FY16/17 PROGRESS IN SRNL RECOVERY OF PLUTONIUM-244 AND HEAVY ACTINIDES FROM MARK-18A TARGETS
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ABSTRACT Fast and accurate large‐eddy simulation (LES) of the atmospheric boundary layer plays a crucial role in advancing wind energy research. Long‐duration wind farm studies at turbine‐resolving scales have become increasingly important to understand the intricate interactions between large wind farms and the atmospheric boundary layer. However, the prohibitive computational cost of these turbulence‐ and turbine‐resolving simulations has precluded such modeling to be exercised on a regular basis. To that end, we implement and validate the generalized actuator disk (GAD) model in the computationally efficient, graphics processing unit (GPU)–resident, LES model FastEddy. We perform single‐turbine simulations under three atmospheric stabilities (neutral, unstable, and stable) and compare them against observations from the Scaled Wind Farm Technology (SWiFT) facility and other LES codes from the recent Wakebench turbine wake model benchmark. Our idealized LES results agree well with observed wake velocity deficit and downstream recovery across stability regimes. Turbine response in terms of rotational speed, generated power, torque, and thrust coefficient are well predicted across stability regimes and are consistent with the LES results from the benchmark. The FastEddy simulations are found to be at least two orders of magnitude more efficient than the traditional CPU‐based LES models, opening the door for realistic LES simulations of full wind plants as a viable standard practice.
The magnetar Swift J1822.3–1606 entered an outburst phase in 2011 July. Previous X-ray studies of its post-outburst rotational evolution yielded inconsistent measurements of the spin-inferred magnetic field. Here we present the timing behavior and flux relaxation from over two years of Swift, RXTE, and Chandra observations following the outburst. We find that the ambiguity in previous timing solutions was due to enhanced spin down that resembles an exponential recovery following a glitch at the outburst onset. After fitting out the effects of the recovery, we measure a long-term spin-down rate of ν-dot =(−3.0 ± 0.3)×10{sup −16} s{sup –2} which implies a dipolar magnetic field of 1.35 × 10{sup 13} G, lower than all previous estimates for this source. We also consider the post-outburst flux evolution, and fit it with both empirical and crustal cooling models. We discuss the flux relaxation in the context of both crustal cooling and magnetospheric relaxation models.
Two-band radiance-ratio in-water algorithms in the visible spectrum have been evaluated for remote oceanic chlorophyll determination. Airborne active-passive (laser-solar) data from coastal, shelf-slope, and blue-water regions were used to generate two-dimensional chlorophyll-fluorescence and radiance-ratio statistical correlation matrices containing all possible two-band ratio combinations from the thirty-two available contiguous 11.25-nm passive bands. The principal finding was that closely spaced radiance-ratio bands yield chlorophyll estimates which are highly correlated with laser-induced chlorophyll fluorescence within several distinct regions of the ocean color spectrum. Band combinations in the yellow, orange-red, spectral regions showed considerable promise for satisfactory chlorophyll pigment estimation in near-coastal Case II waters. Pigment recovery in Case I waters was best accomplished using blue-green radiance ratios in the 490/500-nm region.
Single and dual-beam ion irradiations of silicon carbide (SiC) were performed to study possible Synergetic effects between Nuclear (S{sub n}) and Electronic (S{sub e}) Energy Losses. Results obtained combining Rutherford backscattering in channeling conditions, Raman spectroscopy, and transmission electron microscopy techniques show that dual-beam irradiation of SiC induces a dramatic change in the final sample microstructure with a substantial decrease of radiation damage as compared to single-beam irradiation. Actually, a defective layer containing dislocations is formed upon dual-beam irradiation (S{sub n} and S{sub e}), whereas single low-energy irradiation (S{sub n} alone) or even sequential (S{sub n} + S{sub e}) irradiations lead to full amorphization. The healing process is ascribed to the electronic excitation arising from the electronic energy loss of swift ions. These results shed new light on the long-standing puzzling problem of the existence of a possible synergy between S{sub n} and S{sub e} in ion-irradiation experiments. This work is interesting for both fundamental understanding of the ion-solid interactions and technological applications in the nuclear industry where recovery S{sub n}/S{sub e} effects may preserve the integrity of nuclear devices.
