Design and Synthesis of Heterostructured Quantum Dots with Dual Emission in the Visible and Infrared
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Dramatic enhancement of near-infrared intersubband absorption in c-plane AlInN/GaN superlattices
We report substantial improvement of near-infrared (2–2.6 μm) intersubband absorption in c-plane AlInN/GaN superlattices grown by molecular beam epitaxy. Progress was obtained through optimization of AlInN growth conditions using an AlInN growth rate of 0.9-nm/min at substrate temperature of 550 °C, as well as by judiciously placing the charge into two delta-doping sheets. Structural characterization suggests that AlInN crystal quality is enhanced and interface roughness is reduced. Importantly, near-infrared absorption data indicate that the optical quality of the AlInN/GaN superlattices is now comparable with that of AlN/GaN superlattices designed to exploit near-infrared intersubband transitions.
Shirazi-HD, M.↗
Searching water megamasers by using mid-infrared spectroscopy (I): Possible mid-infrared indicators
ABSTRACT Water megamasers at 22 GHz with a gas disc configuration in galaxies provide the most precise measurements of supermassive black hole masses, as well as independent constraints on the Hubble constant in the nearby universe. The existence of other maser types, such as jet or outflow masers, represents another tracer for AGN science. However, the detection rate of water megamasers in galaxies is extremely low. Over 40 yr, only ∼ 160 galaxies are found to harbour maser emission, and ∼30 per cent of them show features in their maser emission that indicate a disc-like geometry. Therefore, increasing the detection rate of masers is a crucial task to allow expanding on maser studies. We present a comparison of mid-infrared spectroscopic data between a maser galaxy sample and a Seyfert 2 control sample. We find that maser galaxies show significant peculiarities in their mid-infrared spectra: (1) Maser galaxies tend to present stronger silicate absorption at τ9.7 $\mu\mathrm{ m}$ than the control sample, (2) PAH 11.3 $\mu$m emission in maser galaxies is much weaker than in the control sample, (3) spectral indices at 20–30 $\mu$m are steeper in maser galaxies than in the control sample and tend to be mid-infrared enhanced population. We conclude that there may be good indicators in mid-infrared and far-infrared which could differentiate maser and non-maser Seyfert 2 galaxies. Upcoming infrared facilities, such as the James Webb Space Telescope, may be able to exploit these and other useful criteria and tracers for water megamaser observations.
Lam, Man I.↗
Far infrared supplement: Catalog of infrared observations
The development of a new generation of orbital, airborne and ground-based infrared astronomical observatory facilities, including the infrared astronomical satellite (IRAS), the cosmic background explorer (COBE), the NASA Kuiper airborne observatory, and the NASA infrared telescope facility, intensified the need for a comprehensive, machine-readable data base and catalog of current infrared astronomical observations. The Infrared Astronomical Data Base and its principal data product, this catalog, comprise a machine-readable library of infrared (1 micrometer to 1000 micrometers) astronomical observations published in the scientific literature since 1965.
Gezari, D. Y.↗
Infrared astronomical data base and catalog of infrared observations
A computer data base of infrared astronomical observations has been established at NASA/Goddard Space Flight Center. It contains a summary of all infrared (1-100 microns) observations of celestial sources outside the solar system, published in the major scientific journals since 1960, as well as the contents of infrared surveys and catalogs. A Catalog of Infrared Observations (CIO) has been developed from the data base in printed and magnetic tape versions. A bibliographic Guide to the Infrared Astronomical Literature, and an Altas of Infrared Source Names and Positions will be published in conjunction with the catalog. Future plans include development of an interactive data system at Goddard which will give a user direct access to the computerized data.
Schmitz, M.↗
Infrared astronomical data base and catalog of infrared observations
The NASA/Goddard Space Flight Center has developed a computer data base of infrared astronomical observations. The data base represents a machine-readable library of infrared observational data published in the relevant literature since 1960 for celestial sources outside the solar system. It likewise includes the contents of infrared surveys and catalogs. A catalog of infrared observations has been developed in both printed and magnetic-tape formats. The data base will be accessed through a bibliographic guide and an atlas of infrared source names and positions. Future plans also include two-dimensional graphical displays of infrared data and a user-interactive data terminal.
Schmitz, M.↗
Far infrared supplement. Third edition: Catalog of infrared observations (lambda greater than or equal to 4.6 micrometers)
The Far Infrared Supplement contains a subset of the data in the full Catalog of Infrared Observations (all observations at wavelengths greater than 4.6 microns). The Catalog of Infrared Observations (CIO), NASA RP-1294, is a compilation of infrared astronomical observational data obtained from an extensive literature search of scientific journals and major astronomical catalogs and surveys. The literature search is complete for years 1965 through 1990 in this third edition. The catalog contains about 210,000 observations of roughly 20,000 individual sources, and supporting appendices. The expanded third edition contains coded IRAS 4-band data for all CIO sources detected by IRAS. The appendices include an atlas of infrared source positions (also included in this volume), two bibliographies of catalog listings, and an atlas of infrared spectral ranges. The complete CIO database is available to qualified users in printed, microfiche, and magnetic tape formats.
