Standoff analysis of laser-produced plasmas using laser-induced fluorescence
Not Available
Harilal, S. S. (ORCID:0000000322667976)↗
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Results for “PLASMA”
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
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Cold plasma interactions with plants: Morphing and movements of Venus flytrap and Mimosa pudica induced by argon plasma jet
Not Available
Volkov, Alexander G.↗
Interferometry of plasma bursts in helium atmospheric-pressure plasma jets
Not provided.
Materials Science↗
Observation of the plasma boundary layer at lunar distances - Direct injection of plasma into the plasma sheet
The paper presents observational evidence from the Apollo suprathermal ion detector experiments that the injection of magnetosheath particles at the low-latitude magnetopause operates at lunar distances as well. An interface between the magnetosheath and the plasma sheet, termed the plasma sheet boundary layer (PSBL), is identified and believed to be the extension of the magnetospheric boundary layer (also called the plasma boundary layer) observed on the dayside. Using measurements of the PSBL's thickness, magnetic field, and plasma velocity the average electric potential drop across the PSBL is estimated at 4.2 kV and compared with the potential drop which is needed to insure that the magnetopause is an equipotential for a closed magnetosphere. It was concluded though that the magnetosphere is open since this drop is much larger than 4.2 kV.
Sanders, G. D.↗
Production of superheated hydrogen plasma using induction heating of cold plasma and dc plasma enhancement
Production of superheated hydrogen plasma by induction heating of cold plasma and direct current plasma enhancement
HYDROGEN PLASMA↗
Ionospheric plasma flow over large high-voltage space platforms. I - Ion-plasma-time scale interactions of a plate at zero angle of attack. II - The formation and structure of plasma wake
The paper presents the theory and particle simulation results for the ionospheric plasma flow over a large high-voltage space platform at a zero angle of attack and at a large angle of attack. Emphasis is placed on the structures in the large, high-voltage regime and the transient plasma response on the ion-plasma time scale. Special consideration is given to the transient formation of the space-charge wake and its steady-state structure.
Wang, J.↗
Plasma Wall Interaction with 3-D Plasma Boundaries
The interaction of the edge plasma and the material surfaces is one of the most critical challenges on the path to harness fusion power as new, fundamental energy source. This challenge typically combines the thrust to reach high density, low temperature (detached) plasmas in front of the divertor target plates as well as understanding the plasma material interaction (PMI) in particular in this regime. The combination of both research thrusts represents an extraordinarily challenging subject encompassing spatial scales spanning nanometers to meters in all states of matter and across a broad energy range. Modeling capabilities, which help to interpret data from nowadays experiments and enable extrapolation to future devices are urgently required. This is in particular true for toroidal magnetic confinement devices with three-dimensional (3D) plasma boundaries. Such plasma boundary geometries occur in tokamaks, when small amplitude magnetic perturbations are used to stabilize the unruly edge plasma or in stellarators, that are inherently 3D plasma confinement devices. In this project, the impact of 3D plasma boundaries on the plasma material interaction (PMI) was assessed. This work focused on plasma boundary conditions, in which high-density conditions at the material surfaces yield mitigation of the otherwise immense heat and particle loads that these materials would see. These so-called high recycling and eventually detached plasma regimes are of great interest for future reactor operation. In the project, key features that are unique to 3D boundaries were explored in comparison to canonically assumed axisymmetric plasma edge situations in tokamaks. In particular, the relevance of the 3D boundary situation in the extrapolation to the plasma boundary solution at ITER, the next step fusion energy experiment under construction as a multi-national, world-wide large-science experiment in southern France, has been explored. The EMC3-EIRENE plasma edge fluid and kinetic neutral transport code has been advanced to cope with the challenging and unprecedented conditions in the ITER boundary plasma including 