Tetragonally structured BaTiO3 single crystals were irradiated using 635 MeV 238U+ ions to fluences of 1E7, 5E10 and 1.4E12 ions/cm2 at room temperature. Subsequent sample characterizations were performed using ion channeling, x-ray diffraction (XRD), helium ion microscopy, and transmission electron microscopy. The results show that there are lattice relaxation and recovery of pre-existing defects in the irradiated samples. Various structures representing different regimes of electronic and nuclear interactions along the ion track are observed. The track on the surface has an amorphous core of up to ~10 nm in diameter, surrounded by a strained lattice structure. The core size is roughly proportional to the square root of the electronic stopping power. Satellite-like defects around the core are also present. The ring of cubic phase expected to form around the amorphous core does not appear, probably due to a reversible phase transition as confirmed by an in-situ XRD study. Modeling and simulation are also attempted to interpret the data and gain physical insights. We have developed a partial charge model for cubic BaTiO3 that reproduces its lattice constants, elastic constants, and melting temperature. Using the interatomic potential, we have performed molecular dynamics simulations of the irradiation damage in BaTiO3. The results show that an amorphous track of ~1.2 nm in radius forms under thermal energy deposition at dE(T)/dx = 5 keV/nm. At 20 keV/nm, the radius increases to ~4.5 nm with an order of magnitude increase in the number of defects. The simulation also reveals details of the bonding environments and shows that the amorphous zones produced at different dE(T)/dx values have different densities. The combined experimental and computational data suggest that there is a significant interfacial recrystallization of the as-created amorphous cores during the cooling-down stage of thermal spikes.
A conceptual design of a very large aeroballistic range is presented, as are its operational characteristics and procedures. The proposed model launcher is a two-stage light-gas gun, having a launch tube diameter of 254 mm, and the capability of accelerating a 14 kg launch mass to 6.1 km/sec. The gun's 91.4 cm diameter piston is driven by pressurized helium. High pressures in the central breech are contained by a multiple disk arrangement. The blast tank and sabot separation tank are described, as are methods for arresting sabot segments. The conceptual design of the range itself includes a 3.3 m diameter test or flight chamber some 330 m in length. Provisions are made for testing of free flight models and tests in which the model is confined by a track system. Methods for model deceleration and recovery are described. Provisions required for future addition of advanced model launchers such as an electromagnetic launcher or ram accelerator are addressed. Siting and safety issues are also addressed.
A technical assessment of the current inventory [∼70,150 metric tons of heavy metal (MTHM) as of 2011] of U.S.-discharged used nuclear fuel (UNF) has been performed to support decisions regarding fuel cycle strategies and research, development and demonstration (RD and D) needs. The assessment considered discharged UNF from commercial nuclear electricity generation and defense and research programs and determined that the current UNF inventory can be divided into the following three categories: 1. Disposal - excess material that is not needed for other purposes; 2. Research - material needed for RD and D purposes to support waste management (e.g., UNF storage, transportation, and disposal) and development of alternative fuel cycles (e.g., separations and advanced fuels/reactors); and 3. Recycle/Recovery - material with inherent and/or strategic value. A set of key assumptions and attributes relative to the various disposition options were used to categorize the current UNF inventory. Based on consideration of RD and D needs, time frames and material needs for deployment of alternative fuel cycles, characteristics of the current UNF inventory, and possible uses to support national security interests, it was determined that the vast majority of the current UNF inventory should be placed in the Disposal category, without the need to make fuel retrievable from disposal for reuse or research purposes. Access to the material in the Research and Recycle/Recovery categories should be retained to support RD and D needs and national security interests. This assessment does not assume any decision about future fuel cycle options or preclude any potential options, including those with potential recycling of commercial UNF. (authors)