Gezari, Daniel Y.↗
The CubeSat Infrared Atmospheric Sounder (CIRAS), Pathfinder for the Earth Observing Nanosatellite-Infrared (EON-IR)
The CubeSat Infrared Atmospheric Sounder (CIRAS) will measure upwelling infrared radiation of the Earth in the MWIR region of the spectrum from space on a CubeSat. CIRAS will demonstrate two new infrared sounding technologies. The first is a 2D array of High Operating Temperature Barrier Infrared Detector (HOT-BIRD) material, selected for its high uniformity, low cost, low noise and higher operating temperatures than traditional materials. The detectors are hybridized to a commercial ROIC and commercial camera electronics. The second technology is an MWIR Grating Spectrometer (MGS) to be designed and developed by Ball Aerospace to provide imaging spectroscopy for atmospheric sounding in a CubeSat volume. The MGS has no moving parts and is based on heritage spectrometers including the Ball Aerospace Spaceborne Infrared Atmospheric Sounder for GEO (SIRAS-G) IIP of 2007. JPL will develop the mechanical, electronic and thermal subsystems for CIRAS. The spacecraft will be a commercially available CubeSat. The integrated system will be a complete 6U CubeSat capable of measuring temperature and water vapor profiles with good lower tropospheric sensitivity. The CIRAS is the first step towards the development of an Earth Observing Nanosatellite Infrared (EON-IR) for potential use in a future operational forecasting system.
Pagano, Thomas↗
Long-Wavelength Infrared (LWIR) Quantum Dot Infrared Photodetector (QDIP) Focal Plane Array
We have exploited the artificial atomlike properties of epitaxially self-assembled quantum dots for the development of high operating temperature long wavelength infrared (LWIR) focal plane arrays. Quantum dots are nanometer-scale islands that form spontaneously on a semiconductor substrate due to lattice mismatch. QDIPs are expected to outperform quantum well infrared detectors (QWIPs) and are expected to offer significant advantages over II-VI material based focal plane arrays. QDIPs are fabricated using robust wide bandgap III-V materials which are well suited to the production of highly uniform LWIR arrays. We have used molecular beam epitaxy (MBE) technology to grow multi-layer LWIR quantum dot structures based on the InAs/InGaAs/GaAs material system. JPL is building on its significant QWIP experience and is basically building a Dot-in-the-Well (DWELL) device design by embedding InAs quantum dots in a QWIP structure. This hybrid quantum dot/quantum well device offers additional control in wavelength tuning via control of dot-size and/or quantum well sizes. In addition the quantum wells can trap electrons and aide in ground state refilling. Recent measurements have shown a 10 times higher photoconductive gain than the typical QWIP device, which indirectly confirms the lower relaxation rate of excited electrons (photon bottleneck) in QDPs. Subsequent material and device improvements have demonstrated an absorption quantum efficiency (QE) of approx. 3%. Dot-in-the-well (DWELL) QDIPs were also experimentally shown to absorb both 45 deg. and normally incident light. Thus we have employed a reflection grating structure to further enhance the quantum efficiency. JPL has demonstrated wavelength control by progressively growing material and fabricating devices structures that have continuously increased in LWIR response. The most recent devices exhibit peak responsivity out to 8.1 microns. Peak detectivity of the 8.1 micrometer devices has reached approx. 1 x 10(exp 10) Jones at 77 K. Furthermore, we have fabricated the first long-wavelength 640x512 pixels QDP focal plane array. This QDIP focal plane may has produced excellent infrared imagery with noise equivalent temperature difference of 40 mK at 60K operating temperature. In addition, we have managed to increase the quantum efficiency of these devices from 0.1% (according to the data published in literature) to 20% in discrete devices. This is a factor of 200 increase in quantum efficiency. With these excellent results, for the first time QDIP performance has surpassed the QWIP performance. Our goal is to operate these long-wavelength detectors at much higher operating temperature than 77K which can be passively achieved in space. This will be a huge leap in high performance infrared detectors specifically applicable to space science instruments.