3D fields that are planned to be used to suppress harmful edge instabilities, the so-called edge localized modes. This is a vital integration challenge for ITER and the results from this grant have provide a leading capability for this assessment. It was shown that the detachment process in a 3D edge solution for ITER follows the recycling regimes that are known from axisymmetric solutions, but that multiple plasma exhaust channels connected to the material surfaces are established which feature individual recycling characteristics. Because these channels touch the material surfaces in the divertor in a 3D geometry, the compatibility with the plasma material interaction (PMI), including erosion and impurity generation has been found to be an important part of the integration challenge. To address this, the fully 3D plasma material interaction code ERO2 has been adapted to these ITER specific geometries and a homogeneous mixing model was implemented, that allows to consider the mixing of Be and Was used at ITER in the PMI modeling. This model enhancement has been used to study non-local migration of Be in the JET ITER like wall configuration and it has been shown that with this model such complex migration processes in ITER relevant plasma shapes and with ITER relevant plasma boundary conditions can be addressed. The combined modeling approach using EMC3-EIRENE as a plasma boundary transport code and the ERO2 specialized PMI model will be an asset for the continued preparations of ITER operation as well as for Fusion Pilot Plant efforts that have emerged in the U.S. during the evolution of this grant. The predictive capability of this numerical tool has been validated at the DIII-D US national fusion facility. Here, dedicated plasma edge diagnostics were implemented to measure the impurity household around a 3D edge plasma during ELM suppression by 3D fields. Dedicated experiments with local material probes using these diagnostics and the state-of-the-art suite of boundary measurements at DIII-D have shown that the 3D perturbation of the plasma edge that is excreted by such 3D control fields yield a perturbation of the plasma boundary flux structure and hence also of the resulting PMI. The 3D boundary plasma is composed out of helical magnetic flux channels that intersect the divertor targets at an angle relative to the main guiding field, i.e., the toroidal magnetic field component of the tokamak. A similar effect has been measured as well on limiter surfaces during the startup campaign at the new stellarator experiment Wendelstein 7-X. These experiments ad initial analysis with the ERO plasma material interaction model, suggested that the place of erosion for a given particle from the surface and its re-deposition can be different in such 3D field geometries yielding potentially a significant level of net-erosion. This is not the case for axisymmetric solutions, where it was shown in the past that the eroded particles are effectively re-deposited into gaps produced by erosion at the same position and hence the net-erosion levels are small. For ITER, the quest to suppress the ELMs and at the same time maintain the integrity of the divertor is an issue, which these fundamental findings will help to resolve. The coupling of this work to the extrapolation in the ITER program has been addressed by both the PI and the lead numerical scientist being ITER Science Fellows in the duration of the contract and forward. A second focus in the exploration of 3D boundary effects on tokamaks and stellarators has been set on the measurement of helium exhaust features with such 3D fields. This is important because He represents the ash of the fusion process and needs to be exhausted. It was shown that 3D field application compatible with suppression of ELMs yields an increase of the helium exhaust performance. The ratio of the effective helium confinement time over the energy confinement time was reduced by almost 50% which demonstrated that the impact of helium accumulation in the plasma core with respect to the confinement of energy to sustain the fusion reaction is significantly improved with such 3D control fields. It was shown that this is the case for tokamaks as well as stellarators. At the Large helical Device in Japan, a similar enhancement of the helium exhaust features when small amplitude additional 3D fields were applied was measured. This is an important additional function of 3D field application and its impact on ITER is presently being studied in combination with investigations of helium exhaust in 3D field geometries of stellarator devices.
