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At least 37 records · Page 2

Plasmon mediated coherent population oscillations in molecular aggregates

The strong coherent coupling of quantum emitters to vacuum fluctuations of the light field offers opportunities for manipulating the optical and transport properties of nanomaterials, with potential applications ranging from ultrasensitive all-optical switching to creating polariton condensates. Often, ubiquitous decoherence processes at ambient conditions limit these couplings to such short time scales that the quantum dynamics of the interacting system remains elusive. Prominent examples are strongly coupled exciton-plasmon systems, which, so far, have mostly been investigated by linear optical spectroscopy. Here, we use ultrafast two-dimensional electronic spectroscopy to probe the quantum dynamics of J-aggregate excitons collectively coupled to the spatially structured plasmonic fields of a gold nanoslit array. We observe rich coherent Rabi oscillation dynamics reflecting a plasmon-driven coherent exciton population transfer over mesoscopic distances at room temperature. This opens up new opportunities to manipulate the coherent transport of matter excitations by coupling to vacuum fields.

74 ATOMIC AND MOLECULAR PHYSICS↗

Magnetic field imaging in a laboratory plasma

In laboratory plasmas, arrays of probes have typically been used to measure the evolution of the magnetic field topology. Here, we present initial image-based measurements of the magnetic topology in a low-temperature plasma using a purely optical diagnostic. Laser induced fluorescence measurements of neutral velocity distribution functions are made using a fast camera, imaging the Zeeman splitting of σ-peaks in neutral argon. The separation of σ-peaks provides spatially resolved magnetic field magnitude measurements with a detection threshold on the order of 10 G

36 MATERIALS SCIENCE↗

System-on-chip approach microwave imaging reflectometer on DIII-D tokamak

System-on-chip millimeter wave integrated circuit technology is used on the two-dimensional millimeter-wave imaging reflectometer (MIR) upgrade for density fluctuation imaging on the DIII-D tokamak fusion plasma. Customized CMOS chips have been successfully developed for the transmitter module and receiver module array, covering the 55–75 GHz working band. The transmitter module has the capability of simultaneously launching eight tunable probe frequencies (>0 dBm output power each). The receiver enclosure contains 12 receiver modules in two vertical lines. The quasi-optical local oscillator coupling of previous MIR systems has been replaced with an internal active frequency multiplier chain for improved local oscillator power delivery and flexible installation in a narrow space together with improved shielding against electromagnetic interference. The 55–75 GHz low noise amplifier, used between the receiver antenna and the first-stage mixer, significantly improves module sensitivity and suppresses electronics noise. The receiver module has a 20 dB gain improvement compared with the mini-lens approach and better than –75 dBm sensitivity, and its electronics noise temperature has been reduced from 55 000 K down to 11 200 K. Further, the V-band MIR system is developed for co-located multi-field investigation of MHD-scale fluctuations in the pedestal region with W-band electron cyclotron emission imaging on DIII-D tokamak.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Emerging Functionality in Transition-Metal Compounds Driven by Spatial Confinement and Broken Symmetry

This research project investigates the emerging functionality in transition-metal-compounds (TMCs) driven by spatial confinement and broken symmetry. It combines advanced growth capabilities with cutting-edge characterization and first principles theory to probe and control the properties of TMC interfaces, including the utilization and development of state-of-the-art atomically resolved electron microscopy and spectroscopy to determine the structure, composition, and bonding at TMC interfaces. The proposed research will focus on four challenging areas: 1) manipulate interfaces to design new material phases such as magnetic metals with unique polar structure (net dipole) to achieve multiple functionality; 2) explore electronic mismatch or screening at interfaces of insulating/poor metal TMCs to produce novel electronic and magnetic properties; 3) elucidate and exploit the role of defects, both point and extended, on the functionality of interfaces; 4) develop advanced electron microscopy/spectroscopy techniques to explore temperature dependent phase transitions and couple these structural tools with new nonlinear optical probes of the electronic structure. The research team aims to close the materials-by-design loop of make, measure, model, and modify. The program promises to enhance our ability to engineer the desired physical properties at interfaces, superlattices (periodic arrays of films of different compounds), and heterostructures of TMCs.