We investigated thermal transport in swift heavy ion (SHI) irradiated insulating single crystalline oxide materials: yttrium aluminum garnet- Y 3 Al 5 O 12 (YAG), sapphire (Al 2 O 3 ), zinc oxide (ZnO) and magnesium oxide (MgO) irradiated by 167 MeV Xe ions at 10 12 – 10 14 ions/cm 2 fluences. Depth profiling of the thermal transport on nano- and micro- meter scales was assessed by time-domain thermoreflectance (TDTR) and modulated thermoreflectance (MTR) methods, respectively. This combination allowed us to isolate the conductivities of different sub-surface damage-regions characterized by their distinct microstructure evolution regimes. Thermal conductivity degradation in SHI irradiated YAG and Al 2 O 3 is attributed to formation of ion tracks and subsequent amorphization, while in ZnO and MgO it is mostly due to point defects. Additionally, notably lower conductivity when probed by very low penetrating thermal waves is consistent with surface hillock formation. An analytical model based on Klemens-Callaway method for thermal conductivity coupled with a simplified microstructure evolution capturing saturation in defect concentration was used to obtain depth dependent damage across the ion impacted region. The studies showed that YAG has the highest damage profile resulting in the less dependence of thermal conductivity with the depth, while MgO on the contrary has the strongest dependence. The presented work sheds new light on how SHI induced defects affect thermal transport degradation and recovery of oxide ceramics as promising candidates for next generation nuclear reactor applications.
During the past several years symmetric three-band (460-, 490-, 520-nm) spectral curvature algorithm (SCA) has demonstrated rather accurate determination of chlorophyll pigment concentration using low-altitude airborne ocean color data. It is shown herein that the in-water asymmetric SCA, when applied to certain recently proposed OCI (NOAA-K and SPOT-3) and OCM (ERS-1) satellite ocean color bands, can adequately recover chlorophyll-like pigments. These airborne findings suggest that the proposed new ocean color sensor bands are in general satisfactorily, but not necessarily optimally, positioned to allow space evaluation of the SCA using high-precision atmospherically corrected satellite radiances. The pigment concentration recovery is not as good when existing Coastal Zone Color Scanner bands are used in the SCA. The in-water asymmetric SCA chlorophyll pigment recovery evaluations were performed using (1) airborne laser-induced chlorophyll fluorescence and (2) concurrent passive upwelled radiances. Data from a separate ocean color sensor aboard the aircraft were further used to validate the findings.
A computational analysis of a Gulfstream isentropic external compression supersonic inlet coupled to a Rolls-Royce fan has been completed. The inlet was designed for a small, low sonic boom supersonic vehicle with a design cruise condition of M = 1.6 at 45,000 ft. The inlet design included an annular bypass duct that routed flow subsonically around an engine-mounted gearbox and diverted flow with high shock losses away from the fan tip. Two Reynolds-averaged Navier-Stokes codes were used for the analysis: an axisymmetric code called AVCS for the inlet and a three dimensional (3-D) code called SWIFT for the fan. The codes were coupled at a mixing plane boundary using a separate code for data exchange. The codes were used to determine the performance of the inlet/fan system at the design point and to predict the performance and operability of the system over the flight profile. At the design point the core inlet had a recovery of 96 percent, and the fan operated near its peak efficiency and pressure ratio. A large hub radial distortion generated in the inlet was not eliminated by the fan and could pose a challenge for subsequent booster stages. The system operated stably at all points along the flight profile. Reduced stall margin was seen at low altitude and Mach number where flow separated on the interior lips of the cowl and bypass ducts. The coupled analysis gave consistent solutions at all points on the flight profile that would be difficult or impossible to predict by analysis of isolated components.