3D plasma edge transport↗
Dynamics and chemical mode analysis of plasma thermal-chemical instability
The stability of the weakly ionized plasma and the transition from a stable homogeneous discharge to unstable filaments play an important role in gas laser physics, plasma-assisted combustion, chemical reforming, and material synthesis. Here, theoretical stability analysis and thermal-chemical mode analysis were performed to understand the mechanism of plasma thermal-chemical instability by using a zero-dimensional plasma system with both simplified and detailed chemical kinetics of H 2 /O 2 /N 2 mixtures. The plasma dynamic and kinetic models accounted for multiple physical mechanisms in the chemically-reactive weakly ionized plasma, including ionization, attachment/detachment, recombination, vibrational and electronic energy relaxation, convective and diffusive species/heat removal, Joule heating, and detailed chemical kinetics. An analytical criterion and the explosive mode species/temperature pointers were formulated while the representative active species were identified for different thermal-chemical modes. The results showed that in addition to the classical thermal-ionization mechanism, various chemical modes from chemical heat imbalance and elementary kinetics significantly modified the time dynamics and the stability of the weakly ionized plasma. The present analysis provides insights and guidance to control plasma instability using chemical kinetics.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Controlled plasma–droplet interactions: a quantitative study of OH transfer in plasma–liquid interaction
Plasmas in contact with liquids are a rich source of OH radicals and have been extensively studied in the last decade to leverage the ability to generate chemically reactive species in gas phase plasmas to decompose organics. Multiphase transfer of OH radicals is highly transport limited and to overcome transport limits, the plasma activation of aerosols, small liquid droplets, interspersed in the plasma has been proposed. In this work, we report a combined experimental and modeling study of a controlled plasma–droplet interaction experiment using a diffuse RF glow discharge in He + 0.2% H 2 O with detailed plasma diagnostics, ex situ analysis of the plasma-induced chemistry in the droplet containing formate, droplet trajectory and size measurements. This enables a quantitative study of the reactivity transfer of OH from the gas phase plasma to the liquid phase and how its diffusion limitations impact formate decomposition in the water droplet. For a droplet with a diameter of 36 μm, we observed 50% reduction in formate concentration in the droplets after plasma treatment for droplet residence times in the plasma of ~10 ms. These short droplet residence times in the plasma allow in some cases for droplet size reductions of ~5% in spite gas temperatures of 360 K. A one-dimensional reaction–diffusion model was used to calculate the OH transport and formate oxidation inside the droplet and was able to predict the conversion of formate by plasma in a droplet without any fitting parameters. The model further shows that formate conversion is dominated by near-interfacial reactions with OH radicals and is limited by diffusion of formate in the droplet. Here, the results show that a controlled plasma–micro-droplet reactor as reported in this study might be an excellent tool for detailed quantitative plasma–liquid interaction studies.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Active Measurement of Plasma Parameters in Over-Dense MFE Reactor Plasma Using High Frequency Beat-Wave Resonantly Generated Thermal Bernstein Waves
UC Davis was funded to explore the combination of beat-wave excitation and laser scattering to make completely non-invasive determination of local plasma conditions. This involves the use of two high frequency mm-wave sources of differing frequencies (the pump waves) to excite plasma waves at the difference of the frequencies, which is known as the beat frequency. The difference frequency or the frequency of the beat wave is chosen so that we produce plasma waves whose fluctuating electron density is a sensitive function of plasma parameters at the location where the source waves overlap. This fluctuation can be detected from outside the plasma, by measuring the deflection of a probe beam directed at the overlap region between the two pump waves (i.e., collective scattering). This work is an extension of mm-wave frequencies of a 10 GHz beat-wave experiment conducted on the DDT toroidal device (see Fig. 