36 MATERIALS SCIENCE↗

Parallel high-frequency magnetic sensing with an array of flux transformers and multi-channel optically pumped magnetometer for hand MRI application

Here, we investigate an approach for parallel high-frequency magnetic sensing based on a multi-channel radio frequency (RF) optically pumped magnetometer (OPM) coupled to multiple flux transformers (FTs) with a focus on hand magnetic resonance imaging (MRI) application at ultra-low field (ULF). Multiple RF OPM sensing channels are realized by using a single large-area alkali-metal vapor cell and two laser beams for pumping and probing, shared for all the channels. This design leads to significant cost reduction when multi-channel sensing is desirable, as in the case of ULF MRI. The FT, composed of two connected coils, serves as a transmitter of a target magnetic field to the OPM, while decoupling the OPM from untargeted magnetic fields in the sensing area that can limit the OPM performance. For hand MRI application, theoretical and numerical analysis is performed to determine an optimal geometry for the FT array that could improve signal-to-noise ratio (SNR) and sufficiently reduce crosstalk between FTs. We estimate that the optimized multi-channel FT-OPM sensor can achieve a magnetic field sensitivity of the order of 1 fT / Hz 1 / 2 above 100 kHz, which would be sufficient for 1 mm resolution MRI. In general, the multi-channel capability enables simultaneous magnetic measurements, thus reducing the sensing time and improving the SNR, and we anticipate many applications of the multi-channel FT-OPM sensor beyond the targeted here hand MRI: anatomical parallel ULF MRI of the human brain and other parts of the body, airport security screening, magnetic material imaging, and many others.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Four-channel optically pumped magnetometer for a magnetoencephalography sensor array

We present a novel four-channel optically pumped magnetometer (OPM) for magnetoencephalography that utilizes a two-color pump/probe scheme on a single optical axis. We characterize its performance across 18 built sensor modules. The new sensor implements several improvements over our previously developed sensor including lower vapor-cell operating temperature, improved probe-light detection optics, and reduced optical power requirements. The sensor also has new electromagnetic field coils on the sensor head which are designed using stream-function-based current optimization. We detail the coil design methodology and present experimental characterization of the coil performance. The magnetic sensitivity of the sensor is on average 12.3 fT/rt-Hz across the 18 modules while the average gradiometrically inferred sensitivity is about 6.0 fT/rt-Hz. The sensor 3-dB bandwidth is 100 Hz on average. The on-sensor coil performance is in good agreement with the simulations.

Iivanainen, Joonas (ORCID:0000000160344604)↗

Development of the microcalorimeter and anticoincidence detector for the Line Emission Mapper x-ray probe

The Line Emission Mapper (LEM) is an x-ray probe mission concept that is designed to provide unprecedented insight into the physics of galaxy formation, including stellar and black-hole feedback and flows of baryonic matter into and out of galaxies. LEM incorporates a light-weight x-ray optic with a large-format microcalorimeter array. The LEM detector utilizes a 14k pixel array of transition-edge sensors (TESs) that will provide <2.5 eV spectral resolution over the energy range 0.2 to 2 keV, along with a field-of-view of 30 arcmin. The microcalorimeter array and readout builds upon the technology developed for the European Space Agency’s (ESA’s) Athena/x-ray Integral Field Unit. Here, we present a detailed overview of the base- line microcalorimeter design, its performance characteristics, including a detailed energy resolution budget and the expected count-rate capability. In addition, we outline the current status and plan for continued technology maturation. Behind the LEM array sits a high-efficiency TES-based anticoincidence (antico) detector that will reject cosmic-ray background events. We will briefly describe the design of the antico and plan for continued development.

47 OTHER INSTRUMENTATION↗

Demonstration of the neutron tracking capability of NEXT array in time-of-flight measurements to improve energy resolution

Precise neutron-energy measurements are required to probe the nuclear structure effects of neutron-rich nuclei, where β-delayed neutron emission becomes a dominant decay mode. The Neutron dEtector with Xn Tracking (NEXT) array has been designed and constructed to measure β-delayed neutrons with better energy resolution. The new design localizes the neutron interaction position by optically segmenting the detector along the direction of the neutron flight path, reducing the associated uncertainties in the neutron time-of-flight measurements. This significantly improves the energy resolution without losing the necessary detection efficiency. The proof-of-principle and efficiency measurements showed promising results. Herein, this article details the implementation of the neutron tracking capability of NEXT array in time-of-flight measurements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Resolving the Inner Parsec of the Blazar J1924–2914 with the Event Horizon Telescope

