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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Combining Eddy Covariance Towers, Field Measurements, and the MEMS 2 Ecosystem Model Improves Confidence in the Climate Impacts of Bioenergy With Carbon Capture and Storage

ABSTRACT Carbon dioxide removal technologies such as bioenergy with carbon capture and storage (BECCS) are required if the effects of climate change are to be reversed over the next century. However, BECCS demands extensive land use change that may create positive or negative radiative forcing impacts upstream of the BECCS facility through changes to in situ greenhouse gas fluxes and land surface albedo. When quantifying these upstream climate impacts, even at a single site, different methods can give different estimates. Here we show how three common methods for estimating the net ecosystem carbon balance of bioenergy crops established on former grassland or former cropland can differ in their central estimates and uncertainty. We place these net ecosystem carbon balance forcings in the context of associated radiative forcings from changes to soil N 2 O and CH 4 fluxes, land surface albedo, embedded fossil fuel use, and geologically stored carbon. Results from long term eddy covariance measurements, a soil and plant carbon inventory, and the MEMS 2 process‐based ecosystem model all agree that establishing perennials such as switchgrass or mixed prairie on former cropland resulted in net negative radiative forcing (i.e., global cooling) of −26.5 to −39.6 fW m −2 over 100 years. Establishing these perennials on former grassland sites had similar climate mitigation impacts of −19.3 to −42.5 fW m −2 . However, the largest climate mitigation came from establishing corn for BECCS on former cropland or grassland, with radiative forcings from −38.4 to −50.5 fW m −2 , due to its higher plant productivity and therefore more geologically stored carbon. Our results highlight the strengths and limitations of each method for quantifying the field scale climate impacts of BECCS and show that utilizing multiple methods can increase confidence in the final radiative forcing estimates.

Falvo, Grant [Department of Plant, Soil and Microb↗
DOE OSTI2023

A Large Ensemble Global Dataset for Climate Impact Assessments

We present a self-consistent, large ensemble, high-resolution global dataset of long-term future climate, which accounts for the uncertainty in climate system response to anthropogenic emissions of greenhouse gases and in geographical patterns of climate change. The dataset is developed by applying an integrated spatial disaggregation (SD) - bias-correction (BC) method to climate projections from the MIT Integrated Global System Model (IGSM). Four emission scenarios are considered that represent energy and environmental policies and commitments of potential future pathways, namely, Reference, Paris Forever, Paris 2 °C and Paris 1.5 °C. The dataset contains nine key meteorological variables on a monthly scale from 2021 to 2100 at a spatial resolution of 0.5°x 0.5°, including precipitation, air temperature (mean, minimum and maximum), near-surface wind speed, shortwave and longwave radiation, specific humidity, and relative humidity. We demonstrate the dataset’s ability to represent climate-change responses across various regions of the globe. This dataset can be used to support regional-scale climate-related impact assessments of risk across different applications that include hydropower, water resources, ecosystem, agriculture, and sustainable development.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Modeling dust mineralogical composition: sensitivity to soil mineralogy atlases and their expected climate impacts

