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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Extracting halo independent information from dark matter electron scattering data

Direct detection experiments and the interpretation of their results are sensitive to the velocity structure of the dark matter in our galactic halo. Here we extend the formalism that deals with such astrophysics-driven uncertainties, originally introduced in the context of dark-matter-nuclear scattering, to include dark-matter-electron scattering interactions. Using mock data, we demonstrate that the ability to determine the correct dark matter mass and velocity distribution is depleted for recoil spectra which only populate a few low-lying bins, such as models involving a light mediator. We also demonstrate how this formalism allows one to test the compatibility of existing experimental data sets (e.g. SENSEI and EDELWEISS), as well as make predictions for possible future experiments (e.g. GaAs-based detectors).

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2026

New thermal-relic targets for sub-GeV dark matter direct detection

Dark matter direct detection experiments involving electron recoils are beginning to test highly predictive, thermal-relic milestones for sub-GeV dark matter models. Due to the Lee-Weinberg bound, thermal dark matter candidates in this mass range necessarily require comparably light mediator particles to achieve a suitably large annihilation cross section. Here we present new thermal-relic milestones for sub-GeV dark matter candidates that couple to vector mediators. In these models, the mediators are massive gauge bosons of anomaly-free Abelian extensions to the Standard Model, including the dark photon, gauged L i - L j , B - L , and B - 3 L i models, where B is the baryon number, L is the lepton number, and i , j index the lepton families. Since the same interactions that govern cosmological production also govern electron scattering, the targets we present are firmly predictive and allow for these models to be robustly discovered or falsified. Furthermore, since the mediators we study exhaust the minimal anomaly-free U(1) extensions to the Standard Model, our results offer a complete list of predictive milestones for sub-GeV dark matter coupled to vector mediators.

Han, Xu [Chicago U.] (ORCID:0009000821607836)↗
DOE OSTI2025

Strategy for Direct Detection of Chiral Phonons with Phase-Structured Free Electrons

Chiral phonons possessing valley pseudoangular momentum (PAM) underlie a diversity of quantum phenomena of fundamental and applied importance, but are challenging to probe directly. We show that deficiencies of typical momentum-resolved electron energy loss measurements that make it impossible to distinguish the PAM of chiral phonons can be overcome by introducing pinwheel free electron states with well-defined PAM. Transitions between such states generate 2D periodic arrays of in-plane field vortices with polarization textures tailored to selectively couple to desired chiral mode symmetries.

chirality↗
DOE OSTI2024

Direct detection of light dark matter charged under a 𝐿 𝜇 − 𝐿 𝜏 symmetry

A possible extension of the Standard Model able to explain the recent measurement of the anomalous magnetic moment of the muon consists in adding a gauged 𝑈⁢(1) 𝐿𝜇−𝐿𝜏 symmetry. If the dark matter particle is charged under this symmetry, then the kinetic mixing between the new gauge boson and the photon induces dark matter-electron interactions. We derive direct detection constraints on light dark matter charged under a 𝑈⁢(1) 𝐿𝜇−𝐿𝜏 symmetry with electron recoil experiments and explore prospects with XLZD and OSCURA to close in the parameter space able to explain simultaneously the recent measurement on the anomalous magnetic moment of the muon and the observed relic density of dark matter. We further discuss the spin-dependent scattering contribution arising in this model, which was ignored previously in the literature.

extensions of gauge sector↗
DOE OSTI2023

Even lighter particle dark matter

We report on recent progress in the search for dark matter particles with masses from 1 Mev c ^{-2} − 2 to 1 Gev c ^{-2} − 2 . Several dark matter candidates in this mass range are expected to generate measurable electronic-recoil signals in direct-detection experiments. We focus on dark matter particles scattering with electrons in semiconductor detectors since they have fundamentally the highest sensitivity due to their low ionization threshold. Charge-coupled device (CCD) silicon detectors are the leading technology, with significant progress expected in the coming years. We present the status of the CCD program and briefly report on other efforts.

Chavarria, Alvaro E.↗
DOE OSTI2020

Low-diffusion Xe-He gas mixtures for rare-event detection: electroluminescence yield

High pressure xenon Time Projection Chambers (TPC) based on secondary scintillation (electroluminescence) signal amplification are being proposed for rare event detection such as directional dark matter, double electron capture and double beta decay detection. The discrimination of the rare event through the topological signature of primary ionisation trails is a major asset for this type of TPC when compared to single liquid or double-phase TPCs, limited mainly by the high electron diffusion in pure xenon. Helium admixtures with xenon can be an attractive solution to reduce the electron diffusion significantly, improving the discrimination efficiency of these optical TPCs. We have measured the electroluminescence (EL) yield of Xe-He mixtures, in the range of 0 to 30% He and demonstrated the small impact on the EL yield of the addition of helium to pure xenon. For a typical reduced electric field of 2.5 kV/cm/bar in the scintillation region, the EL yield is lowered by ~ 2%, 3%, 6% and 10% for 10%, 15%, 20% and 30% of helium concentration, respectively. This decrease is less than what has been obtained from the most recent simulation framework in the literature. The impact of the addition of helium on EL statistical fluctuations is negligible, within the experimental uncertainties. The present results are an important benchmark for the simulation tools to be applied to future optical TPCs based on Xe-He mixtures.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

