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All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Nuclear Data Sheets for A=170☆

Nuclear structure data pertaining to all nuclei with mass number A=170 have been evaluated, and incorporated into the ENSDF data file. This evaluation supersedes the previous evaluation (Coral M. Baglin), Nuclear Data Sheets 96, 611 (2002), (cutoff date 15 August 2002) and subsequent updates of the ENSDF file for Yb to Dy (cutoff 15 April 2010), Lu (cutoff 8 October 1998), Pt (cutoff 17 February 1999) and Ta, Os (cutoff 7 April 1998). Since the previous evaluation, {sup 170}Gd has been observed and the ground state T{sub 1/2} measured. New excited states have also been observed in the neutron rich {sup 170}Dy. The ground state T{sub 1/2} of {sup 170}Tb has been determined, however, there are currently still no excited states observed in this nucleus. There remains some uncertainty in the ground state and longer-lived isomer in {sup 170}Ir which could warrent further experimental investigation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

Nuclear Data Sheets for A = 183

Evaluated nuclear structure and decay data for all nuclides with mass number A=183 (Yb, Lu, Hf, Ta, W, Re, Os, Ir, Pt, Au, Hg, Tl, Pb) are presented here. At, Po and Fr have not yet been observed, but for prediction of ground state and/or isomer properties see, e.g., 2015Bh08 (At, Fr), 2013Ba41 (Tl), 2013Ho05 (Po). This evaluation includes structure and decay data information available by 15 April 2015 and supersedes that by R.B. Firestone published in Nuclear Data Sheets65, 589 (1992) (literature cutoff 9 January 1991), and subsequent revisions by C.M. Baglin for {sup 183}Au in ENSDF database (literature cutoff 13 March 1999), {sup 183}Hg in Nuclear Data Sheets91, 117 (2000) (literature cutoff 25 September 2000), {sup 183}Tl in Nuclear Data Sheets95, 49 (2002) (literature cutoff 1 January 2002) and {sup 183}Pb in ENSDF (literature cutoff 6 January 2003). Since the prior Nuclear Data Sheets publication of this mass chain: {sup 183}Yb (2012Ku26) and {sup 183}Pb (2006An11, 2006Se18, 2007De09, 2009Se13) have been observed; our knowledge of high–spin states has been significantly expanded for {sup 183}Ta (2009Sh17), {sup 183}W (1999Sa60), {sup 183}Re (1998Ha51, 2001Sh41), {sup 183}Au (2002Jo18, 2005So01) and {sup 183}Tl (2001Mu26, 2004Ra28); a large amount of new structure information for {sup 183}W has been obtained from transfer reactions (1997Pr02, 2011Bo09), (n,n'γ) (1993Pr09) and thermal neutron capture (1993Pr09, 1997Pr02, 2011Bo09, 2014Hu02), as well as from the two–photon cascade study by 2005Su29.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2014

Working Party on International Nuclear Data Evaluation Cooperation (WPEC)

The OECD Nuclear Energy Agency (NEA) organizes cooperation between the major nuclear data evaluation projects in the world. The NEA Working Party on International Nuclear Data Evaluation Cooperation (WPEC) was established to promote the exchange of information on nuclear data evaluation, measurement, nuclear model calculation, validation, and related topics, and to provide a framework for cooperative activities between the participating projects. The working party assesses nuclear data improvement needs and addresses these needs by initiating joint activities in the framework of dedicated WPEC subgroups. Studies recently completed comprise a number of works related to nuclear data covariance and associated processing issues, as well as more specific studies related to the resonance parameter representation in the unresolved resonance region, the gamma production from fission product capture reactions, the {sup 235}U capture cross section, the EXFOR database, and the improvement of nuclear data for advanced reactor systems. Ongoing activities focus on the evaluation of {sup 239}Pu in the resonance region, scattering angular distribution in the fast energy range, and reporting/usage of experimental data for evaluation in the resolved resonance region. New activities include two subgroups on improved fission product yield evaluation methodologies and on modern nuclear database structures. Future activities under discussion include a pilot project for a Collaborative International Evaluated Library Organization (CIELO) and methods to provide feedback from nuclear and covariance data adjustment for improvement of nuclear data. In addition to the above mentioned short-term task-oriented subgroups, WPEC also hosts a longer-term subgroup charged with reviewing and compiling the most important nuclear data requirements in a high priority request list (HPRL)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

JRC-IRMM/ORNL Collaboration on Nuclear Data for Nuclear Criticality Safety - 14486

