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All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

LAMP Technical Readiness Evaluation Report (Rev. 1)

An internal preliminary evaluation of Critical Technology Elements (CTEs) for the LANSCE Modernization Project (LAMP) was completed. Corresponding Technical Readiness Levels (TRLs) were also determined for all subsystems using the criteria of DOE G 413.3-4A, Technical Readiness Assessment Guide. The scope of the evaluation was limited to the project Work Breakdown Structure (WBS) elements as defined for the RFQ Injector and Drift Tube Linac (DTL) systems only. Integration of Instrumentation and Controls (I&C) and Safety Systems was not considered, although specific technologies as related to the RFQ and DTL systems were included. Other elements of the project such as Shielding, System Design, Technical Management, and additional facility integration needed to enable off-line testing and pre-installation commissioning were also not evaluated. Each technical subsystem element was evaluated for technical readiness, however, not all were found to meet the criteria for a CTE. Only two subsystem elements were determined to meet the CTE criteria. Their associated TRLs are summarized in the table below. These subsystem elements of the project have the lowest technical readiness due to either being new, novel or modified, requiring additional R&D before being capable of meeting the project Key Performance Parameters (KPPs) and subsystem requirements, or present technology exists but has not yet been demonstrated in a relevant environment. All other subsystems were determined to have a TRL of 8, indicating that actual operating systems exist having similar performance requirements as needed for LAMP. Details of the technical readiness evaluation for each subsystem is given in the following sections of this report.

43 PARTICLE ACCELERATORS↗
DOE OSTI2025

LAMP Technical Readiness Evaluation Report

An internal preliminary evaluation of Critical Technology Elements (CTEs) for the LANSCE Modernization Project (LAMP) was completed in 2023. This included determining corresponding Technical Readiness Levels (TRLs) for all subsystems using the criteria of DOE G 413.3-4A, Technical Readiness Assessment Guide. This revised report includes a summary of the recent design modifications required to meet the project Key Performance Requirements (KPPs), some of which may reduce technical risk to the project. These recent design modifications include: • Further optimization of the low-energy and medium-energy beam transport regions (LEBT and MEBT, respectively), including relocation of various functional elements (ie choppers, kickers, and bunchers). • An additional H - ion source to separate ion-source function based on beam delivery requirements. • A high-repetition-rate pulsed kicker magnet to select/merge the two H ion beams into a common low-energy beam transport. • Modification and further optimization to a more conventional RFQ design. Performance of the RFQ has been optimized to deliver the required three types of beams while meeting the project KPPs. • The addition of a second chopper in the medium-energy beam transport (MEBT) line to reduce the required pulser voltages. The scope of the evaluation was limited to the project Work Breakdown Structure (WBS) elements as defined for the RFQ Injector and Drift Tube Linac (DTL) systems only. Integration of Instrumentation and Controls (I&C) and Safety Systems was not considered, although specific technologies as related to the RFQ and DTL systems were included. Other elements of the project such as Shielding, System Design, Technical Management, and additional facility integration needed to enable off-line testing and pre-installation commissioning were also not evaluated. Each technical subsystem element was evaluated for technical readiness, however, not all were found to meet the criteria for a CTE. Three subsystem elements were determined to meet the CTE criteria. Their associated TRLs are summarized in the table below. These subsystem elements of the project have the lowest technical readiness due to either being new, novel or modified, requiring additional R&D before being capable of meeting the project Key Performance Parameters (KPPs) and subsystem requirements, or present technology exists but has not yet been demonstrated in a relevant environment. All other subsystems were determined to have a TRL of 8, indicating that actual operating systems exist having similar performance requirements as needed for LAMP. Details of the technical readiness evaluation for each subsystem is given in the following sections of this report.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

