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At least 37 records · Page 2

Behavior of fuel with zirconium alloy cladding in reactivity-initiated accident and loss-of-coolant accident - 2016-0090

Along with our colleagues at the Japan Atomic Energy Research Institute (JAERI) and Japan Atomic Energy Agency (JAEA), we have performed extensive research programs for more than 2 decades and have developed a better understanding of fuel behavior under accident conditions. Data and findings from these research programs have provided the technical basis directly and indirectly for regulatory criteria in Japan and other countries. This paper reviews and summarizes the major outcomes from the research programs performed at JAERI and JAEA facilities and identifies further research needs. The programs aim to generate data and models to (1) evaluate the adequacy of present safety criteria and safety margins; (2) create a database for the future regulation of higher-burnup UO{sub 2} and mixed-oxide (MOX) fuels, new cladding, and pellets; (3) provide adequately mechanistic computer codes for regulatory application; (4) promote a better understanding of phenomena that appear in high-burnup regions and MOX fuels, such as rim effect and an effect of plutonium agglomerates in MOX fuels, and to evaluate those effects on fuel behavior in accident conditions; and (5) to assess fuel behaviors with higher fuel duty, such as plant power uprates, longer operating cycles, and water chemistry changes. The programs comprise reactivity-initiated accident studies, including pulse-irradiation experiments in the Nuclear Safety Research Reactor, cladding mechanical tests, and the development and verification of RANNS; loss-of-coolant accident tests, including integral thermal shock tests, oxidation rate measurements, and cladding mechanical tests; development and verification of a computer code FEMAXI-6 that simulates high-burnup fuel behavior under normal operating and abnormal transient conditions; and studies on phenomena specific to high-burnup regions, including thermal property measurements, experimental and analytical simulation of rim structure formation, cladding mechanical tests on effects of hydrides, etc. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Analysis of the FeCrAl Accident Tolerant Fuel Concept Benefits during BWR Station Blackout Accidents

Iron-chromium-aluminum (FeCrAl) alloys are being considered for fuel concepts with enhanced accident tolerance. FeCrAl alloys have very slow oxidation kinetics and good strength at high temperatures. FeCrAl could be used for fuel cladding in light water reactors and/or as channel box material in boiling water reactors (BWRs). To estimate the potential safety gains afforded by the FeCrAl concept, the MELCOR code was used to analyze a range of postulated station blackout severe accident scenarios in a BWR/4 reactor employing FeCrAl. The simulations utilize the most recently known thermophysical properties and oxidation kinetics for FeCrAl. Overall, when compared to the traditional Zircaloy-based cladding and channel box, the FeCrAl concept provides a few extra hours of time for operators to take mitigating actions and/or for evacuations to take place. A coolable core geometry is retained longer, enhancing the ability to stabilize an accident. Finally, due to the slower oxidation kinetics, substantially less hydrogen is generated, and the generation is delayed in time. This decreases the amount of non-condensable gases in containment and the potential for deflagrations to inhibit the accident response.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

New intrinsically smart severe accident instrumentation saves costs and enhances severe accident management - 302

The Severe Accidents (SA) at Fukushima in 2011, identified the need for enhanced I and C to follow the progress of SA. Since SA environments are significantly Beyond DBA conditions, some new advanced Inherently Smart sensors had to be developed and tested. Nuclear plant designers and operators have helped focus the I and C enhancement based upon lessons learned from the Fukushima accidents. The result has been the addition of I and C for direct measurement of SA conditions hydrogen concentration, oxygen concentration, temperature, and pressure that provide unambiguous information for management of Severe Accident scenarios. The benefits are immediate from three important aspects. First, they deliver on the nuclear promise for enhanced safety at reduced costs. These Inherently Smart sensors have no maintenance and replace equipment that has high maintenance costs. Secondly, these sensors provide multiple benefits, such as condition monitoring information all the time and direct measurement of SA conditions if they are needed. Thirdly, and most importantly, simplify operator actions and training for SA. SA scenarios and SA Management can now rely on direct measurements to know such things as, the extent of fuel damage, integrity of the reactor pressure vessel, when corium is on the floor of containment, and conditions upon which to activate the hardened vent. (authors)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

A review of inherent safety characteristics of metal alloy sodium-cooled fast reactor fuel against postulated accidents

