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NASA NTRS2004

Lunar and Planetary Science XXXV: Early Solar System Chronology

The titles in this section discuss: 1) Mg Isotopic Systematics in Eutectites; 2) Diffusion Kinetics of Cr in Olivine; 3) The W Isotope Composition of Eucrite Metals; 4) U-Pb and Hf-W Chronometry; 5) Fe-60 in Silicate from a Semarkona Chondrule; 6) The Isotope Geochemistry of Nickel in Chondrites and Iron Meteorites; 7) Iron-60 in the Early Solar System; 8) Endemic Mo Isotopic Anomalies in Iron and Carbonaceous Meteorites; 9) Solar System Iron and Tungsten Isotope Abundances; 10) Li and B Isotope Variations in CAI; 11) Short-lived Radionuclides and Early Solar System Irradiation; Ru Endemic Isotope Anomalies in Meteorites; 12) Cl-36 in Ca-Al rich inclusions from a carbonaceous chondrite.

Source record↗
NASA NTRS1974

The movement of small particulate matter in the early solar system and the formation of satellites

The motions of the abundant small particulate matter in the early solar system are discussed. The effects of gas drag and resonance effects of perturbing forces could have led to accretion and differentiation of the matter. The composition of the moon and the existence of the rings of Saturn can be explained on the basis of the assembly of small particulate matter in satellite orbits around the planets.

Gold, T.↗
NASA NTRS1993

Energetic particle environment in the early solar system - Extremely long pre-compaction meteoritic ages or an enhanced early particle flux

Individual mineral grains from meteorites have been exposed to energetic particles prior to inclusion in the host meteorite matrix, an event which occurred quite early in solar system history. Spallation-produced noble gases in such grains are observed to be orders of magnitude greater in abundance than could be produced after meteorite formation and thus provide a record of precompaction irradiation by energetic particles. If attributed to the contemporary particle environment (current galactic and solar cosmic rays) a minimum exposure time for these grains in the CM parent-body regolith of 150 Myr is obtained, with more realistic models suggesting an active parent body regolith for 300 Myr. Constraints on when meteorite compaction occurred and current models for meteorite evolution suggest that this is unreasonably long, that the time available for exposure to energetic particles on the surface of the parent-body regolith is much less than this. Pre-compaction exposure, compressed into a shorter span of time by constraints on the compaction times of carbonaceous meteorites, would require energetic particle fluxes in excess of those in the contemporary solar system and point toward an active early (T Tauri) sun as its source.

Woolum, Dorothy S.↗
NASA NTRS1973

Deuterium in the early solar system.

An attempt is made to construct a self-consistent picture of the deuterium abundance in the early solar system based on the assumption of chemical equilibrium in the solar nebula. A recent determination of the D/H ratio for the atmosphere of Jupiter is consistent with a previous estimate of the D/H ratio for the protosun. The high (greater than .00015) D/H ratios determined from analyses of carbonaceous meteorites imply an equilibrium temperature less than 270 K, in marked disagreement with the equilibrium temperature determined for the same material by oxygen isotope cosmothermometry.

Black, D. C.↗
NASA NTRS1993

Development of a molecular beam technique to study early solar system silicon reactions

