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DOE OSTI2024

Electromagnetic Radioisotope Separator for Methods Development, Testing, and Training

The major goal of the project is the construction and operation of an electromagnetic isotope separator. Included in that goal is the construction and installation of a high throughput surface ion source, with specific applicability to the Lanthanides. The surface ion source features a single-piece titanium crucible insert that mates with a tantalum hot surface ionizer. The titanium crucible, which does not readily activate, can be loaded with samarium and then irradiated simultaneously, greatly reducing operator dose.

07 ISOTOPE AND RADIATION SOURCES↗

NASA NTRS1994

Compact radio sources in the starburst galaxy M82 and the Sigma-D relation for supernova remnants

We have obtained an 8.4 GHz Very Large Array (VLA) A-array map of the starburst galaxy M82 with a resolution Full Width at Half Maximum (FWHM) approximately 0.182 sec. About 50 compact radio sources in the central region of M82 were detected with a peak surface brightness approximately greater than 10(exp -17) W/Hz/sq m/sr. Comparison with previous observations shows that most sources are declining in flux. Three previously visible sources have faded into the background of our map (approximately less than 0.2 mJy/beam), while a few sources, including the second and third brightest radio sources in M82, may have increased slightly in flux over the last decade. No new radio supernova was found. The birth rate of the compact radio sources is estimated to be 0.11 + or - 0.05/yr. We attribute the population of such bright, small supernova remnants (SNRs) in M82 to the high pressure in the central region that can truncate the mass loss during a red supergiant phase or allow dense ionized clouds to be present. The compact radio sources obey a Sigma(radio surface brightness) - D(diameter) relation which is remarkably similar to that followed by supernova remnants in the Galaxy and the Magellanic Clouds and by two of the strongest known extragalactic radio supernovae: SN 1986J and SN 1979C. A least-squares fit to the SNR data gives: Sigma(sub 8.4 GHz) (W/Hz/sq m/sr) = 4.4 x 10(exp -16) D(sub pc)(exp -3.5 +/- 0.1) covering seven orders of magnitude in Sigma. Possible selection effects are discussed and a theoretical discussion of the correlation is presented.

Huang, Z. P.↗

NASA NTRS2011

Calcium in Mercury's Exosphere: Modeling MESSENGER Data

Mercury is surrounded by a surface-bounded exosphere comprised of atomic species including hydrogen, sodium, potassium, calcium, magnesium, and likely oxygen. Because it is collisionless. the exosphere's composition represents a balance of the active source and loss processes. The Mercury Atmospheric and Surface Composition Spectrometer (MASCS) on the MErcury Surface. Space ENvironment. GEochemistry. and Ranging (MESSENGER) spacecraft has made high spatial-resolution observations of sodium, calcium, and magnesium near Mercury's surface and in the extended, anti-sunward direction. The most striking feature of these data has been the substantial differences in the spatial distribution of each species, Our modeling demonstrates that these differences cannot be due to post-ejection dynamics such as differences in photo-ionization rate and radiation pressure. but instead point to differences in the source mechanisms and regions on the surface from which each is ejected. The observations of calcium have revealed a strong dawn/dusk asymmetry. with the abundance over the dawn hemisphere significantly greater than over the dusk. To understand this asymmetry, we use a Monte Carlo model of Mercury's exosphere that we developed to track the motions of exospheric neutrals under the influence of gravity and radiation pressure. Ca atoms can be ejected directly from the surface or produced in a molecular exosphere (e.g., one consisting of CaO). Particles are removed from the system if they stick to the surface or escape from the model region of interest (within 15 Mercury radii). Photoionization reduces the final weighting given to each particle when simulating the Ca radiance. Preliminary results suggest a high temperature ( I-2x 10(exp 4) K) source of atomic Ca concentrated over the dawn hemisphere. The high temperature is consistent with the dissociation of CaO in a near-surface exosphere with scale height <= 100 km, which imparts 2 eV to the freshly produced Ca atom. This source region and energy are consistent with data from the three MESSENGER flybys; whether this holds true for the data obtained in orbit is under investigation.