1) in a magnetized plasma where the excited Langmuir wave is replaced by the magnetized upper hybrid wave. Here, two high power (> 1 kW) ~94 GHz pump sources will be employed to match the upper hybrid resonance. The primary envisioned experiment is to drive the electron Bernstein wave (EBW) in the interior of a magnetized plasma. The EBW is a hot-plasma electrostatic wave, which cannot propagate in vacuum. Roots of the EBW dispersion relation occur at frequencies slightly higher than harmonics of the electron cyclotron frequency. Use of the EBW has particular advantages for measuring plasma magnetic field in plasmas with relatively high density and low magnetic field, as is the case in spherical tokamaks. This is the “over dense” condition of future efficient high beta magnetic confinement fusion reactors such as the spherical tokamak (STs). The overarching goal of the proposed project is to demonstrate beat wave EBW excitation in low density and temperature parameters that are directly scalable to over-dense spherical tokamaks such as NSTX or MAST, where measurement of magnetic field by electron cyclotron emission (ECE) is experimentally complex, and requires models of plasma profiles in order to interpret results. In such experiments, availability of point measurements of magnetic field strength provided by a beat-wave diagnostic would serve as a powerful independent check on the ECE results, serving to validate the assumed profiles and wave-propagation models used. The first step was to assemble/modify the target chamber in which the beat-wave plasma experiments will take place. Here, the target chamber of the CTIX compact-toroid (spheromak) injector was chosen. At the time that the proposal was submitted, the aim was to conduct the experiments in the CTIX experimental facilities located at the Livermore campus of UC Davis using microwave/mm-wave equipment brought from the main campus., However, by the time DoE funds for this project were awarded, the CTIX experimental facilities located at the Livermore campus of UC Davis were in the process of being shut down due to the closure of the Livermore campus by Lawrence Livermore National Laboratory (LLNL). Consequently, the equipment needed for this project was crated up and shipped from Livermore to Davis as part of the laboratory shutdown after space on campus was secured and College of Engineering approval secured. Once it arrived in Davis on December 20, 2018, work on the project began in earnest with the initial efforts directed toward developing a new plasma target source. Because of the shutdown of the CTIX facility, the scope of the project thus had to be reduced due to the abbreviated amount of time allocated to the project once the shutdown/move had been completed. Chamber modifications have been completed, including the fabrication and installation of a 38 GHz interferometer, as described in Sec. 3. The thermionic plasma source has been tested and characterized. The magnetic field required for the EBW experiments will be generated by permanent magnets mounted on plates positioned above and below the chamber. Magnetic simulations have been performed, and show that a 3-ring magnet arrangement on each plate, with a plate separation of 50 cm, is required to achieve the ~100 G uniform magnetic field in the interaction region that we feel is necessary to ensure good EBW coupling. We proved unable to successfully revive either of Prof. Luhmann’s two high power (≥20 kW) 94 GHz millimeter-wave sources after their extended time in storage and decided to postpone further efforts and concentrate on slightly lower power sources. Consequently, we were successful in reviving a ~2 kW extended klystron amplifier (EIK), which together with a ~2 kW extended interaction oscillator (EIO) will provide the two pump sources required for the project. Safe operation of the EIO requires extensive modifications to one of Prof. Luhmann’s pulse modulators - these modulator modifications are ongoing, which has unfortunately delayed the planned beat-wave experiments. Details of this work are provided in Sec. 3. Even though project funding has now ended, we still plan to proceed to complete the EIO pulse modulator modifications, install the two ~94 GHz pump wave sources on the target chamber, and conduct unmagnetized tests of the beat-wave concept which involve coupling to unmagnetized electron plasma waves rather than magnetized EBWs. Should these experiments prove successful, we plan to submit a follow-up proposal for additional funding which would allow us to undertake the magnetized EBW experiments.