Silicon monoxide is one of the major gas phase silicon bearing components observed in astronomical environments. Silicon oxide serves as the major rock forming material for terrestrial and meteoritic bodies. It is known that several gas phase reactions produce mass independent isotopic fractionations which possess the same delta(O-17)/delta(O-18) ratio observed in Allende inclusions. The general symmetry dependence of the chemically produced mass independent isotopic fractionation process suggests that there are several plausible reactions which could occur in the early solar system which may lead to production of the observed meteoritic oxygen isotopic anomalies. An important component in exploring the role of such processes is the need to experimentally determine the isotopic fractionations for specific reactions of relevance to the early solar system. It has already been demonstrated that atomic oxygen reaction with CO, a major nebular oxygen bearing species, produces a large (approximately 90 percent), mass independent isotopic fractionation. The next hurdle regarding assessing the involvement of symmetry dependent isotopic fractionation processes in the pre-solar nebula is to determine isotopic fractionation factors associated with gas phase reactions of metallic oxides. In particular, a reaction such as O + SiO yields SiO2 is a plausible nebular reaction which could produce a delta(O-17) is approximately delta(O-18) fractionation based upon molecular symmetry considerations. While the isotopic fractionations during silicate evaporation and condensation have been determined, there are no isotopic studies of controlled, gas phase nucleation processes. In order to carefully control the reaction kinetics, a molecular beam apparatus has been constructed. This system produces a supersonic, collimated beam of SiO molecules which is reacted with a second beam of oxygen atoms. An important feature of molecular beams is that they operate at sufficiently low pressures and high temperatures in the jet that avalanche nucleation and clustering processes may be avoided.

Dong, Q. W.↗
NASA NTRS1983

Samarium-146 in the early solar system - Evidence from neodymiun in the Allende meteorite

A carbon-chromite fraction from the Allende C3V chondrite shows strikingly large isotopic enrichments of neodymium-142 (0.47 percent) and neodymium-143 (36 percent). Both apparently formed by alpha decay of samarium-146 and samarium-147 (half-lives 1.03 x 10 to the 8th and 1.06 x 10 to the 11th years), but the isotopic enrichment was greatly magnified by recoil of residual nuclei into a carbon film surounding the samarium-bearing grains. These data provide an improved estimate of the original abundance of extinct samarium-146 in the early solar system, Sm-146/Sm-144 = (4.5 + or - 0.5) x 10 to the -3rd, higher than predicted by some models of p-process nucleosynthesis. It may be possible to use this isotopic pair as a chronometer of the early solar system.

Lugmair, G. W.↗
NASA NTRS1977

Aluminum-26 in the early solar system - Fossil or fuel

The isotopic composition of Mg was measured in different phases of a Ca-Al-rich inclusion in the Allende meteorite. Large excesses of Mg-26 of up to 10% were found. These excesses correlate strictly with the Al-27/Mg-24 ratio for four coexisting phases with distinctive chemical compositions. Models of in situ decay of Al-26 within the solar system and of mixing of interstellar dust grains containing fossil Al-26 with normal solar system material are presented. The observed correlation provides definitive evidence for the presence of Al-26 in the early solar system. This requires either injection of freshly synthesized nucleosynthetic material into the solar system immediately before condensation and planet formation, or local production within the solar system by intense activity of the early sun. Planets promptly produced from material with the inferred Al-26/Al-27 would melt within about 300,000 years.

Lee, T.↗
NASA NTRS1985

Short-lived nuclei in the early solar system

An overview is given of the existence and abundance of short-lived nuclei that were present in the early solar system. It is shown that there are excesses of certain isotopes that may be assigned to the decay of short-lived radioactive nuclei corresponding to an abundance of about 0.0001 relative to a neighboring stable isotope. This abundance is roughly similar to the level of general nonlinear isotopic anomalies present in meteoritic material (excluding oxygen) which are not attributable to short-lived nuclei. If these results are representative of the bulk solar system, they indicate that about 0.0001 solar mass of freshly synthesized material of peculiar composition was added to the protosolar nebula as it was formed from the interstellar medium. This material must have been synthesized about three million yr before the formation of the solar system.