Soil dust aerosols are a key component of the climate system, as they interact with short- and long-wave radiation, alter cloud formation processes, affect atmospheric chemistry and play a role in biogeochemical cycles by providing nutrient inputs such as iron and phosphorus. The influence of dust on these processes depends on its physicochemical properties, which, far from being homogeneous, are shaped by its regionally varying mineral composition. The relative amount of minerals in dust depends on the source region and shows a large geographical variability. However, many state-of-the-art Earth system models (ESMs), upon which climate analyses and projections rely, still consider dust mineralogy to be invariant. The explicit representation of minerals in ESMs is more hindered by our limited knowledge of the global soil composition along with the resulting size-resolved airborne mineralogy than by computational constraints. In this work we introduce an explicit mineralogy representation within the state-of-the-art Multiscale Online Nonhydrostatic AtmospheRe CHemistry (MONARCH) model. We review and compare two existing soil mineralogy datasets, which remain a source of uncertainty for dust mineralogy modeling and provide an evaluation of multiannual simulations against available mineralogy observations. Soil mineralogy datasets are based on measurements performed after wet sieving, which breaks the aggregates found in the parent soil. Our model predicts the emitted particle size distribution (PSD) in terms of its constituent minerals based on brittle fragmentation theory (BFT), which reconstructs the emitted mineral aggregates destroyed by wet sieving. Our simulations broadly reproduce the most abundant mineral fractions independently of the soil composition data used. Feldspars and calcite are highly sensitive to the soil mineralogy map, mainly due to the different assumptions made in each soil dataset to extrapolate a handful of soil measurements to arid and semi-arid regions worldwide. For the least abundant or more difficult-to-determine minerals, such as iron oxides, uncertainties in soil mineralogy yield differences in annual mean aerosol mass fractions of up to ~ 100 %. Although BFT restores coarse aggregates including phyllosilicates that usually break during soil analysis, we still identify an overestimation of coarse quartz mass fractions (above 2 µm in diameter). In a dedicated experiment, we estimate the fraction of dust with undetermined composition as given by a soil map, which makes up ~ 10 % of the emitted dust mass at the global scale and can be regionally larger. Changes in the underlying soil mineralogy impact our estimates of climate-relevant variables, particularly affecting the regional variability of the single-scattering albedo at solar wavelengths or the total iron deposited over oceans. All in all, this assessment represents a baseline for future model experiments including new mineralogical maps constrained by high-quality spaceborne hyperspectral measurements, such as those arising from the NASA Earth Surface Mineral Dust Source Investigation (EMIT) mission.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Climate impacts in scenarios: time to close the loop?

Reaching a full understanding of the consequences of climate change for society and ecosystems, and the ensuing needs for adaptation, requires a consideration of the interactions between human and Earth systems. Currently, however, climate research largely separates the influence of society on climate from the influence of climate on society; that is, it doesn’t “close the loop.” A primary example of this approach is the generation and use of earth system model (ESM) simulations in the climate change research community. Large-scale socio-economic models, known as integrated assessment models (IAMs), are used to project emissions and land use change which serve as input to ESMs. ESM projections then serve as input to models of impacts on society and ecosystems. But, according to this modeling chain, those impacts do not affect the emissions and land use that drove the ESMs in the first place. Previous work has not drawn firm conclusions on whether this feedback would be large enough to warrant explicitly accounting for it. Two prominent possibilities, however, are that emissions and land use scenarios representing the high and low ends of the plausible range of future climate change are both too extreme. The high-end scenario may miss damaging impacts that would reduce economic activity, and therefore emissions, while the low-end scenario may ignore climate feedbacks that would make large-scale land-based carbon removal ineffective and therefore would hamper mitigation at the level assumed by the scenario. In this piece, we identify the opportunities and challenges that implementing such feedback loops would face. We argue that recent developments in climate impact research, human system modeling and ESM emulation make the time ripe to use IAMs in a structured model intercomparison exercise. Model intercomparison projects have benefitted the climate modeling community for decade snow, and more recently have also benefitted the impact modeling community. An IAM intercomparison focused on integrating impacts could make large strides in testing the implications of these feedbacks and assessing whether closing the loop would fundamentally change our outlook on future climate changes and their consequences.

Tebaldi, Claudia↗
DOE OSTI2021

Assessing the Relative Climate Impact of Carbon Utilization for Concrete, Chemical, and Mineral Production

Estimates show that 6.2 gigatons of carbon dioxide (CO2) can be captured and utilized across three pathways, concrete, chemical, and minerals, by 2050. However, it is difficult to compare the climate benefit across these three carbon capture and utilization (CCU) pathways to determine the most effective use of captured CO2. The life cycle assessment methods to evaluate the climate benefit of CCU chemicals should additionally account for the change in material properties of concrete due to CO2 utilization. Furthermore, with most CO2 utilization technologies being in the early stages of research and development, the uncertainty and variability in process and inventory data present a significant challenge in evaluating the climate benefit. We present a stochastically determined climate return on investment (ROI) metric to rank and prioritize CO2 utilization across 20 concrete, chemical and mineral pathways based on the realized climate benefit. We show that two concrete pathways, which use CO2 during concrete mixing, and two chemical pathways, which produce formic acid through hydrogenation of CO2 and carbon monoxide through dry reforming of methane, generate the greatest climate ROI and are the only CCU pathways with a higher likelihood of generating a climate benefit than a climate burden.