Burger, Matthew H.↗

NASA NTRS1973

The open-source neutral-mass spectrometer on Atmosphere Explorer-C, -D, and -E.

The open-source mass spectrometer will be used to obtain the number densities of the neutral atmospheric gases in the mass range 1 to 48 amu at the satellite location. The ion source has been designed to allow gas particles to enter the ionizing region with the minimum practicable number of prior collisions with surfaces. This design minimizes the loss of atomic oxygen and other reactive species due to reactions with the walls of the ion source. The principal features of the open-source spectrometer and the laboratory calibration system are discussed.

Nier, A. O.↗

NASA NTRS2018

Hall Current Plasma Source Having a Center-Mounted or a Surface-Mounted Cathode

A miniature Hall current plasma source apparatus having magnetic shielding of the walls from ionized plasma, an integrated discharge channel and gas distributor, an instant-start hollow cathode mounted to the plasma source, and an externally mounted keeper, is described. The apparatus offers advantages over other Hall current plasma sources having similar power levels, including: lower mass, longer lifetime, lower part count including fewer power supplies, and the ability to be continuously adjustable to lower average power levels using pulsed operation and adjustment of the pulse duty cycle. The Hall current plasma source can provide propulsion for small spacecraft that either do not have sufficient power to accommodate a propulsion system or do not have available volume to incorporate the larger propulsion systems currently available. The present low-power Hall current plasma source can be used to provide energetic ions to assist the deposition of thin films in plasma processing applications.

Martinez, Rafael A.↗

DOE OSTI2022

Simulation of Liquid Lithium Divertor Geometry Using SOLPS-ITER

Here, plasma-facing component (PFC) geometries are evaluated for a Fusion Nuclear Science Facility (FNSF) design to find solutions that are compatible with flowing liquid lithium components while satisfying requirements from the perspective of plasma and neutral particle transport. Flowing liquid metal (LM) divertor systems offer important advantages due to continual regeneration of the surface material, but may require modifications from standard optimized tokamak divertor designs. Scrape Off Layer Plasma Simulator for the International Thermonuclear Experimental Reactor (SOLPS-ITER) simulations are used to compare standard vertical target, open, and balanced baffled geometries. It is found that the open geometry offers little control of neutral particles and has narrow operating windows where the divertor fluxes can be lowered to acceptable levels, while maintaining the required upstream density. The addition of neutral baffles allows greater control over the divertor conditions with less impact on the upstream density. The divertor neutral pressure in the baffled geometry is slightly higher than the open divertor, but not as large with a vertical target. A first-pass coupling of the SOLPS solution with sheath and implantation/erosion models to compute the lithium emission shows that the lithium is largely confined to the near-surface region due to the small ionization mean free path and large main ion flow toward the surface. The lithium source was varied by three orders of magnitude. At the highest rate, when the sourced lithium approaches the level of the main ion recycling flux, a high core lithium concentration (~10%) is observed with only moderate power dissipation to affect the divertor plasma.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1991

Origins of the 12-200 micron flux in NGC 6946 - Starlight and continuum dust emission from AN Sc galaxy

Infrared maps and optical CCD images of NGC 6946, a nearly face-on spiral with evidence of active star formation, are presented. Consideration is given, at 1-3 kpc spatial scales, to the relationship of the infrared continuum to spiral and radial structure, tracers of the interstellar medium, and ionizing and nonionizing sources of stellar radiation. Two infrared components were revealed - one with surface brightnesses of 20-60 Jy per 45 arcsec aperture at 160 microns, and the other with a surface brightness of less than 20 Jy. Various continuum distributions show discrete sources coinciding with giant H II regions superposed on a smooth unresolved disk background which decreases exponentially with the radius. The optical and spectral properties of the nuclear source and the disk are described. Dust properties and heating conditions, and far-infrared emitting phases are discussed.

