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At least 37 records · Page 2

Tidal influences on vertical diffusion and diurnal variability of ozone in the mesosphere

Possible dynamical influences on the diurnal behavior of ozone are investigated. A time dependent one-dimensional photochemical model is developed for this purpose; all model calculations are made at 70 deg N during summer. It is shown that the vertical diffusion can vary as much as 1 order of magnitude within a day as a result of large changes in the zonal wind induced by atmospheric thermal tides. It is found that by introducing a dissipation time scale for turbulence produced by breaking gravity waves, the agreement with Poker Flat echo data is improved. Comparisons of results from photochemical model calculations, where the vertical diffusion is a function of height only, with those in which the vertical diffusion coefficient is changing in time show large differences in the diurnal behavior of ozone between 70 and 90 km. By including the dynamical effect, much better agreement with the Solar Mesosphere Explorers data is obtained. The results are, however, sensitive to the background zonally averaged wind. The influence of including time-varying vertical diffusion coefficient on the OH densities is also large, especially between 80 and 90 km. This suggests that dynamical effects are important in determining the diurnal behavior of the airglow emission from the Meinel bands.

Bjarnason, Gudmundur G.↗

Simultaneous spectroscopic determination of the latitudinal, seasonal, and diurnal variability of stratospheric N2O, NO, NO2, and HNO3

A program for the measurement of latitudinal, seasonal, and diurnal variations in stratospheric N2O, NO, NO2 and HNO3 is described, which uses airborne Fourier transform absorption spectroscopy to simultaneously determine columns, above 12 km, of the four molecules. The data may prove useful for comparison with two-dimensional models of stratospheric chemistry, since simultaneous measurement of several species with the same technique provides an inherently more reliable set for model comparisons, by eliminating uncorrelated atmospheric variability and reducing differences in instrumental biases.

Coffey, M. T.↗

Diurnal variability of the planetary albedo - An appraisal with satellite measurements and general circulation models

An atmospheric radiation model is used here to illustrate several features associated with modeling the diurnal cycle of the planetary albedo. It is found that even for clear regions there appear to be deficiencies in our knowledge of how to model this quantity. The diurnal amplitude factor, defined as the ratio of the diurnally averaged planetary albedo to that at noon, between two GCMs and measurements made from a geostationary satellite. While reasonable consistency is found, the comparisons underscore difficulties associated with converting local-time albedo measurements, as made from sun-synchronous satellites, to diurnally averaged albedos.

Potter, G. L.↗

A New Method to Retrieve the Diurnal Variability of Planetary Boundary Layer Height from Lidar Under Different Thermodynamic Stability Conditions

The planetary boundary layer height (PBLH) is an important parameter for understanding the accumulation of pollutants and the dynamics of the lower atmosphere. Lidar has been used for tracking the evolution of PBLH by using aerosol backscatter as a tracer, assuming aerosol is generally well-mixed in the PBL; however, the validity of this assumption actually varies with atmospheric stability. This is demonstrated here for stable boundary layers (SBL), neutral boundary layers (NBL), and convective boundary layers (CBL) using an 8-year dataset of micropulse lidar (MPL) and radiosonde (RS) measurements at the ARM Southern Great Plains, and MPL at the GSFC site. Due to weak thermal convection and complex aerosol stratification, traditional gradient and wavelet methods can have difficulty capturing the diurnal PBLH variations in the morning and forenoon, as well as under stable conditions generally. A new method is developed that combines lidar-measured aerosol backscatter with a stability dependent model of PBLH temporal variation (DTDS). The latter helps “recalibrate” the PBLH in the presence of a residual aerosol layer that does not change in harmony with PBL diurnal variation. The hybrid method offers significantly improved PBLH detection, with better correlation and smaller biases, under most thermodynamic conditions, especially for SBL and CBL. Relying on the physical process of PBL diurnal development, different schemes are developed for growing, maintenance, and decaying periods. Comprehensive evaluation of this new method shows much better tracking of diurnal PBLH variation and significantly smaller biases under various pollution levels.