The thermal, mechanical, and neutronic performance of the metal alloy fast reactor fuel design complements the safety advantages of the liquid metal cooling and the pool-type primary system. Together, these features provide large safety margins in both normal operating modes and for a wide range of postulated accidents. In particular, they maximize the measures of safety associated with inherent reactor response to unprotected, double-fault accidents, and to minimize risk to the public and plant investment. High thermal conductivity and high gap conductance play the most significant role in safety advantages of the metallic fuel, resulting in a flatter radial temperature profile within the pin and much lower normal operation and transient temperatures in comparison to oxide fuel. Despite the big difference in melting point, both oxide and metal fuels have a relatively similar margin to melting during postulated accidents. When the metal fuel cladding fails, it typically occurs below the coolant boiling point and the damaged fuel pins remain cool-able. Metal fuel is compatible with sodium coolant, eliminating the potential of energetic fuel coolant reactions and flow blockages. All these, and the low retained heat leading to a longer grace period for operator action, are significant contributing factors to the inherently benign response of metallic fuel to postulated accidents. This paper summarizes the past analytical and experimental results obtained in past sodium-cooled fast reactor safety programs in the United States, and presents an overview of fuel safety performance as observed in laboratory and in-pile tests.

inherent safety↗

Modular Accident Analysis Program (MAAP) - MELCOR Crosswalk: Phase II Analyzing a Partially Recovered Accident Scenario

Following the conclusion of the first phase of the crosswalk analysis, one of the key unanswered questions was whether or not the deviations found would persist during a partially recovered accident scenario, similar to the one that occurred in TMI - 2. In particular this analysis aims to compare the impact of core degradation morphology on quenching models inherent within the two codes and the coolability of debris during partially recovered accidents. A primary motivation for this study is the development of insights into how uncertainties in core damage progression models impact the ability to assess the potential for recovery of a degraded core. These quench and core recovery models are of the most interest when there is a significant amount of core damage, but intact and degraded fuel still remain in the cor e region or the lower plenum. Accordingly this analysis presents a spectrum of partially recovered accident scenarios by varying both water injection timing and rate to highlight the impact of core degradation phenomena on recovered accident scenarios. This analysis uses the newly released MELCOR 2.2 rev. 966 5 and MAAP5, Version 5.04. These code versions, which incorporate a significant number of modifications that have been driven by analyses and forensic evidence obtained from the Fukushima - Daiichi reactor site.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Preliminary Modeling of Accident Tolerant Fuel Concepts under Accident Conditions

The catastrophic events that occurred at the Fukushima-Daiichi nuclear power plant in 2011 have led to widespread interest in research of alternative fuels and claddings that are proposed to be accident tolerant. Thus, the United States Department of Energy through its NEAMS (Nuclear Energy Advanced Modeling and Simulation) program has funded an Accident Tolerant Fuel (ATF) High Impact Problem (HIP). The ATF HIP is funded for a three-year period. The purpose of the HIP is to perform research into two potential accident tolerant concepts and provide an in-depth report to the Advanced Fuels Campaign (AFC) describing the behavior of the concepts, both of which are being considered for inclusion in a lead test assembly scheduled for placement into a commercial reactor in 2022. The initial focus of the HIP is on uranium silicide fuel and iron-chromium-aluminum (FeCrAl) alloy cladding. Utilizing the expertise of three national laboratory participants (INL, LANL, and ANL) a comprehensive mulitscale approach to modeling is being used including atomistic modeling, molecular dynamics, rate theory, phase-field, and fuel performance simulations. In this paper, we present simulations of two proposed accident tolerant fuel systems: U3Si2 fuel with Zircaloy-4 cladding, and UO2 fuel with FeCrAl cladding. The simulations investigate the fuel performance response of the proposed ATF systems under Loss of Coolant and Station Blackout conditions using the BISON code. Sensitivity analyses are completed using Sandia National Laboratories’ DAKOTA software to determine which input parameters (e.g., fuel specific heat) have the greatest influence on the output metrics of interest (e.g., fuel centerline temperature). Early results indicate that each concept has significant advantages as well as areas of concern. Further work is required prior to formulating the proposition report for the Advanced Fuels Campaign.

36 MATERIALS SCIENCE↗

Accident-tolerant fuel: quantifying relative risks and timescales in severe accidents

