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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2011

Synthesis and characterization of monodisperse, mesoporous, and magnetic sub-micron particles doped with a near-infrared fluorescent dye

Recently, multifunctional silica nanoparticles have been investigated extensively for their potential use in biomedical applications. We have prepared sub-micron monodisperse and stable multifunctional mesoporous silica particles with a high level of magnetization and fluorescence in the near infrared region using an one-pot synthesis technique. Commercial magnetite nanocrystals and a conjugated-NIR-dye were incorporated inside the particles during the silica condensation reaction. The particles were then coated with polyethyleneglycol to stop aggregation. X-ray diffraction, N{sub 2} adsorption analysis, TEM, fluorescence and absorbance measurements were used to structurally characterize the particles. These mesoporous silica spheres have a large surface area (1978 m{sup 2}/g) with 3.40 nm pore diameter and a high fluorescence in the near infrared region at {lambda}=700 nm. To explore the potential of these particles for drug delivery applications, the pore accessibility to hydrophobic drugs was simulated by successfully trapping a hydrophobic ruthenium dye complex inside the particle with an estimated concentration of 3 wt%. Fluorescence imaging confirmed the presence of both NIR dye and the post-grafted ruthenium dye complex inside the particles. These particles moved at approximately 150 {mu}m/s under the influence of a magnetic field, hence demonstrating the multifunctionality and potential for biomedical applications in targeting and imaging. - Graphical Abstract: Hydrophobic fluorescent Ruthenium complex has been loaded into the mesopores as a surrogate drug to simulate drug delivery and to enhance the multifunctionality of the magnetic NIR emitting particles. Highlights: > Monodisperse magnetic mesoporous silica particles emitting in the near infrared region are obtained in one-pot synthesis. > We prove the capacity of such particles to uptake hydrophobic dye to mimic drug loading. > Loaded fluorescent particles can be moved under a magnetic field in a microfluidic device.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Experimental evidence for the formation of CoFe{sub 2}C phase with colossal magnetocrystalline-anisotropy

Attainment of magnetic order in nanoparticles at room temperature is an issue of critical importance for many different technologies. For ordinary ferromagnetic materials, a reduction in size leads to decreased magnetic anisotropy and results in superparamagnetic relaxations. If, instead, anisotropy could be enhanced at reduced particle sizes, then it would be possible to attain stable magnetic order at room temperature. Herein, we provide experimental evidence substantiating the synthesis of a cobalt iron carbide phase (CoFe{sub 2}C) of nanoparticles. Structural characterization of the CoFe{sub 2}C carbide phase was performed by transmission electron microscopy, electron diffraction and energy electron spectroscopy. X-ray diffraction was also performed as a complimentary analysis. Magnetic characterization of the carbide phase revealed a blocking temperature, T{sub B}, of 790 K for particles with a domain size as small as 5 ± 1 nm. The particles have magnetocrystalline anisotropy of 4.6 ± 2 × 10{sup 6 }J/m{sup 3}, which is ten times larger than that of Co nanoparticles. Such colossal anisotropy leads to thermally stable long range magnetic order. Moreover, the thermal stability constant is much larger than that of the commonly used FePt nanoparticles. With thermal stability and colossal anisotropy, the CoFe{sub 2}C nanoparticles have huge potential for enhanced magnetic data storage devices.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Induced versus intrinsic magnetic moments in ultrafast magnetization dynamics

Ferromagnetic metal alloys are today commonly used in spintronic and magnetic data storage devices. These multicompound structures consist of several magnetic sublattices exhibiting both intrinsic and induced magnetic moments. Here, we study the response of the element-specific magnetization dynamics for thin film systems based on purely intrinsic (CoFeB) and partially induced (FePt) magnetic moments using extreme ultraviolet pulses from high-harmonic generation (HHG) as an element-sensitive probe. In FePt, on the one hand, we observe an identical normalized transient magnetization for Fe and Pt throughout both the ultrafast demagnetization and the subsequent remagnetization. On the other hand, Co and Fe show a clear difference in the asymptotic limit of the remagnetization process in CoFeB, which is supported by calculations for the temperature-dependent behavior of the equilibrium magnetization using a dynamic spin model. Furthermore, in this work, we provide a vital step toward a comprehensive understanding of ultrafast light-induced magnetization dynamics in ferromagnetic alloys with sublattices of intrinsic and induced magnetic moments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2010