Diagnostics for PSR Upgrade

This report discusses the diagnostics upgrade plan for the PSR. The PSR diagnostics under discussion include beam position and phase monitor (BPPM), wirescanners, wall current monitors, bunch shape monitors, laser notchers, and diamond array detectors. Existing diagnostics at the PSR include beam position monitors (BPM), a wirescanner, and a wall current monitor. All existing diagnostics need modernization, as part of the PSR upgrade plan. Meanwhile, we will introduce minor changes to improve the existing setups, which will enhance the performance and the longevity of the diagnostics equipment and components in the upgraded PSR operation. On the other hand, new, advanced, and available diagnostic technologies at a high technology readiness level (TRL) can also be considered for implementation for the PSR upgrade. In this note, we go through all types of diagnostics, introducing their basic principle, operating status, and plans for the PSR upgrade.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Flow Measurements in Pressurized Helium Gas Cooling Channels

Production of metastable Technetium-99 (Tc-99m) is vital to the medical imaging community. It is a radioactive tracer that emits gamma rays as it decays and it is these gamma rays that are then detected through imaging. Tc-99m is extracted from the decay of Molybdenum-99 (Mo-99) which has a half-life of about 2-3 days. One method of generating Mo-99 is using accelerator based technology, through the irradiation of Mo-100 using an electron beam. This is part of the NNSA’s mission to produce Mo-99 commercially, within the US, without the use of highly enriched uranium (HEU) in support of nonproliferation and global security. Los Alamos National Laboratory (LANL) is working with NorthStar medical Radioisotopes (NMR) on their efforts to produce Mo-99 from the irradiation of Mo-100 targets. The NMR target consists of an Inconel window that allows the electron beam to penetrate and irradiate a stack of Mo-100 discs. The irradiation process generates large amounts of heat and requires extensive cooling of the Mo-100 targets and target housing using pressurized helium gas. Before beam on target, the design of the target stack and target housing is tested at LANL using laser based diagnostics experiments. We quantify the velocity field of the helium gas around the target housing to estimate whether the cooling provided is sufficient for the design and to validate computational fluid dynamics (CFD) models. Fiber optic imaging is also developed for use during cold testing (without beam on target) as well as during irradiation, to obtain real time information on disc performance.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2022

Evaluation of Synthetic Diamond Detectors for Fast Neutron and X-ray Detection [Slides]

Element6 has come out of a two year production pause (pre-COVID) with material that lacks their previous QC – some is excellent, but screening is needed. Applied Diamond can now make usable polycrystalline material, for applications not requiring absolute flux calibration. A large area possible (1cm 2 ). Great Lakes Crystal Technology has made great progress in two years, but still needs development to become a trusted supplier of single crystal material. LANL staff (Dongsung Kim) has developed proficient lithography and bonding expertise at CINT to make devices from vendor supplied material. LANL staff has continued and expanded capabilities for device testing at NSLS-II.

42 ENGINEERING↗
DOE OSTI2023

805 Stepped Plan Project Description

The 805 MHz system utilizes 1.25 MW class klystron amplifiers. The Solid-State Amplifier (SSA) technology has been utilized in the SC accelerator technology, but more powerful sources are needed for use in the NC accelerator facilities such as LASNCE. The SSA topologies that are widely used need to be scaled and tested for reliability and operation in a high impact accelerator facility, such as the 805 MHz SCCL in Los Alamos. Operational experience with high power SSA needs to be assessed prior to installation of an SSA unit at LANSCE. The RFE group at LANSCE is looking for collaboration in the development of the Solid-State Amplifier.

43 PARTICLE ACCELERATORS↗
DOE OSTI2023

Development of an accelerator-based neutron source to prototype Mo-99 production, Part II: A liquid LBE loop under a high vacuum

