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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Measurement of ambient radon progeny decay rates and energy spectra in liquid argon using the MicroBooNE detector

We report measurements of radon progeny in liquid argon within the MicroBooNE time projection chamber (LArTPC). The presence of specific radon daughters in MicroBooNE’s 85 metric tons of active liquid argon bulk is probed with newly developed charge-based low-energy reconstruction tools and analysis techniques to detect correlated Bi 214 − Po 214 radioactive decays. Special datasets taken during periods of active radon doping enable new demonstrations of the calorimetric capabilities of single-phase neutrino LArTPCs for β and α particles with electron-equivalent energies ranging from 0.1 to 3.0 MeV. By applying Bi 214 − Po 214 detection algorithms to data recorded over a 46-day period, no statistically significant presence of radioactive Bi 214 is detected, and a limit on the activity is placed at < 0.35 mBq / kg at the 95% confidence level. This bulk Bi 214 radiopurity limit—the first ever reported for a liquid argon detector incorporating liquid-phase purification—is then further discussed in relation to the targeted upper limit of 1 mBq / kg on bulk Rn 222 activity for the DUNE neutrino detector. Published by the American Physical Society 2024

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Removal of radon progeny from delicate surfaces

210 Po α-decay-driven neutron background is a concern for many rare event search experiments. It is a difficult to control background because its radiogenic component depends on the air exposure history of parts. In this study, we demonstrate that about half of the radon progeny 210 Po can be removed from copper and silicon surfaces relatively easily by wiping a copper sample with acetone-wetted tissue and a silicon detector with acetone soaked cotton balls. For a copper sample, we demonstrate that long-lived 210 Pb is removed with similar effectiveness. For copper, allocated the longest counting time, additional wiping was found to be largely ineffective. For silicon, the removal effectiveness has large uncertainties. Additional cleaning showed a small but statistically significant effect. Here, capitalizing on this trivial cleaning step will allow experiments to relax their requirements on the allowable air exposure time during construction, leading to cost and time savings.

Radioactivity↗
DOE OSTI2025

Utilization of traceable standards to validate plutonium isotopic purification and separation of plutonium progeny using AG MP-1M resin for nuclear forensic investigations

Radio-chronometric studies on plutonium (Pu) materials require independent measurement of the Pu (parent) content and isotopic distribution as well as concentration and isotopic distribution of the plutonium isotopic decay products. We performed a series of experiments to demonstrate the consistency of separations using the Lewatit MP 800 macroporous anion exchange resin and the AG MP-1M resin with traceable Pu isotopic certified reference material (CRM) standards 136, 137, 138, and 126-A. Two different mesh-sizes of the AG MP-1M resin were tested and the 50–100 mesh size resin was found to work more efficiently for the separation task. Both Lewatit and AG MP-1M resins were found to perform satisfactorily for quantitatively extracting the americium (Am) and uranium (U) progeny as well as gallium (Ga) present as a tracer in the Pu material. Both resins were effective in removing isobaric interferences from the Pu fraction used in isotopic measurements by thermal ionization mass spectrometry (TIMS). To address the co-elution of uranium and gallium, Alizarin red S (ARS) was used as a colorimetric dye to determine the behavior of UO 2 2+ and Ga 3+ on AG MP-1M resin with various acidic solutions as eluents using UV–vis spectra. Poor resolution of these peaks complicated quantitative analysis by UV–vis spectroscopy, but these results were informative in planning automated separation experiments by HPLC. LA-UR-24-28919.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2016

Electrical capacitance as a predictor of root dry weight in shrub willow ( Salix ; Salicaceae) parents and progeny