Tianning Su↗

Diurnal variability of regional cloud radiative parameters from geostationary satellite data

In the discussed study, Geostationary Operational Environmental Satellite visible and infrared brightness measurements are used to infer regional cloud cover and several associated radiative parameters on an hourly basis. Several techniques are utilized to derive the parameters of interest. These parameters include the areal cloud fraction, cloud-atmosphere albedo, surface-atmosphere albedo, and equivalent blackbody surface and cloud-top temperatures. Attention is given to clear radiance temperature determinations, surface temperature modeling, the infrared threshold method, narrowband-broadband correlations, and albedo determination. Monthly mean values were computed for each parameter as a function of local time. Cloud amounts and temperatures are considered along with longwave emission and shortwave albedo, and composite results.

Minnis, P.↗

Nonmethane hydrocarbon chemistry in the remote marine boundary layer

A photochemical model of the remote marine boundary layer (MBL) is presented, with focus placed on the role of reactive nonmethane hydrocarbons (NMHC). A wide range of NMHC air-sea fluxes with various relative distributions of NMHC regions are considered. In particular, the flux magnitude at which NMHC emissions become significant, and then dominant, players in MBL chemistry is identified. Emphasis is placed on diurnal variability, diurnal ozone variations and sensitivity to NMHC emission fluxes, to CO, O3, H2O, and UV light, and to kinetics and isometric composition. Model runs indicate that, in the range consistent with current observations, the NMHCs may either dominate MBL chemistry, or simply be contributors at the 10-percent level. These model runs also show that existing observations of NMHCs in ocean water find them to scarce for fluxes from bulk-flux air-sea gas exchange models to be consistent with the fluxes needed in the proposed model to maintain the lowest observed MBL NMHC.

Donahue, Neil M.↗

The observed day-to-day variability of Mars water vapor

The diurnal variability of atmospheric water vapor as derived from the Viking MAWD data is discussed. The detection of day to day variability of atmospheric water would be a significant finding since it would place constraints on the nature of surface reservoirs. Unfortunately, the diurnal variability seen by the MAWD experiment is well correlated with the occurrence of dust and/or ice hazes, making it difficult to separate real variations from observational effects. Analysis of the day to day variability of water vapor in the Martian atmosphere suggests that the observations are, at certain locations and seasons, significantly affected by the presence of water-ice hazes. Because such effects are generally limited to specific locations, such as Tharsis, Lunae Planum, and the polar cap edge during the spring, the seasonal and latitudinal trends in water vapor that have been previously reported are not significantly affected.

Jakosky, Bruce M.↗

SAGE III/ISS Ozone and NO2 Validation Using Diurnal Scaling Factors

We developed a set of solar zenith angle, latitude- and altitude-dependent scaling factors to account for the diurnal variability in ozone (O3) and nitrogen dioxide (NO2) when comparing Stratospheric Aerosol and Gas Experiment (SAGE) III/ISS observations to observations from other times of day. The scaling factors are calculated as a function of solar zenith angle from the four-dimensional output of a global atmospheric chemistry model simulation of 2017–2020 that shows good agreement with observed vertical profiles. Using a global atmospheric chemistry model allows us to account for both chemically and dynamically driven variability. Both year-specific scale factors and a multi-year monthly climatology are available to decrease the uncertainty in inter-instrument comparisons and allow consistent comparisons between observations from different times of day. We describe the variability in the diurnal scale factors as a function of space and time. The quasi-biennial oscillation (QBO) appears to be a contributing factor to interannual variability in the NO2 scaling factors, leading to differences between years that switch sign with altitude. We show that application of these scaling factors improves the comparison between SAGE III/ISS and OSIRIS NO2 and between SAGE III/ISS and OMPS LP, OSIRIS, and ACE-FTS O3 observations. The comparisons between SAGE III/ISS O3 for sunrise or sunset vs. Microwave Limb Sounder (MLS) daytime or nighttime observations are also more consistent when we apply the diurnal scaling factors. There is good agreement between SAGE III/ISS V5.2 ozone and correlative measurements, with differences within 5 % between 20 and 50 km when corrected for diurnal variability. Similarly, the SAGE III/ISS V5.2 NO2 agreement with correlative measurement is mostly within 10 %. While the scale factors were designed for use with SAGE III/ISS observations, they can easily be applied to other observation intercomparisons as well.

