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Early Career Award: Single Molecule Fluorescence Imaging for a Background-Free Neutrinoless Double Beta Decay Search

This project aimed to develop a suite of novel technologies targeted at detecting individual barium ions produced in neutrinoless double beta decays of 136 Xe, as part of the NEXT program of gaseous xenon detectors. We realized novel molecules which could sense Ba 2+ ions in dry conditions; new microscopy techniques operable in dry noble gases, including the required operating conditions of xenon at 10 bar pressure; and new radiofrequency ion transport methods (developed both theoretically and experimentally) that can transport ions in dense xenon gas. Together, these developments represent a major advance toward a background-free neutrinoless double beta decay experiment based on single molecule fluorescence imaging of Ba 2+ daughter ions.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Neutrinoless double beta decay rates in the presence of light sterile neutrinos

We investigate neutrinoless double-beta decay (0νββ) in minimal extensions of the Standard Model of particle physics where gauge-singlet right-handed neutrinos give rise to Dirac and Majorana neutrino mass terms. We argue that the standard treatment of these scenarios, based on mass-dependent nuclear matrix elements, is missing important contributions to the 0νββ amplitude. First, new effects arise from the exchange of neutrinos with very small (ultrasoft) momenta, for which we compute the associated nuclear matrix elements for the decays of 76 Ge and 136 Xe. These contributions can dominate the 0νββ rate in cases with light sterile neutrinos. The ultrasoft terms are also relevant in the more standard scenario of just three light Majorana neutrinos where they lead to a 10% reduction of the total 0νββ amplitude. Secondly, we highlight the importance of short-range terms associated with medium-heavy sterile neutrinos and provide explicit formulae that can be used in phenomenological analyses. As examples we discuss impact of these new effects in several explicit scenarios, including a realistic 3 + 2 model with two right-handed gauge-singlet neutrinos.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

A method to load tellurium in liquid scintillator for the study of neutrinoless double beta decay

Herein, a method has been developed to load tellurium into liquid scintillator so as to permit searches for neutrinoless double beta decay with high sensitivity. The approach involves the synthesis of an oil-soluble tellurium compound from telluric acid and an organic diol. The process utilises distillable chemicals that can be safely handled underground and affords low radioactive backgrounds, low optical absorption and high light yields at loading levels of at least several percent Te by weight.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Scalar-induced neutrinoless double beta decay in SU(5)

We discuss the role of heavy scalar fields in mediating neutrinoless double beta decay (0νββ) within the SU(5) Grand Unified Theory framework, extended suitably to include neutrino mass. In such a minimal realistic SU(5) setup for fermion masses, the scalar contributions to 0νββ are extremely suppressed as a consequence of the proton decay bound. We circumvent this problem by imposing a discrete Z 3 symmetry. However, the scalar contributions to 0νββ remain suppressed in this SU(5) x Z 3 model due to the neutrino mass constraint. We find that the 0νββ contribution can be enhanced by extending the scalar sector with an additional 15-dimensional scalar representation with suitable Z 3 charge. Such an extension not only yields realistic fermion mass spectra but also leads to experimentally testable predictions in upcoming ton-scale 0νββ searches, which can be used as a sensitive probe of the new scalars across a broad range, from LHC-accessible scales up to ∼ 10 10 GeV.

Baryon/Lepton Number Violation↗

The implication of the atomic effects in neutrinoless double beta decay

In the planned ton-scale neutrinoless double beta [Formula: see text] decay experiments, the used [Formula: see text] value is the mass-energy difference between the ground states of mother and daughter atoms, without correcting the atomic energy difference due to the alteration in the nuclear charge before and after the decay process. We show that the atomic energy change between the two ground states can potentially reduce the [Formula: see text] value by 5.502, 12.103, and 12.372 keV for the decays from [Formula: see text], [Formula: see text], and [Formula: see text], respectively. The available kinetic energy for two electrons can be 2033.51 keV for [Formula: see text] decay, 2515.41 keV for [Formula: see text] decay, and 2445.45 keV for [Formula: see text] decay after correcting for atomic effects. This implies that the planned experiments could potentially miss the decay signature if a narrow energy window is designated to reduce background events including [Formula: see text] decay events.