The blazar J1924–2914 is a primary Event Horizon Telescope (EHT) calibrator for the Galactic center’s black hole Sagittarius A*. Here we present the first total and linearly polarized intensity images of this source obtained with the unprecedented 20 μas resolution of the EHT. J1924–2914 is a very compact flat-spectrum radio source with strong optical variability and polarization. In April 2017 the source was observed quasi-simultaneously with the EHT (April 5–11), the Global Millimeter VLBI Array (April 3), and the Very Long Baseline Array (April 28), giving a novel view of the source at four observing frequencies, 230, 86, 8.7, and 2.3 GHz. These observations probe jet properties from the subparsec to 100 pc scales. We combine the multifrequency images of J1924–2914 to study the source morphology. We find that the jet exhibits a characteristic bending, with a gradual clockwise rotation of the jet projected position angle of about 90° between 2.3 and 230 GHz. Linearly polarized intensity images of J1924–2914 with the extremely fine resolution of the EHT provide evidence for ordered toroidal magnetic fields in the blazar compact core.

79 ASTRONOMY AND ASTROPHYSICS↗

Shock wave formation in the thermosphere by an earthgrazing fireball: Empirical evidence for volatile-enhanced hydrodynamic shielding

Hydrodynamic shielding is a theoretically well-established but observationally elusive and experimentally difficult-to-replicate phenomenon with implications that extend far beyond meteor physics. Rare earthgrazing meteoroids with infrasound signatures that penetrate to the ground can be used to probe hydrodynamic shielding that leads to strong shock formation at high altitude. Here, we report the first coordinated optical and multi-station infrasound observations of a centimeter-scale earthgrazing fireball that generated sustained cylindrical line shock at thermospheric altitudes near 92 km. The event was recorded by numerous optical stations and three infrasound arrays, allowing trajectory reconstruction, ablation behavior, acoustic source localization, and shock characteristics. Optical observations indicate early mechanical erosion and ablation/evaporation at exceptionally low dynamic pressure, consistent with a cometary or a porous, volatile-bearing CM chondritic object. Independent infrasound detections localize shock generation to multiple points along a 164 km trajectory segment near perigee. Weak-shock modeling yields a consistent blast radius of ∼30 m, implying an acoustic-equivalent source size far exceeding the physical dimensions of the ∼45 g nucleus. We demonstrate that classical gas dynamics and ablation-driven hydrodynamic shielding alone cannot account for these observations under ambient thermospheric conditions. We show that volatile release provides the additional flow-field density enhancement required to amplify hydrodynamic shielding, reduce the effective local Knudsen number, and sustain a shock envelope capable of radiating detectable infrasound. Furthermore, these results demonstrate that small, volatile-rich meteoroids can transiently establish continuum-like flow in rarefied environments.

Astrometry↗

Multi-scale time-resolved electron diffraction: A case study in moiré materials

Ultrafast-optical-pump — structural-probe measurements, including ultrafast electron and x-ray scattering, provide direct experimental access to the fundamental timescales of atomic motion, and are thus foundational techniques for studying matter out of equilibrium. High-performance detectors are needed in scattering experiments to obtain maximum scientific value from every probe particle. Here we deploy a hybrid pixel array direct electron detector to perform ultrafast electron diffraction experiments on a WSe 2 /MoSe 2 2D heterobilayer, resolving the weak features of diffuse scattering and moiré superlattice structure without saturating the zero order peak. Enabled by the detector’s high frame rate, we show that a chopping technique provides diffraction difference images with signal-to-noise at the shot noise limit. Finally, we demonstrate that a fast detector frame rate coupled with a high repetition rate probe can provide continuous time resolution from femtoseconds to seconds, enabling us to perform a scanning ultrafast electron diffraction experiment that maps thermal transport in WSe 2 /MoSe 2 and resolves distinct diffusion mechanisms in space and time.