Sarah A. Strode↗

How Can TOLNet Help to Better Understand Tropospheric Ozone? A Satellite Perspective

Potential sources of a priori ozone (O3) profiles for use in Tropospheric Emissions: Monitoring of Pollution (TEMPO) satellite tropospheric O3 retrievals are evaluated with observations from multiple Tropospheric Ozone Lidar Network (TOLNet) systems in North America. An O3 profile climatology (tropopause-based O3 climatology (TB-Clim), currently proposed for use in the TEMPO O3 retrieval algorithm) derived from ozonesonde observations and O3 profiles from three separate models (operational Goddard Earth Observing System (GEOS-5) Forward Processing (FP) product, reanalysis product from Modern-Era Retrospective analysis for Research and Applications version 2 (MERRA2), and the GEOS-Chem chemical transport model (CTM)) were: 1) evaluated with TOLNet measurements on various temporal scales (seasonally, daily, hourly) and 2) implemented as a priori information in theoretical TEMPO tropospheric O3 retrievals in order to determine how each a priori impacts the accuracy of retrieved tropospheric (0-10 km) and lowermost tropospheric (LMT, 0-2 km) O3 columns. We found that all sources of a priori O3 profiles evaluated in this study generally reproduced the vertical structure of summer-averaged observations. However, larger differences between the a priori profiles and lidar observations were observed when evaluating inter-daily and diurnal variability of tropospheric O3. The TB-Clim O3 profile climatology was unable to replicate observed inter-daily and diurnal variability of O3 while model products, in particular GEOS-Chem simulations, displayed more skill in reproducing these features. Due to the ability of models, primarily the CTM used in this study, on average to capture the inter-daily and diurnal variability of tropospheric and LMT O3 columns, using a priori profiles from CTM simulations resulted in TEMPO retrievals with the best statistical comparison with lidar observations. Furthermore, important from an air quality perspective, when high LMT O3 values were observed, using CTM a priori profiles resulted in TEMPO LMT O3 retrievals with the least bias. The application of time-specific (non-climatological) hourly/daily model predictions as the a priori profile in TEMPO O3 retrievals will be best suited when applying this data to study air quality or event-based processes as the standard retrieval algorithm will still need to use a climatology product. Follow-on studies to this work are currently being conducted to investigate the application of different CTM-predicted O3 climatology products in the standard TEMPO retrieval algorithm. Finally, similar methods to those used in this study can be easily applied by TEMPO data users to recalculate tropospheric O3 profiles provided from the standard retrieval using a different source of a priori.

Satellite↗

Computationally Efficient Modeling and Data Assimilation of Near-Surface Variability

Near-surface (< 20m) ocean exhibits high variability due to coupled interactions, for e.g., with the atmosphere, sea ice, land, etc. Here we focus on atmospheric heat and momentum (wind) forcing, which are known to cause diurnal variability within the mixed layer. Only recently with a combination of sufficiently high vertical/horizontal resolution (75L, 1/4deg) and sub-daily atmospheric forcing fields, ocean models are starting to resolve this diurnal variability. However, the computation expense of such a high vertical resolution is burdensome in the context of coupled modeling and data assimilation. An alternative approach is to parameterize this diurnal variability with a prognostic model, that is embedded into the ocean model.In the first part of this presentation, we will demonstrate results with the above two approaches, by comparing them to profiles of near-surface temperature and salinity. In the context of data assimilation and reanalysis, this modeling capability opens the door to re-examine and perhaps improve specification of background (or, ensemble) error characteristics. The second half of this talk will focus on illustrating diurnally varying errors within an ensemble DA, and possible approaches to improve localization (horizontal/vertical) to extract maximum possible observational information content from in-situ and satellite observations of sea surface temperature.

Akella, Santha↗

A 10-Year Climatology of Amazonian Rainfall Derived from Passive Microwave Satellite Observations

In this study we present and describe a satellite-derived precipitation climatology over northern South America using a passive microwave technique, the Goddard Profiling Algorithm. A period of data slightly longer than 10 years is examined. The climatologies take the form of the mean estimated (adjusted) rainfall for a 10-year (+) period, with sub-divisions by month and meteorological season. For the six-year period 1992-1997, when two satellites were in operation, diurnal variability (to the extent it is discerned by four unequally spaced observations) is presented. We find an alternating pattern of morning and maxima stretching from the northeast (Atlantic coast) clear across the continent to the Pacific. The effects of topography, coastlines and geography (river valleys) on the rainfall patterns are clear. Interannual variability is examined by computing the deviations of yearly and warm season (DJF) rainfall from their respective long-term means. Interannual variability of the diurnal nature of the rainfall is presented, and the strong El Nino event of 1997-1998 is discussed.

