positive velocity changes were observed for active sensor pairs with ray paths passing through the generated hydraulic fracture indicating fluid permeation, whereas isolated dry deformation was characterized by a slight but permanent velocity decrease. Compared to velocity, the energy of the active signals was 1–2 orders of magnitude more sensitive to different hydraulic fracturing processes. However, the sensitivity and signatures of the active signal attributes were found to be dependent on the frequency range and direction of ray path with respect to the location of the generated fracture network. Using the coupled evaluation of the active and passive signals we were able to systematically identify various hydraulic fracturing processes including: (1) aseismic deformation, (2) fracture initiation and fluid permeation, (3) pressure build-up, (4) fracture propagation and (5) pressure release and leak-off. The results of this study showed that combining the respective advantages of active and passive seismic techniques and using both of them to monitor the failure processes can facilitate a more comprehensive understanding and better control of the hydraulic stimulations in subsurface operations.

Geochemistry & Geophysics↗
NASA NTRS1976

Laminar flow at a three-dimensional stagnation point with large rates of injection

Exact calculations of the titled flow are presented and compared to the predictions of an asymptotic analysis for large rates of injection. The inner layer of the boundary layer is found to involve outflow in both orthogonal directions whether the external flow along the y axis is inward or outward. As a result, the flow at a nearly two-dimensional stagnation point involves drastic changes as a weak outflow changes to a weak inflow. It is also found that the velocity profiles in the two directions in the inner layer are quite different.

Libby, P. A.↗
NASA NTRS1971

Experiment T001: Entry communication on the Gemini 3 mission

Water addition to the Gemini 3 exhaust plasma was studied to determine its effectiveness in the establishment of communication links during the entry portion of the flight. Attenuation levels were measured with and without water injection at uhf frequencies of 230.4 and 296.8 megahertz and at the C-band frequency of 5690 megahertz. Ultrahigh frequency signals that had been blacked out were restored to significant levels, during early portions of the water-injection sequence, by the high flow rate injection. The C-band signal was enhanced by medium and high flow rate injections during the latter portion of the injection period. The uhf signal recovered during water injection resulted in an antenna pattern that was beamed in the radial direction of injection from the spacecraft. Postflight analysis showed that the uhf recovery data were consistent with injection-penetration theory.

Schroeder, L. C.↗
DOE OSTI2022

Modeling the effect of nitrogen recycling on the erosion and leakage of tungsten impurities from the SAS-VW divertor in DIII-D during nitrogen gas injection

The new SAS-VW divertor in DIII-D has tungsten-coated components to enable the study of tungsten erosion and leakage from a closed, slot-like divertor. A proposed method of actively managing the tungsten impurities is to inject low-Z impurities, such as nitrogen, into the Scrape-off-Layer (SOL) to modify the conditions in the plasma boundary and in turn manipulate both the erosion and subsequent transport of tungsten. Nitrogen injection from the SOL crown has been modeled using SOLPS-ITER to calculate the background plasma including the intrinsic carbon and the injected nitrogen impurities, and subsequently DIVIMP has been used to calculate the tungsten erosion and transport on top of the background plasma solution. This workflow has been used to model scenarios at a variety of nitrogen injection rates with different assumptions about the nitrogen recycling at the target. In the scenario modeled here, an optimal nitrogen injection rate around 3-4 x 10 20 N/s is found to reduce the amount of tungsten reaching the core by a factor of about 2.4. However, when the nitrogen recycling rate at the divertor targets is high, the nitrogen redistributes within the slot leading to increased tungsten sputtering, and the range of injection rates resulting in tungsten mitigation becomes narrower.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2026

The effectiveness of D 2 pellet and gas injection in reducing intra-ELM tungsten erosion and heat flux in the DIII-D small angle slot divertor

Edge localized modes (ELMs) in H-mode plasmas can melt and erode plasma-facing components (PFCs) and lead to impurities in the core, reducing confinement. This study analyzes the use of D 2 pellet and gas injection for ELM mitigation on the DIII-D tokamak during the 2022 Small Angle Slot V-shaped Tungsten (W) (SAS-VW) divertor campaign, reducing W erosion and heat flux during ELMs. D α (656 nm) and WI (400.9 nm) filterscopes and Langmuir probes provide photon emission and electron density/temperature to estimate W atom erosion using the S/XB method, while surface eroding thermocouples measured ELM peak heat flux at the outer strike point (OSP). Thomson Scattering measurements of pedestal T e and n e provided input to predict W divertor erosion and heat flux during ELMs via the Free-Streaming plus Recycling Model (FSRM). While a greater D 2 mass injection rate decreased the ELM peak heat flux, the impact on W erosion was not monotonic. The average ‘large’ intra-ELM W erosion was lower for plasma shots with D 2 mass injection compared to the plasma shots without any D 2 mass injection in the SAS-VW divertor. However, plasma shots did not see significant changes in ‘large’ intra-ELM W divertor erosion as the D 2 mass injection rate increased. On average, the FSRM overestimated SAS-VW experimental intra-ELM W erosion by a factor of 6.9, but the overestimation is reduced to a factor of 3.6 with the implication of C deposition effects. Generally, experimentally measured and predicted quantities were worse for plasma shots with a lower D 2 mass injection rate and corresponding higher plasma carbon (C) impurity percentage (f C ). The discrepancies are postulated to be due to C/W material mixing, for which a simple analytic mixed-material model is presented. These results highlight the importance of incorporating and improving the robustness of a mixed-material layer model in the analysis of PFC erosion on present and future tokamak devices.