42 ENGINEERING↗
Ion Fluxes and Neutral Gas Ionization Efficiency of the 100-kW Light-Ion Helicon Plasma Source Concept for the Material Plasma Exposure eXperiment
Linear plasma devices are cost-effective alternatives for testing materials under reactor-relevant divertor plasma conditions. In this work, we describe how an intense radio-frequency (RF) plasma source concept for the Material Plasma Exposure eXperiment (MPEX) is under development at Oak Ridge National Laboratory. The source concept, Proto-MPEX, aims to produce high-density background deuterium helicon plasmas ( n e > 3 × 10 19 m - 3 ) that are subsequently heated with additional RF and microwave systems to deliver reactor-relevant conditions for studies on plasma-material interaction. In this work, we focus on the plasma-producing stage and its effectiveness in converting input neutral gas into plasma, namely, the neutral gas ionization efficiency. We provide a direct quantitative measurement of the ionization efficiency by measuring the total ion flux arriving at the target region relative to the neutral gas injected at the source. Using 80 kW at 13.56 MHz and a source magnetic field of 0.05 T, the helicon plasma source delivers ion fluxes up to 1 × 10 24 m - 2 s - 1 and heat fluxes greater than 1 M W m - 2 to a target plate located 2 m away from the source. Under these conditions, we observe that the plasma source converts ~89% of the input neutral gas into plasma that arrives at the target as ion flux at a rate of 5 × 10 20 s - 1 . We demonstrate that because of the large pumping capacity of the plasma, neutral gas pumping systems are required only in the target region to maintain optimal plasma operation.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Infrared studies of gas phase and surface processes of the enhancement of catalytic methane decomposition by low temperature plasma
Catalyst enhancement by atmospheric pressure plasma is a recently emerging field of research that embodies a complex system of reactive species and how they interact with surfaces. In this work we use an atmospheric pressure plasma jet integrated with a nickel on Al 2 O 3 /SiO 2 support catalyst material to decompose methane gas by partial oxidation reaction. We use Fourier-transform Infrared spectroscopy (FTIR) analysis of the gas phase post reaction to measure the loss of methane and the production of CO, CO 2 , and H 2 O and diffuse reflectance Fourier-transform Infrared spectroscopy (DRIFTs) in situ analysis of the catalyst surface as a function of both catalyst temperature and plasma operating parameters. We find reduction of methane by both plasma alone, catalyst alone, and an increase when both plasma and catalyst were simultaneously used. The production of CO appears to be due primarily to the plasma source as it only appears above 2.5 W plasma dissipated power and decreases as catalyst temperature increases. CO 2 production is enhanced by having the catalyst at high temperature and H 2 O production depends on both plasma power and temperature. Using DRIFTs we find that both heating and plasma treatment remove absorbed water on the surface of the catalyst. Plasma treatment alone however leads to the formation of CO and another IR spectral feature at 1590 cm -1 , which may be attributed to carboxylate groups, bonded to the catalyst surface. These species exhibit a regime of plasma treatment where they are formed on the surface and where they are significantly removed from the catalyst surface. We see the formation of a new spectral feature at 995 cm -1 and discuss the behavior and possible origins of this feature. Furthermore, this research highlights the potential for plasma regeneration of catalyst materials as well as showing enhancement of the catalytic behavior under low temperature plasma treatment.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Classical trajectory Monte Carlo simulation of plasma fueling using magnetic plasma expulsion
The possibility of fueling a magnetically confined plasma using particle sources located inside of the plasma is studied by computer simulation. Magnetic plasma expulsion [R. E. Phillips and C. A. Ordonez, Phys. Plasmas 25, 012508 (2018)] would serve to keep the magnetically confined plasma away from the particle sources without adversely affecting plasma confinement. The simulations show how charged particles can be injected into a plasma by using particle sources located directly between two current-carrying wires that create a magnetic expulsion field. Plasma fueling with the average energy of injected particles greater than the average energy of plasma particles may serve for heating the plasma. Also, plasma fueling with positive and negative particles injected at different rates may serve for changing the neutrality of the plasma. Conditions for plasma fueling are investigated using a classical trajectory Monte Carlo simulation. Two types of particle sources are considered, and the fraction of emitted particles that reach (and fuel) the magnetically confined plasma is evaluated for each.
71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
Laser cooling of ions in a neutral plasma
Laser cooling of a neutral plasma is a challenging task because of the high temperatures typically associated with the plasma state. By using an ultracold neutral plasma created by photoionization of an ultracold atomic gas, we avoid this obstacle and demonstrate laser cooling of ions in a neutral plasma. After 135 microseconds of cooling, we observed a reduction in ion temperature by up to a factor of four, with the temperature reaching as low as 50(4) millikelvin. This pushes laboratory studies of neutral plasmas deeper into the strongly coupled regime, beyond the limits of validity of current kinetic theories for calculating transport properties. The same optical forces also retard the plasma expansion, opening avenues for neutral-plasma confinement and manipulation.