Negri, Andrew J.↗

Convective Transport and Evolution of Clouds and aerosols in the Asian Summer Monsoon Region

The existence of a persistent layer in the lowermost stratosphere in the Asian Monsoon region is well-known and has been observed by satellites and also in situ by balloon-borne sensors. This aerosol layer has been observed to persist every year by both SAGE sensors and by CALIOP, between the tropopause and the lower boundary of the Junge stratospheric sulfate layer. But how does this layer form and why? Apparently, aerosols are lofted by convection form the Indian and Asian continents, into the upper troposphere/lower stratosphere (UT/LS) area in the middle of a persistent anticyclone associate with the Asian summer monsoon. But some mysteries remain. The top of this aerosol layer is well above the altitude of maximum convective outflow, so why is the top of the aerosol layer so high? Are the aerosols coming from China or from India? And finally, is there an observable impact of these aerosol on thin cirrus distributions in the UT/LS? We explore the interesting difference in altitude between the ATAL layer and the convective cloud top height, using observations from CALIOP and from SAGE. In the process of doing this we examine the accuracy of both CALIOP and SAGE cloud/aerosol discrimination, and the impact of various averaging lengths. We compare the apparent "observational tropopause" with observations from COSMIC, CALIOP (clouds), and with modeled interpolation from MERRA-2. We also compare CALIOP and CloudSat daytime cloud top heights for convective clouds with the vertical aerosol distribution, and evaluate convection in this region as represented by MERRA-2. Finally, and maybe most importantly we compare convective cloud top heights and temperatures with diurnal variability during the most recent years by using observations from the geostationary Himawari satellite. How representative are the twice-daily A-Train observations, when compared to the natural diurnal variability of convection? The goal is to establish the origins of these UT/LS aerosols, whether these aerosol distributions can be completely explained by convective transport, and to evaluate convective lofting of aerosol by models. Ultimately, the convective lofting of aerosols as modeled is needed to explain the Asian Monsoon aerosol distributions. The observations contribute much-needed information to enhance the model accuracy.

clouds↗

The Diurnal Cycle of Cloud Profiles over Land and Ocean Between 51degS and 51degN, Seen by the CATS Spaceborne Lidar from the International Space Station

We document, for the first time, how detailed vertical profiles of cloud fraction (CF) change diurnally between 51 deg S and 51 deg N, by taking advantage of 15 months of measurements from the Cloud-Aerosol Transport System (CATS) lidar on the non-sun-synchronous International Space Station (ISS). Over the tropical ocean in summer, we find few high clouds during daytime. At night they become frequent over a large altitude range (11-16 km between 22:00 and 04:00 LT). Over the summer tropical continents, but not over ocean, CATS observations reveal mid-level clouds (4-8 km above sea level or a.s.l.) persisting all day long, with a weak diurnal cycle (minimum at noon). Over the Southern Ocean, diurnal cycles appear for the omnipresent low-level clouds (minimum between noon and 15:00) and high-altitude clouds (minimum between 08:00 and 14:00). Both cycles are time shifted, with high-altitude clouds following the changes in low-altitude clouds by several hours. Over all continents at all latitudes during summer, the low-level clouds develop upwards and reach a maximum occurrence at about 2.5 km a.s.l. in the early afternoon (around 14:00). Our work also shows that (1) the diurnal cycles of vertical profiles derived from CATS are consistent with those from ground-based active sensors on a local scale, (2) the cloud profiles derived from CATS measurements at local times of 01:30 and 13:30 are consistent with those observed from CALIPSO at similar times, and (3) the diurnal cycles of low and high cloud amounts (CAs) derived from CATS are in general in phase with those derived from geostationary imagery but less pronounced. Finally, the diurnal variability of cloud profiles revealed by CATS strongly suggests that CALIPSO measurements at 01:30 and 13:30 document the daily extremes of the cloud fraction profiles over ocean and are more representative of daily averages over land, except at altitudes above 10 km where they capture part of the diurnal variability. These findings are applicable to other instruments with local overpass times similar to CALIPSO's, such as all the other A-Train instruments and the future Earth-CARE mission.

