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FY26 Mid-Year Report

The goal of this project is to develop specific aspects of ultra-high-resolution microcalorimeter technologies that support IAEA Nuclear Material Laboratory needs and the goals of SP-1 19/NML-003 "Microcalorimetry Analysis Technique for NML" but are outside the scope of the SP-1. The focus is on commissioning, assembly, and testing of the microcalorimeter decay energy spectrometer with superconducting transition-edge sensors (TESs) and magnetic microcalorimeters (MMCs) in preparation for transfer to the IAEA Nuclear Material Laboratory.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Microcalorimeters for IAEA NML (FY2019 NA-241 Annual Report)

The primary goal of this project was to better understand the analytical needs of the IAEA and the applications where magnetic microcalorimeter (MMC) radiation detectors might be able to address some of these needs. In support of this, the second goal was to use MMC gamma detectors in an application of potential interest for the IAEA.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Microcalorimeters for IAEA NML (Annual Report FY2020)

Based on input from Andrey Bosko (IAEA NML) during a visit to LLNL October 17-18, 2019, the project focused on adapting magnetic microcalorimeters (MMCs) for high-resolution decay energy (Q) spectroscopy of actinides. This included fabricating an MMC detector suitable for MeV signals, testing different approaches on how to embed an alpha source inside an absorber, and demonstrating Q-spectroscopy with MMCs.

42 ENGINEERING↗

Thermal links and position resolution in multi-absorber hydra microcalorimeters

The “hydra” style of position-sensitive, multi-absorber microcalorimeter is used in some imaging x-ray spectroscopy detector arrays to thermally multiplex multiple pixels to one sensor, thereby enabling readout of larger arrays for a given number of sensor readout channels. We describe the benefit of choosing a set of thermal conductance values for the links between absorbers and sensor such that the probability of misidentifying the absorber hit location is minimized while still achieving a specified x-ray energy resolution for all pixels. We illustrate the benefit of this approach as applied in our current prototype 25-pixel hydra magnetic microcalorimeter arrays for the Lynx x-ray astrophysics mission concept.

microcalorimeter↗

Radioisotope dating of nuclear materials using cryogenic decay energy spectrometry

Cryogenic decay energy spectrometry provides high energy resolution and enables absolute decay counting, offering an alternative measurement technique for radiochronometry. A cryogenic decay energy spectrometry experiment was conducted using a magnetic microcalorimeter to determine the age of a plutonium sample. The energy resolution was measured at 0.05% from 5 to 6 MeV. The time since sample purification was determined using the measured concentration ratio of the 241 Am/ 241 Pu radiochronometer. Sample age estimates based on 241 Pu alpha-decay and beta-decay counts, along with 241 Am decay counts, align with the expected sample age within expanded uncertainty (k = 2), supporting the accuracy of cryogenic decay energy spectrometry as a radiochronometric method.

and nuclear chemistry↗

Absolute decay counting of 146 Sm with 4π cryogenic microcalorimetry

We present a methodology for absolute activity counting of long-lived isotopes based on cryogenic Decay Energy Spectroscopy. A 146 Sm source was produced at the TRIUMF Laboratory and then processed and purified at Lawrence Livermore National Laboratory, yielding a pure sample. The source was embedded within a 4π thermal absorber coupled to a magnetic microcalorimeter achieving nearly 100% counting efficiency. Experimental uncertainties were studied and modeled, including thermal coupling of the source to the absorber, pulse pile-up, trigger, and event selection efficiencies. Here, the absolute activity of the pure 146 Sm source was measured to better than 1% uncertainty.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Dark Matter Search in Pu-241 Beta Decays

Our universe is predominantly composed of mysterious unknowns: Dark Matter (DM) and Dark Energy. DM constitutes approximately 27% of the universe, yet its nature and origins remain elusive. Among the various candidates for dark matter, this project focuses on the search for keV-scale sterile neutrinos. A sterile neutrino is a hypothetical particle that belongs to the neutrino family and may possess a higher mass than ordinary neutrinos. They are considered a compelling warm dark matter candidate if their mass is on the order of kilo-electronvolts. Existence of sterile neutrinos can be investigated via high precision beta spectroscopy. Sterile neutrinos can be produced during nuclear beta decay processes, similar to ordinary active neutrinos, but they uniquely alter the beta decay spectrum. The emission of sterile neutrinos will introduce a distinctive "kink" structure in the middle of the beta spectrum. This project investigated the existence of sterile neutrino dark matter by employing high-precision decay energy spectroscopy of Pu-241 beta decays using magnetic microcalorimeters (MMCs). The Pu-241 source material is embedded within the microcalorimeter detectors, enabling the measurement of full beta decay energies with ultra-high energy resolution. In this project, the most precise Pu-241 spectrum to date was obtained by collecting a total of 1 billion beta decay events in the MMC detectors. This extensive data set allows us to investigate evidence of keV sterile neutrino emission in beta decays with unprecedented sensitivity.