36 MATERIALS SCIENCE↗

Small footprint optoelectrodes using ring resonators for passive light localization

The combination of electrophysiology and optogenetics enables the exploration of how the brain operates down to a single neuron and its network activity. Neural probes are in vivo invasive devices that integrate sensors and stimulation sites to record and manipulate neuronal activity with high spatiotemporal resolution. State-of-the-art probes are limited by tradeoffs involving their lateral dimension, number of sensors, and ability to access independent stimulation sites. Here, we realize a highly scalable probe that features three-dimensional integration of small-footprint arrays of sensors and nanophotonic circuits to scale the density of sensors per cross-section by one order of magnitude with respect to state-of-the-art devices. For the first time, we overcome the spatial limit of the nanophotonic circuit by coupling only one waveguide to numerous optical ring resonators as passive nanophotonic switches. With this strategy, we achieve accurate on-demand light localization while avoiding spatially demanding bundles of waveguides and demonstrate the feasibility with a proof-of-concept device and its scalability towards high-resolution and low-damage neural optoelectrodes.

42 ENGINEERING↗

First Results from the Thomson Scattering Diagnostic on the Large Plasma Device

We present the first Thomson scattering measurements of electron density and temperature in the Large Plasma Device (LAPD), a 22 m long magnetized linear plasma device at the University of California Los Angeles (UCLA). The diagnostic spectrally resolves the Doppler shift imparted on light from a frequency-doubled Nd:YAG laser when scattered by plasma electrons. A fiber array coupled to a triple-grating spectrometer is used to obtain high stray light rejection and discriminate the faint scattering signal from a much larger background. In the center of the plasma column, the measured electron density and temperature are about ne≈1.5×1013 cm−3 and Te≈ 3 eV, respectively, depending on the discharge parameters and in good agreement with Langmuir probe data. Optical design considerations to maximize photon count while minimizing alignment sensitivity are discussed in detail and compared to numerical calculations. Raman scattering off of a quartz crystal probe is used for an absolute irradiance calibration of the system.

Kaloyan, Marietta (ORCID:0000000182593038)↗

Probing the Impact of Radio-mode Feedback on the Properties of the Cool Circumgalactic Medium

We explore the influence of radio-mode feedback on the properties of the cool circumgalactic medium (CGM). To this end, we assemble a statistical sample of approximately 30,000 radio galaxies with background quasars by combining optical spectroscopic measurements of luminous red galaxies and quasars from the year 1 data set of the Dark Energy Spectroscopic Instrument and radio sources from the LOw-Frequency ARray Two-metre Sky Survey (LoTSS) DR2 catalog and the Very Large Array Sky Survey (VLASS) quick-look catalog. Galaxies with similar optical properties but with no radio counterparts in LoTSS and VLASS are selected as the control group. We measure the cool CGM properties of radio galaxies and their control samples traced by Mg ii absorption lines, including covering fraction, rest equivalent width, and gas kinematics. Our results show no significant difference in the properties of gas around radio galaxies and their control sample, indicating that the operating radio-mode feedback of massive galaxies does not produce detectable effects on the properties of the cool CGM. Finally, we show that the CGM of radio galaxies contains a nonnegligible amount of cool gas with approximately 10 10 M ⊙ . This abundance can place a stringent constraint on the radio-mode feedback models.

79 ASTRONOMY AND ASTROPHYSICS↗

Results from the DUNE ND-LAr 2x2 Demonstrator Run 2

The Deep Underground Neutrino Experiment (DUNE) is a cutting-edge, long-baseline experiment under construction in the United States, based on large liquid-argon time projection chambers (LArTPCs). The DUNE Near Detector LArTPC (ND-LAr) will employ a novel modular architecture using a pixelated LArPix charge readout. To validate this design and characterize detector response, the 2×2 demonstrator—an array of eight optically isolated LArTPC modules—was deployed at Fermilab in 2024. During winter 2025, the 2x2 demonstrator was operated for a second data-taking campaign (Run 2) with the aim of studying the low-energy response of the detector. Run 2 focused on calibration and response studies using a suite of deployed radioactive sources. Gamma sources (²²Na, ⁶⁰Co, and ⁸⁸Y) were used to probe module-to-module performance variations, energy resolution, and calibrations. Neutron sources (AmBe and a pulsed neutron generator) enabled studies of neutron interactions in liquid argon, including inelastic scatters and neutron capture signals, relevant for low-energy backgrounds and detector modeling. In addition, the detector was doped with ²²⁰Rn, providing Bi–Po coincidence signals that allow precise calibration of the charge and scintillation response. This poster will present results from these calibration campaigns. These studies provide critical validation of the ND-LAr modular LArTPC concept and inform calibration and reconstruction strategies for the full DUNE near detector.