Noel, Vincent↗

The effects of UV radiation A and B on diurnal variation in photosynthesis in three taxonomically and ecologically diverse microbial mats

Photosynthetic primary production, the basis of most global food chains, is inhibited by UV radiation. Evaluating UV inhibition is therefore important for assessing the role of natural levels of UV radiation in regulating ecosystem behavior as well as the potential impact of stratospheric ozone depletion on global ecosystems. As both photosynthesis and UV fluxes are subject to diurnal variations, we examined the diurnal variability of the effect of UV radiation on photosynthesis in three diverse algal mats. In one of the mats (Cyanidium caldarium) a small mean decrease in primary productivity over the whole day occurred when both UVA and UVB were screened out. In two of the mats (Lyngbya aestuarii and Zygogonium sp.) we found a mean increase in the total primary productivity over the day when UVB alone was screened and a further increase when UVA and UVB were both screened out. Variations in the effects of UV radiation were found at different times of the day. This diurnal variability may be because even under the same solar radiation flux, there are different factors that may control photosynthetic rate, including nutritional status and other physiological processes in the cell. The results show the importance of assessing the complete diurnal productivity. For some of the time points the increase in the mean was still within the standard deviations in primary productivity, illustrating the difficulty in dissecting UV effects from other natural variations.

Ultraviolet Rays↗

A New Technique for Retrieval of Tropospheric and Stratospheric Ozone Profiles using Sky Radiance Measurements at Multiple View Angles: Application to a Brewer Spectrometer

This paper describes and applies a new technique for retrieving diurnal variability in tropospheric ozone vertical distribution using ground-based measurements of ultraviolet sky radiances. The measured radiances are obtained by a polarization-insensitive modified Brewer double spectrometer located at Goddard Space Flight Center, in Greenbelt, Maryland, USA. Results demonstrate that the Brewer angular (0-72deg viewing zenith angle) and spectral (303-320 nm) measurements of sky radiance in the solar principal plane provide sufficient information to derive tropospheric ozone diurnal variability. In addition, the Brewer measurements provide stratospheric ozone vertical distributions at least twice per day near sunrise and sunset. Frequent measurements of total column ozone amounts from direct-sun observations are used as constraints in the retrieval. The vertical ozone profile resolution is shown in terms of averaging kernels to yield at least four points in the troposphere-low stratosphere, including good information in Umkehr layer 0 (0-5 km). The focus of this paper is on the derivation of stratospheric and tropospheric ozone profiles using both simulated and measured radiances. We briefly discuss the necessary modifications of the Brewer spectrometer that were used to eliminate instrumental polarization sensitivity so that accurate sky radiances can be obtained in the presence of strong Rayleigh scattering and aerosols. The results demonstrate that including a site-specific and time-dependent aerosol correction, based on Brewer direct-sun observations of aerosol optical thickness, is critical to minimize the sky radiance residuals as a function of observing angle in the optimal estimation inversion algorithm and improve the accuracy of the retrieved ozone profile.

Tzortziou, Maria↗

Toward Realistic Simulation of low-Level Clouds Using a Multiscale Modeling Framework With a Third-Order Turbulence Closure in its Cloud-Resolving Model Component

This study presents preliminary results from a multiscale modeling framework (MMF) with an advanced third-order turbulence closure in its cloud-resolving model (CRM) component. In the original MMF, the Community Atmosphere Model (CAM3.5) is used as the host general circulation model (GCM), and the System for Atmospheric Modeling with a first-order turbulence closure is used as the CRM for representing cloud processes in each grid box of the GCM. The results of annual and seasonal means and diurnal variability are compared between the modified and original MMFs and the CAM3.5. The global distributions of low-level cloud amounts and precipitation and the amounts of low-level clouds in the subtropics and middle-level clouds in mid-latitude storm track regions in the modified MMF show substantial improvement relative to the original MMF when both are compared to observations. Some improvements can also be seen in the diurnal variability of precipitation.

Xu, Kuan-Man↗