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At least 37 records · Page 2

ENDF/B-VIII.1: Neutron Reaction Sublibrary

The neutrons sublibrary aims to describe nuclear reactions between incident neutron particles and different nuclei. For ENDF/B-VIII.1, many neutron files were re-evaluated or received major changes. A new 239Pu evaluation was jointly-produced by IAEA, LANL, LLNL and ORNL bringing important updates to fission neutron multiplicity, Prompt Fission Neutron Spectrum, resonance and fast regions. Around one third of the new neutron evaluations were performed as part of the INDEN collaboration, including 16,18 O, 19 F, 28,29,30 Si, 63,65 Cu, 50,51,52,53,54 Cr, 55 Mn, 54,56,57 Fe, 139 La, 233,235,238 U, 240,241 Pu. Important non-INDEN evaluations include 234,236 U, 206,207,208 Pb, 181 Ta, 88 Sr, 140,142 Ce, Pt and Dy isotopes, and many others. Also, dosimetry reactions from IRDFF-II were adopted for many materials.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Neutron Induced Fission Product Yields Sublibrary

The neutron-induced fission yields (NFY) sublibray aims to describe fission yields in neutron-induced reactions. For ENDF/B-VIII.1, there were no new fission yields complete evaluations. However, an important fix the 241 Pu NFY file was implemented, solving a long-standing anomalous discontinuity issue accidentally introduced in ENDF/B-VI.2, decades ago. Additionally, many erroneously large uncertainties, present in NFY from ENDF/B-VIII.0, were corrected.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Photoatomic Reaction Sublibrary

The photo-atomic sublibrary aims to describe atomic photon cross section data, corresponding to the interaction between photons and the different atoms. For ENDF/B-VIII.1 we adopted the EPICS2023 EPDL evaluations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Proton Reaction Sublibrary

The protons sublibrary aims to describe nuclear reactions between incident proton particles and different nuclei. For ENDF/B-VIII.1, compared to ENDF/B-VIII.0, there were only evaluation updates for 4 He.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Spontaneous Fission Product Yields Reaction Sublibrary

The spontaneous fission yields (SFY) sublibray aims to describe fission yields that happen spontaneous, without any incident particle. For ENDF/B-VIII.1, there were no new fission yields complete evaluations. However, many erroneously large uncertainties, present in both SFY from ENDF/B-VIII.0, were corrected.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Neutron Standards Sublibrary

The neutron standards sublibrary describes specific reaction cross sections, in a limited range, that are so well-known that they are used as ratios or references in other measurements. ENDF/B-VIII.1 remains unchanged from ENDF/B-VIII.0 for the neutron standards sublibrary

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Thermal Neutron Scattering Sublibrary

The thermal neutron scattering law (TSL) sublibrary aims to describe the interaction of incident neutrons at thermal or sub-thermal energies with different compound materials such fuels, moderators and special-purpose materials. In ENDF/B-VIII.1 there was a large number of new and updated TSL evaluations, including traditional moderators (light water, Beryllium metal, Beryllium Oxide, Calcium Hydride, plastics (Polystyrene and Lucite), graphite (reactor-grade and crystalline), anhydrous Hydrogen Fluoride, and heavy paraffinic oil); exotic moderators (Beryllium Carbide, Zirconium Hydride, Yttrium Hydride, Lithium-7 Hydride and Deuteride), FLiBe molten salt, structural materials and cladding (Silicon Carbide, Silicon Dioxide, Zirconium Carbide), fuels (Plutonium Dioxide, Uranium Carbide, Uranium metal, Uranium Nitride, Uranium Dioxide, Uranium Hydride), and special purpose materials. In ENDF/B-VIII.1 we also distribute alongside the evaluated files, a comma-separated file (CSV), named TSL_MAT_numbers.csv, which lists all evaluated files in the current release and their corresponding unique MAT number.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

ENDF/B-VIII.1: Triton Reaction Sublibrary

The tritons sublibrary aims to describe nuclear reactions between incident triton particles and different nuclei. For ENDF/B-VIII.1, compared to ENDF/B-VIII.0, there were only evaluation updates for 4 He.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Adaptive-in-temperature method for fast on-the-fly sampling of thermal neutron scattering data in MCNP6 [Slides]

The project objective and motivation is to develop thermal data libraries for selected isotopes in MCNP6 to support on-the-fly S(alpha, beta) sampling for temperature ranges applicable to nuclear criticality safety, thereby enhancing the physics treatment in MCNP6 so that it can perform fast on-the-fly sampling of S(alpha, beta) data at arbitrary temperature.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Fast On-The-Fly Monte Carlo Sampling of Temperature Dependent Thermal Scattering [Slides]

This presentation highlights the process of developing a thermal data library for MCNP6 to support on-the-fly S(alpha, beta) sampling for temperature ranges applicable to nuclear criticality safety. Advanced on-the-fly (OTF) strategy driven libraries have been developed for six materials based on ENDF/B-VIII.0. Validation of the OTF libraries is being conducted currently.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The PARADIGM Project: Case Study in Balancing Experiment Uncertainty with Design simplicity