infrared imaging↗
NEAR-INFRARED THERMAL EMISSION DETECTIONS OF A NUMBER OF HOT JUPITERS AND THE SYSTEMATICS OF GROUND-BASED NEAR-INFRARED PHOTOMETRY
We present detections of the near-infrared thermal emission of three hot Jupiters and one brown dwarf using the Wide-field Infrared Camera (WIRCam) on the Canada-France-Hawaii Telescope (CFHT). These include Ks-band secondary eclipse detections of the hot Jupiters WASP-3b and Qatar-1b and the brown dwarf KELT-1b. We also report Y-band, K {sub CONT}-band, and two new and one reanalyzed Ks-band detections of the thermal emission of the hot Jupiter WASP-12b. We present a new reduction pipeline for CFHT/WIRCam data, which is optimized for high precision photometry. We also describe novel techniques for constraining systematic errors in ground-based near-infrared photometry, so as to return reliable secondary eclipse depths and uncertainties. We discuss the noise properties of our ground-based photometry for wavelengths spanning the near-infrared (the YJHK bands), for faint and bright stars, and for the same object on several occasions. For the hot Jupiters WASP-3b and WASP-12b we demonstrate the repeatability of our eclipse depth measurements in the Ks band; we therefore place stringent limits on the systematics of ground-based, near-infrared photometry, and also rule out violent weather changes in the deep, high pressure atmospheres of these two hot Jupiters at the epochs of our observations.
79 ASTRONOMY AND ASTROPHYSICS↗
LOW-RESOLUTION NEAR-INFRARED STELLAR SPECTRA OBSERVED BY THE COSMIC INFRARED BACKGROUND EXPERIMENT (CIBER)
We present near-infrared (0.8–1.8 μm) spectra of 105 bright (m{sub J} < 10) stars observed with the low-resolution spectrometer on the rocket-borne Cosmic Infrared Background Experiment. As our observations are performed above the Earth's atmosphere, our spectra are free from telluric contamination, which makes them a unique resource for near-infrared spectral calibration. Two-Micron All-Sky Survey photometry information is used to identify cross-matched stars after reduction and extraction of the spectra. We identify the spectral types of the observed stars by comparing them with spectral templates from the Infrared Telescope Facility library. All the observed spectra are consistent with late F to M stellar spectral types, and we identify various infrared absorption lines.
79 ASTRONOMY AND ASTROPHYSICS↗
Complementary Barrier Infrared Detector (CBIRD) with Double Tunnel Junction Contact and Quantum Dot Barrier Infrared Detector (QD-BIRD)
The InAs/GaSb type-II superlattice based complementary barrier infrared detector (CBIRD) has already demonstrated very good performance in long-wavelength infrared (LWIR) detection. In this work, we describe results on a modified CBIRD device that incorporates a double tunnel junction contact designed for robust device and focal plane array processing. The new device also exhibited reduced turn-on voltage. We also report results on the quantum dot barrier infrared detector (QD-BIRD). By incorporating self-assembled InSb quantum dots into the InAsSb absorber of the standard nBn detector structure, the QD-BIRD extend the detector cutoff wavelength from approximately 4.2 micrometers to 6 micrometers, allowing the coverage of the mid-wavelength infrared (MWIR) transmission window. The device has been observed to show infrared response at 225 K.
antimonide↗
Simultaneous far-infrared, near-infrared, and radio observations of OH/IR stars
Simultaneous far-infrared, near-infrared, and radio observations have been made of five infrared stars which show OH maser emission at 1612 MHz. These stars have very thick circumstellar dust shells and are not seen optically. The data permit a direct comparison of the far-infrared and maser emission from these sources, which strongly supports the hypothesis that the maser emission is pumped by 35 micron photons. A comparison with data obtained at earlier epochs suggests that the maser emission is saturated. The infrared and radio data are used together with estimates of the source distances to determine the luminosities and mass loss rates for these objects. The luminosities lie in the range 2000-30,000 solar luminosities and are consistent with either Mira variable or M supergiant classifications for the underlying stars. The estimated mass loss rates lie between 0.000005-0.00007 solar mass/year.
Werner, M. W.↗
Far infrared supplement: Catalog of infrared observations
The Far Infrared Supplement: catalog of infrared observations summarizes all infrared astronomical observations at far infrared wavelengths published in the scientific literature between 1965 and 1982. The Supplement list contains 25% of the observations in the full catalog of infrared observations (C10), and essentially eliminates most visible stars from the listings. The Supplement is more compact than the main Catalog (it does not contain the bibliography and position index of the C10), and is intended for easy reference during astronomical observations.