Astronomy & Astrophysics↗

Neutrinoless Double Beta Decay of 136 Xe and Related Nuclear Structure Studies (Final Scientific Report)

The search for neutrinoless double-beta decay (0nbb) explores new physics by directly probing the unknown mass scale and possible Majorana nature of the neutrino. The nEXO experiment, one of the two leading proposed ton-scale projects in the US, has a projected sensitivity to the 136 Xe 0nbb half-life of 10 28 years. The interpretation of possible signals in this next generation of experiments would be complicated by significant variations in theoretical calculations of the nuclear matrix elements (NMEs) of the decay, and nuclear structure measurements testing those theories can help address that uncertainty. We have 136 Xe(p,n) 136 Cs reaction at TUNL to deduce the level-scheme of states in 136 Cs through which the lowest-lying 1+ state decays. We find that over 99% of such decays will proceed through at least one isomeric state with a lifetime of order 100ns, which would enable large xenon detectors to employ a delayed-coincidence technique to search for charge-exchange processes including solar neutrino interactions. We have carried out measurements at TUNL of the 134 Xe( 3 He,n) 136 Ba and 136 Xe( 3 He,n) 138 Ba reactions to low-lying 0 + states in the residuals to probe the BCS assumption for QRPA NME calculations for the initial and final nuclei in 136 Xe 0nbb. While the analyses of these reactions is not yet complete and is ongoing, our initial results indicate tension with the BCS assumption. We have assembled a thermosyphon cooling R&D system for nEXO which has demonstrated up to 500 W of cooling in vacuum. We have developed a simple thermosyphon cooling simulation for nEXO and planned laboratory tests with the R&D system to benchmark it.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Lattice calculation of short-range contributions to neutrinoless double-beta decay 𝜋 − → 𝜋 + ⁢𝑒⁢𝑒 at physical pion mass

Neutrinoless double-beta (0⁢𝜈⁢𝛽⁢𝛽) decays provide an excellent probe for determining whether neutrinos are Dirac or Majorana fermions. The short-range matrix elements associated with the 𝜋 − → 𝜋 + ⁢𝑒⁢𝑒 process contribute at leading order in the 0⁢𝜈⁢𝛽⁢𝛽 decay channel 𝑛⁢𝑛 → 𝑝⁢𝑝⁢𝑒⁢𝑒 through pion exchange between nucleons. However, current lattice calculations show notable discrepancies in predicting these short-range contributions. To address this issue, we perform a lattice QCD calculation of the 𝜋 − → 𝜋 + ⁢𝑒⁢𝑒 matrix elements using domain wall fermion ensembles at the physical pion mass generated by the RBC/UKQCD Collaboration. To mitigate contamination from around-the-world effects, we develop a new method to reconstruct and subtract them directly from lattice data. We then perform nonperturbative renormalization in the regularization-independent symmetric momentum-subtraction scheme (RI/SMOM), using the (𝛾 𝜇 , 𝛾 𝜇 ) and ($\not{𝑞}$, $\not{𝑞}$) projectors. Compared with previous studies, this work reduces the uncertainties in the matrix elements and provides an independent cross-check that helps to reconcile the discrepancies among previous lattice calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Beyond-mean-field approaches for nuclear neutrinoless double beta decay in the standard mechanism