Premise of the study: Root biomass is an important trait often disregarded in woody perennial selection due to the challenge and expense of accurately and efficiently measuring large populations. In this study, we aim to develop a simple method that can predict root dry weight within a diverse shrub willow ( Salix ) breeding population representing species hybrids and their parents using root electrical capacitance (REC). Methods: The REC method was tested on plants started from cuttings and grown in pots with potting mix in the greenhouse for 11 wk to assess the relationship of REC with 24 biomass traits and its usefulness in allometric models for root and stem dry biomass. Results: Strong linear and positive correlations were found between REC and root dry biomass ( r = 0.88). The total proportion of variance of root and stem dry biomass explained by predictors in multiple regression was 85% and 69%, respectively. The relative importance of predictor variables in allometric models was dominated by the contribution of REC. Discussion: This work provides an efficient and nondestructive technique to indirectly quantify root biomass of genetically diverse shrub willow progeny, which has great promise for selection of genotypes with varying root biomass and for the accurate estimation of belowground carbon sequestration.

59 BASIC BIOLOGICAL SCIENCES↗
NASA NTRS2002

Nonhereditary enhancement of progeny growth

The im electroporated injection of a protease-resistant GH-releasing hormone cDNA into rat dams at 16 d gestation resulted in enhanced long-term growth of the F(1) offspring. The offspring were significantly heavier by 2 wk of age, and the difference was sustained to 10 wk of age. Consistent with their augmented growth, the plasma IGF-I concentration of the F(1) progeny was increased significantly. The pituitary gland of the offspring was significantly heavier and contained an increased number of somatotrophs and PRL-secreting cells, which is indicative of modification of cell lineage differentiation. These unique findings demonstrate that enhanced GH-releasing hormone expression in pregnant dams can result in intergenerational growth promotion by altering development of the pituitary gland in the offspring.

Non-NASA Center↗
DOE OSTI2024

Fractionation of UF6 and daughter progeny in storage cylinders from external heating

Abstract Uranium hexafluoride (UF 6 ) is a significant concern for material accountancy and verification in the international safeguards community. Verification of the contents of UF 6 cylinders is generally attempted with gamma spectroscopy but the current methods assume a uniform, homogeneous UF 6 mass distribution within the cylinder. In this work, it was found experimentally and confirmed via modeling, that under an external heat load (the sun), the UF 6 and its daughter products undergo fractionation in the cylinder. This fractionation of the UF 6 and daughter products can cause an errant measurement of the enrichment of the cylinder when using the current verification methods.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2017

Multiple Paternity Benefits Female Marbled Salamanders by Increasing Survival of Progeny to Metamorphosis

Abstract Multiple paternity occurs in most species and animal groups that have been studied. Because mating involves fitness costs to individual females, theory predicts that polyandrous females gain greater fitness benefits than costs, allowing the behavior to be maintained. Genetic, rather than material, benefits often occur in species where males provide females with little more than sperm and seminal fluid. We compared fitness correlates of single‐ and double‐sire clutches from female marbled salamanders ( Ambystoma opacum ) at the egg, hatchling, and metamorph stages of offspring development. Because clutches were collected from experimental breeding groups, strict paternity exclusion of offspring using microsatellite data allowed us to categorize each clutch as having either one or two fathers. Early offspring viability and size of hatchlings were not different between single‐ and multiple‐paternity clutches. Larvae from the two clutch types were allowed to develop together in field enclosures until metamorphosis. Although there was no difference in size at metamorphosis, survival to metamorphosis was significantly higher in multiple‐paternity clutches (44% vs. 40%) suggesting a benefit for females. The results were consistent with genetic benefits, although maternal effects could not be ruled out. The data did not support predictions of the genetic bet‐hedging and good sperm hypotheses for genetic benefits of polyandry.

Croshaw, Dean A.↗
DOE OSTI2014

Genetic and Epigenetic Changes in Chromosomally Stable and Unstable Progeny of Irradiated Cells