Gezari, D. Y.↗
Application of infrared radiometers for airborne detection of clear air turbulence and low level wind shear, airborne infrared low level wind shear detection test
The feasibility of infrared optical techniques for the advance detection and avoidance of low level wind shear (LLWS) or low altitude wind shear hazardous to aircraft operations was investigated. A primary feasibility research effort was conducted with infrared detectors and instrumentation aboard the NASA Ames Research Center Learjet. The main field effort was flown on the NASA-Ames Dryden B57B aircraft. The original approach visualized a forward-looking, infrared transmitting (KRS-5) window through which signals would reach the detector. The present concept of a one inch diameter light pipe with a 45 deg angled mirror enables a much simpler installation virtually anywhere on the aircraft coupled with the possibility of horizontal scanning via rotation of the forward directed mirror. Present infrared detectors and filters would certainly permit ranging and horizontal scanning in a variety of methods. CRT display technology could provide a contoured picture with possible shear intensity levels from the infrared detection system on the weather radar or a small adjunct display. This procedure shoud be further developed and pilot evaluated in a light aircraft such as a Cessna 207 or equivalent.
Kuhn, P. M.↗
Direct Aqueous-Phase Synthesis of Sub-10 nm “Luminous Pearls” with Enhanced in vivo Renewable Near-Infrared persistent luminescence
Near-infrared persistent luminescence nanoparticles (PLNPs) possess unique near-infrared persistent luminescence properties. They have recently been emerging as important materials for a wide variety of applications in chemistry and biology. Yet, they must endure high-temperature solid-state annealing reactions and subsequent complicated physical post-treatments. Herein, we report on a first direct aqueous-phase chemical synthesis route of NIR PLNPs and present their enhanced in vivo renewable near-infrared persistent luminescence. Our method leads to monodisperse PL nanoparticles as small as ca. 8 nm. More importantly, such sub-10 nm nanocrystals are readily dispersed, functionalized as well as form stable colloidal solutions in aqueous solution and cell culture medium for biological applications. Under bio-tissue penetrable red-light excitation, we found that such nanocrystals possess superior renewable PL photoluminescence in vitro and in vivo than current larger counterparts made by existing methods. We believe that this solid-state-reaction-free chemical approach overcomes the current key roadblock in regard to PLNP development, and thus will pave the way to broad use of these advanced miniature “luminous pearls” in photonics and biophotonics.
Luminous Pearls, Near-Infrared persistent luminesc↗
Improved signal to noise ratio and sensitivity of an infrared imaging video bolometer on large helical device by using an infrared periscope
An Infrared imaging Video Bolometer (IRVB) diagnostic is currently being used in the Large Helical Device (LHD) for studying the localization of radiation structures near the magnetic island and helical divertor X-points during plasma detachment and for 3D tomography. This research demands high signal to noise ratio (SNR) and sensitivity to improve the temporal resolution for studying the evolution of radiation structures during plasma detachment and a wide IRVB field of view (FoV) for tomography. Introduction of an infrared periscope allows achievement of a higher SNR and higher sensitivity, which in turn, permits a twofold improvement in the temporal resolution of the diagnostic. Higher SNR along with wide FoV is achieved simultaneously by reducing the separation of the IRVB detector (metal foil) from the bolometer's aperture and the LHD plasma. Altering the distances to meet the aforesaid requirements results in an increased separation between the foil and the IR camera. This leads to a degradation of the diagnostic performance in terms of its sensitivity by 1.5-fold. Using an infrared periscope to image the IRVB foil results in a 7.5-fold increase in the number of IR camera pixels imaging the foil. This improves the IRVB sensitivity which depends on the square root of the number of IR camera pixels being averaged per bolometer channel. Despite the slower f-number (f/# = 1.35) and reduced transmission (τ{sub 0} = 89%, due to an increased number of lens elements) for the periscope, the diagnostic with an infrared periscope operational on LHD has improved in terms of sensitivity and SNR by a factor of 1.4 and 4.5, respectively, as compared to the original diagnostic without a periscope (i.e., IRVB foil being directly imaged by the IR camera through conventional optics). The bolometer's field of view has also increased by two times. The paper discusses these improvements in apt details.
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
Reactive intermediates in {sup 4}He nanodroplets: Infrared laser Stark spectroscopy of dihydroxycarbene
Singlet dihydroxycarbene (HOC{sup ¨}OH) is produced via pyrolytic decomposition of oxalic acid, captured by helium nanodroplets, and probed with infrared laser Stark spectroscopy. Rovibrational bands in the OH stretch region are assigned to either trans,trans- or trans,cis-rotamers on the basis of symmetry type, nuclear spin statistical weights, and comparisons to electronic structure theory calculations. Stark spectroscopy provides the inertial components of the permanent electric dipole moments for these rotamers. The dipole components for trans, trans- and trans, cis-rotamers are (μ{sub a}, μ{sub b}) = (0.00, 0.68(6)) and (1.63(3), 1.50(5)), respectively. The infrared spectra lack evidence for the higher energy cis,cis-rotamer, which is consistent with a previously proposed pyrolytic decomposition mechanism of oxalic acid and computations of HOC{sup ¨}OH torsional interconversion and tautomerization barriers.
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