Accurate nuclear data are required for simulations of many applications including nuclear criticality safety. Actinide nuclear data at intermediate energies (from 1 to 100s of keV) are imprecise and inaccurate, because of scarce differential data, and an insufficient theory approach to capture the structures expected in the data to yield evaluated nuclear data, and lack of integral data for proper validation. This is a known deficiency but has proved challenging to address. More specifically, only 5% of integral experiments in the International Criticality Safety Benchmark Evaluation Project (ICSBEP) benchmark suite address intermediate energies (Fig. 1). Associated calculated effective multiplication factor, k eff , values for these experiments are far outside the experimental uncertainties and are 25× further from experiment than for fast energies. These differences could either stem from systematic biases in nuclear data, experiments or both. The goal of the PARADIGM (PARallel Approach of Differential and InteGral Measurements) project is to significantly reduce (by more than tens of percent) the uncertainties of intermediate energy actinide nuclear data. The PARADIGM project designed and intends to execute LANSCE (Los Alamos Neutron Science CEnter) and NCERC (National Criticality Experiments Research Center) intermediate experiments in parallel. They will specifically address a high priority nuclear data need—reducing bias and uncertainty in intermediate plutonium nuclear data. The two experiment will achieve that by informing each other and nuclear theory. By doing all these steps in parallel, the timeline to deliver improved nuclear data to users will significantly be reduced. This work will focus on the integral experiment final design and the balance of design and modeling simplicity while minimizing experiment uncertainty.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nuclear Criticality Safety Margin and Handbook Data: Concepts and Applications [Slides]

At the end of this briefing, personnel should be able to: • Define concepts associated with criticality safety margin • Provide and understand practical applications that illustrate safety margin concepts • Describe how safety margin is addressed in criticality safety evaluations • Improve documentation and communication of safety margin • Connect these concepts to related statements in the ANS-8 Standards • Find numerous applications for handbook data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Gaussian Process Optimization of Sensitivity-Based Similarity Metrics between New Nuclear Applications and New/Existing Benchmarks [Slides]

This presentation discusses Nuclear Criticality Safety (NCS) and how designing safe, new nuclear criticality experiments requires expert judgement, which could take years of experience. Sensitivity/uncertainty (S/U) analysis can be utilized by less experienced individuals to conservatively estimate uncertainties in important parameters, such as k eff , in newly proposed nuclear experiments. The presentation poses the question of how this analysis can be performed and states that the answer lies in matching new nuclear experiments with existing benchmark experiments using similarity metrics. By increasing the criticality safety of the application in this work, higher mass limits could be used in PF-4 operations. Additionally, the presentation discusses MCNP6.2®, Whisper-1.1, the software that can be used in this analysis. Also discussed is the fact that International Criticality Safety Benchmark Evaluation Project (ICSBEP) benchmarks rarely match new nuclear applications and that there are significant differences in given set of materials and/or geometry. If there are no benchmarks that match the application, the presentation discusses the possibility of creating new benchmarks. In conclusion, this work presents a Gaussian process (GP) optimization scheme that was used to generate new benchmarks with the highest sensitivity-based similarity metrics to user-defined nuclear applications. The Gaussian process optimization successfully designed 3 new experimental benchmarks that were highly correlated to the application of interest and had k eff values near critical. Optimization over c k,i-r has shown that investigating specific isotope reactions for different applications is crucial to designing benchmark experiments. Partial contribution from Pu dominates c k similarity metric. Future work includes testing new stand-alone similarity metrics or new combinations of similarity metrics as the design criterion of this optimization – design criterion is application dependent.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

On the Feynman-alpha method for reflected fissile assemblies

The Feynman-alpha method is a neutron noise technique that is used to estimate the prompt neutron period of fissile assemblies. The method and quantity are of widespread interest including in applications such as nuclear criticality safety, safeguards and nonproliferation, and stockpile stewardship; the prompt neutron period may also be used to infer the k eff multiplication factor. The Feynman-alpha method is predicated on time-correlated neutron detections that deviate from a Poisson random variable due to multiplication. Traditionally, such measurements are diagnosed with one-region point kinetics, but two-region models are required when the fissile assembly is reflected. This paper presents a derivation of the two-region point kinetics Feynman-alpha equations based on a double integration of the Rossi-alpha equations, develops novel propagation of measurement uncertainty, and validates the theory. Validation is achieved with organic scintillator measurements of weapons-grade plutonium reflected by various amounts of copper to achieve k eff values of 0.83–0.94 and prompt periods of 5–75 ns. The results demonstrate that Feynman-alpha measurements should use the two-region model instead of the one-region model. The simplified one-region model deviates from the validated two-region models by as much as 10% in the estimate of the prompt neutron period, and the two-region model reduces to the one-region model for small amounts of reflector. The Feynman-alpha estimates of the prompt neutron period are compared to those of the Rossi-alpha approach. The comparative results demonstrate that the Feynman-alpha method is more precise than the Rossi-alpha method and more accurate for k eff < 0.92, whereas the Rossi-alpha method is generally more accurate for higher multiplications. Here, the uncertainty propagation developed in this work should be used for all Feynman-alpha measurements and will therein improve fitting accuracy and appropriate precision estimates.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Physics-based hybrid machine learning for critical heat flux prediction with uncertainty quantification