29 ENERGY PLANNING, POLICY, AND ECONOMY↗
DOE OSTI2023

Climate Impacts of Convective Cloud Microphysics in NCAR CAM5

Here we improved the treatments of convective cloud microphysics in the NCAR Community Atmosphere Model version 5.3 (CAM5.3) by 1) implementing new terminal velocity parameterizations for convective ice and snow particles, 2) adding graupel microphysics, 3) considering convective snow detrainment, and 4) enhancing rain initiation and generation rate in warm clouds. Furthermore, we evaluated the impacts of improved microphysics on simulated global climate, focusing on simulated cloud radiative forcing, graupel microphysics, convective cloud ice amount, and tropical precipitation. Compared to CAM5.3 with the default convective microphysics, the too-strong cloud shortwave radiative forcing due primarily to excessive convective cloud liquid is largely alleviated over the tropics and midlatitudes after rain initiation and generation rate is enhanced, in better agreement with the CERES-EBAF estimates. Geographic distributions of graupel occurrence are reasonably simulated over continents; whereas the graupel occurrence remains highly uncertain over the oceanic storm-track regions. When evaluated against the CloudSat–CALIPSO estimates, the overestimation of convective ice mass is alleviated with the improved convective ice microphysics, among which adding graupel microphysics and the accompanying increase in hydrometeor fall speed play the most important role. The probability distribution function (PDF) of rainfall intensity is sensitive to warm rain processes in convective clouds, and enhancement in warm rain production shifts the PDF toward heavier precipitation, which agrees better with the TRMM observations. Common biases of overestimating the light rain frequency and underestimating the heavy rain frequency in GCMs are mitigated.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Impacts of climate and biophysical variability on global agriculture markets

Agricultural production is highly sensitive to changes in climate and weather patterns. The focus of the great majority of studies assessing climate impacts on agriculture has been on mean changes in agricultural responses. However, the manner in which global agricultural markets respond to the interannual variability of the climate and biophysical shocks is poorly understood. Here we show a strong transmission of interannual variations in climate-induced biophysical yield shocks to agriculture markets, which is magnified further by endogenous market fluctuations. We demonstrate the importance of imperfect versus perfect expectations of market and weather in generating the market fluctuations that play a key role in transferring the interannual variations to markets. We find that the volatility of market prices and consumption could be potentially reduced on average by 55% and 41%, respectively, with improved expectations, where agricultural producers make better decisions to adapt to climate and biophysical variability. We also find much heterogeneity in interannual variability across crops and regions, which is considerably mediated by trade as part of the economic response. Our study provides new insights on climate impacts on agricultural market variability and lays a foundation for further investigating the full range of climate impacts on biophysical and human systems.

Zhao, Xin↗
DOE OSTI2021

Climate impacts associated with reduced diet diversity in children across nineteen countries

