Engineering Papers⌕ Search

SEARCH · Engineering Papers

Results for “Nuclear decay data”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 37 records · Page 2

Nuclear Structure and Decay Data for A=169 Isobars

Experimental data pertaining to all nuclei with mass number A=169 (Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, Lu, Hf, Ta, W, Re, Os, Ir, Pt) have been evaluated. Level schemes from both radioactive decay and reaction studies are presented, along with associated tables of experimental data and adopted properties for levels and γ rays. The present evaluation for A=169 supersedes the 2008 evaluation, 2008Ba31, by C.M. Baglin. A few highlights of this evaluation: More extensive work on ε decay from 169W is needed and new experimental work will be required to resolve a discrepancy between the J π values deduced for a 180-keV level in 169Ta based on extensive band structure from (HI,xnγ) work (J π =1/2−) and TDPAD measurements (J=5/2). Low lying states of 169Os were studied via fine structure of 173Pt α decay in 2014ThZZ. The Eαs feeding the g.s. of 169Os in 2008Ba31 are separated well into two consistent groups to feed the g.s. and the newly proposed state at 34.84 keV. Based on the studies of 2014ThZZ and 2021Zh52, the g.s. spin-parity assignment of 169Os has been proposed to be (7/2−) from (5/2−). The 169Ir g.s. half-life and alpha emission branching reported in 2012Th13 from 173Au α decay measurements are preferred over the values in 2005Sc22. The reported half-life value in 2005Sc22 for 169Ir g.s. is discrepant and the research work was carried out in the same lab of 2012Th13.

Basunia, M Shamsuzzoha↗

In search of truth: In memory of Balraj Singh

Born in Punjab (India) in December 1941, Balraj Singh is not only the single most prolific nuclear data evaluator and disseminator of nuclear structure and decay data with 148 evaluations in Nuclear Data Sheets — 85 as the first and often only author — plus other journals, but his upmost curiosity and dedication brought him to be one of the finest nuclear physicists, with an everlasting influence on many of us. Furthermore, Balraj passed away about a year ago on 9 October 2023 in Ottawa, Ontario (Canada) at the age of 81, and at Atomic Data and Nuclear Data Tables we would like to commemorate some of his scientific achievements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

CONFLUX: A standardized framework to calculate reactor antineutrino flux

Nuclear fission reactors are abundant sources of antineutrinos for neutrino physics experiments. The flux and spectrum of antineutrinos emitted by a reactor can indicate its activity and composition, suggesting potential applications of neutrino measurements beyond fundamental scientific studies that may be valuable to society. The utility of reactor antineutrinos for applications and fundamental science is dependent on the availability of precise predictions of these emissions. For example, in the last decade, disagreements between reactor antineutrino measurements and models have inspired revision of reactor antineutrino calculations and standard nuclear databases as well as searches for new fundamental particles not predicted by the Standard Model of particle physics. Past predictions and descriptions of the methods used to generate them are documented to varying degrees in the literature, with different modeling teams incorporating a range of methods, input data, and assumptions. The resulting difficulty in accessing or reproducing past models and reconciling results from differing approaches complicates the future study and application of reactor antineutrinos. The CONFLUX (Calculation Of Neutrino FLUX) software framework is a neutrino prediction tool built with the goal of simplifying, standardizing, and democratizing the process of reactor antineutrino flux calculations. CONFLUX includes three primary methods for calculating the antineutrino emissions of nuclear reactors or individual beta decays that incorporate common nuclear data and beta decay theory. The software is prepackaged with the current nuclear databases, including ENDF.B/VIII, JEFF-3.3, and ENSDF, and it includes the capability to predict time-dependent reactor emissions, adjust nuclear database or beta decay inputs/assumptions, and propagate related sources of uncertainty. Here, this paper describes the CONFLUX software structure, details the methods used for flux and spectrum calculations, and provides examples of potential use cases.

Zhang, Xianyi [Lawrence Livermore National Laborat↗

First observation of a high-𝐾 band structure in 162 Er and implications in the context of the identical bands phenomenon

The first ever identification of a high-𝐾 band structure in 162 Er is reported. Based on a 𝐾 𝜋 = 7 (−) isomer, it is found to be identical in nature to the corresponding 𝐾 𝜋 = 7 − sequence in 164 Er up to its highest observed spin. Furthermore, the phenomenon of identical high-K bands built on a two-quasiparticle configuration in an isotopic chain is reported here for the first time. While this is a notable addition to the systematics of known identical bands in nuclei at normal deformation, a satisfactory global understanding of the phenomenon remains elusive.