Concerns about using cross sections recommended in the main evaluated data libraries (i.e. ENDF/B, JEFF and JENDL) for nuclear criticality calculations have been a prime motivator for new cross section measurements. The measurements and evaluations discussed in this work are part of a collaboration between the Oak Ridge National Laboratory (ORNL) and the Institute for Reference Material and Measurements of the Joint Research Center (JRC-IRMM) of the European Commission (EC). They are performed in response to the US Nuclear Criticality Safety Program (NCSP) data needs. In particular, the NCSP five-year plan encompasses a listing of elements that have been identified for measurements and evaluations to address issues on criticality safety applications. This listing is based on data deficiency concerns in practical applications that are conveyed by criticality safety practitioners. In general these deficiencies are obtained through the analysis of benchmark calculations. A wealth of evaluations in the main libraries were derived from results of measurements made with poor time-of-flight resolution, and also the description of some data in the neutron energy range above several tens of keV is crude. This impacts both the resolved and unresolved resonance region, and leads to bias effects when resonance structures play an important role. As a consequence only average corrections can be applied in calculations for nuclear criticality calculations where self-shielding, multiple scattering, or Doppler broadening are important. This can lead to erroneous results. Furthermore, many evaluations for nuclides having small neutron-capture cross sections show erroneously high cross sections because the influence of the neutron sensitivity of the old measurement systems was underestimated. Although their neutron capture cross sections are small, these nuclides, if occurring in large amounts, can be important absorbers in criticality calculations, so an accurate determination of these cross sections is required. Over the last seven years the JRC-IRMM/ORNL collaboration has produced many neutron induced cross section data using the Geel Electron Linear Accelerator (GELINA) neutron time-of-flight facility. This facility is ideally suited to measure total, fission and capture cross sections in the energy range from 1 eV to ∼600 keV, which is important for nuclear criticality calculations. In this paper the facility and experimental set-ups at GELINA will be described together with the data reduction and analysis procedures which result in experimental observables including their full covariance information. The importance of combining transmission and partial cross section data will be emphasized. We will give a list of the measured nuclides and discuss the impact of the resulting data and evaluations. (authors)

42 ENGINEERING↗
DOE OSTI2018

Nuclear Data Sheets for A=171

Experimental data pertaining to all nuclei with mass number A=171 (Tb, Dy, Ho, Er, Tm, Yb, Lu, Hf, Ta, W, Re, Os, Ir, Pt, Au, Hg) have been evaluated. Level schemes from both radioactive decay and reaction studies are presented, along with associated tables of experimental data and adopted properties for levels and γ rays. This evaluation for A=171, which considers data received by 30 June 2018, supersedes the 2002 evaluation (with a literature cutoff date of August 2002) by Coral M. Baglin, published in Nuclear Data Sheets 96, 399 (2002) and the subsequent evaluation of the ENSDF file for 171Pt by C. Baglin (literature cutoff date of 15 April 2010).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2013

Nuclear Data Sheets for A = 215

The evaluated spectroscopic data are presented for 12 known nuclides of mass 215 (Hg, Tl, Pb, Bi, Po, At, Rn, Fr, Ra, Ac, Th, Pa). For {sup 215}Hg, {sup 215}Tl, {sup 215}Pb, and {sup 215}Pa nuclei, no excited states are known. The decay characteristics of {sup 215}Hg and {sup 215}Tl are unknown. The decay scheme of {sup 215}Pb is considered as incomplete. Ordering of γ cascades in the decay of 36.9–s isomer of {sup 215}Bi and for high–spin states above 2251 keV in {sup 215}Fr are not established. High–spin excitations, including several isomeric states, are well known in {sup 215}Bi, {sup 215}Po, {sup 215}Rn, {sup 215}Fr, {sup 215}Ra, and {sup 215}Ac. No particle–transfer reaction data are available for any of the A=215 nuclei. The rms charge radii for {sup 215}Pb, {sup 215}Bi, {sup 215}Po, {sup 215}Rn, {sup 215}Fr and {sup 215}Ra have been evaluated by Daniel Abriola, from extrapolation or interpolation of available evaluated data in 2013An02 for radii of respective Z chains using formula 9 in 2004An14. This evaluation was carried out as part of ENSDD–workshop at VECC, Kolkata for Nuclear Structure and Decay Data, organized and hosted by VECC and Board of Research in Nuclear Sciences (BRNS) in Kolkata, India, November 26–29, 2012. This work supersedes the previous A = 215 evaluation (2001Br31) published by E. Browne which covered literature prior to May 2001.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Automated Resonance Fitting for Nuclear Data Evaluation

Global and national efforts to deliver high-quality nuclear data to users have a wide-ranging impact, affecting applications in national security, reactor operations, basic science, medicine, and more. Cross section evaluation is a major part of this effort, combining theory and experimentation to produce recommended values and uncertainties for reaction probabilities. Resonance region evaluation is a specialized type of nuclear data evaluation that can require significant manual effort and months of time from expert scientists. In this article, non-convex non-linear optimization methods are combined with concepts of inferential statistics to infer a resonance model from experimental data in an automated manner that is not dependent on prior evaluation(s). This methodology aims to enhance the workflow of a resonance evaluator by minimizing time, effort, and the potential for bias from prior assumptions, while enhancing reproducibility and documentation, thereby addressing well-known challenges in the field.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2017