79 ASTRONOMY AND ASTROPHYSICS↗

Prototype Magnetic Calorimeter Arrays with Buried Wiring for the Lynx X-Ray Microcalorimeter

Metallic magnetic calorimeter (MMC) technology is a leading contender for detectors for the Lynx X-ray Microcalorimeter, which is an imaging spectrometer consisting of an array of greater than 100,000 pixels. The fabrication of such large arrays presents a challenge when attempting to route the superconducting wiring from the pixels to the multiplexed readout. If the wiring is designed to be planar, then an aggressive, submicron scale wiring pitch has to be employed, which is technically challenging to design and fabricate on account of the requirements of low inductance, low cross-talk, high critical currents and high yield. An alternative way to achieve large scale, high density wiring is through the use of multiple buried metal layers, planarized by Chemical Mechanical Planarization. This approach is well-suited for connecting thousands of pixels on a large focal plane to readout chips, and also for fabricating sensor meander coils with narrow line widths, which helps in increasing the sensor inductance and thus alleviates stray inductance issues associated with the wiring in large size arrays. In this work we describe the fabrication of high sensor inductance MMC arrays implementing Lynx concepts and incorporating multiple layers of buried Nb wiring. The detector array is composed of three sub-arrays with pixels optimized to meet the different science driven performance requirements of Lynx. In two of the sub-arrays we adopt a thermal multiplexing scheme to read out pixels by coupling 25 absorbers to a single sensor through thermal links of varied thermal conductance. We demonstrate the successful fabrication of multi-absorber MMCs with fine pitch pixels in very large size arrays.

Solid-State Physics↗

Development of Position-Sensitive Magnetic Calorimeters for X-Ray Astronomy

Metallic magnetic calorimeters (MMC) are one of the most promising devices to provide very high energy resolution needed for future astronomical x-ray spectroscopy. MMC detectors can be built to large detector arrays having thousands of pixels. Position-sensitive magnetic (PoSM) microcalorimeters consist of multiple absorbers thermally coupled to one magnetic micro calorimeter. Each absorber element has a different thermal coupling to the MMC, resulting in a distribution of different pulse shapes and enabling position discrimination between the absorber elements. PoSMs therefore achieve the large focal plane area with fewer number of readout channels without compromising spatial sampling. Excellent performance of PoSMs was achieved by optimizing the designs of key parameters such as the thermal conductance among the absorbers, magnetic sensor, and heat sink, as well as the absorber heat capacities. Micro fab ri - cation techniques were developed to construct four-absorber PoSMs, in which each absorber consists of a two-layer composite of bismuth and gold. The energy resolution (FWHM full width at half maximum) was measured to be better than 5 eV at 6 keV x-rays for all four absorbers. Position determination was demonstrated with pulse-shape discrimination, as well as with pulse rise time. X-ray microcalorimeters are usually designed to thermalize as quickly as possible to avoid degradation in energy resolution from position dependence to the pulse shapes. Each pixel consists of an absorber and a temperature sensor, both decoupled from the cold bath through a weak thermal link. Each pixel requires a separate readout channel; for instance, with a SQUID (superconducting quantum interference device). For future astronomy missions where thousands to millions of resolution elements are required, having an individual SQUID readout channel for each pixel becomes difficult. One route to attaining these goals is a position-sensitive detector in which a large continuous or pixilated array of x-ray absorbers shares fewer numbers of temperature sensors. A means of discriminating the signals from different absorber positions, however, needs to be built into the device for each sensor. The design concept for the device is such that the shape of the temperature pulse with time depends on the location of the absorber. This inherent position sensitivity of the signal is then analyzed to determine the location of the event precisely, effectively yielding one device with many sub-pixels. With such devices, the total number of electronic channels required to read out a given number of pixels is significantly reduced. PoSMs were developed that consist of four discrete absorbers connected to a single magnetic sensor. The design concept can be extended to more than four absorbers per sensor. The thermal conductance between the sensor and each absorber is different by design and consequently, the pulse shapes are different depending upon which absorber the xrays are received, allowing position discrimination. A magnetic sensor was used in which a paramagnetic Au:Er temperature-sensitive material is located in a weak magnetic field. Deposition of energy from an x-ray photon causes an increase in temperature, which leads to a change of magnetization of the paramagnetic sensor, which is subsequently read out using a low noise dc-SQUID. The PoSM microcalorimeters are fully microfabricated: the Au:Er sensor is located above the meander, with a thin insulation gap in between. For this position-sensitive device, four electroplated absorbers are thermally linked to the sensor via heat links of different thermal conductance. One pixel is identical to that of a single-pixel design, consisting of an overhanging absorber fabricated directly on top of the sensor. It is therefore very strongly thermally coupled to it. The three other absorbers are supported directly on a silicon-nitride membrane. These absorbers are thermally coupled to the sensor via Ti (5 nm)/Au250 nm) metal links. The strength of the links is parameterized by the number of gold squares making up the link. For detector performance, experimentally different pulse-shapes were demonstrated with 6 keV x-rays, which clearly show different rise times for different absorber positions. For energy resolution measurement, the PoSM was operated at 32 mK with an applied field that was generated using a persistent current of 50 mA. Over the four pixels, energy resolution ranges from 4.4 to 4.7 eV were demonstrated.