It is widely anticipated that climate change will negatively affect both food security and diet diversity. Diet diversity is especially critical for children as it correlates with macro and micronutrient intake important for child development. Despite these anticipated links, little empirical evidence has demonstrated a relationship between diet diversity and climate change, especially across large datasets spanning multiple global regions and with more recent climate data. Here we use survey data from 19 countries and more than 107 000 children, coupled with 30 years of precipitation and temperature data, to explore the relationship of climate to child diet diversity while controlling for other agroecological, geographic, and socioeconomic factors. We find that higher long-term temperatures are associated with decreases in overall child diet diversity, while higher rainfall in the previous year, compared to the long-term average rainfall, is associated with greater diet diversity. Examining six regions (Asia, Central America, North Africa, South America, Southeast Africa, and West Africa) individually, we find that five have significant reductions in diet diversity associated with higher temperatures while three have significant increases in diet diversity associated with higher precipitation. In West Africa, increasing rainfall appears to counterbalance the effect of rising temperature impacts on diet diversity. In some regions, the statistical effect of climate on diet diversity is comparable to, or greater than, other common development efforts including those focused on education, improved water and toilets, and poverty reduction. These results suggest that warming temperatures and increasing rainfall variability could have profound short- and long-term impacts on child diet diversity, potentially undermining widespread development interventions aimed at improving food security.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Assessing the climate impact of an improved volcanic sulfate aerosol representation in E3SM

Accurately simulating historical surface temperature variations is essential for evaluating climate models, yet many struggle to reproduce the mid-20th-century temperature trends associated with significant volcanic eruptions. This study examines the impact of volcanic sulfate aerosol representation on these biases using the Energy Exascale Earth System Model (E3SM). The standard CMIP6 protocol prescribes volcanic forcing through radiative perturbations, omitting volcanic aerosol–cloud interactions (VACIs). Here, we implement an emission-based approach with an updated volcanic eruption inventory that directly incorporates volcanic sulfur dioxide (SO 2 ) emissions, enabling a more process-based representation of volcanic forcing. This approach leads to improved surface temperature variability and a modest reduction in cold biases between 1940 and 1980 compared to the CMIP6 setup. Additionally, we assess cloud property responses to a more realistic volcanic sulfate aerosol representation, which weakens cloud-induced cooling during periods of lower volcanic activity. However, despite these refinements, a significant temperature cold bias remains, indicating that further improvements in atmospheric chemistry, aerosol microphysics, cloud processes, and model parameterizations are needed to fully resolve this issue in E3SM.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Elastic functional changepoint detection of climate impacts from localized sources

Detecting changepoints in functional data has become an important problem as interest in monitoring of climate phenomenon has increased, where the data is functional in nature. Here, the observed data often contains both amplitude (y-axis) and phase (x-axis) variability. If not accounted for properly, true changepoints may be undetected, and the estimated underlying mean change functions will be incorrect. In this article, an elastic functional changepoint method is developed which properly accounts for these types of variability. The method can detect amplitude and phase changepoints which current methods in the literature do not, as they focus solely on the amplitude changepoint. This method can easily be implemented using the functions directly or can be computed via functional principal component analysis to ease the computational burden. We apply the method and its nonelastic competitors to both simulated data and observed data to show its efficiency in handling data with phase variation with both amplitude and phase changepoints. We use the method to evaluate potential changes in stratospheric temperature due to the eruption of Mt. Pinatubo in the Philippines in June 1991. Using an epidemic changepoint model, we find evidence of a increase in stratospheric temperature during a period that contains the immediate aftermath of Mt. Pinatubo, with most detected changepoints occurring in the tropics as expected.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

HSW-V v1.0: localized injections of interactive volcanic aerosols and their climate impacts in a simple general circulation model

Abstract. A new set of standalone parameterizations is presented for simulating the injection, evolution, and radiative forcing by stratospheric volcanic aerosols against an idealized Held–Suarez–Williamson (HSW) atmospheric background in the Energy Exascale Earth System Model version 2 (E3SMv2). In this model configuration (HSW with enabled volcanism, HSW-V), sulfur dioxide (SO2) and ash are injected into the atmosphere with a specified profile in the vertical, and they proceed to follow a simple exponential decay. The SO2 decay is modeled as a perfect conversion to a long-living sulfate aerosol which persists in the stratosphere. All three species are implemented as tracers in the model framework and are transported by the dynamical core's advection algorithm. The aerosols contribute simultaneously to local heating of the stratosphere and cooling of the surface by a simple plane-parallel Beer–Lambert law applied on two zonally symmetric radiation broadbands in the longwave and shortwave ranges. It is shown that the implementation parameters can be tuned to produce realistic temperature anomaly signatures of large volcanic events. In particular, results are shown for an ensemble of runs that mimic the volcanic eruption of Mt. Pinatubo in 1991. The design requires no coupling to microphysical subgrid-scale parameterizations and thus approaches the computational affordability of prescribed aerosol forcing strategies. The idealized simulations contain a single isolated volcanic event against a statistically uniform climate, where no background aerosols or other sources of externally forced variability are present. HSW-V represents a simpler-to-understand tool for the development of climate source-to-impact attribution methods.