General Guidelines on Criteria for Adoption or Rejection of Evaluated Libraries and Data by the Nuclear Data Team

This memo contains general guidelines on what documentation and tools need to be in place as well as format and data testing requirements such that evaluated nuclear data sets or entire libraries can be adopted by the nuclear data team. Additional requirements beyond this memo might apply for specific nuclear data observables. These guidelines were established based on discussions between J.L. Conlin, M.G. Gray, A.P. McCartney, D. Neudecker, D.K. Parsons and M.C. White.

96 KNOWLEDGE MANAGEMENT AND PRESERVATION↗
DOE OSTI2019

Nuclear Data Sheets for A=73☆

Experimental nuclear structure data for the known A=73 isobaric nuclides (Mn, Fe, Co, Ni, Cu, Zn, Ga, Ge, As, Se, Br, Kr, Rb and Sr) have been evaluated, and presented together with Adopted properties of level energies, and associated γ rays. The decay data for these nuclides have also been evaluated, providing Adopted values of γ and β radiations, and log ft values. For {sup 73}Mn, only the isotopic identification has been established, with no knowledge of its g.s. half-life. For {sup 73}Fe, {sup 73}Co and {sup 73}Sr, only the ground states and their half-lives are known with no information about the excited states. For {sup 73}Ni, {sup 73}Cu, {sup 73}Zn and {sup 73}Rb, little data are available for excited states. The half-life and decay modes of possibly proton-unbound {sup 73}Rb need firmly established. {sup 73}Ga structure presents a special challenge in that the 1/2{sup −} ground state and the first 3/2{sup −} state have recently been proposed, in a Coulomb excitation experiment by 2010Di14, to form an almost degenerate doublet with an estimated spacing of 229 Th with its first excited state at 7.8 eV, and {sup 235}U with its first excited state at 76 eV. Ultra-high resolution gamma-ray spectroscopic studies are warranted to search for the low-lying (73 Ga, and to determine its half-life. Level structures of {sup 73}Ga, {sup 73}Ge, {sup 73}As, {sup 73}Se, {sup 73}Br and {sup 73}Kr are quite well known, although decay schemes of radioactive ground states of {sup 73}Co, {sup 73}Cu and {sup 73}Br are considered incomplete. The reactions and decays for which no new experimental information has become available since the 2003 update have undergone revisions to incorporate conversion coefficients from BrIcc code, and evaluated Q values from 2017Wa10, but essential content of such datasets may have remained the same as in previous evaluations. In this respect the present work greatly benefited from all the previous NDS evaluations (2004Si08,1993Ki25,1987Ki13, 1980Ek01,1974Al33), but at the same time data presented herein supersede all the previous published evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2014

Nuclear Data Sheets for A = 148

The experimental nuclear structure data available through October 2013 have been reviewed. A summary of information obtained in various reaction and decay experiments is presented, together with adopted level schemes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Nuclear Data Sheets for A=164

Experimental nuclear structure data for the known A=164 isobaric nuclides (Sm, Eu, Gd, Tb, Dy, Ho, Er, Tm, Yb, Lu, Hf, Ta, W, Re, Os, Ir) have been evaluated, and presented together with Adopted properties of level energies, and associated γ rays. The decay data for these nuclides have also been evaluated, providing Adopted values of γ and β radiations, and log ft values. No excited states are known in 164 Eu, 164 Tb, and 164 Ir. Information for 164 Gd, 164 Re and 164 Os is limited due to insufficient experimental data. For radioactive nuclides, decay schemes of 164 Sm, 164 Gd and 164 Re are not known, and those of 164 W, 164 Tb, 164 Lu, 164 Hf, 164 Ta and 164 W are incomplete. The decay schemes of 164 Ho and the two activities of 164 Tm seem fairly complete. The decay scheme of 164 Yb presents a major problem that the Q(ε) value of 887 keV 29 recommended in 2017Wa10 is in disagreement with the population of levels at 928, 952 and 1060 keV in the daughter nucleus. This decay scheme, which so far has been mainly reported in a secondary reference (1982AdZZ) needs further investigation. Also the masses of 164 Yb and 164 Tm need either new measurements or a re-evaluation to resolve discrepancy of about 220 keV in the Q value of 164 Yb decay to 164 Tm. The reactions and decays for which no new experimental information has become available since the 2001 update have undergone revisions to incorporate conversion coefficients from BrIcc code, and evaluated Q values from 2017Wa10, but the essential content of such datasets may have remained the same as in previous evaluations. Finally, in this respect the present work greatly benefited from all the previous NDS evaluations (2001Si27,1992Sh07, 1986Sh03,1974Bu30), but at the same time data presented herein supersede all the previous published evaluations.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2014