Sub-Ångström-resolution MicroED Using a Direct Detection Camera

The recent development of microcrystal electron diffraction (MicroED) in electron cryo-microscopy (cryo-EM) has addressed many of the challenges of X-ray crystallography [1], filling a long-standing need in organic chemistry for rapid and accurate high-resolution structural characterization [2]. Like X-ray crystallography, this is also a diffraction technique requiring crystalline specimens, but because high energy electrons have a more favorable ration of elastic to inelastic scattering [3], MicroED can acquire data using crystals that are orders of magnitude smaller than those needed for X-ray crystallography—even as small as 50 nm in length [4]. Additionally, the instrumentation required for MicroED is readily available, as many chemistry and biology labs already have access to cryo-capable transmission electron microscopes (TEM).

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Hydrogen Analysis by Gas Chromatography–Mass Spectrometry

The detection of hydrogen in complex gas mixtures is essential for many applications. Conventional approaches such as gas chromatography (GC) with thermal conductivity detection (TCD) and residual gas analyzers (RGAs) face significant limitations: TCD exhibits poor response when helium is used as a carrier gas, whereas RGAs lack chromatographic separation, preventing reliable quantification of hydrogen because of interference from other species. Traditional GC methods rely on dual-column configurations with packed or molecular-sieve porous layer open tubular (PLOT) columns to separate hydrogen from O2, N2, CO, CO2, CH4, and other hydrocarbons, increasing system complexity and limiting compatibility with mass spectrometry (MS) detection. In this work, we developed and validated a robust GC–MS method capable of directly detecting and quantifying hydrogen using electron ionization (EI) without dopants, reagent gases, or ion–molecule reaction schemes. By integrating a modified EI source and a cryogenically cooled single capillary column configuration, we achieved baseline separation of hydrogen from all major permanent gases and hydrocarbons in a refinery gas mixture using helium as the carrier gas. The method demonstrated excellent linearity, high sensitivity, and exceptional reproducibility. Adjustable sample-loop volumes and split ratios enabled optimization of peak shape and signal-to-noise performance for trace-level and percent-level hydrogen concentrations. Beyond hydrogen quantitation, the method provides simultaneous compositional profiling of other gases in a mixture in a single run, making it valuable for a wide range of tasks.

Lobodin, Vlad [ORNL]↗
DOE OSTI2023

Examination of Exogenous and Endogenous Irradiation Effects on PuO2 and its Precursors via EPR Spectroscopy

The spectroscopic examination of actinide compounds are of con-siderable interest for elucidating the role of 5f electrons in chemical bonding. For example, this could be directly detected via EPR spectroscopy through the hyperfine interaction of an unpaired Pu electron with a given ligand. However, typically fast spin-lattice re-laxation times [1] require the use of low temperatures, multiplying the difficulty of working with radio-toxic Pu compounds. Instead, we looked for radicals at room temperature produced from endoge-nous α-decay or exogenous γ-irradiation. PuO2 and its precursor PuIII2(C2O4)3∙nH2O were used as examples because of their ubiquity in the literature.

Kinyon, Jared S.↗
DOE OSTI2020

From Atom to Engine: Understanding Fundamental Effects of Structure on Combustion Using Tandem Experiment and Computation

The ability to tie structural features to a fuel candidate’s ignition properties provides a path for rational design of advantaged fuels that facilitate higher-efficiency, lower-emitting combustion in engines. The time evolution of a fuel’s radical population directly correlates with global combustion parameters, and because the generated radicals depend on the initial structure and reaction pathways of the fuel molecule, it follows that the molecular structure of a fuel has a direct impact on this cascade, and therefore salient ignition-tied fuel properties. This work aims to understand the impact of structural features in the context of global combustion properties for direct application to emerging engine technologies. Specifically, we highlight the ability to identify potential fuel blendstocks for specific engine strategies by examining and elucidating the radical cascade tied to ignition. A representative subset of alcohols possessing a variety of structural features (e.g. branching, chain length) was selected for study using a robust combination of experimental and computational methods. The approach begins with identifying short-lived radicals and likely abstraction sites upon pyrolysis in a microreactor coupled with photoionization mass spectrometry for direct detection of product species. In tandem, electronic structure calculations were performed to calculate the relevant potential energy surfaces for fuel pyrolysis as well as the subsequent O2 addition-isomerization reactions, which govern ignition behavior. Furthermore, the theoretical energetic and ro-vibrational data are used to calculate rate constants for direct ignition modeling to explore how structural effects impact NTC behavior. The microreactor data combined with electronic structure theory calculations provide a well-informed picture of the reactions relevant to ignition for each fuel in this study, as well as the most likely radicals generated under engine conditions. This thorough fundamental picture of fuel decomposition and ignition chemistry is used to correlate the observed ignition behavior to molecular structural effects.