Hollowed, Joseph P. (ORCID:0000000286581672)↗
DOE OSTI2023

The Atlantic Multidecadal Oscillation: Key Drivers and Climate Impacts (Final Technical Report)

The goal of this project was to investigate the Atlantic multidecadal variability (AMV) using a hierarchical modeling framework to advance our process-level understanding on the respective roles of, and the feedback between, the key drivers of the AMV, in particular the ocean circulation associated with the Atlantic meridional overturning circulation and stochastic atmospheric forcing, primarily due to the North Atlantic Oscillation. The focus was primarily on the AMV due to natural variability, but the investigation will be extended to the possible modulation on the main characteristics of AMV under external climate forcing. Furthermore, we examined the impact of the AMV, with a special emphasis on the possible augmentation of predictability the AMV may bring to the regional weather and climate of North America, Western Europe, and the Arctic. Under this goal, we have published 15 peer-reviewed journal papers, and presented our results in more than 30 conferences over the project duration.

58 GEOSCIENCES↗
DOE OSTI2026

Indirect climate impacts of the Hunga eruption

Injection of sulfur and water vapour by the Hunga volcanic eruption significantly altered chemical composition and radiative budget of the stratosphere. Yet, whether the eruption could also affect surface climate, especially via indirect pathways, remains poorly understood. Here we investigate these effects using large ensembles of simulations with the CESM2(WACCM6) Earth system model, incorporating interactive chemistry and aerosols in both coupled ocean and atmosphere-only configurations. We find some statistically significant extratropical regional climate responses to the eruption driven by circulation changes; these are partially linked to the modulation of El Niño–Southern Oscillation, and its associated teleconnections, and to perturbations of the stratospheric polar vortex in both hemispheres. The stratospheric anomalies affect surface climate through modulating the North Atlantic Oscillation in the Northern Hemisphere (up to three boreal winters following the eruption) and the Southern Annular Mode in the Southern Hemisphere in late 2023. The latter is partly related to a concurrent reduction in Antarctic ozone, as increased stratospheric aerosols and water vapor reach the polar vortex. Our study suggests that the eruption could have had a non-negligible influence on regional surface climate, and discusses the mechanisms via which such an influence could occur. However, the results also highlight that this forcing is relatively weak compared to interannual variability, and is subject to model uncertainties in the representation of key processes. More research is thus needed before definitive statements on the role of the eruption in contributing to surface climate and weather events in the following years are made.

Geosciences↗
DOE OSTI2023

Pyrocumulonimbus Events Over British Columbia in 2017: An Ensemble Model Study of Parameter Sensitivities and Climate Impacts of Wildfire Smoke in the Stratosphere