Science & Technology - Other Topics↗
Ground-Based Simulation of Low-Earth Orbit Plasma Conditions: Plasma Generation and Characterization
A 16-cm diameter plasma source operated on argon is described that is capable of producing a plasma environment that closely simulates the low Earth orbit (LEO) conditions experienced by satellites in the altitude range between 300 to 500 km. The plasma source uses a transverse-field magnetic filter, and has been successful in producing low electron temperature plasmas that contain streaming ion populations. Both of these characteristics are important because the plasma in LEO is relatively cold (e.g., Te approx. 0.1 eV) and the ram energy of the ions due to the motion of the satellite relative to the LEO plasma is high (e.g., 7,800 m/s which corresponds to approx. 5 eV for O+ ions). Plasma source operational conditions of flow rate and discharge power are presented that allow the electron temperature to be adjusted over a range from 0.14 to 0.4 eV. The expanding plasma flow field downstream of the source contains both low-energy, charge-exchange ions and streaming ions with energies that are adjustable over a range from 4 eV to 6 eV. At low flow rates and low facility pressures, the streaming ion component of the ion population comprises over 90% of the total plasma density. In the work described herein, a large area retarding potential analyzer was used to measure both electron and ion energy distribution functions in the low density, expanding plasma produced downstream of the plasma source. The benefits of using this type of plasma diagnostic tool in easily perturbed, low-density plasma are identified, and techniques are also discussed that can be used to perform real-time measurements of electron temperature. Finally, recommendations are made that may enable lower electron temperatures to be produced while simultaneously decreasing the plasma source flow rate below 1 to 2 sccm.
Williams, John D.↗
Plasma-Coupled Flow Reactor Studies of Low-Temperature Plasma Assisted Kinetics of Methanol Blended with CO2
Ignition technologies based on low-temperature plasmas (LTP) have the potential to operate next generation engines at elevated pressures and increased dilution limits promoting higher efficiencies. From a practical standpoint, research on LTP igniters has shown to enhance combustion and ignition, improve flame stability, and extend the dilution limits of combustion. All of the aforementioned gains are complemented with higher ignition efficiencies. However, the biggest challenge with incorporating this technology into engines is the knowledge gap of how exactly plasma chemistry effects can enhance the basic combustion phenomena. This coupled with the lack of validated kinetic mechanisms for plasma-combustion chemistry is the biggest obstruction to recognize efficient ignition, especially for application relevant fuels and biofuels. In order to comprehensively evaluate the effects of LTP on an oxygenated fuel specific system, this present study examines the kinetics of methanol plasma-assisted pyrolysis and oxidation using a custom-built plasma flow reactor (PFR). Experimental regimes are also further extended to understand the effects of adding CO2 to the mixture and its consequence on reaction kinetics. The PFR is installed with a dielectric-barrier discharge (DBD) configuration to induce LTP into the fuel mixture. Non-equilibrium plasmas are generated by high-voltage pulses (nearing 20 KV) administered by a plasma pulser at high-pulse repetition rates (up to 10 kHz). In order to better understand and isolate plasma chemistry and its effect on neutral chemistry, the experiments were carried out by heavily diluting reactive mixtures in nitrogen at near isothermal conditions. This suppresses the effect of exothermic reactions on chemistry allowing stable intermediates and products to be detected and quantified using ex-situ GC/MS diagnostic methods. Experiments were carried out at 0.5 atm pressure and over a wide range of temperatures from 523 K to 1203 K. Experimental results depicted the enhancement in intermediates production as well as overall lower temperatures required for complete fuel consumption in the plasma specific cases as opposed to their pure thermal counterpart. Formation of oxygenated and nitrile compounds specific to plasma assisted pyrolysis cases illustrated the efficacy of LTP to introduce new reaction pathways accelerating fuel decomposition. Increase in reactivity at lower temperatures is sought to be an effect induced by plasma chemistry postulating the acceleration in intermediates production. The onset of thermal ignition in plasma assisted oxidation is seen 200 K earlier than thermal oxidation highlighting efficient fuel conversion to final byproducts. Enhanced collisional processes afforded by LTP is seen to perturb reaction pathways between oxygenated fuel radicals and N-atoms to alter overall chemical reactivity. New insights into kinetics are gained from this study highlighting governing plasma assisted combustion (PAC) pathways for oxygenated fuel reaction chemistry. The results from this study can be used to develop future mechanisms specific to plasma chemistry which can bridge the mechanistic knowledge gap for LTP ignition so that future engines can adopt LTPs in their design for efficient combustion.