Bandler, SImon↗

Progress Toward Fast Decay Energy Spectroscopy for Actinide Analysis

Decay energy spectroscopy (DES) is an increasingly popular technique for measuring isotopic composition of actinide samples for nuclear safeguards applications. Current approaches for actinide DES utilize milligram-scale external gold absorbers (> 0.1 nJ/K) that are integrated with actinide samples through mechanical kneading and are thermally connected to microcalorimeters using indium or gold wire bonds. This leads to relatively slow sensor rise time and, consequently, limits counting speed to a few counts per second. We are developing faster metallic magnetic calorimeter-based DES by integrating actinide samples with magnetic sensor materials. This reduces signal rise time and enables high counting speed while maintaining the ability to knead the radioactive source with the absorber. We have measured signal rise time of 0.7 μs with a 1.5 mg external gold absorber using this approach. Here, we also demonstrated online DES operation using an Ortec DSPEC 50, a commercially available data acquisition system developed for semiconductor detectors.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Magnetic Calorimeter Arrays with High Sensor Inductance and Dense Wiring

We describe prototype arrays of magnetically coupled microcalorimeters fabricated with an approach scalable to very large format arrays. The superconducting interconnections and sensor coils have sufficiently low inductance in the wiring and sufficiently high inductance in the coils in each pixel, to enable arrays containing greater than 4000 sensors and 100,000 X-ray absorbers to be used in future astrophysics missions such as Lynx. We have used projection lithography to create submicron patterns (e.g., 400-nanometer-lines and spaces) in our niobium sensor coils and wiring, integrated with gold-erbium sensor films and gold X-ray absorbers. Our prototype devices will explore the device physics of metallic magnetic calorimeters as feature sizes are reduced to nanoscale.

Magnetism↗

Microcalorimeter measurement of x-ray spectra from a high-temperature magnetically confined plasma

A NASA-built x-ray microcalorimeter spectrometer has been installed on the MST facility at the Wisconsin Plasma Physics Laboratory and has recorded x-ray photons emitted by impurity ions of aluminum in a majority deuterium plasma. Much of the x-ray microcalorimeter development has been driven by the needs of astrophysics missions, where imaging arrays with few-eV spectral resolution are required. The goal of our project is to adapt these single-photon-counting microcalorimeters for magnetic fusion energy research and demonstrate the value of such measurements for fusion science. Microcalorimeter spectrometers combine the best characteristics of the x-ray instrumentation currently available on fusion devices: high spectral resolution similar to an x-ray crystal spectrometer and the broadband coverage of an x-ray pulse height analysis system. Fusion experiments are increasingly employing high-Z plasma-facing components and require measurement of the concentration of all impurity ion species in the plasma. This diagnostic has the capability to satisfy this need for multi-species impurity ion data and will also contribute to measurements of impurity ion temperature and flow velocity, Zeff, and electron density. Here, we introduce x-ray microcalorimeter detectors and discuss the diagnostic capability for magnetic fusion energy experiments. We describe our experimental setup and spectrometer operation approach at MST, and we present the results from an initial measurement campaign.

Eckart, M. E. (ORCID:0000000338945889)↗

Superconducting detectors for rare event searches in experimental astroparticle physics

Superconducting detectors have become an important tool in experimental astroparticle physics, which seeks to provide a fundamental understanding of the Universe. In particular, such detectors have demonstrated excellent potential in two challenging research areas involving rare event search experiments, namely, the direct detection of dark matter (DM) and the search for neutrinoless double beta decay. Here, we review the superconducting detectors that have been and are planned to be used in these two categories of experiments. We first provide brief histories of the two research areas and outline their significance and challenges in astroparticle physics. Then, we present an extensive overview of various types of superconducting detectors with a focus on sensor technologies and detector physics, which are based on calorimetric measurements and heat flow in the detector components. Finally, we introduce leading experiments and discuss their future prospects for the detection of DM and the search for neutrinoless double beta decay employing superconducting detectors.

transition edge sensors↗

Final Summary of On-Orbit ADR Operation on Hitomis Soft X-Ray Spectrometer Instrument