Abstract The Pyrocumulonimbus (pyroCb) events over British Columbia in 2017 were observed in the lower stratosphere for about 8–10 months after the smoke injections. Several previous studies used global climate models to investigate the physical parameters for the 2017 pyroCb events, but the conclusions show strong model dependency. In this study, we use the Energy Exascale Earth System Model (E3SM) and complete an ensemble of runs exploring three injection parameters: smoke aerosol mass, the percentage of black carbon within the smoke aerosols, and plume injection height. Additionally, we consider the heterogeneous reaction of ozone and primary organic matter. According to the satellite daily observed aerosol optical depth (AOD), we find that the best ensemble member is the simulation with 0.4 Tg of smoke, 3% of which is black carbon, a 13.5 km smoke injection height, and a 10 −5 probability factor of the heterogeneous reaction. Besides AOD, we examine the ensemble score based on the metrics used in previous studies: the metrics of the extinction coefficient at 18 km altitude and the maximum plume height. The conclusion of the best estimate of the injection parameters for 2017 pyroCb events shows strong not only model but also evaluation metric dependency. We use the Random Forest machine learning technique to quantify the relative importance of each parameter in accurately simulating the 2017 pyroCb events and find that the injection height is the most critical feature, no matter which metric is used to score the ensemble members.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Climate Impact of Primary Plastic Production

Plastics show the strongest production growth of all bulk materials over the last decade. The industry’s current growth trajectory is exponential and plastic production is expected to double or triple by 2050. The rapidly increasing production of plastics and the continued reliance on fossil fuels for production, have contributed to numerous environmental problems and health harms. As a result, plastic pollution has become an increasing threat to natural ecosystems, human health and climate. However, there is a lack of granularity on the contribution of the primary plastics specifically to greenhouse gas (GHG) emissions and their impact on the remaining global carbon budget needed to stay below a 1.5°C or 2°C global average temperature rise. In this report, we explore the contribution of primary plastic production to climate change disaggregated by polymer and technology. To this end, we have developed comprehensive bottom-up modeling of GHG emissions from global primary plastic production, with a special focus on polymer value chains. We have analyzed the results under various growth scenarios in the context of carbon budgets compatible with a 1.5°C global trajectory. Modeling includes the material flows of all production stages, processes and technologies used in primary plastic production value chains, including from the extraction of fossil fuels required for production to shaping the final product. We specifically focus on nine major types of fossil fuelbased plastic polymers that are produced and consumed in large quantities: three types of polyethylene (PE) – low-density (LDPE), linear low-density (LLDPE), and high-density (HDPE) – as well as polypropylene (PP); polyethylene terephthalate (PET); polyvinyl chloride (PVC); polystyrene (PS) and other key styrene-based plastics such as styrene acrylonitrile (SAN) and acrylonitrile butadiene styrene (ABS), and polyurethane (PU). Together these account for about 80% of plastics production.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Climate Impact of Primary Plastic Production

Plastics show the strongest production growth of all bulk materials over the last decade. The industry’s current growth trajectory is exponential and plastic production is expected to double or triple by 2050. The rapidly increasing production of plastics and the continued reliance on fossil fuels for production, have contributed to numerous environmental problems and health harms. As a result, plastic pollution has become an increasing threat to natural ecosystems, human health and climate. However, there is a lack of granularity on the contribution of the primary plastics specifically to greenhouse gas (GHG) emissions and their impact on the remaining global carbon budget needed to stay below a 1.5°C or 2°C global average temperature rise. In this report, we explore the contribution of primary plastic production to climate change disaggregated by polymer and technology. To this end, we have developed comprehensive bottom-up modeling of GHG emissions from global primary plastic production, with a special focus on polymer value chains. We have analyzed the results under various growth scenarios in the context of carbon budgets compatible with a 1.5°C global trajectory. Modeling includes the material flows of all production stages, processes and technologies used in primary plastic production value chains, including from the extraction of fossil fuels required for production to shaping the final product. We specifically focus on nine major types of fossil fuel-based plastic polymers that are produced and consumed in large quantities: three types of polyethylene (PE) – low-density (LDPE), linear low-density (LLDPE), and high-density (HDPE) – as well as polypropylene (PP); polyethylene terephthalate (PET); polyvinyl chloride (PVC); polystyrene (PS) and other key styrene-based plastics such as styrene acrylonitrile (SAN) and acrylonitrile butadiene styrene (ABS), and polyurethane (PU). Together these account for about 80% of plastics production.

54 ENVIRONMENTAL SCIENCES↗