32 ENERGY CONSERVATION, CONSUMPTION, AND UTILIZATI↗
Effect of hydrogen isotope on plasma impedance and thermal pinching induced by single aerosol droplets injected into an inductively coupled plasma
The mass of the hydrogen isotope in micrometer-sized aqueous droplets introduced into an ICP has been found to affect the degree of resulting plasma perturbation. Studied plasma perturbations include local plasma cooling, plasma shrinkage due to thermal pinching, and changes in plasma impedance. The local cooling effect caused by a vaporizing aerosol droplet was found to be similar between H 2 O and D 2 O. This finding is likely a result of the similar heat capacities and vaporization rates of H 2 O and D 2 O droplets and of the comparable thermal conductivities and dissociation kinetics of H 2 O and D 2 O vapor. In contrast, a clear isotope effect was observed for plasma shrinkage and impedance change, with H 2 O causing a considerably stronger effect. Plasma shrinkage, gauged by the reduction in Ar emission at the edge of the plasma, was detected at all observation heights within the load-coil region, with D 2 O droplets causing as much as 30% less of an effect than H 2 O. Likewise, D 2 O droplets induce significantly less change in plasma impedance than H 2 O droplets. Depending on experimental conditions and the probing method, changes in plasma impedance caused by monodisperse D 2 O droplets were only 52%–80% that of H 2 O. The lower influence on plasma shrinkage and impedance change for D 2 O droplets is believed to be related to the much lower thermal conductivity of atomic deuterium, around 70% that of atomic hydrogen (protium). The time required for the plasma impedance to return to its original steady-state value was comparatively long (~10 ms) and similar for H 2 O and D 2 O droplets.
70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
Perspectives on Machine Learning-assisted Plasma Medicine: Towards Automated Plasma Treatment
Cold atmospheric plasmas (CAPs) have shown great promise for medical applications through their synergistic chemical, electrical, and thermal effects, which can induce therapeutic outcomes. However, safe and reproducible plasma treatment of complex biological surfaces poses a major hurdle to the widespread adoption of CAPs for medical applications. Predictive modeling of the mutual interactions between the plasma and biological surfaces and, thus, systematic approaches to quantify and predict plasma treatment outcomes remain largely elusive due to the lack of mechanistic understanding of plasma-surface interactions that can span across vastly different length-and time-scales. In addition, real-time sensing capabilities in biomedical CAP devices are often limited, which can be detrimental to plasma treatment due to the intrinsic plasma and surface variability during the treatment, as well as sensitivity to external perturbations. All of these challenges can make reproducible and effective plasma treatment of biological surfaces difficult to realize, which is further compounded by errors due to human operation of hand-held CAP devices. Machine learning and data-driven approaches can be particularly useful in addressing these challenges in three major ways: (i) data-driven modeling of hard-to-model plasma-surface interactions and plasma treatment outcomes; (ii) learning data analytics for plasma and surface diagnostics in real-time; and (iii) developing predictive controllers that enable reliable and effective CAP treatments. Furthermore, this paper discusses the promise of machine learning to accelerate plasma medicine research in these areas, toward machine learning-assisted and automated CAP treatment of complex biological surfaces.
60 APPLIED LIFE SCIENCES↗