Engargiola, G.↗

NASA NTRS1974

A new approach to mass spectrometer measurements of thermospheric density

The gas sampling problem in satellite and high velocity probes was investigated by applying the theory of a drifting Maxwellian gas. A lens system using a free stream ion source was developed and experimentally evaluated over the pressure range of 0.00001 to 0.01 N/m sq (approx. 10 to the minus 7th power to 0.0001 torr). The source has high beam transparency, which minimizes gas-surface collisions within, or near, the ionization volume. It is shown that for high ion energy (60 eV), the extracted ion beam has an on-axis energy spread of less than 4 eV, and that 90 percent of the ions are within 2.5 deg of the beam axis. It is concluded that the molecular beam mass spectrometer concept, developed for gas density measurements in the upper atmosphere, substantially reduces gas-surface scattering and gas-surface reactions in the sample, and preserves the integrity of the gas sample during the analysis process. Studies show that both the Scout and Delta launch vehicles have adequate volume, control, velocity, and data acquisition capability necessary to obtain thermospheric number density in real time.

Melfi, L. T., Jr.↗

NASA NTRS1983

Accretion disks, precessing jets and the asymmetric emission lines of QSOs

The broad line profiles of active galaxies are consistent with emission from the surface of an accretion disk ionized by an ultraviolet continuum emitted from a linear or point source of continuum above the disk. If the point source is offset from the axis of the disk, then the line peak is shifted from zero velocity in a way that resembles observed cases. This misalignment could result from the Lense-Thirring precession of a rotating black hole.

Shields, G. A.↗

NASA NTRS1991

Limits to the lunar atmosphere

Apollo UV spectrometer experiment set limits on the density of oxygen of less than 500/cu cm, and the Apollo Lunar Atmospheric Composition Experiment data imply a value less than 50/cu cm above the subsolar point. These limits are surprisingly small relative to the measured value for sodium. A simple consideration of sources and sinks predicts significantly greater densities of oxygen. It is possible but doubtful that the Apollo measurements occurred during an epoch in which source rates were small. A preferential loss process for oxygen on the darkside of the moon is considered in which ionization by electron capture in surface collisions leads to escape through acceleration in the local electric field. Cold trapping in permanently shadowed regions as a net sink is considered and discounted, but the episodic nature of cometary insertion may allow formation of ice layers which act as a stabilized source of OH. On the basis of an assumed meteoroid impact source, a possible emission brightness of 50 R in the OH(A - X)(0,0) band above the lunar bright limb is predicted.

Morgan, T. H.↗

DOE OSTI2022

Plasma production and composition from hypervelocity impacts on solar cell cover glass

Satellites are subjected to detrimental effects from the space environment, including impacts by orbital debris and meteoroids that can cause mechanical or electrical damage. While mechanical damage is well studied, electrical effects resulting from hypervelocity impact (HVI) remain poorly understood. In HVIs, where the projectile speed exceeds the speed of sound in the target material, the impact energy ionizes the material near the surface, creating a plasma that can cause radio frequency emission. This emission is the main source of electrical anomalies in satellites, but the mechanism behind its creation is still unknown. Ground-based experiments have been used to characterize HVI plasma, including the empirical power law relations that describe the impact charge produced as a function of impactor mass and speed. Quantifying these power law relations gives us a better understanding of the species formed in the impact which can eventually lead to plasma evolution models and help us first, understand the mechanism behind radio frequency emission and second, ways to prevent its damage to the satellites. In this paper, we interpret the results of the HVI experiments on solar cell coverglass targets and identify the potential chemical or molecular reactions that form the impact ion species. This is done by looking simultaneously at multiple data sets for different species within the same impact configuration, and using a new technique for quantifying the power law relations for each emitted species. We use time of flight analysis (TOF) to detect the charged particle compositions and determine their initial speeds. The results suggest that the charge production power law is species specific, with different formation mechanisms involved in a single HVI event, some of which are associated with dissociation and some with ionization of a molecule. Furthermore, our results also show that electrons have different power laws that depend on the spacecraft surface charge. TOF measurements of ions from impact events on solar cell cover glass shows the presence of SiO + and SiO – 2 as the dominant species present in plasmas on positively and negatively charged targets, respectively, as well as the formation of FeO + .