Core magnetic islands and plasma confinement in the H-1NF heliac

Plasma confinement in the vicinity of vacuum magnetic islands near the magnetic axis in the H-1NF heliac [S. M. Hamberger et al., Fusion Technol. 17, 123 (1990)] has been experimentally studied in a low temperature argon plasma. Experimental results indicate that, under favorable conditions, these low order (m=2) islands near the core of the plasma serve as 'pockets' of higher electron density. This results in significant profile modifications including enhancement of the core radial electric field to a large positive value, possibly through an electron-root ambipolar condition. The characteristics of islands are found to be dependent on the plasma collisionality and island width.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Tunable, room-temperature multiferroic Fe-BaTiO 3 vertically aligned nanocomposites with perpendicular magnetic anisotropy

Room-temperature ferromagnetic materials with perpendicular magnetic anisotropy are widely sought after for spintronics, magnetic data storage devices, and stochastic computing. To address this need, a new Fe-BaTiO 3 vertically aligned nanocomposite (VAN) has been fabricated—combining both the strong room-temperature ferromagnetic properties of Fe nanopillars and the strong room-temperature ferroelectric properties of the BaTiO 3 matrix. Furthermore, the Fe-BaTiO 3 VAN allows for highly anisotropic magnetic properties with tunable magnetization and coercivity. Additionally, to demonstrate the multiferroic properties of the Fe-BaTiO 3 system, the new metal-oxide hybrid material system has been incorporated in a multilayer stack. Overall, this new multiferroic VAN system possesses great potential in magnetic anisotropy and property tuning and demonstrates a new material family of oxide-metal hybrid systems for room-temperature multiferroic material designs.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Thermal effects on transverse domain wall dynamics in magnetic nanowires

Magnetic domain walls are proposed as data carriers in future spintronic devices, whose reliability depends on a complete understanding of the domain wall motion. Applications based on an accurate positioning of domain walls are inevitably influenced by thermal fluctuations. In this letter, we present a micromagnetic study of the thermal effects on this motion. As spin-polarized currents are the most used driving mechanism for domain walls, we have included this in our analysis. Our results show that at finite temperatures, the domain wall velocity has a drift and diffusion component, which are in excellent agreement with the theoretical values obtained from a generalized 1D model. The drift and diffusion component are independent of each other in perfect nanowires, and the mean square displacement scales linearly with time and temperature.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2011

The double electrostatic ion ring experiment: A unique cryogenic electrostatic storage ring for merged ion-beams studies

We describe the design of a novel type of storage device currently under construction at Stockholm University, Sweden, using purely electrostatic focussing and deflection elements, in which ion beams of opposite charges are confined under extreme high vacuum cryogenic conditions in separate ''rings'' and merged over a common straight section. The construction of this double electrostatic ion ring experiment uniquely allows for studies of interactions between cations and anions at low and well-defined internal temperatures and centre-of-mass collision energies down to about 10 K and 10 meV, respectively. Position sensitive multi-hit detector systems have been extensively tested and proven to work in cryogenic environments and these will be used to measure correlations between reaction products in, for example, electron-transfer processes. The technical advantages of using purely electrostatic ion storage devices over magnetic ones are many, but the most relevant are: electrostatic elements which are more compact and easier to construct; remanent fields, hysteresis, and eddy-currents, which are of concern in magnetic devices, are no longer relevant; and electrical fields required to control the orbit of the ions are not only much easier to create and control than the corresponding magnetic fields, they also set no upper mass limit on the ions that can be stored. These technical differences are a boon to new areas of fundamental experimental research, not only in atomic and molecular physics but also in the boundaries of these fields with chemistry and biology. For examples, studies of interactions with internally cold molecular ions will be particular useful for applications in astrophysics, while studies of solvated ionic clusters will be of relevance to aeronomy and biology.