The Soft X-ray Spectrometer (SXS) on the Astro-H observatory contains a 6x6 array of x-ray microcalorimeters that are cooled to 50 mK by an adiabatic demagnetization refrigerator (ADR). The ADR consists of three stages in order to provide stable detector cooling using either a 1.2 K superfluid helium bath or a 4.5 K Joule-Thomson (JT) cryocooler as its heat sink. Astro-H was renamed Hitomi after it was successfully launched in February 2016. The SXS carried approximately 36 liters of helium into orbit, and by day 5 the helium had cooled sufficiently (1.4 K) to allow operation of the ADR. This paper summarizes the ADRs performance during the 38 days that the satellite was operational.

space astronomy↗

Superconducting Effects in Optimization of Magnetic Penetration Thermometers for X-ray Microcalorimeters

We have made high resolution x-ray microcalorimeters using superconducting MoAu bilayers and Nb meander coils. The temperature sensor is a Magnetic Penetration Thermometer (MPT). Operation is similar to metallic magnetic calorimeters, but instead of the magnetic susceptibility of a paramagnetic alloy, we use the diamagnetic response of the superconducting MoAu to sense temperature changes in an x-ray absorber. Flux-temperature responsivtty can be large for small sensor heat capacity, with enough dynamic range for applications. We find models of observed flux-temperature curves require several effects to explain flux penetration or expulsion in the microscopic devices. The superconductor is non-local, with large coherence length and weak pinning of flux. At lowest temperatures, behavior is dominated by screening currents that vary as a result of the temperature dependence of the magnetic penetration depth, modified by the effect of the nonuniformity of the applied field occurring on a scale comparable to the coherence length. In the temperature regime where responslvity is greatest, spadal variations in the order parameter become important: both local variations as flux enters/leaves the film and an intermediate state is formed, and globally as changing stability of the electrical circuit creates a Meissner transition and flux is expelled/penetrates to minimize free energy.

Stevenson, Thomas R.↗

Magnetic Calorimeter Option for the Lynx X-Ray Microcalorimeter

One option for the detector technology to implement the Lynx x-ray microcalorimeter (LXM) focal plane arrays is the metallic magnetic calorimeter (MMC). Two-dimensional imaging arrays of MMCs measure the energy of x-ray photons by using a paramagnetic sensor to detect the temperature rise in a microfabricated x-ray absorber. While small arrays of MMCs have previously been demonstrated that have energy resolution better than the 3 eV requirement for LXM, we describe LXM prototype MMC arrays that have 55,800 x-ray pixels, thermally linked to 5688 sensors in “hydra” configurations, and that have sensor inductance increased to avoid signal loss from the stray inductance in the large-scale arrays when the detectors are read out with microwave superconducting quantum interference device multiplexers, and that use multilevel planarized superconducting wiring to provide low-inductance, low-crosstalk connections to each pixel. We describe the features of recently tested MMC prototype devices and simulations of expected performance in designs opti- mized for the three subarray types in LXM.

Stevenson, Thomas R.↗

Superconducting Effects in Optimization of Magnetic Penetration Thermometers for X-ray Microcalorimeters

Like MMCs, MPTs enable high energy microcalorimeters with zero bias power dissipation and potential resolution < 1 eV. MPTs can provide d(phi)/dT as large as 1000 (Phi)(sub 0)/K, with no excess noise, thereby reducing the importance of SQUID noise. Long coherence length in a Type-I superconducting MoAu film offers multiple advantages for efficient flux expulsion in MPT. Region of steepest d(phi)/dT is the Meissner effect in the small device; flux is expelled/penetrates to minimize free energy. Steepness of transition can be engineered with choice of film thickness and coil pitch relative to lambda(sub eff)(0), ratio of T/T(sub c), and bias circuit inductance.

Stevenson, T. R.↗

Design of Magnetic Shielding and Field Coils for a TES X-Ray Microcalorimeter Test Platform

The performance of transition-edge sensors (TES) and their SQUID multiplexed readouts is very sensitive to ambient magnetic field and its fluctuations. In order to run ground experiments on thousands of X-ray TES microcalorimeters with a small uniform ambient magnetic field (< 1 μT, with a uniformity < 0.1 μT), we need a very low ambient field to be trapped into the superconducting magnetic shields. We have designed a sub-Kelvin test platform to reach these specifications. For this purpose, we modeled a new design for the shielding consisting of a series of different mu-metal and superconducting shields, including a niobium shield at 50 mK, a cryoperm (A4K) shield at 3 K, and a mu-metal shield at 300 K. A magnetic field coil is used to vary the local perpendicular magnetic field over the TES array. To optimize this field, we have studied a number of different field-coil designs and the impact of the different shield geometries, in order to reach the required field uniformity.

Miniussi, Antoine R.↗