Radiation induced genomic instability is a well-studied phenomenon, the underlying mechanisms of which are poorly understood. Persistent oxidative stress, mitochondrial dysfunction, elevated cytokine levels and epigenetic changes are among the mechanisms invoked in the perpetuation of the phenotype. To determine whether epigenetic aberrations affect genomic instability we measured DNA methylation, mRNA and microRNA (miR) levels in well characterized chromosomally stable and unstable clonally expanded single cell survivors of irradiation. While no changes in DNA methylation were observed for the gene promoters evaluated, increased LINE-1 methylation was observed for two unstable clones (LS12, CS9) and decreased Alu element methylation was observed for the other two unstable clones (115, Fe5.0-8). These relationships also manifested for mRNA and miR expression. mRNA identified for the LS12 and CS9 clones were most similar to each other (261 mRNA), while the 115 and Fe5.0-8 clones were more similar to each other, and surprisingly also similar to the two stable clones, 114 and 118 (286 mRNA among these four clones). Pathway analysis showed enrichment for pathways involved in mitochondrial function and cellular redox, themes routinely invoked in genomic instability. The commonalities between the two subgroups of clones were also observed for miR. The number of miR for which anti-correlated mRNA were identified suggests that these miR exert functional effects in each clone. The results of this study demonstrate significant genetic and epigenetic changes in unstable cells, but similar changes almost equally common in chromosomally stable cells. Possible conclusions might be that the chromosomally stable clones have some other form of instability, or that some of the observed changes represent a sort of radiation signature for and that other changes are related to genomic instability. Irrespective, these findings again suggest that a spectrum of changes both drive genomic instability and permit unstable cells to persist and proliferate.

Baulch, Janet E.↗
NASA NTRS1974

The progeny of Skylab - The pioneering phase of our expansion into space

The opportunities provided by such near-earth space resources as the continuous view of the earth, sun, and stars, the presence of ultrahigh vacuum, and the absence of gravitational stress are briefly reviewed, along with the significance of manned observation and experimentation in near-earth space. The stimulation triggered in young minds by a week or summer in space, as the Apollo and Skylab experiences show, simply defies the imagination. The plea is made not to miss these opportunities.

Schmitt, H. H.↗
NASA NTRS2013

Rotational Variation of Daughter Species Production Rates in Comet 103P/Hartley: Implications for the Progeny of Daughter Species and the Degree of Chemical Heterogeneity

We present analysis of high spectral resolution optical spectra of Comet 103P/Hartley taken during its Fall 2010 apparition. These spectra include transitions belonging to CN, C2, CH, NH2, and OI. We measure production rates and mixing ratios from these spectra. We find evidence for large changes in production rates (factors of a few) over the course of a nucleus rotation, in agreement with other measurements. We also measure variability with rotational phase in the CN/H2O and C2/CN ratios, which has not been previously reported for any comet. There may also be variability in the NH2/H2O ratio with rotational phase, but this trend is not as clear as for CN/H2O. We interpret the changing mixing ratios as due to H2O and C2 being released primarily from the icy grain halo, while the CN parent molecule comes directly from the nucleus. There is evidence that the CH/CN ratio is higher pre-perihelion than post-perihelion. We conclude that the observed CN and NH2 abundances are consistent with HCN and NH3 being the dominant parent molecules for these species. The C2 and CH abundances are higher than those of candidate parent molecules (C2H2 and CH4 respectively), so there must be another source for these molecules in 103P's coma. Carbonaceous dust grains could serve as this source.

Comets↗
DOE OSTI2026

Accelerating Surface Radiation Content to Investigate the Impact of Radon Progeny on Superconducting Qubits

Ionizing radiation in the form of $α$, $β$, $γ$, and additional high-energy particles can induce decoherence via phonon and quasiparticle poisoning in superconducting qubits. Recent studies have explored this effect using cosmic rays or controlled radioactive sources held in the proximity of a qubit package, and have concluded that reductions in such ``external'' environmental radiation may benefit stable operation of qubit devices. However, the effect of long-lived, unstable daughters of $^{222}$Rn that ``plate out'' directly on device and packaging surfaces has not been as extensively explored. This plate-out process, well-known to the dark matter direct detection field, occurs throughout the fabrication and testing lifecycle of a device and (separately) its packaging, and produces a local source of $α$-decays which can remain active for decades. As this scales with chip area, understanding and managing this source of ionizing radiation is relevant for successfully scaling quantum computing architectures to larger numbers of qubits in a radiation-robust way. We present a setup capable of accelerating and enhancing radon daughter plateout by a factor of $7\times10^4$ over ambient, in order to study, \textit{in situ}, the impact of these events on superconducting qubits. We also provide outlook on the potential impact of this source of ionizing radiation on current and future qubit arrays.