43 PARTICLE ACCELERATORS↗
DOE OSTI2010

Magnetoelectric coupling at metal surfaces

Magnetoelectric coupling allows the magnetic state of a material to be changed by an applied electric field. To date, this phenomenon has mainly been observed in insulating materials such as complex multiferroic oxides. Bulk metallic systems do not exhibit magnetoelectric coupling, because applied electric fields are screened by conduction electrons. We demonstrate strong magnetoelectric coupling at the surface of thin iron films using the electric field from a scanning tunnelling microscope, and are able to write, store and read information to areas with sides of a few nanometres. Our work demonstrates that high-density, non-volatile information storage is possible in metals.

36 MATERIALS SCIENCE↗
DOE OSTI2010

Observation of coupled vortex gyrations by 70-ps-time- and 20-nm-space-resolved full-field magnetic transmission soft x-ray microscopy

We employed time- and space-resolved full-field magnetic transmission soft x-ray microscopy to observe vortex-core gyrations in a pair of dipolar-coupled vortex-state Permalloy (Ni{sub 80}Fe{sub 20}) disks. The 70 ps temporal and 20 nm spatial resolution of the microscope enabled us to simultaneously measure vortex gyrations in both disks and to resolve the phases and amplitudes of both vortex-core positions. We observed their correlation for a specific vortex-state configuration. This work provides a robust and direct method of studying vortex gyrations in dipolar-coupled vortex oscillators.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2012

Delayed switching applied to memristor neural networks

Magnetic flux and electric charge are linked in a memristor. We reported recently that a memristor has a peculiar effect in which the switching takes place with a time delay because a memristor possesses a certain inertia. This effect was named the ''delayed switching effect.'' In this work, we elaborate on the importance of delayed switching in a brain-like computer using memristor neural networks. The effect is used to control the switching of a memristor synapse between two neurons that fire together (the Hebbian rule). A theoretical formula is found, and the design is verified by a simulation. We have also built an experimental setup consisting of electronic memristive synapses and electronic neurons.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2011

MAGNETIC FLUX EXPULSION IN STAR FORMATION

Stars form in dense cores of magnetized molecular clouds. If the magnetic flux threading the cores is dragged into the stars, the stellar field would be orders of magnitude stronger than observed. This well-known 'magnetic flux problem' demands that most of the core magnetic flux be decoupled from the matter that enters the star. We carry out the first exploration of what happens to the decoupled magnetic flux in three dimensions, using a magnetohydrodynamic (MHD) version of the ENZO adaptive mesh refinement code. The field-matter decoupling is achieved through a sink particle treatment, which is needed to follow the protostellar accretion phase of star formation. We find that the accumulation of the decoupled flux near the accreting protostar leads to a magnetic pressure buildup. The high pressure is released anisotropically along the path of least resistance. It drives a low-density expanding region in which the decoupled magnetic flux is expelled. This decoupling-enabled magnetic structure has never been seen before in three-dimensional MHD simulations of star formation. It generates a strong asymmetry in the protostellar accretion flow, potentially giving a kick to the star. In the presence of an initial core rotation, the structure presents an obstacle to the formation of a rotationally supported disk, in addition to magnetic braking, by acting as a rigid magnetic wall that prevents the rotating gas from completing a full orbit around the central object. We conclude that the decoupled magnetic flux from the stellar matter can strongly affect the protostellar collapse dynamics.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2010