Carbon (C)↗
DOE OSTI2025

A Model Intercomparison Study of Aerosol‐Cloud‐Turbulence Interactions in a Cloud Chamber: 1. Model Results

This study presents the first model intercomparison of aerosol‐cloud‐turbulence interactions in a controlled cloudy Rayleigh‐Bénard Convection chamber environment, utilizing the Pi Chamber at Michigan Technological University. We analyzed simulated cloud chamber‐averaged statistics of microphysics and thermodynamics in a warm‐phase, cloudy environment under steady‐state conditions at varying aerosol injection rates. Simulation results from seven distinct models (DNS, LES, and a 1D turbulence model) were compared. Our findings demonstrate that while all models qualitatively capture observed trends in droplet number concentration, mean radius, and droplet size distributions at both high and low aerosol injection rates, significant quantitative differences were observed. Notably, droplet number concentrations varied by over two orders of magnitude between models for the same injection rates, indicating sensitivities to the model treatments in droplet activation and removal and wall fluxes. Furthermore, inconsistencies in vertical relative humidity profiles and in achieving steady‐state liquid water content suggest the need for further investigation into the mechanisms driving these variations. Despite these discrepancies, the models generally reproduced consistent power‐law relationships between the microphysical variables. This model intercomparison underscores the importance of controlled cloud chamber experiments for validating and improving cloud microphysical parameterizations. Recommendations for future modeling studies are also highlighted, including constraining wall conditions and processes, investigating droplet/aerosol removal (including sidewall losses), and conducting simplified experiments to isolate specific processes contributing to model divergence and reduce model uncertainties.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Methane foam performance in oil-wet unconsolidated porous media: A systematic experimental investigation at reservoir conditions

Methane foam performance was systematically evaluated using high-pressure and high-temperature experiments performed on oil-wet proppant packs. The sensitivities of foam performance to various key factors, including surfactant concentration, foam quality, total injection rate, salinity, operating pressure, and initial oil saturation were examined. The results showed that even though the foamability and foam strength in oil-wet proppant packs were adversely affected by wettability and presence of oil, the steady-state pressure drops across the proppant packs were insensitive to the quantity of oil initially present. The presence of oil above the critical oil saturation impeded the onset of foam generation. This suggested that the foamability of surfactants depends on the synergetic effects of surfactant’s ionic nature and foam parameters, such as foam quality and total injection rate, on their ability to reduce the oil saturation to a threshold value below which favorable bubble generation sites could be created. It was observed that, for low injection rate, anionic surfactant was ineffective at low salinity conditions, while amphoteric agent performed well at all salinities. Additionally, an increase in salinity resulted in enhanced pressure drop across the proppant packs for both anionic and amphoteric surfactants. Further, the results also established that too high operating pressures are somewhat detrimental to the foam strength and stability, irrespective of the ionic nature of foaming agents and the wettability of the porous medium. For the anionic surfactant, the increase in the total flow rate was found to mitigate the adverse effects of low salt concentration and operating pressure. Results from quality-sensitivity foam tests identified two regions for the foam behavior, named low-quality and high-quality regimes, separated by the transition foam quality. Finally, we discuss the implications of the results for the design and effective implementation of enhanced oil recovery (EOR) schemes that deploy hydrocarbon-based foams.

02 PETROLEUM↗
DOE OSTI2022

The Synchrotron Low-energy Spectrum Arising from the Cooling of Electrons in Gamma-Ray Bursts

This work is a continuation of a previous effort (Panaitescu) to study the cooling of relativistic electrons through radiation (synchrotron and self-Compton) emission and adiabatic losses, with application to the spectra and light curves of the synchrotron gamma-ray burst (GRB) produced by such cooling electrons. Here, we derive the low-energy slope β LE of a GRB pulse-integrated spectrum and quantify the implications of the measured distribution of β LE . Radiative processes that produce soft integrated spectra can accommodate the harder slopes measured by CGRO/BATSE and Fermi/GBM only if the magnetic field lifetime t B is shorter than the time during which the typical GRB electrons cool to radiate below 1–10 keV, which is less than (at most) 10 radiative cooling timescales t rad of the typical GRB electron. In this case, there is a one-to-one correspondence between t B and β LE . To account for low-energy slopes β LE > -3/4, the adiabatic electron-cooling requires a similar restriction on t B . In this case, the diversity of slopes arises mostly from how the electron-injection rate varies with time (temporal power-law injection rates yield power-law low-energy GRB spectra) and not from the magnetic field timescale.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Minimizing exposure to legacy wells and avoiding conflict between storage projects: Exploring area of review as a screening tool