Poudel, Sagar S. [South Dakota Sch. Mines Tech.]↗
DOE OSTI2016

The long-term effects of acute exposure to ionising radiation on survival and fertility in Daphnia magna

The results of recent studies have provided strong evidence for the transgenerational effects of parental exposure to ionising radiation and chemical mutagens. However, the transgenerational effects of parental exposure on survival and fertility remain poorly understood. To establish whether parental irradiation can affect the survival and fertility of directly exposed organisms and their offspring, crustacean Daphnia magna were given 10, 100, 1000 and 10,000 mGy of acute γ-rays. Exposure to 1000 and 10,000 mGy significantly compromised the viability of irradiated Daphnia and their first-generation progeny, but did not affect the second-generation progeny. The fertility of F{sub 0} and F{sub 1}Daphnia gradually declined with the dose of parental exposure and significantly decreased at dose of 100 mGy and at higher doses. The effects of parental irradiation on the number of broods were only observed among the F{sub 0}Daphnia exposed to 1000 and 10,000 mGy, whereas the brood size was equally affected in the two consecutive generations. In contrast, the F{sub 2} total fertility was compromised only among progeny of parents that received the highest dose of 10,000 mGy. We propose that the decreased fertility observed among the F{sub 2} progeny of parents exposed to 10,000 mGy is attributed to transgenerational effects of parental irradiation. Our results also indicate a substantial recovery of the F{sub 2} progeny of irradiated F{sub 0}Daphnia exposed to the lower doses of acute γ-rays. - Highlights: • Viability of irradiated daphnids and their F{sub 1} progeny is compromised. • Viability of the F{sub 2} progeny of irradiated parents is not affected. • Total fertility of irradiated daphnids and their F{sub 1} progeny declines with the dose. • Total fertility of the F{sub 2} progeny of parents exposed to 10,000 mGy is compromised. • The decreased fertility among the F{sub 2} progeny is transgenerational phenomenon.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Environmental Characterization Scans Using Sodium-Iodide Gamma Spectroscopy to Determine Ra-226 Concentration in Surface Soil - 16326