EMERGENCE OF PROTOPLANETARY DISKS AND SUCCESSIVE FORMATION OF GASEOUS PLANETS BY GRAVITATIONAL INSTABILITY

We use resistive magnetohydrodynamical (MHD) simulations with the nested grid technique to study the formation of protoplanetary disks around protostars from molecular cloud cores that provide the realistic environments for planet formation. We find that gaseous planetary-mass objects are formed in the early evolutionary phase by gravitational instability in regions that are decoupled from the magnetic field and surrounded by the injection points of the MHD outflows during the formation phase of protoplanetary disks. Magnetic decoupling enables massive disks to form and these are subject to gravitational instability, even at {approx}10 AU. The frequent formation of planetary-mass objects in the disk suggests the possibility of constructing a hybrid planet formation scenario, where the rocky planets form later under the influence of the giant planets in the protoplanetary disk.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2010

THE EFFECT OF THE RADIAL PRESSURE GRADIENT IN PROTOPLANETARY DISKS ON PLANETESIMAL FORMATION

The streaming instability provides a promising mechanism for planetesimal formation because of its ability to concentrate solids into dense clumps. The degree of clumping strongly depends on the height-integrated solid to gas mass ratio Z in protoplanetary disks. In this Letter, we show that the magnitude of the radial pressure gradient that drives the streaming instability (characterized by {Pi} {identical_to} {eta}v{sub K} /c{sub s} , where {eta}v{sub K} is the reduction of Keplerian velocity due to the radial pressure gradient and c{sub s} is the sound speed) also strongly affects clumping. We present local two-dimensional hybrid numerical simulations of aerodynamically coupled particles and gas in the midplane of protoplanetary disks. Magnetic fields and particle self-gravity are ignored. We explore three different radial pressure gradient values appropriate for typical protoplanetary disks: {Pi} = 0.025, 0.05, and 0.1. For each {Pi} value, we consider four different particle size distributions ranging from submillimeter to meter sizes and run simulations with solid abundance from Z = 0.01 up to Z = 0.07. We find that a small radial pressure gradient strongly promotes particle clumping in that: (1) at fixed particle size distribution, the critical solid abundance Z {sub crit} above which particle clumping occurs monotonically increases with {Pi} and (2) at fixed Z, strong clumping can occur for smaller particles when {Pi} is smaller. Therefore, we expect planetesimals to form preferentially in regions of protoplanetary disks with a small radial pressure gradient.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2010

Quantum defragmentation algorithm

In this addendum to our paper [D. Burgarth and V. Giovannetti, Phys. Rev. Lett. 99, 100501 (2007)] we prove that during the transformation that allows one to enforce control by relaxation on a quantum system, the ancillary memory can be kept at a finite size, independently from the fidelity one wants to achieve. The result is obtained by introducing the quantum analog of defragmentation algorithms which are employed for efficiently reorganizing classical information in conventional hard disks.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2010

Superradiant scattering of electromagnetic waves emitted from disk around Kerr black holes

We study electromagnetic perturbations around a Kerr black hole surrounded by a thin disk on the equatorial plane. Our main purpose is to reveal the black hole superradiance of electromagnetic waves emitted from the disk surface. The outgoing Kerr-Schild field is used to describe the disk emission, and the superradiant scattering is represented by a vacuum wave field which is added to satisfy the ingoing condition on the horizon. The formula to calculate the energy flux on the disk surface is presented, and the energy transport in the disk-black hole system is investigated. Within the low-frequency approximation we find that the energy extracted from the rotating black hole is mainly transported back to the disk, and the energy spectrum of electromagnetic waves observed at infinity is also discussed.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2011

Characterization of the plastic substrates, the reflective layers, the adhesives, and the grooves of today's archival-grade recordable DVDs

The plastic substrates, reflective layers, dyes, and adhesives of four archival-grade DVDs and one standard-grade recordable DVD were analyzed to determine their chemical compositions and/or physical dimensions. Chemical analyses by ATR-FTIR, ToF-SIMS, XPS, EDX/STEM, and RBS show that all these DVDs use very similar polycarbonate plastic substrates and acrylate-based adhesives, but different reflective layers and dye write layers. In addition, physical measurements by AFM show differences in the DVD groove depth, width, and other dimensions. These chemical and physical analyses may help explain variations in DVD lifetimes and facilitate development of the next generation of archival-grade DVDs.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