150 ≤ A ≤ 189↗

Nuclear Data Sheets for A=201

Evaluated nuclear structure and decay data for all nuclei with mass number A=201 ( 201 Os, 201 Ir, 201 Pt, 201 Au, 201 Hg, 201 Tl, 201 Pb, 201 Bi, 201 Po, 201 At, 201 Rn, 201 Fr, 201 Ra) are presented. All available experimental data are compiled and evaluated, and best values for level and γ-ray energies, quantum numbers, lifetimes, γ-ray intensities and transition probabilities, as well as other nuclear properties, are recommended. Inconsistencies and discrepancies that exist in the literature are discussed. A number of computer codes (https://wwwnds.iaea.org/public/ensdf pgm/index.htm) developed by members of the NSDD network were used during the evaluation process. For example, the reported absolute γ-ray emission probabilities and their uncertainties in various decay data sets were determined using the GABS code. The γ-ray transition probabilities were determined using the RULER code and the corresponding uncertainties were determined using a Monte-Carlo approach. In conclusion, this work supersedes the earlier evaluation by F.G. Kondev (2007Ko06), published in Nuclear Data Sheets 108, 365 (2007).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Impact of Newly Measured 𝛽-Delayed Neutron Emitters around 78 Ni on Light Element Nucleosynthesis in the Neutrino Wind Following a Neutron Star Merger

Neutron emission probabilities and half-lives of 37 𝛽-delayed neutron emitters from 75 Ni to 92 Br were measured at the RIKEN Nishina Center in Japan, including 11 one-neutron and 13 two-neutron emission probabilities and six half-lives for the first time that supersede theoretical estimates. These nuclei lie in the path of the weak 𝑟 process occurring in neutrino-driven winds from the accretion disk formed after the merger of two neutron stars synthesizing elements in the 𝐴∼80 abundance peak. The presence of such elements dominates the accompanying kilonova emission over the first few days and have been identified in the AT2017gfo event, associated to the gravitational wave detection GW170817. Abundance calculations based on over 17,000 simulated trajectories describing the evolution of matter properties in the merger outflows show that the new data lead to an increase of 50%–70% in the abundance of Y, Zr, Nb, and Mo. This enhancement is large compared to the scatter of relative abundances observed in old very metal poor stars and thus is significant in the comparison with other possible astrophysical processes contributing to the light-element production. These results underline the importance of including experimental decay data for very neutron-rich 𝛽 -delayed neutron emitters into 𝑟 -process models.

59 ≤ A ≤ 89↗

Multimessengers from the Radioactive Decay of r -process Nuclei

The radioactive β-decay of nuclei synthesized in the rapid neutron capture process (r-process) releases a variety of particles, including electrons, γ-rays, neutrinos, and neutrons. These particles provide a rich set of multimessenger signals that carry information about the astrophysical environments where neutron-rich nucleosynthesis occurs. In this work, we calculate from first principles the emission spectra resulting from the β-decay of r-process nuclei. Our approach incorporates detailed nuclear structure and decay data to model the energy distributions of each particle species. We couple the spectra with a nuclear reaction network simulation to obtain the temporal evolution of these distributions. We find that the emission distributions vary significantly in time and are nonthermal, with substantial average energies. We investigate these nuclear signals as a direct probe of heavy element formation and show that they are complementary observables to kilonova.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Precise half-life determination of 131 Ba and 125 Xe

Barium-131 and Xenon-125 are valuable radioisotopes with numerous scientific and medical applications. Here, we produced both isotopes via proton irradiation of a cesium iodide (CsI) target at the Brookhaven Tandem Van de Graaff accelerator (BTVG). Following irradiation, we conducted systematic γ-ray spectroscopy measurements at the National Nuclear Data Center (NNDC) decay station using a calibrated High-Purity Germanium (HPGe) detector, collecting data over a 2-month period (spanning approximately 4.5 half-lives for 131 Ba). Through careful analysis of the characteristic γ-ray emissions from both isotopes, we determined the half-life of 131 Ba to be 11.55(6) days, which agrees with the previously evaluated value. For 125 Xe, we measured a half-life of 16.56(8) hours, slightly lower than the evaluated value.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Decay Reaction Sublibrary

The decay sublibrary aims to describe all known spontaneous decays and branching ratios for all nuclei across the nuclide chart. ENDF/B-VIII.1 remains unchanged from ENDF/B-VIII.0 for the decay sublibrary.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Calculation Of Neutrino Flux

The CONFLUX software framework, Calculation Of Neutrino FLUX, is built with the goal to simplify and standardize the calculation. CONFLUX packages three methods to calculate neutrinos generated from reactor neutrinos or individual beta decays with common nuclear data and beta theories for direct cross-method comparison. The software prepacked the latest nuclear database, including ENDF.B/VIII, JEFF 3.3, and ENSDF, as well as methods to process the uncertainties. It also allows customized nuclear data and beta theories and user generated time dependent reactor models for convenient adjustment of fission products, theoretical corrections.