Nuclear Data Sheets for A = 248

Detailed level schemes, decay schemes, and the experimental data on which they are based are presented for all nuclei with mass number A=248. The experimental reaction and decay data are evaluated; inconsistencies and discrepancies are noted; and adopted values are given for various level properties (including spin and parity, halflife, and configuration), γ properties (including energy, intensity, and multipole character) and α properties (including energy, intensity, and hindrance factor). This evaluation replaces the A=248 evaluation published by A. Akovali in Nuclear Data Sheets 87, 249 (1999)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Nuclear Data Sheets for A=177

Evaluated nuclear structure and decay data for all nuclei with mass number A=177 (Ho,Er,Tm,Yb,Lu, Hf,Ta,W,Re,Os,Ir,Pt,Au,Hg,Tl) are presented. Here, the experimental data are compiled and evaluated, and best values for level and gamma-ray energies, quantum numbers, lifetimes, gamma-ray intensities and transition probabilities, and other nuclear properties are recommended. Inconsistencies and discrepancies that exist in the literature are discussed.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2016

Nuclear Data Sheets for A = 79

Nuclear spectroscopic information for known nuclides of mass number 79 (Ni,Cu,Zn,Ga,Ge,As,Se,Br,Kr,Rb, Sr,Y,Zr) has been evaluated and presented together with adopted energies, Jπ, and decay modes of levels in these nuclei. No data are yet available for excited states in {sup 79}Ni, {sup 79}Cu and {sup 79}Zr. The half–life of {sup 79}Se, a nuclide of importance in reactor–irradiated fuel composition has been measured by several independent groups and reported in a number of publications after 1995, and seems to be converging to a narrow margin of experimental values. These measurements were likely prompted by a recommendation made in the 1993 update of A = 79 nuclides (1993Si28), that since a 1949PaZZ report, there had been no measurement until 1993, and that based on simulation studies by 1993HeZW, the value listed in 1949PaZZ, and cited in all data tables and charts for 44 years, was quite likely in error, being too low by a factor of 10. According to conclusions in recent papers such as 2014Do20, there is still room for improvement in the measurement of this half–life, and further experiments are expected. This evaluation supersedes earlier Nuclear Data Sheets for A = 79 (2002Si13,1993Si28, 1982Si21,1975Ur03).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Covariances in the Generalized Nuclear Data (GND) Structure

The Generalized Nuclear Data structure (GND) is being designed as a new standard for storing evaluated nuclear data. It is intended as an eventual replacement for the ENDF-6 format, and as such must be capable of handling at a minimum all the types of data supported by ENDF-6, including central values and covariances. Containers for storing covariances in GND are being developed, with the goal of representing covariance data in a simple and concise manner, that is easy to read, understand and use. This paper presents an overview of the status of covariances in GND, and on the tools for generating and using covariance data that are being implemented in LLNL's nuclear data toolkit ‘Fudge’.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Nuclear Data Sheets for A = 112

Evaluated nuclear structure and decay data for all nuclei within the A = 112 mass chain are presented. The experimental data are evaluated and best values for level and gamma-ray energies, quantum numbers, lifetimes, gamma-ray intensities, and other nuclear properties are recommended. Inconsistencies and discrepancies that exist in the literature are noted. This work supersedes the earlier evaluation by D. De Frenne and E. Jacobs (1996De55), published in Nuclear Data Sheets79, 639 (1996)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

Nuclear Data Sheets for A = 86

The experimental nuclear spectroscopic data for known nuclides of mass number 86 (Ga, Ge, As, Se, Br, Kr, Rb, Sr, Y, Zr, Nb, Mo, Tc) have been evaluated and presented together with Adopted properties for levels and γ rays. New high-spin data are available for {sup 86}Se, {sup 86}Br, {sup 86}Kr, {sup 86}Sr, {sup 86}Y, {sup 86}Zr and {sup 86}Mo; and lifetime data for high-spin states in {sup 86}Y and {sup 86}Zr. No significant new data since the 2001 NDS for A=86 have been reported for {sup 86}Rb and {sup 86}Nb. No data are yet available for excited states in {sup 86}Ga and {sup 86}As. The decay scheme of radioactive {sup 86}Ge is unknown, while those for {sup 86}Ga, {sup 86}As, 47.4 min isomer of {sup 86}Y, {sup 86}Nb and {sup 86}Tc are deemed as incomplete. Isomerism in {sup 86}Nb remains unconfirmed. This work supersedes the data presented in the previous NDS evaluation of A=86 published by 2001Si43.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