Mora-Lepin, Luis [Florida State U.] (ORCID:0000000↗

Topological steering of light by nematic vortices and analogy to cosmic strings

Liquid crystals are widely known for their technological uses in displays, electro-optics, photonics and nonlinear optics, but these applications typically rely on defining and switching non-topological spatial patterns of the optical axis. Here, we demonstrate how a liquid crystal’s optical axis patterns with singular vortex lines can robustly steer beams of light. External stimuli, including an electric field and light itself, allow us to reconfigure these unusual light–matter interactions. Here, periodic arrays of vortices obtained by photo-patterning enable the vortex-mediated fission of optical solitons, yielding their lightning-like propagation patterns. Predesigned patterns and spatial trajectories of vortex lines in high-birefringence liquid crystals can steer light into closed loops or even knots. Our vortex lattices might find technological uses in beam steering, telecommunications, virtual reality implementations and anticounterfeiting, as well as possibly offering a model system for probing the interaction of light with defects, including the theoretically predicted, imagination-capturing light-steering action of cosmic strings, elusive defects in cosmology.

36 MATERIALS SCIENCE↗

Photophysical Properties and Electronic Structure of Hydroporphyrin Dyads Exhibiting Strong Through-Space and Through-Bond Electronic Interactions

Electronic interactions between tetrapyrroles are utilized in natural photosynthetic systems to tune the light-harvesting and energy/charge-transfer processes in these assemblies. Such interactions also can be employed to tailor the electronic properties of tetrapyrrolic dyads and larger arrays for use in materials science and biomedical research. Here we have utilized static and time-resolved optical spectroscopy to characterize the optical absorption and emission properties of a set of chlorin and bacteriochlorin dyads with varied degrees of through-bond (TB) and through-space (TS) interactions between the constituent macrocycles. The dyads consist of two chlorins or two bacteriochlorins joined by a linker that utilizes a triple-double-triple bond (enediyne) motif in which the double bond portion is a ester-substituted ethylene or o-phenylene unit. The photophysical studies are coupled with density functional theory (DFT) calculations to probe the ground-state molecular orbital (MO) characteristics of the dyads and time-dependent calculations (TDDFT) to elucidate excited-state properties. The latter include electronic characteristics of the singlet excited state manifold and the absorption transitions to these states from the electronic ground state. Comparison of the MO and calculated spectral properties of each dyad with the linker present versus disrupted (by eliminating the double-bond portion) gives insight into the relative contributions of TB versus TS interactions to the electronic properties of the dyads. The results show that the TB and TS contributions are additive (constructively interfere), which is not always the case for molecular dyads. Most of the dyads have shorter lifetimes of the lowest singlet excited state compared to the parent monomer, which derives from increased S 1 → S 0 internal conversion. The enhancement is greater for the dyads in benzonitrile than in toluene. Furthermore, the studies provide insights into the nature of the electronic interactions between the constituents in the tetrapyrrole arrays and how these interactions dictate the spectral properties and excited-state decay characteristics.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

94 GHz microplasma sustained by a photonic crystal

A photonic crystal (PhC) with a single vacancy sustains an argon microplasma at 94 GHz. The PhC consists of a 7 × 13 array of small alumina rods, each 250 μm in radius. The PhC has a forbidden bandgap from 70–105 GHz. The vacancy creates an internal electromagnetic resonance at 94 GHz that intensifies the electric field of an incident wave to 5 × 10 5 V m –1 . Breakdown of low-pressure argon gas (80 mbar) occurs and forms a stable, ellipsoidal plasma inside the crystal. The central core of the microplasma is probed using a 200 μm optical fiber inserted into the PhC. The rotational temperature of the CH molecule is estimated from a numerical fit of the plasma emission and is found to increase from 450–650 K with both pressure (200–1000 mbar) and incident wave power (100 mW–1100 mW). Under these conditions, the electron density increases with both power and pressure from 0.5–1.5 × 10 20 m –3 . Furthermore, this plasma density range brackets the electron plasma frequency at 94 GHz. The results are compared with a similar microplasma operating at 44 GHz.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