For such severe accident scenarios, a key objective for alternative 'accident tolerant' fuels (or ATFs) is to increase the threshold temperature for possible accelerated hydrogen production and/or fuel damage and core degradation. By reducing hydrogen production, this change to more ATF should also give more time for restoring power and cooling, for mitigating actions like emergency equipment deployment, and consequently effect on- and off-site evacuation decisions. There is always a finite and non-zero probability of core damage due to the likelihood and chance of not restoring power and cooling. Using the Fukushima complete Station Black Out (SBO) and Loss-of-Cooling (LOC) scenario as a starting point, this paper establishes a simple limiting estimate for the potential changes in the timescales available for power and cooling recovery and for emergency evacuation decision-making made possible by using ATFs. The straightforward analysis also provides a basis for estimating the realistic probability of avoiding core damage for a range of assumed ATF failure properties or criteria, and the needed backup cooling requirements. The analysis includes the effects on the recovery probability caused by significant disruption and chaos. The results show that for this accident scenario, there is a relatively small benefit or increase in recovery probability due to only having higher ATF failure limits. The largest relative benefit arises from not only having ATF but also assuring longer cooling by extending the boil off or time before core uncover and damage onset, from somehow adding and/or injecting sufficient make up water, and/or rejecting decay heat, say for five or more days. Obviously, as an added benefit, some ATF concepts avoid or reduce hydrogen production, which improves containment integrity but does not significantly alter the core damage or failure probability.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Testing Accident Tolerant Fuels in Reactivity Initiated Accident Conditions

The Transient Reactor Test Facility (TREAT) at Idaho National Laboratory (INL) has been successfully restarted. A principal goal of restarting the reactor was to perform transient testing of Accident Tolerant Fuels (ATF), supporting their safe adoption by the commercial Light Water Reactor (LWR) fleet. This paper will describe the efforts underway at INL to conduct testing of ATF under Reactivity Initiated Accident (RIA) conditions in an inert helium atmosphere. Tests in an inert helium atmosphere capsule provide valuable information about initial deposition and distribution of energy in the nuclear fuel. Tests in an inert helium atmosphere are especially suited for ATF concepts where the thermophysical properties of the new fuel material differ from UO2 such as the U3Si2 fuel concept and other non-oxide materials. These tests are also useful for exploring the thermal mechanical interaction of pellets with cladding where the cladding mechanical properties do not change much with temperature such as Silicon Carbide Cladding. Tests with nominal dimensions will be used to determine how fresh fuel failure and core coolability limits of ATF pellet and cladding materials compare with that of standard LWR fuel made up of UO2 pellets and Zircaloy cladding. Tests with a reduced pellet cladding gap will be used as a preliminary indicator of any pellet cladding mechanical interaction (PCMI) vulnerabilities of the new fuel concepts. The materials, methods, and schedule for the ATF RIA tests will be discussed in the paper.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Hydrothermal Corrosion of SiC Materials for Accident Tolerant Fuel Cladding with and Without Mitigation Coatings

As a candidate material for accident-tolerant fuel cladding for light water reactors (LWR), SiCf–SiC composite materials possess many attractive properties. However, prior work has shown that SiC is susceptible to aqueous dissolution in LWR coolant environments. To address this issue, candidate coatings have been developed to inhibit dissolution. For this study, CVD SiC samples were prepared with Cr, CrN, TiN, ZrN, NiCr, and Ni coatings. Uncoated SiC and SiCf–SiC samples were also prepared. The samples were exposed for 400 h in 288 °C water with 2 wppm DO in a constantly-refreshing autoclave to simulate BWR–NWC. Cr and Ni coated samples lost less mass than the uncoated SiC sample, indicating an improvement in performance. The CrN coating resisted oxidation, but some of the coating was lost due to poor adhesion. The TiN coated sample gained significant mass due to oxidation of the coating. ZrN and NiCr coatings showed significant corrosion attack. SiCf–SiC ceramic matrix composite materials dissolved much faster than the CVD SiC sample, demonstrating the need for mitigation coatings if CMCs are to be used in LWRs. This work demonstrates the promise of Cr, Ni and CrN coatings for corrosion mitigation in LWRs, and shows that NiCr and ZrN are not promising coating materials.

Raiman, Stephen S.↗

Estimate of radiation release from MIT reactor with un-finned LEU core during Maximum Hypothetical Accident

The Massachusetts Institute of Technology Reactor (MITR-II) is a research reactor in Cambridge, Massachusetts designed primarily for experiments using neutron beam and in-core irradiation facilities. At 6 MW, it delivers neutron flux and energy spectrum comparable to light water reactor (LWR) power reactors in a compact core using highly enriched uranium (HEU) fuel. In the framework of nonproliferation policy, the international community aims to minimize the use of HEU in civilian facilities. Within this context, research and test reactors have started a program to convert HEU fuel to low enriched uranium (LEU) fuel. A new type of LEU fuel based on a high density alloy of uranium and molybdenum (U-10Mo) is expected to allow the conversion of U.S. domestic high performance reactors like MITR. The current study focuses on the impacts of MITR Maximum Hypothetical Accident (MHA), which is also the Design Basis Accident (DBA), with LEU fuel. The MHA for the MITR is postulated to be a coolant flow blockage in the fuel element that contains the hottest fuel plate. It is assumed that the entire active portion of five fuel plates melts. The analysis shows that, within a 2-h period and by considering all the possible radiation sources and dose pathways, the overall off-site dose is 302.1 mrem (1 rem ¼ 0.01 Sv) Total Effective Dose Equivalent (TEDE) at 8 m exclusion area boundary (EAB) and a higher dose of 392.8 mrem TEDE is found at 21 m EAB. In all cases the dose remains below the 500 mrem total TEDE limit goal based on NUREG-1537 guidelines.