To provide US domestic supply of Mo-99 without using high-enriched uranium (HEU), a subcritical uranium target assembly (UTA) is irradiated by an accelerator-based neutron source to create Mo-99 through fission. Part I of this work discusses the design of a liquid lead–bismuth eutectic (LBE) windowless target for an accelerator-based neutron source development. Part II discusses how to couple this windowless target to an accelerator operating at an ultra-high vacuum and the subcritical UTA cooled by water at room temperature. Due to the windowless design of the target, the liquid LBE flow shares an ultra-high vacuum (<1.3 × 10 -7 Pa or 10 -9 Torr) space with the accelerator. As a result of this shared vacuum space, the LBE system must operate at a high vacuum (10 -3 ~10 -6 Pa or 10 -5 ~10 -8 Torr). A magnetic rotary motion feedthrough unit utilizes magnetic fluid to allow rotation of the pump while maintaining a high vacuum environment. Prior to testing the LBE system under vacuum, a pump curve measurement is performed to estimate flowrate in the system. This measurement also generates data on orifice loss coefficients, which are compared to correlations in literature. The second experiment investigates vacuum level in the LBE system during operation. High vacuum is maintained (10 -3 ~10 -5 Pa or 10 -5 ~10 -7 Torr) during system operation, and a residual gas analyzer (RGA) scan shows that partial pressures of residual gases in the LBE system lower over the duration of LBE system operations. The third experiment investigates the gravity driven liquid LBE flowing out of the target chamber in the return line, which is partially full. If the liquid LBE is not drained quickly enough, flooding in the target chamber could occur. The coefficient n in the Manning equation is found to be around 0.008 s/m 1/3 . The last experiment performed is a demonstration that a vacuum jacket could provide sufficient thermal insulation to allow coupling between 300 °C LBE loop and a water tank at room temperature. In conclusion, the results from these experiments have influenced the development of the neutron source for the future commercial scale Mo-99 production system.

43 PARTICLE ACCELERATORS↗
DOE OSTI2021

Systematic evaluation of magnetic sensitivities of anisotropic magnetoresistive sensors at liquid helium temperature for superconducting cavities

Trapped magnetic flux in bulk superconductors reduces the quality factor Q in superconducting radio-frequency (SRF) cavities. However, the mechanisms underlying flux trapping and radio-frequency loss are not well understood. Detailed observation of the magnetic distributions is important for understanding such phenomena. Magnetic field mapping is useful for observing the magnetic field distribution around SRF cavities. Measuring the change in the magnetic field around the cavity elucidates the flux trapping behavior. Anisotropic magnetoresistive (AMR) sensors are inexpensive and small devices that can detect magnetic flux density. The magnetic sensitivities of AMR sensors need to be evaluated at liquid helium temperature for the magnetic field mapping of SRF cavities. In this study, a test stand was constructed to calibrate the magnetic sensitivities of AMR sensors in liquid helium, and 110 AMR sensors were tested using this stand. The magnetic sensitivities were evaluated systematically. A solenoid coil was used to control the uniform external magnetic field and to measure the magnetic sensitivity at low temperatures. All AMR sensors exhibited suitable sensitivities to the magnetic field around the SRF cavity. The variation in these sensitivities in all AMR sensors was ~1%. Further, the AMR sensors were found to have sufficient sensitivity for mapping the magnetic field around the exterior surface of the SRF cavity.

43 PARTICLE ACCELERATORS↗
DOE OSTI2021

FEbeam: Cavity and electron emission data conversion, processing, and analysis. A freeware toolkit for rf injectors

FEbeam is an all-in-one field emission data processing interface with the capability to analyze the field emission cathode performance in an rf injector by extracting the field enhancement factor, local field, and effective emission area from the Fowler–Nordheim equations. It also has the capability of processing beam imaging micrographs using its sister software, FEpic. Furthermore, the current version of FEbeam was designed for the Argonne Cathode Test-stand of the Argonne Wakefield Accelerator facility switch yard. With slight modifications, FEbeam could work for many rf field emission injectors. This software is open-source and can be found at GitHub.