Zhang, Xianyi [Lawrence Livermore National Laborat↗

ENDF/B-VIII.1: Alpha Reaction Sublibrary

The alphas sublibrary aims to describe nuclear reactions between incident alpha particles and different nuclei. For ENDF/B-VIII.1, the LLNL ECPL evaluation for 6Li, and the JENDL-based NNL evaluations of 9 Be and 16,17 O were adopted. Also, there were minor fixes done to 4 He.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Deuteron Reaction Sublibrary

The deuterons sublibrary aims to describe nuclear reactions between incident deuteron particles and different nuclei. For ENDF/B-VIII.1, we adopted additions and corrections to the ENDF/B-VIII.0 d+t file, as well as new LANL evaluation updates for 3 He and 6 Li.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Electron Reaction Sublibrary

The electrons sublibrary aims to describe electron-atomic cross section data, corresponding to the interaction between electrons and the different atoms. For ENDF/B-VIII.1 we adopted the EPICS2023 EEDL evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1

The ENDF/B-VIII.1 release is the newest evaluated nuclear data library produced, distributed, and recommended by CSEWG for use in nuclear science and technology applications. Among the many key advances, relative to the previous version ENDF/B-VIII.0, are: re-evaluation of 239Pu file by a joint international effort; updated 16,18O, 19F, 28-30Si, 50-54Cr, 55Mn, 54,56,57Fe, 63,65Cu, 139La, 233,235,238U, and 240,241Pu neutron nuclear data by the IAEA-coordinated INDEN collaboration; significant changes for 3He, 6Li, 9Be, 51V, 88Sr, 103Rh, 140,142Ce, Dy, 181Ta, Pt, 206-208Pb, and 234,236U neutron data; new nuclear data for the photo-nuclear, being 196 adopted from the IAEA2019 Photonuclear Data Library and one new file from JENDL-5; and new evaluations for the charged-particle and atomic sublibraries. Numerous thermal neutron scattering kernels were re-evaluated or provided for the very first time. Additionally, new covariance testing was implemented. ENDF/B-VIII.1 reduced bias in the simulations of many integral experiments with particular progress noted for fluorine, copper and stainless steel containing benchmarks. Data issues which had hindered the deployment of ENDF/B-VIII.0 for commercial nuclear power applications in high burn-up situations, were addressed. ENDF/B-VIII.1 data are distributed in both ENDF-6 and GNDS formats.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Photonuclear Sublibrary

The photonuclear sublibrary aims to describe nuclear reactions between incident gamma particles and different nuclei. For ENDF/B-VIII.1, we adopted around 200 evaluations from the IAEA Coordinated Research Project (CRP) on photonuclear data while, for a few select mission-critical materials, evaluations from ENDF/B-VIII.0 were maintained. Additionally, many fixes to many files were implemented. Finally, ENDF/B-VIII.1 includes a new photonuclear file, 242 Pu, which was adopted from JENDL-5.0.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Helium-3 Reaction Sublibrary

The Helium-3 (Helions) sublibrary aims to describe nuclear reactions between incident 3 He particles and different nuclei. For ENDF/B-VIII.1, we adopted a new 4He evaluation from the INDEN collaboration and the LLNL ECPL evaluation for 7 Li.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Neutron Reaction Sublibrary

The neutrons sublibrary aims to describe nuclear reactions between incident neutron particles and different nuclei. For ENDF/B-VIII.1, many neutron files were re-evaluated or received major changes. A new 239Pu evaluation was jointly-produced by IAEA, LANL, LLNL and ORNL bringing important updates to fission neutron multiplicity, Prompt Fission Neutron Spectrum, resonance and fast regions. Around one third of the new neutron evaluations were performed as part of the INDEN collaboration, including 16,18 O, 19 F, 28,29,30 Si, 63,65 Cu, 50,51,52,53,54 Cr, 55 Mn, 54,56,57 Fe, 139 La, 233,235,238 U, 240,241 Pu. Important non-INDEN evaluations include 234,236 U, 206,207,208 Pb, 181 Ta, 88 Sr, 140,142 Ce, Pt and Dy isotopes, and many others. Also, dosimetry reactions from IRDFF-II were adopted for many materials.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