A computational analysis of a Gulfstream isentropic external compression supersonic inlet coupled to a Rolls-Royce fan was completed. The inlet was designed for a small, low sonic boom supersonic vehicle with a design cruise condition of M = 1.6 at 45,000 feet. The inlet design included an annular bypass duct that routed flow subsonically around an engine-mounted gearbox and diverted flow with high shock losses away from the fan tip. Two Reynolds-averaged Navier-Stokes codes were used for the analysis: an axisymmetric code called AVCS for the inlet and a 3-D code called SWIFT for the fan. The codes were coupled at a mixing plane boundary using a separate code for data exchange. The codes were used to determine the performance of the inlet/fan system at the design point and to predict the performance and operability of the system over the flight profile. At the design point the core inlet had a recovery of 96 percent, and the fan operated near its peak efficiency and pressure ratio. A large hub radial distortion generated in the inlet was not eliminated by the fan and could pose a challenge for subsequent booster stages. The system operated stably at all points along the flight profile. Reduced stall margin was seen at low altitude and Mach number where flow separated on the interior lips of the cowl and bypass ducts. The coupled analysis gave consistent solutions at all points on the flight profile that would be difficult or impossible to predict by analysis of isolated components.
The solar wind interaction with the geomagnetic field is studied using global auroral images obtained by the Ultraviolet Imager (UVI) on Polar. We study the dynam,cs of the poleward and equatorward boundaries of the auroral oval in response to the solar wind IMF on January 10, 1997 using a neural network algorithm to perform an automated morphological analysis. Poleward and equatorward boundaries identified by the algorithm demonstrate a clear growth motion with the southward turning of the IMF and growth and poleward expansion at substorm onset. The area poleward of the oval (polar cap) is found to increase in size coincident with the'southward turning of the IMF Bz component at 0220 UT and peaks at substorm onset at 0334 UT. The area of the oval, however, decreases continuously throughout the period of the polar cap area increase with a slight recovery observed during the substorm onset. These observations are consistent with the concept that magnetospheric dynamics are directly driven by the solar wind-geomagnetic field interactions.
We introduce a new capability of the Neil Gehrels Swift Observatory to provide event-level data from the Burst Alert Telescope (BAT) on demand in response to transients detected by other instruments. We show that the availability of these data can effectively increase the rate of detections and arcminute localizations of gamma-ray bursts (GRB) like GRB 170817 by >400%. We describe an autonomous spacecraft-commanding pipeline purpose built to enable this science; to our knowledge, this is the first fully autonomous extremely low-latency commanding of a space telescope for scientific purposes. This pipeline has been successfully run in its complete form since 2020 January, and has resulted in the recovery of BAT event data for >800 externally triggered events to date (gravitational waves, GWs; neutrinos; GRBs triggered by other facilities; fast radio bursts; and very high-energy detections), now running with a success rate of ∼90%. We exemplify the utility of this new capability by using the resultant data to (1) set the most sensitive upper limits on prompt 1 s duration short GRB-like emission within ±15 s around the unmodeled GW burst candidate S200114f, and (2) provide an arcminute localization for short GRB 200325A and other bursts. We also show that using data from GUANO to localize GRBs discovered by other instruments, we can increase the net rate of arcminute-localized GRBs by 10%–20% per year. Along with the scientific yield of more sensitive searches for subthreshold GRBs, the new capabilities designed for this project will serve as the foundation for further automation and rapid target of opportunity capabilities for the Swift mission, and have implications for the design of future rapid-response space telescopes.