43 PARTICLE ACCELERATORS↗
DOE OSTI2021

Robust method for broadband efficiency enhancement of electron photocathodes using optical interferences

In this work, we demonstrate the key features of an interference cathode using both simulations and experiments. We deposit Cs 3 Sb photocathodes on Ag to produce an interference enhanced photocathode with 2–5× quantum efficiency (QE) enhancement using a robust procedure that requires only a smooth metal substrate and QE monitoring during growth. We grow both an interference cathode (Ag substrate) and a typical photocathode (Si reference substrate) simultaneously to confirm that the effects are due to optical interactions with the substrate rather than photocathode composition or surface electron affinity differences. Growing the cathodes until the QE converges shows both the characteristic interference peaks during growth and the identical limiting case where the cathode is “infinitely thick,” in agreement with simulations. We also grow a cathode until the QE on Ag peaks and then stop the growth, demonstrating broadband QE enhancement.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Photoelectron spectroscopy of CsK2Sb photocathode at Synchrotron Radiation Facility using vacuum transport system

As accelerators and electron microscopes become more advanced, high-performance photocathodes are required. In particular, Cesium potassium antimonide (CsK 2 Sb) photocathode is of interest because of its low emittance, excitability in visible light, and high quantum efficiency (QE). The challenge is its high susceptibility to environment that lead to low operating vacuum pressure and short lifetime/low extraction charge. To resolve these issues, it is necessary to understand the molecular structure of the cathode and its degradation mechanism. In this study, we transported CsK 2 Sb photocathode to a beamline of synchrotron radiation facility using a vacuum transport system for molecular structure analysis. Specifically, the cathode was deposited in an evaporation system at Nagoya University. We transported it to Aichi Synchrotron Radiation Center (Aichi SR) located 15 km away, and analyzed it in the depth direction by X-ray photoelectron spectroscopy (XPS) at BL7U. Based on the results, we quantitatively evaluated the composition ratios and stoichiometry of the cathode elements (Sb, K, Cs). A Cs ex-cess state of surface was observed at the surface, and it is consistent with previous studies. The intended atomic structure of CsK 2 Sb was formed only at a few nanometres of the surface on the Mo substrate. On the other hand, the CsK 2 Sb cathode structure on the graphene substrate was preserved further in the depth direction.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Observation of quenching-induced magnetic flux trapping using a magnetic field and temperature mapping system

Highly efficient superconducting radio-frequency cavities exhibit low heat loss and are used as components in accelerators and superconducting devices due to their high Q-values. The precise location of magnetic flux trapping in cavities is necessary to identify its effects on the performance of superconducting cavities. In this study, we report a new combined mapping system to measure the temperature and magnetic field on the equator. The proposed system comprehensively maps local magnetic field changes as magnetic flux trapping due to quenching. Our experimental results show that magnetic flux trapping due to quenching increases the local surface resistance of superconducting cavities at 2 K. Thus, the proposed system elucidates the relationship between local flux trapping due to quenching and surface resistance in superconducting cavities and highlights the effect of quenching on the surface resistance. This system can aid in the development of superconducting cavities with higher Q values.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Mitigation of Beam Losses in LANSCE Linear Accelerator

Suppression of beam losses is essential for successful operation of high-intensity accelerator facility. The LANSCE accelerator started routine operation in 1972 as a 0.8 MW average proton beam power facility for meson physics research, and delivered highpower beam for a quarter century. The accelerator currently delivers 100 MeV proton beam to Isotope Production Facility (IPF) and 800 MeV H- beams to various experimental areas. The accelerator is equipped with two independent injectors for H + and H - beams, merging at the entrance of a 201.25 MHz Drift Tube Linac (DTL). The DTL performs acceleration up to the energy of 100 MeV. After the DTL, the Transition Region beamline directs a 100 MeV proton beam to the Isotope Production Facility, while the H - beam is accelerated up to the final energy of 800 MeV in an 805- MHz Coupled Cavity Linac. The H - beams, created with different time structure by a lowenergy chopper, are distributed in the Switch Yard (SY) to four experimental areas: the Lujan Neutron Scattering Center equipped with a Proton Storage Ring (PSR), the Weapons Neutron Research facility (WNR), the Proton Radiography facility (pRad), and the Ultra-Cold Neutron facility (UCN). Multi-beam operation requires careful control of accelerator tune to minimize beam losses. In this paper we review main effects affecting beam losses in LANSCE linear accelerator and discuss methods to reduce them.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Northstar Accelerator Based Mo99 Production Facility Design Support (LANL FY20 Quarters 1 and 2 Facility Design Support Report)