Nuclear weak decays provide important probes to fundamental symmetries in nature. A precise description of these processes in atomic nuclei requires comprehensive knowledge on both the strong and weak interactions in the nuclear medium and on the dynamics of quantum many-body systems. In particular, an observation of the hypothetical double beta decay without emission of neutrinos (0νββ) would unambiguously demonstrate the Majorana nature of neutrinos and the existence of the lepton-number-violation process. It would also provide unique information on the ordering and absolute scale of neutrino masses. The next-generation tonne-scale experiments with sensitivity up to 10 28 years after a few years of running will probably provide a definite answer to these fundamental questions based on our current knowledge on the nuclear matrix element (NME), the precise determination of which is a challenge to nuclear theory. Beyond-mean-field approaches have been frequently adapted for the study of nuclear structure and decay throughout the nuclear chart for several decades. In this review, we summarize the status of beyond-mean-field calculations of the NMEs of 0νββ decay assuming the standard mechanism of an exchange of light Majorana neutrinos. In conclusion, the challenges and prospects in the extension and application of beyond-mean-field approaches for 0νββ decay are discussed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutrinoless Double Beta Decay

This White Paper, prepared for the Fundamental Symmetries, Neutrons, and Neutrinos Town Meeting related to the 2023 Nuclear Physics Long Range Plan, makes the case for double beta decay as a critical component of the future nuclear physics program. The major experimental collaborations and many theorists have endorsed this white paper.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Xenon-Doped Liquid Argon TPCs as a Neutrinoless Double Beta Decay Platform

Next-generation large liquid argon time-projection chambers offer an unprecedented amount of active detector mass in a deep location. Modifications to the detector design could enable neutrinoless double beta decay searches, with the possibility of reaching the normal ordering region. These modifications include adding external neutron moderation, filling the detector with argon depleted in Ar42, doping with xenon, and a method to achieve percent-level energy resolution at the MeV scale. One way to achieve this desired level of energy resolution is to introduce a photosensitive dopant into the argon, converting the isotropic scintillation photons into a directional ionization signal. This would enhance the achievable energy resolution in large LArTPCs, and would lead to sizeable improvements to many facets of the broad physics program such a detector could offer.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Final Results of the M AJORANA D EMONSTRATOR ’s Search for Double-Beta Decay of 76 Ge to Excited States of 76 Se

76 Ge can 𝛽⁢𝛽 decay into three possible excited states of 76 Se , with the emission of two or, if the neutrino is Majorana, zero neutrinos. None of these six transitions have yet been observed. The M AJORANA D EMONSTRATOR was designed to study 𝛽⁢𝛽 decay of 76 Ge using a low background array of high purity germanium detectors. With 98.2 kg-y of isotopic exposure, the demonstrator sets the strongest half-life limits to date for all six transition modes. For 2⁢𝜈⁢𝛽⁢𝛽 to the 0$^+_1$ state of 76 Se , this search has begun to probe for the first time half-life values predicted using modern many-body nuclear theory techniques, setting a limit of 𝑇 1/2 > 1.5 × 10 24 y (90% CL).

Majorana neutrinos↗

Neutrinoless double beta decay sensitivity of the XLZD rare event observatory

The XLZD collaboration is developing a two-phase xenon time projection chamber with an active mass of 60–80 t capable of probing the remaining weakly interacting massive particle-nucleon interaction parameter space down to the so-called neutrino fog. In this work we show that, based on the performance of currently operating detectors using the same technology and a realistic reduction of radioactivity in detector materials, such an experiment will also be able to competitively search for neutrinoless double beta decay in 136 Xe using a natural-abundance xenon target. XLZD can reach a 3σ discovery potential half-life of 5.7 × 10 27 years (and a 90% CL exclusion of 1.3 × 10 28 years) with 10 years of data taking, corresponding to a Majorana mass range of 7.3–31.3 meV (4.8–20.5 meV). XLZD will thus exclude the inverted neutrino mass ordering parameter space and will start to probe the normal ordering region for most of the nuclear matrix elements commonly considered by the community.