Wasserburg, G. J.↗
NASA NTRS1977

Pre-mare cratering and early solar system history

An evaluation of the application of the high extralunar flux in pre-mare times to more general problems of early solar system history is attempted by combining the results of dynamic studies with lunar chronological data. There is a twofold to fourfold contrast in the integral impact flux between the Apollo 14 and 16 sites and the older mare surfaces. This is judged insufficient to account for the contrasting lithology between these two sites: basalts and soil breccias in the maria, annealed breccias and impact melts in the highlands. Therefore, these rocks and their ages (3.9-4.0 b.y.) are thought to predate the surfaces in which they are found. Estimation of the flux needed to produce these lithologies, and difficulties associated with extrapolating this further back in lunar history give support to the "cataclysm" hypothesis of Tera, Papanastassiou, and Wasserburg. Dynamical studies permit separate evaluation of the possible sources for both the "normal" flux during the first 600 million years of lunar history and the "peak" that apparently occurred 4.0 billion years ago. The most likely sources for the normal flux are comets from the vicinity of Uranus and Neptune. The most promising source for the peak is tidal disruption by Earth or Venus of a Ceres-size asteroid initially in a Mars-crossing orbit. Alternative possibilities are suggested.

Wetherill, G. W.↗
NASA NTRS2011

Progress in the Early Solar System Chronology: A Sketch of an Ever-Changing Landscape

The years since the Workshop on the Chronology of Meteorites and the Early Solar System, are marked with ongoing progress in cosmochronology. Rapid improvements in techniques, discovery of new meteorites unlike any previously known, and findings that what was deemed well established constants are actually variables, will be reflected in an updated review of the solar system chronology we are currently preparing. Along with updating the database of meteorite ages, it will involve development of a set of criteria for evaluation of accuracy and consistency of isotopic dates across the entire range of meteorite classes and isotope chronometer systems. Here we present some ideas on what we think is important in meteorite chronology, and invite the cosmochemistry community to discuss them.

Amelin, Yuri↗
NASA NTRSDate not supplied

Direct Analysis of Early Solar System Aqueous Fluids by TOF-SIMS

We lack fundamental information related to the location and timing of the aqueous alteration in the early solar system, and the detailed nature of the aqueous fluid itself [1,2,3]. Two thermally-metamorphosed ordinary chondrite regolith breccias (Monahans 1998, hereafter simply “Monahans” (H5) and Zag (H3-6)) contain fluid inclusion-bearing halite (NaCl) crystals [4,5]. The halites were dated by K-Ar, Rb-Sr and I-Xe systematics to be ~4.5 billion years old [4,6,7] and thus the trapped aqueous fluids are at least as ancient. Through previously-published O, H, Cr isotopic work we have established that the fluid-bearing halite originated in the outer solar system[8].

M Zolensky↗
NASA NTRS1974

Pre-mare cratering and early solar system history

An evaluation of the application of the high extra-lunar flux in pre-mare times to more general problems of early solar system history is attempted by combining the results of dynamic studies with lunar chronological data. Dynamical studies permit separate evaluation of the possible sources for both the normal flux during the first 600 m.y. years of lunar history as well as the peak which apparently occurred 4.0 b.y. ago. Dynamical studies have been carried out in order to determine the extent to which a heliocentric flux could be confined to the Moon (and Earth). A Monte Carlo method has been used to calculate the relative impact rates of planet-crossing bodies with the moon and the terrestrial planets. It is concluded that the time-variation of the flux on these planets is closely related to that on the moon.

Wetherill, G. W.↗
NASA NTRS1980

Evidence for live Cm-247 in the early solar system

Variations of the U-238/U-235 ratio in the Allende meteorite, ranging from -35% to +19% are interpreted as evidence of live Cm-247 in the early solar system. The amounts of these and other r-products in the solar system indicate values of (9000 + or - 3000) million years for the age of the Galaxy and approximately 8 million years for the time between the end of nucleosynthesis and the formation of meteoritic grains. Three possible explanations are presented for the different values of the latter time period which are indicated by the decay of products of Cm-247, Al-27, Pu-244, and I-129.

Tatsumoto, M.↗
NASA NTRS1978

Meteorites - Relics from the early solar system

Data on meteorite mineralogy, texture, and composition are reviewed and analyzed in order to obtain constraints on the temperatures, pressures, time-spans, and chemical environments that existed in the early solar system. It emerges that the temperature in the nebula was above 1400 K. Accretion into small bodies appears to have begun just below this temperature, when the major condensates, metal and silicate, appeared. Pressures inferred are about 0.000001 to 0.001 atm, suggesting a massive nebula with low accretion efficiency.