Facility design support this quarter centered on transfer of the target insertion and design details to MBraun and Springs, the companies under contract via Northstar to do the hot cell, target insertion and the local target shielding. A significant number of changes have been introduced by these vendors which have been reviewed and critiqued. In addition, the company contracted to produce the Mo100 disks announced that the tolerance on the thickness of 0.5 mm would be ±25%. An alternative design of the target holder was proposed. Bulk shielding and local target shielding design work has continued also and will be reported.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Northstar Mo100 Target Beam Spot Size Sensitivity Study

Northstar Mo100 target for production of the medical isotope Mo99 is particularly sensitive to beam over focusing because of the intended high power density. At 38 MeV and 6.32 mA (240 kW beam power, nominally 160 kW th in the target), small deviation from the nominal 12 mm FWHM beam can significantly increase the target disk temperatures and more importantly the load bearing target window temperature. A rhodotron will be the source of the electron beam to be used in the isotope production. This machine operates in a pulsed beam mode, currently expected to be at 50 Hz, which results in a 100 C temperature oscillation above and below the steady state temperature that is the focus of this study. This must be considered in the determination of minimum beam spot size that can be accepted by the target without risk of failure. In addition to the nominal beam spot size of 12 mm, the analysis of 10, 11 and 14.5 mm beam spot sizes are analyzed. The primary conclusion is that an over focused beam to just 11 mm FWHM is the minimum beam spot allowable, based on window temperature and the Ultimate Tensile Stress (UTS) of the window material Inconel 718 as a function of temperature. In contrast an under focused beam of 14.5 mm FWHM has much reduced target and window temperatures, but there is a resulting 6% drop in isotope production, all other factor staying the same. These results are presented herein.

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2020

Niowave Power Converter Modeling and Testing

Niowave has designed, built and is now using in-beam a low power (up to 10 kW) lead bismuth eutectic (LBE) converter. In this concept, an electron beam is passed through a falling layer of LBE, converting the electron to neutrons which then pass into a vessel which is functionally a subcritical reactor configuration. A detailed report has been written by Niowave, entitled “LBE Neutron Converter Manual.” The LANL contribution has been modeling, followed by a flow visualization model made in quartz. The LANL contribution is reported herein.

43 PARTICLE ACCELERATORS↗
DOE OSTI2020

Design and Analysis of a Double Wall, Water Cooled Window for Accelerator Based Mo-99 Production

The electron accelerator based Mo-99 production technique requires the use of Rhodotrons to generate 38 MeV, 6.32 mA pulsed electron beams. The introduction of the pulsed beam structure has introduced fatigue concerns in the vacuum-helium windows that did not exist previously for electron beam production via linear accelerators. Previous analysis has shown that temperature fluctuations of approximately 100°C above and below the steady state operating temperature of ~500°C will occur within the windows. A water cooled window will eliminate this concern by reducing the primary mechanical stress due to the 300-psig helium pressure load as well as the secondary thermally induced stress. Although a water cooled window was considered years ago, the complexities of adding an additional water line was unattractive until now. A double wall, water cooled window has been designed and analyzed for this reason. The water cooled window design is shown to decrease the helium-side window temperature to as low as 125°C, while the vacuum-side window is maintained at 161°C at a water flow rate of 3.2 GPM. These low steady state temperatures reduce the thermal stress of the helium-side window significantly. Also, the primary mechanical stress has been reduced by roughly 50% due to the reduced pressure gradient across the helium-side window (150-psig water and 300-psig helium). Considering a Mo-99 production loss of roughly 1%, the water cooled window is a drastic improvement over the previous helium cooled designs and should be greatly considered for future upgrades and redesign.

43 PARTICLE ACCELERATORS↗