2-phase xenon TPCs↗

Neutrinoless double beta decay via light neutralinos in R-parity violating supersymmetry

We perform a study of neutrinoless double beta (0νββ) decay mediated by the lightest neutralino of arbitrary mass in the minimal supersymmetric Standard Model (MSSM) under the presence of R-parity violating trilinear interactions. In this scenario, the exchange of the lightest neutralino can result in 0νββ decay of either long-range or short-range behaviour, depending on the neutralino mass. Using nuclear matrix elements calculated in the interacting boson model, we use an interpolation between the long- and short-range behaviours with an approximate formula. The non-observation of 0νββ decay is then used to place constraints on the supersymmetry parameter space, compatible with constraints from collider experiments. We compare these constraints to bounds from pion decays, CKM unitarity and big bang nucleosynthesis.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Majorana phases beyond neutrinoless double beta decay

The ν M SM is defined as the SM extended to include dimension-5 operators. In this model neutrino masses violate lepton number, and two parameters of the lepton mixing matrix, the Majorana phases, are yet to be constrained. One combination of these phases and the neutrino masses, often denoted by m ee , is probed by neutrinoless double beta decays (0νββ). We explore what information may be obtained beyond 0νββ, and how it depends on the lightest neutrino mass. We point out that with current central values of the mixing parameters, ΔL e = 2 and ΔL e = ΔL μ = 1 (or ΔL e = 2 and ΔL μ = 2) processes cannot simultaneously vanish, providing a no-lose theorem, in principle, for excluding the ν M SM, even in the case of normal mass ordering.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Search for two-neutrino double-beta decay of 136 Xe to the $0$$^{+}_{1}$ excited state of 136 Ba with the complete EXO-200 dataset*

A new search for two-neutrino double-beta (2νββ) decay of 136 Xe to the $0$$^{+}_{1}$ excited state of 136 Ba is performed with the full EXO-200 dataset. A deep learning-based convolutional neural network is used to discriminate signal from background events. Signal detection efficiency is increased relative to previous searches by EXO-200 by more than a factor of two. With the addition of the Phase II dataset taken with an upgraded detector, the median 90% confidence level half-life sensitivity of 2νββ decay to the $0$$^{+}_{1}$ state of 136 Ba is 2.9 x 10 24 yr using a total 136 Xe exposure of 234.1 kg yr. Furthermore, no statistically significant evidence for 2νββ decay to the $0$$^{+}_{1}$ state is observed, leading to a lower limit of $T$$^{2v}_{1/2}$(0 + → $0$$^{+}_{1}$) > 1.4 x 10 24 yr at 90% confidence level, improved by 70% relative to the current world's best constraint.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

New Direct Limit on Neutrinoless Double Beta Decay Half-Life of 128 $\mathrm{Te}$ with CUORE

The Cryogenic Underground Observatory for Rare Events (CUORE) at Laboratori Nazionali del Gran Sasso of INFN in Italy is an experiment searching for neutrinoless double beta (0νββ) decay. Its main goal is to investigate this decay in 130 Te, but its ton-scale mass and low background make CUORE sensitive to other rare processes as well. Here, in this Letter, we present our first results on the search for 0νββ decay of 128 Te, the Te isotope with the second highest natural isotopic abundance. We find no evidence for this decay, and using a Bayesian analysis we set a lower limit on the 128 Te 0νββ decay half-life of T 1/2 > 3.6 x 10 24 yr (90% CI). This represents the most stringent limit on the half-life of this isotope, improving by over a factor of 30 the previous direct search results, and exceeding those from geochemical experiments for the first time.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

TeV-scale lepton number violation: Connecting leptogenesis, neutrinoless double beta decay, and colliders

In the context of TeV-scale lepton number violating (LNV) interactions, we illustrate the interplay between leptogenesis, neutrinoless double beta ( 0 ν β β ) decay, and LNV searches at proton-proton colliders. Using a concrete model for illustration, we overcome the limitations of previous effective field theory analyses and are able to identify the parameter space where standard thermal leptogenesis is rendered unviable due to washout processes. Moreover, we show how 0 ν β β decay and p p collisions provide complementary probes. We find that the new particle spectrum can have a decisive impact on the relative sensitivity of these two probes. Published by the American Physical Society 2024

Astronomy & Astrophysics↗