Critical heat flux (CHF) is a key quantity in nuclear system modeling due to its impact on heat transfer, safety margins, and reactor performance. This study develops and validates an uncertainty-aware hybrid modeling approach that combines machine learning with physics-based models to predict CHF in cases of dryout. The Biasi and Bowring empirical correlations were paired with three ML uncertainty quantification (UQ) techniques: deep neural network (DNN) ensembles, Bayesian neural networks (BNNs), and deep Gaussian processes (DGPs). A pure ML model without a base model was evaluated for comparison. Model performance was assessed under plentiful (7,350 points) and limited (9 points) training data scenarios using parity, uncertainty distributions, and calibration curves. Results show that the Biasi hybrid DNN ensemble achieved the best overall performance, with a mean absolute relative error of 1.846%, and well-calibrated uncertainty estimates. The BNN-based hybrids showed slightly higher error (2.14%) but superior uncertainty calibration. DGP models underperformed, with over 6% error and poor uncertainty calibration. All hybrid models outperformed pure machine learning configurations, demonstrating resistance against data scarcity. These findings indicate that hybrid modeling significantly improves predictive accuracy, interpretability, and resilience to data scarcity. The integration of uncertainty awareness provides actionable confidence in CHF predictions, which is vital for safety-critical decisions in nuclear applications. This hybrid approach offers a viable pathway for deploying ML models in reactor analysis tools while preserving domain knowledge and physical consistency.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Advancing the Theory of Nuclear Data Evaluations [Abstract]

We present recent advances in the R-matrix formalism as well as the Bayesian evaluation framework for improved nuclear data evaluations. The advances in the R matrix formalism include: 1) direct processes, 2) doorway, as well as multistep, processes, and 3) various forms of the Reich-Moore approximation for eliminated capture channels. Furthermore, to address unreasonably small posterior uncertainties often encountered in nuclear data evaluations of large data sets using the conventional form of the Bayes’ theorem, we introduce imperfections (of the data or the model) as a formal evaluation tool for taming the evaluated uncertainties in harmony with Bayes’ theorem. These theoretical advances were motivated by the nuclear data evaluations of differential resolved resonance cross section data using the code SAMMY, as well as the integral benchmark experiments using the SCALE code system, being performed at Oak Ridge National Laboratory for the Nuclear Criticality Safety Program. Some pedagogical applications of the new formalism, as well as a snapshot of the SAMMY modernization efforts, will be presented.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Sensitivity Studies, Gap Analysis, and Benchmark Experiment Optimization for Reactor Physics and Criticality Safety Applications

Many new reactor designs, such as advanced reactors and micro reactors, have materials that lack nuclear data validation. This is also true for many other applications in criticality safety and global security. Both differential and integral experiments are needed to validate cross-section data. Without this, a user cannot have confidence in the predicted results of a radiation-transport code. This work describes an approach called ARCHIMEDES (Application Relevant Critical/Subcritical HEU/Pu-based Integral Measurements for Enhancing Data and Evaluating Sensitivities) to design new criticality experiments that have similar k eff cross-section sensitivities to an application of interest. This process involves simulations to generate cross-section sensitivities to a parameter of interest (such as k eff ), a gap analysis to determine which existing benchmarks are most similar to the application, and an experiment optimization. Recently, there has been a great deal of interest in the reactor physics community on advanced reactors, micro reactors, and accelerator driven systems (ADS). This work will apply the described method to specific examples in this area. The focus of this work will be on the sensitivity study and gap analysis, while future work will include experiment design.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

An Alternative to Solution Experiments for Nuclear Data Validation: Reflection and Interaction of Juxtaposed Uranium (RAIJU) Experiment Design

The need for solution experiments was thoroughly discussed at the recent NCERC (National Criticality Experiments Research Center) Futures Meeting in September 2022 for multiple applications including criticality safety, training, and nuclear data. However, this capability does not exist anywhere in the United States. NCERC, located at the Nevada National Security Site and operated by LANL (Los Alamos National Laboratory) is the only general-purpose critical experiments laboratory in the United States. However, solution experiments are not authorized at NCERC, and obtaining that authorization would be too time consuming and costly to happen in the foreseeable future. An alternative is needed – an experimental configuration with the homogeneity of liquid experiments, but without being a liquid. This project, Reflection and Interaction of Juxtaposed Uranium (RAIJU) will fill the gap in capability within LANL, the U.S. Department of Energy, and the international community and will support current and future nuclear material processing needs.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