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1993

Galactic fine-structure lines - Morphologies of the warm ionized interstellar medium

Far-infrared ionic fine-structure emission lines associated with the large-scale structure of the Galactic ionized medium are interpreted in terms of a heuristic model in which three distinct source morphologies are considered: ionization-bounded H II regions, an extended, low-density medium, and externally ionized surfaces of neutral clouds. The model reveals that the overall luminosity of the Galaxy in the fine-structure lines of both C II and N II is due, in comparable proportions, to diffuse medium and the boundaries between ionized and neutral regions. Limits are set on the luminosity of the diffuse component in the plane of the Galaxy. Some individual lines of sight of the COBE FIRAS instrument are dominated, in these spectral lines, by H II regions, even with its 7 deg field of view. Average densities of both H II regions and photodissociation regions are estimated on a Galactic scale.

Petuchowski, S. J.↗

DOE OSTI2020

Interactions between atmospheric pressure plasmas and metallic catalyst particles in packed bed reactors

Atmospheric-pressure plasmas sustained in packed bed reactors (PBRs) are being investigated for chemical conversion of gases and pollution control. Metallic catalysts added to the surfaces of the dielectric beads of PBRs can increase the energy efficiency and selectivity of chemical processes by reducing operating temperature and providing additional reaction pathways. In this paper, results from a computational investigation of plasma surface interactions between micron-scale metallic catalysts and humid-air plasmas in PBRs are discussed. Here we found that high plasma density regions form in the proximity of the metallic catalysts. These higher-density plasma regions were confirmed experimentally using ICCD imaging. The intense plasmas result from geometrical electric field enhancement and redistribution of charges within the conductive particles, leading to further enhancement. The high electric field at the triple points of the catalysts can produce electric field emission of electrons, which provides a pre-ionization source or additional source of electrons. These regions of high electric field and sources of electrons guide discharges towards the catalysts and increases fluxes of excited species, ions, electrons and photons to their surfaces. These fluxes are focused primarily at the triple points between the metal, dielectric and gas. As a result, the catalyst is locally heated, which could lead to further increased rates of thermocatalytic reactions on the surface. Surface roughness of the metal inclusions can lead to additional electric field enhancement, which changes the character of the discharges in the vicinity of the catalysts while reducing breakdown voltage.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1978

Europa - Ultraviolet emissions and the possibility of atomic oxygen and hydrogen clouds

Emission signals from Europa with wavelength below 800 A were detected by the Pioneer 10 ultraviolet photometer. In the present paper, improved procedures for data reduction are used to determine the spatial region as well as the intensity of the suggested emission sources. The observations indicate a cloud with a radius of about 1.5 Jupiter radii and an apparent brightness of approximately 10 rayleighs for a wavelength of 500 A. It is argued that neutral oxygen atoms, along with neutral hydrogen, are produced through dissociation of water ice on the surface of Europa by particle impact. Electron impact ionization excitation of oxygen atoms in the resulting cloud then gives rise to the observed emission. The present source brightness and cloud radius results are used to estimate an oxygen column density of the order of 10 trillion per sq cm, while the density of atomic hydrogen is at most 100 billion per sq cm and 1 trillion per sq cm for molecular hydrogen.