Swift heavy ion (2 GeV 181 Ta) irradiation-induced amorphization and temperature-induced recrystallization of cubic pyrochlore Gd 2 Ti 2 O 7 (Fd3¯m) are compared with the response of a compositionally-similar material with a monoclinic-layered perovskite-type structure, La 2 Ti 2 O 7 (P2 1 ). The averaged electronic energy loss, dE/dx, was 37 keV/nm and 35 keV/nm in Gd 2 Ti 2 O 7 and La 2 Ti 2 O 7 , respectively. Systematic analysis of the structural modifications was completed using transmission electron microscopy, synchrotron X-ray diffraction, Raman spectroscopy, and small-angle X-ray scattering. Increasing ion-induced amorphization with increasing ion fluence was evident in the X-ray diffraction patterns of both compositions by a reduction in the intensity of the diffraction maxima concurrent with the growth in intensity of a broad diffuse scattering halo. Transmission electron microscopy analysis showed complete amorphization within ion tracks (diameter: ~10 nm) for the perovskite-type material; whereas a concentric, core–shell morphology was evident in the ion tracks of the pyrochlore, with an outer shell of disordered yet still crystalline material with the fluorite structure surrounding an amorphous track core (diameter: ~9 nm). The radiation response of both titanate oxides with the same stoichiometry can be understood in terms of differences in their structures and compositions. While the radiation damage susceptibility of pyrochlore A 2 B 2 O 7 materials decreases as a function of the cation radius ratio rA/rB, the current study correlates this behavior with the stability field of monoclinic structures, where rLa/rTi > rGd/rTi. Isochronal annealing experiments of the irradiated materials showed complete recrystallization of La 2 Ti 2 O 7 at 775 °C and of Gd 2 Ti 2 O 7 at 850 °C. The annealing behavior is discussed in terms of enhanced damage recovery in La 2 Ti 2 O 7 , compared to the pyrochlore compounds Gd 2 Ti 2 O 7 . As a result, the difference in the recrystallization behavior may be related to structural constraints, i.e., reconstructing a low symmetry versus a high symmetry phase.
We report that pressure-driven shock waves in solid materials can cause extreme damage and deformation. Understanding this deformation and the associated defects that are created in the material is crucial in the study of a wide range of phenomena, including planetary formation and asteroid impact sites, the formation of interstellar dust clouds, ballistic penetrators, spacecraft shielding and ductility in high-performance ceramics. At the lattice level, the basic mechanisms of plastic deformation are twinning (whereby crystallites with a mirror-image lattice form) and slip (whereby lattice dislocations are generated and move), but determining which of these mechanisms is active during deformation is challenging. Experiments that characterized lattice defects have typically examined the microstructure of samples after deformation, and so are complicated by post-shock annealing and reverberations. In addition, measurements have been limited to relatively modest pressures (less than 100 gigapascals). In situ X-ray diffraction experiments can provide insights into the dynamic behaviour of materials, but have only recently been applied to plasticity during shock compression and have yet to provide detailed insight into competing deformation mechanisms. Here we present X-ray diffraction experiments with femtosecond resolution that capture in situ, lattice-level information on the microstructural processes that drive shock-wave-driven deformation. To demonstrate this method we shock-compress the body-centred-cubic material tantalum—an important material for high-energy-density physics owing to its high shock impedance and high X-ray opacity. Tantalum is also a material for which previous shock compression simulations and experiments have provided conflicting information about the dominant deformation mechanism. Our experiments reveal twinning and related lattice rotation occurring on the timescale of tens of picoseconds. In addition, despite the common association between twinning and strong shocks, we find a transition from twinning to dislocation-slip-dominated plasticity at high pressure (more than 150 gigapascals), a regime that recovery experiments cannot accurately access. Lastly, the techniques demonstrated here will be useful for studying shock waves and other high-strain-rate phenomena, as well as a broad range of processes induced by plasticity.
Described herein is a series of design studies concerning the Assured Crew Return Vehicle (ACRV). Study topics include a braking and landing system for the ACRV, ACRV growth options, and the design impacts of ACRV's role as a medical emergency vehicle. Four alternate designs are presented for the ACRV braking and landing system. Options presented include ballistic and lifting body reentries; the use of high-lift, high-payload aerodynamic decelerators, as well as conventional parachutes; landing systems designed for water landings, land landings or both; and an aerial recovery system. Uses of the ACRV or a similarly designed vehicle in several roles for possible future space missions are discussed, along with the required changes to the ACRV to allow it to perform these missions optimally. The impacts on the design of the ACRV due to its role as an emergency vehicle were studied and are presented here. This study included the design of a stretcher-like system to transport an ill or injured crewmember safely within the ACRV; a compilation of necessary medical equipment and decisions on how or where to store it; and recommendations about internal and external vehicle characteristics that will ease the transport of the ill or injured crewmember and allow for swift and easy ingress/egress of the vehicle.
Abstract not provided