The recent natural gas drilling boom has brought heightened attention to the issue of TENORM waste management. Radioactive residues from the extraction, treatment, and purification of materials containing uranium and thorium, or their progeny, pose a public health hazard primarily in the form of ground water contamination. Hydraulic fracturing can liberate formation waters from shale; the high salinity of which can cause radium to move with the water to the surface. The disposal and handling of this water has been a subject of public controversy. For soil remediation projects, radium-226 is generally one of the radionuclides of concern due to its alpha emissions. However performing a survey scan for Ra-226 is difficult because its photon emissions are low energy and have minimal probability of emission per decay (186.2 keV, 3.3% abundance). Additionally resolving its emission from U-235 (185.7 keV, 57% abundance) with field instrumentation is not feasible. Therefore detection of Ra-226 relies on the presence and photon emissions of its progeny. This paper outlines methodology for calculating the minimum detectable concentration of Ra-226 in characterization scans using a sodium-iodide detector array coupled with a multi-channel analyzer. Using progeny ingrowth as a detection proxy requires knowing decay time in order to determine progeny emission rates. Knowledge of site history, process, and prior survey results can be key in determining an accurate decay time. However in the absence of such information in-situ measurements can be used to estimate decay time by comparing observed progeny emission ratios against established values. These values are determined using Oak Ridge National Laboratory's ORIGEN-ARP program to generate photon energy spectra for Ra-226 and its progeny at specified time intervals. Once decay time is established, the detector's minimum detectable concentration can be calculated by synthesizing the expected emission spectra and Los Alamos National Laboratory's Monte Carlo N-Particle transport code to simulate detector response. Traditionally, one of the steps in calculating a system's minimum detectable concentration is to place an appropriate button source under the detector, record the response, and then move the source by a specified increment. This process is repeated until the detector's spatial efficiency has been mapped. Due to the impracticality of performing this with Ra-226 button sources of varying decay times, Monte Carlo N-Particle transport code was utilized to determine the detector's spatial efficiency. A dime sized source with the established emission spectra was placed into the center of a rectangle of soil. This rectangle, including the source, was used as a lattice element to fill the region of space below the detector. The simulation was designed to track the energy distribution of pulses created in the sodium iodide crystal using the F8 tally, and was setup to isolate each source; thereby correlating detector response to source position. The simulation output required post-processing to determine conversion factors from counts per second to disintegrations per second. Post-processing accounted for subtraction of the Compton continuum, and average the data over the scanning pattern to obtain the expected spatial sensitivity during a characterization study. This was performed for the following photo-peaks: 609 keV (Bi-214), and 1764 keV (Bi-214). For calculation of the scan minimum detectable concentration, the surveyor efficiency coefficient from NUREG 1507 was supplanted in favor of a scan speed deviation factor. This was used because the detector utilizes computerized data collection (spatial and spectral). This report finds that, for two shielded 10.16 cm x 10.16 cm x 40.64 cm sodium-iodide crystals with integrated multi-channel analyzers, the minimum detectable concentration in surface soils is less than 1 pCi per gram Ra-226 for a 1 second survey measurement. These results assume a volumetric source with a maximum depth of 15.24 cm and a minimum decay time of 21 days. Verification of the system's capabilities was performed by sending soil samples from scanned areas, and locations where in-situ measurements were performed, to an independent laboratory for analysis. The laboratory results demonstrated that scanned area was principally comprised of soil containing less than 1 pCi per gram Ra-226. This borders the system MDC and it underestimated the concentration of radium in the soil. The probable causes of this is escape of radon gas from the surface soil. Radon is the daughter of radium, and has a high mobility in soil. If the gas escapes, then the progeny used as the detection proxy will be present in lower than expected concentrations. Radionuclide identification using high volume sodium-iodide crystals in low level characterization scans is demonstrated to be possible. Further system refinement will focus on developing a methodology to estimate a radon escape factor for site specific use. Accounting for radon escape in the top 15.24 cm of soil will allow the system to better estimate Ra-226 concentrations in soil. This is a significant advancement over the gross counting statistics used in most studies to satisfy MARSSIM survey requirements, because it will increase stakeholder confidence. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗
DOE OSTI2018

Preliminary Work Toward a Transuranic Activity Estimation Method for Rapid Discrimination of Anthropogenic from Transuranic Activity in Alpha Air Samples

Radon ( 222 Rn) and thoron ( 220 Rn) progeny (primarily bismuth and polonium) are known interferents when rapid evaluation of transuranic content on air filters is of interest. These complexities stem from the overlapping energies of the progeny alpha particles onto the transuranic region of interest (3–5.5 MeV) where naturally-occurring alpha emitters can overwhelm the spectra. Due to the immediacy of the alpha counting methods employed, coupled with the half-life of thoron progeny dominated by 212 Pb (t 1/2 =10.6 h), a conservative transuranic activity estimate with rigorous uncertainty is being sought. A successful transuranic activity estimation method will incorporate any thoron progeny present on the filter providing 95% confidence decision levels in which a filter may be evaluated for emergency response applications. Twenty-three pairs of samples of various duration having no transuranic content were taken over a 2-mo period. The resulting filters were counted in a time series before non-linear least squares decay curve fitting was applied to the decay profile. For the samples considered, a transuranic activity estima-tor decision level was determined at 0.2 Bq for the given geographic location and months analyzed. In conclusion, validation of this method for other seasonal and geographic regions could provide enhanced emergency response capability when the presence of transuranic activity is suspected.

54 ENVIRONMENTAL SCIENCES↗