advanced biofuels↗
DOE OSTI2026

Anomalous Spin‐Optical Helical Effect in Ti‐Based Kagome Metal

The kagome lattice stands as a rich platform for hosting a wide array of correlated quantum phenomena, ranging from charge density waves and superconductivity to electron nematicity and loop current states. Direct detection of loop currents in kagome systems has remained a formidable challenge due to their intricate spatial arrangements and the weak magnetic field signatures they produce, and this has made their identification experimentally subtle. This has left their existence and underlying mechanisms a topic of intense debate. In this work, we uncover signatures compatible with loop currents: spin handedness-selective signals that surpass conventional dichroic, spin, and spin-dichroic responses. We observe this phenomenon in the kagome metal CsTi 3 ⁢Bi 5 and we call it the anomalous spin-optical helical effect. This effect arises from the coupling of light's helicity with spin-orbital electron correlations, thereby providing an indirect yet sensitive approach to probe loop-current–related electronic correlations in quantum materials. Our discovery not only enriches the debate surrounding loop currents but also offers new experimental strategies to exploit the electronic phases of quantum materials via light–matter interaction.

anomalous spin-optical helical effect↗
DOE OSTI2026

Testing thermal-relic dark matter with a dark-photon mediator

In light of recent DAMIC-M results, we present the status of thermal-relic dark matter χ coupled to a kinetically mixed dark photon A ′ . In the predictive “direct annihilation” regime, m A ′ > m χ , the relic abundance depends on the kinetic mixing parameter, and there is a minimum value compatible with thermal freeze-out. Using only electron- and nuclear-recoil direct-detection results, we find that, for complex scalar dark matter, the direct annihilation regime is now excluded for nearly all values of m χ ; the only exception is the resonant annihilation regime where m A ′ ≈ 2 m χ . Direct annihilation relic targets for other representative models, including Majorana and pseudo-Dirac candidates, remain viable across a wide range of model parameters but will be tested with a combination of dedicated accelerator searches in the near future. In the opposite “secluded annihilation” regime, where m χ > m A ′ , this scenario is excluded by cosmic microwave background measurements for all m χ ≲ 30 GeV . Similar conclusions in both the direct and secluded regimes hold for all anomaly-free vector mediators that couple to the first generation of electrically charged Standard Model particles.

Krnjaic, Gordan [Fermilab; Chicago U., KICP] (ORCI↗
DOE OSTI2022

Characterization of an aerosolized nanoparticle beam beyond the diffraction limit through strong field ionization

Abstract The study of nanomaterials is an active area of research for technological applications as well as fundamental science. A common method for studying properties of isolated nanoparticles is by an in-vacuum particle beam produced via an aerodynamic lens. Despite being common practice, characterization of such beams has proven difficult as light scattering detection techniques fail for particles with sizes beyond the diffraction limit. Here we present a new technique for characterizing such nanoparticle beams using strong field ionization. By focusing an ultrafast, mJ-level laser into the particle beam, a nanoparticle within the laser focus is ionized and easily detected by its ejected electrons. This method grants direct access to the nanoparticle density at the location of the focus, and by scanning the focus through the transverse and longitudinal profiles of the particle beam we attain the 3-dimensional particle density distribution for a cylindrically symmetric beam. Further, we show that strong field ionization is effective in detecting spherical nanoparticles as small as 10 nm in diameter. Additionally, this technique is an effective tool in optimizing the particle beam for specific applications. As an example we show that the particle beam density and width can be manipulated by restricting the gas flow into the aerodynamic lens.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2023

Fully depleted charge‐coupled device design and technology development

Abstract We describe the advancement of fully depleted charge‐coupled device (CCD) technology for scientific applications. Recent efforts on 650–725 m‐thick CCDs for direct dark‐matter and radiation detection with single‐electron sensitivity are described, as well as the technology transfer of the fully depleted CCD technology to 200 mm‐wafer fabrication facilities.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

Surface Analysis and Hydrogen Permation Measurements for Super-Permeating Membrane Materials

In this report, we summarize preliminary surface characterization results for Nb surfaces, using low energy ion scattering, direct recoil spectrometry, and Auger electron spectroscopy. While most surface analysis tools cannot detect hydrogen, the low energy ion beam techniques described here are among the few techniques that are directly sensitive to it. For this study, we examined chemisorption using both molecular and atomic hydrogen (using an heated tungsten capillary to dissociate the hydrogen.) To complement these results, we have been performing ex-situ spectroscopic ellipsometry as a means of detecting the surface oxide.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Studies of BONuS12 Radial GEM Detector and TCS Beam Spin Asymmetry in CLAS12