Elevated pressure from large-volume injection is a key driver of risk and project cost. If transmissive features (e.g., non-isolating wells or fracture systems) are present, increased injection-zone pressure can drive fluids from depth toward protected freshwater resources. In US Carbon Capture and Storage (CCS) law, the area at risk is known as the Area of Review (AoR). The size and number of potentially transmissive features to be evaluated and possibly remediated or managed is a function of the size and location of the AoR. The size of the AoR depends on several variables, including properties of the injection zone, properties of protected resources, and injection rate and duration. Evaluation of the intersection of these variables across a portfolio of sites highlights the injection zone depth and boundary conditions as top-level controls. Deep injection, use of multiple stacked injection zones, reduced injection rate and choice of injection well location can all be used to minimize AoR and the number of potentially transmissive features within it. Here, we introduce the concept of pressure space (defined as connected pore volume times pressure) as the key subsurface commodity for CO 2 storage and we suggest that it forms a more robust basis for leasing and regulation than pore space alone.

58 GEOSCIENCES↗
DOE OSTI2026

Basin-scale analysis of Mokelumne River Formation for multi-well CO 2 injection

Large-scale carbon sequestration will likely require multiple projects injecting CO 2 into the same subsurface formation, raising concerns about safe operation and efficient use of storage capacity. This study evaluates the long-term response of the Mokelumne River Formation in California’s Sacramento Basin to multi-megaton CO 2 injection using three geologic models of the formation and the open-source simulator GEOS. The analysis focuses on three aspects of reservoir performance: (1) average pressure increase and dissolved CO 2 mass after 30 years for varying well counts and injection rates, (2) pressure interference in a multi-well configuration, and (3) dynamic storage capacity with identification of overpressure-prone regions. The results show that average formation pressure increases linearly with injected mass, while CO 2 dissolution exhibits mixed scaling: approximately linear with the number of wells but sublinear with injection rate, indicating that distributing injection across more wells enhances dissolution more effectively than increasing per-well rates. Pressure-interference effects are significant, with lower-permeability conditions delaying their onset but amplifying their magnitude at later times. Dynamic capacity, defined by the first occurrence of pressure exceeding the local overburden-based limit anywhere in the formation, varies across geologic models and assumed overburden pressure gradients. A lower fidelity geologic model predicts nearly twice the storage capacity of the two higher fidelity models, which consistently estimate approximately 1 Gt under the upper-bound overburden pressure gradient considered for the Sacramento Basin. In all model scenarios, overpressure develops away from injection wells, particularly in higher-elevation regions, highlighting the importance of basin-scale modelling for identifying risks beyond the immediate well vicinity.

Basin-scale↗
NASA NTRS1987

Sputtering of sulfur by kiloelectronvolt ions - Application to the magnetospheric plasma interaction with Io

Accurate measurements of the yields, mass spectra, and energy spectra of ejected sulfur are presented based on vapor deposits of sulfur at temperatures and ion energies relevant to the plasma interaction with the surface of Io. The measured sputtering yields are much lower than previous estimates for room temperature sulfur films, but are comparable to previous measurements of low-temperature keV ion sputtering of SO2. Results suggest that if ions reach the surface of Io its atmosphere will have a nonnegligible sulfur component which is primarily S2. Comparison of injection rates determined for sulfur with those for SO2 indicates that injection from sulfur deposits contributes 13 percent to the total mass injection rate of about 2-3 x 10 to the 29th amu/sec.

Chrisey, D. B.↗
DOE OSTI2025

Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud Response

Abstract Cloud responses to surface‐based sources of aerosol perturbation partially depend on how turbulent transport of the aerosol to cloud base affects the spatial and temporal distribution of aerosol. Here, scenarios of plume injection below a marine stratocumulus cloud are modeled using large eddy simulations coupled to a prognostic bulk aerosol and cloud microphysics scheme. Both passive plumes, consisting of an inert tracer, and active plumes are investigated, where the latter are representative of saltwater droplet plumes such as have been proposed for marine cloud brightening. Passive plume scenarios show higher in‐plume cloud brightness (relative to out‐of‐plume) due to the predominant transport of the passive plume tracer from the near‐surface to the cloud layer within updrafts. These updrafts rise into brighter areas within the cloud deck, even in the absence of an aerosol perturbation associated with an active plume. Comparing albedo at in‐plume to out‐of‐plume locations associates the inert plume with the brightest cloud locations, without any causal effect of the plume on the cloud. Numerical sensitivities are first assessed to establish a suitable model configuration. Then sensitivity to particle injection rate is investigated. Trade‐offs are identified between the number of injected particles and the suppressive effect of droplet evaporation on plume loft and spread. Furthermore, as the near‐field in‐plume brightening effect does not depend significantly on injection rate given a suitable definition of perturbed versus unperturbed regions of the flow, plume area is a key controlling factor on the overall cloud brightening effect of an aerosol perturbation.

54 ENVIRONMENTAL SCIENCES↗