Sun, Kaichao (ORCID:0000000285871918)↗

Preliminary modeling of accident tolerant fuel concepts under accident conditions

In this paper, we present simulations of two proposed accident tolerant fuel systems for light-water reactors: U{sub 3}Si{sub 2} fuel with Zircaloy-4 cladding, and UO{sub 2} fuel with FeCrAl cladding. The simulations investigate the fuel performance response of the proposed ATF systems under Loss of Coolant (LOCA) and Station Blackout (SBO) conditions using the BISON code. It was observed that U{sub 3}Si{sub 2}/Zircaloy4 and UO{sub 2}/FeCrAl have superior performance during a 90 s LOCA than traditional UO{sub 2}/Zircaloy4 fuel rods. This is based upon reduced fuel centerline temperatures and lower cladding strains experienced during the LOCA. For the postulated SBO analyzed in this work, it was found that the centerline temperature and cladding strains remained well below any values of concern. This is attributed to the shortness of the rod studied and how the coolant channel model treats the inlet as the bottom of the rod. An analysis of a full-length fuel rod is required to obtain improved qualitative comparisons between the 3 systems under SBO conditions. Sensitivity analyses have been performed using Sandia National Laboratories' DAKOTA software to determine which input parameters (e.g., fuel specific heat) have the greatest influence on the output metrics of interest (e.g., fuel centerline temperature). Early results indicate that each concept has significant advantages as well as areas of concern. Further work is required prior to formulating the proposition report for the Advanced Fuels Campaign.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

TRISO SiC Failure Probability for Reactivity Initiated Accidents in High-Temperature Gas-Cooled Reactors

This work analyzes the failure process of the silicon carbide (SiC) layer in tristructural isotropic (TRISO) during reactivity-initiated accident scenarios for a high-temperature gas-cooled reactor (HTGR) with BISON. Two cases are considered—a group control rod withdrawal (CRW) and a control rod ejection (CRE)—reproduced from a previous study. Failure probability is modeled using Weibull statistics, and worst-case scenario Weibull parameters are adopted to simulate the envelopes in BISON with a one-dimensional TRISO model. CRW scenario results are characterized by higher values of maximum energy deposition and final temperature and volumetric strain with respect to the CRE ones, but the latter have remarkably higher SiC failure probability, mainly due to the offset in strain rates between the two cases. This work also confirms the validity and conservatism of the performance envelopes produced in a previous work by replicating the envelope formulation using RELAP5-3D and RAVEN with a different sampling technique and obtaining consistent results. A sensitivity analysis using the Sobol variance decomposition method on SiC failure probability is then performed involving a set of inputs on both CRW and CRE. The two most important parameters are Weibull modulus and characteristic stress, and their relative importance depends on the specific case. The proposed interpretation of the results is that both energy deposition and strain rate influence the relative degree of importance of the failure parameters. Computation of 95% confidence intervals around worst-case scenario SiC failure probability values is also carried out for four different sets of Weibull parameters. Heren a new criterion for SiC TRISO quality classification built upon safety-based ranges of Weibull parameters is proposed to be integrated in future Fuel-Production Quality Assurance Plans.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

A Look at Aircraft Accident Analysis in the Early Days: Do Early 20th Century Accident Investigation Techniques Have Any Lessons for Today?

In the early years of powered flight, the National Advisory Committee on Aeronautics in the United States produced three reports describing a method of analysis of aircraft accidents. The first report was published in 1928; the second, which was a revision of the first, was published in 1930; and the third, which was a revision and update of the second, was published in 1936. This paper describes the contents of these reports, and compares the method of analysis proposed therein to the methods used today.

Holloway, C. M.↗

The Columbia Accident: Synopsis of CAIB Report Regarding the Physical Cause of the Accident and and Personal Thoughts

This seminar describes the process of determining the physical cause of The Shuttle Columbia Accident. The presentation is based on the published CIAB Report, and is based mainly on Appendix F2, Vol IV of the CIAB report by J. O. Arnold, H. E. Goldstein and D. J. Rigalli. As a part of the seminar, I would also indicate how my education in Engineering Physics at the University of Kansas helped prepare me to accept the assignment to serve as an investigator for the CAIB. A similar presentation was given at Purdue in 2005. Presentation charts are attached.

Arnold, James O.↗