Larimer, J. W.↗
NASA NTRS1993

On possible Mn-53 heterogeneity in the early solar system

The effects of influence of shock wave propagation on the energy spectrum of accelerated particles that lead to different production rates of radionuclides, in particular, Mn-53, on small scales in the early solar system are shown. Search for evidence for extinct Mn-53 has stimulated investigations of Cr isotope anomalies in meteorites. The linear correlation between the magnitude of the Cr-53* excesses and the Mn/Cr ratio that unambiguously proves the in situ decay of Mn-53 was detected, really, in different mineral phases of some carbonaceous and enstatite chondrites, primitive achondrites, pallasites and iron meteorites. However, the data on the Cr-53* excess rarely defines a single linear array on a Mn-53-Cr-52 evolution diagram even for meteorites of the same chemical group. A clear isochron with Mn-53/Mn-55 = 4.4 plus or minus 1.0 x 10(exp -5) (in range of approximately 2.4 to approximately 9 x 10(exp -5)) is observed for CAI of the Allende C3-chondrite while the data for the Murchison C2- and Orgueil C1-chondrites fall much lower corresponding rather to Mn-53/Mn-55 less than 2 x 10(exp -5). In the case of iron meteorites it ranges from less than 5 x 10(exp -8) to less than 5 x 10(exp -5).

Lavrukhina, A. K.↗
NASA NTRS2015

Early Solar System Alkali Fractionation Events Recorded by K-Ca Isotopes in the Yamato-74442 LL-Chondritic Breccia

Radiogenic ingrowth of Ca-40 due to decay of K-40 occurred early in the solar system history causing the Ca-40 abundance to vary within different early-former reservoirs. Marshall and DePaolo ] demonstrated that the K-40/Ca-40 decay system could be a useful radiogenic tracer for studies of terrestrial rocks. Shih et al. [3,4] determined 40K/40Ca ages of lunar granitic rock fragments and discussed the chemical characteristics of their source materials. Recently, Yokoyama et al. [5] showed the application of the K-40/Ca-40 chronometer for high K/Ca materials in ordinary chondrites (OCs). High-precision calcium isotopic data are needed to constrain mixing processes among early solar system materials and the time of planetesimal formation. To better constrain the solar system calcium isotopic compositions among astromaterials, we have determined the calcium isotopic compositions of OCs and an angrite. We further estimated a source K/Ca ratio for alkali-rich fragments in a chondritic breccia using the estimated solar system initial Ca-40/Ca-44.

Tatsunori, T.↗
NASA NTRS1991

An ion microprobe study of corundum in the Murchison meteorite - Implications for Al-26 and O-16 in the early solar system

Results are presented from measurements of O, Mg, and Ti isotopes and the abundances of Mg, Ca, Sc, Ti, V, Sr, Y, Zr, La, and Ce in 26 individual corundum grains from the Murchison CM2 chondrite. The results provide further evidence for live Al-26 in the early solar system and set strict upper limits on the amounts of fossil Mg-26. The analyses suggest that corundum in this chondrite formed from two components with live Al-26 and a mass fraction of 43 percent dead Al.

Virag, Alois↗
NASA NTRS1989

The presence of Sm-146 in the early solar system and implications for its nucleosynthesis

A correlation of Nd-142/Nd-144 with Sm-144/Nd-144 in two meteorites which have a large range in Sm-144/Nd-144 in their constituent mineral phases is presented as evidence for the presence of the p-process nucleus Sm-146 in the early solar system and its alpha-decay into Nd-142. The ratio Sm-146/Sm-144 is estimated to be about 0.015 at the time of solar system formation, 4.56 AE ago. It is suggested that the abundance of Sm-146 is compatible with p-proc ess production rate estimates, but not with the production rate for Sm-146 based on a photodisintegration model for the production of p-process nuclides.

Prinzhoffer, A.↗