Wu, F.-M.↗

NASA NTRS1980

Plasmas in Saturn's magnetosphere

The solar wind plasma analyzer on board Pioneer 2 provides first observations of low-energy positive ions in the magnetosphere of Saturn. Measurable intensities of ions within the energy-per-unit charge (E/Q) range 100 eV to 8 keV are present over the planetocentric radial distance range about 4 to 16 R sub S in the dayside magnetosphere. The plasmas are found to be rigidly corotating with the planet out to distances of at least 10 R sub S. At radial distances beyond 10 R sub S, the bulk flows appear to be in the corotation direction but with lesser speeds than those expected from rigid corotation. At radial distances beyond the orbit of Rhea at 8.8 R sub S, the dominant ions are most likely protons and the corresponding typical densities and temperatures are 0.5/cu cm and 1,000,000 K, respectively, with substantial fluctuations. It is concluded that the most likely source of these plasmas in the photodissociation of water frost on the surface of the ring material with subsequent ionization of the products and radially outward diffusion. The presence of this plasma torus is expected to have a large influence on the dynamics of Saturn's magnetosphere since the pressure ratio beta of these plasmas approaches unity at radial distances as close to the planet as 6.5 R sub S. On the basis of these observational evidences it is anticipated that quasi-periodic outward flows of plasma, accompanied with a reconfiguration of the magnetosphere beyond about 6.5 R sub S, will occur in the local night sector in order to relieve the plasma pressure from accretion of plasma from the rings.

Frank, L. A.↗

NASA NTRS1996

Externally Induced Evaporation of Young Stellar Disks in Orion

In this paper we propose a model for the evaporation of disks around young low-mass stars by external sources of high energy photons. Two evaporation techniques are possible. Lyman continuum radiation can ionize hydrogen at the disk surface powering a steady thermal ionized disk-wind, or FUV radiation can heat the disk through photo-electric grain processes powering a slower thermal neutral disk-wind. Applying these two models to the evaporating objects in the Trapezium produces a satisfactory solution to both the mass-loss rate and size of the ionized envelopes.

Johnstone, D.↗

DOE OSTI2020

Design and Evaluation of a Tethered, Open Port Sampling Interface for Liquid Extraction-Mass Spectrometry Chemical Analysis

Presented in this work is a tethered, liquid-extraction-sampling interface designed for the mass spectrometric surface sampling/analysis of 3D objects. The tethered, open port sampling interface (TOPSI) incorporates a vacuum line between the sampling probe and ionization source, which enables the ability for an extended, tethered sample transfer line. Herein, several designs of the hand-held TOPSI are presented and evaluated on the basis of the analytical metrics of analyte transport time, peak width, and analyte sensitivity. The best analytical metrics were obtained with capillary flow resistances arranged in a particular order and the vacuum region set at 6.2 kPa. This TOPSI design incorporated a transfer capillary 1 m in length, while retaining a fast analyte transport time (12 s), short signal peak width (5 s baseline-to-baseline), and high analyte signal at 90% of that obtained with a regular open port sampling interface (OPSI). The hand-held TOPSI was demonstrated for the characterization of extracted small molecules and metabolites from the surface of mint and rosemary leaves.

47 OTHER INSTRUMENTATION↗

DOE OSTI2026

Accelerating Surface Radiation Content to Investigate the Impact of Radon Progeny on Superconducting Qubits

Ionizing radiation in the form of $α$, $β$, $γ$, and additional high-energy particles can induce decoherence via phonon and quasiparticle poisoning in superconducting qubits. Recent studies have explored this effect using cosmic rays or controlled radioactive sources held in the proximity of a qubit package, and have concluded that reductions in such ``external'' environmental radiation may benefit stable operation of qubit devices. However, the effect of long-lived, unstable daughters of $^{222}$Rn that ``plate out'' directly on device and packaging surfaces has not been as extensively explored. This plate-out process, well-known to the dark matter direct detection field, occurs throughout the fabrication and testing lifecycle of a device and (separately) its packaging, and produces a local source of $α$-decays which can remain active for decades. As this scales with chip area, understanding and managing this source of ionizing radiation is relevant for successfully scaling quantum computing architectures to larger numbers of qubits in a radiation-robust way. We present a setup capable of accelerating and enhancing radon daughter plateout by a factor of $7\times10^4$ over ambient, in order to study, \textit{in situ}, the impact of these events on superconducting qubits. We also provide outlook on the potential impact of this source of ionizing radiation on current and future qubit arrays.

Poudel, Sagar S. [South Dakota Sch. Mines Tech.]↗