The Barely Offshell Nucleon Structure (BONuS12) experiment adopted the concept of spectator tagging technique to study the nearly-free neutron structure function Fn2 in the CLAS12 of Jefferson Lab. A novel Radial Time Projection Chamber (RTPC) detector was built, tested and integrated into the CLAS12 system to detect a back-moving low momentum tagged proton in d(e,ep)X deep-inelastic scattering. It was a 40 cm long gaseous detector consisting of 3 layers of cylindrical GEM foils for the charge amplification, with the data readout directly from the surrounding padboard. The RTPC detected the recoiling spectator proton, in coincidence with the scattered electron in the CLAS12. Nucleon structure functions are directly related to the partonic functions, quarks momentum distribution in one dimension. A Generalized Parton Distribution (GPD) came to the lime-light as it encodes the information of both longitudinal momentum and transverse position of partons inside the nucleons. Factorization of hard process such as DVCS allows to access GPDs. Timelike Compton Scattering (TCS), ?p ? ??p, is another process that allows to access the GPDs. TCS is studied experimentally in the CLAS12 of Jefferson lab using the quasi-real photoproduction of time-like photon which eventually decays to lepton pair. This dissertation presents the concept of spectator tagging in BONuS12, and the research and development efforts during the BONuS12 preparation leading up to the successful data-taking during spring and summer 2020. In addition, analysis framework to extract the beam spin asymmetry of TCS events through the CLAS12 Run group A data is presented.

Poudel, Jiwan↗
DOE OSTI2024

Search for New Physics with the Compact Muon Solenoid Experiment and QIS-enabled Technology

Understanding the fundamental nature of dark matter (DM)---its cosmological origin, constituents, and interactions---is one of the most important questions in fundamental science today. In this thesis, I present two novel and highly complementary approaches to cover the gaps in sensitivity of current DM searches. The searches are enabled by a first-of-its-kind reconstruction technique to search for hidden-sector particles using the Compact Muon Solenoid (CMS) and by new advances in quantum sensing technology to search for axions and hidden-sector DM. In the first part of this thesis, I present a search for long-lived hidden sector particles, predicted by many extensions of the SM, using a novel technique to reconstruct decays of long-lived particles (LLPs) in the CMS muon detector. The innovative LLP reconstruction technique is sensitive to a broad range of LLP decays and to LLP masses below GeV. The search yields competitive sensitivity for proper lifetime 0.1--1000 m with the full Run 2 dataset recorded at the LHC between 2016--2018 at $\sqrt{s} = 13~$TeV. To extend the physics reach of this novel muon detector shower (MDS) signature, I present the model-independence of MDS and the reinterpretation of the search to a large number of LLP models, demonstrating its complementarity with proposed and existing dedicated LLP experiments. Finally, I present a new dedicated MDS trigger that improves the trigger efficiency by at least an order of magnitude and was deployed in 2022, at the start of Run 3 of the LHC operations. In the second part of the thesis, I present for the first time, the use of a novel quantum sensor, the low-noise and single-photon sensitive superconducting nanowire single photon detectors (SNSPDs), to directly detect dark matter. The low detection threshold and ultra-low dark count rate of SNSPDs can close the gap in DM discovery reach due to the current limitations in detector sensitivity. I will present my work on the development and characterization of SNSPDs for two entirely new experiments to directly detect axions via absorption and hidden-sector DM via electron scattering. The search for axions employs a novel broadband reflector technique with the Broadband Reflector Experiment for Axion Detection (BREAD). A unique parabolic mirror is then used to focus axion-converted photons to the SNSPDs, extending the reach to axion masses of 0.04--1 eV. On the other hand, by coupling the SNSPDs with gallium arsenide, a bright cryogenic scintillator well matched to SNSPD detection, a prototype sensing system can be built as a basis of new direct DM detection experiments capable of extending the discovery to DM masses as low as 1 MeV.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Diffractive Imaging of Conical Intersections Amplified by Resonant Infrared Fields

The fate of virtually all photochemical reactions is determined by conical intersections. These are energetically degenerate regions of molecular potential energy surfaces that strongly couple electronic states, thereby enabling fast relaxation channels. Their direct spectroscopic detection relies on weak features that are often buried beneath stronger, less interesting contributions. For azobenzene photoisomerization, a textbook photochemical reaction, we demonstrate how a resonant infrared field can be employed during the conical intersection passage to significantly enhance its coherence signatures in time-resolved Xray diffraction while leaving the product yield intact. Furthermore, this transition-state amplification holds promise to bring signals of conical intersections above the detection threshold.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