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At least 37 records · Page 2

Large-Scale Production of Carbon Nanotubes Using the Jefferson Lab Free Electron Laser

We report on our interdisciplinary program to use the Free Electron Laser (FEL) at the Thomas Jefferson National Accelerator Facility (J-Lab) for high-volume pulsed laser vaporization synthesis of carbon nanotubes. Based in part on the funding of from this project, a novel nanotube production system was designed, tested, and patented. Using this new system nanotube production rates over 100 times faster than conventional laser systems were achieved. Analysis of the material produced shows that it is of as high a quality as the standard laser-based materials.

Holloway, Brian C.

TerraHertz Free Electron Laser Applications for Satellite Remote Sensing

The development of a Free Electron Laser (EL) operating in the terahertz frequency regime by the group at the University of Hawaii (Elias et al.) represents a significant new opportunity in the area of atmospheric remote sensing. The FEL has 2 salient features that create a unique opportunity. First of all it represents the only source in this frequency range with sufficient power to enable lidar instrumentation. Secondly its very high electrical efficiency (several times more efficient than any currently employed spaceborne laser) renders it a strong candidate for use in satellite remote sensing. On the negative side the atmosphere is rather strongly absorbing throughout this frequency range due primarily to the water vapor continuum absorption. This means that the instruments using this laser will not be able to access the lower troposphere because of its very high water concentration.. However the instrument will be very capable of measurements in the upper troposphere and stratosphere. A passive instrument, the Microwave Limb Sounder on the UARS satellite operated by Jet Propulsion Laboratory, has already demonstrated that this wavelength region can be used for chemical species with strong emission lines. A lidar would complement the capabilities of this instrument by providing the capability to measure absorbing species in the upper atmosphere. I will discuss the design of such an instrument in greater detail and estimate its performance in measuring a number of chemical species of interest to the Earth Science community.

Heaps, William S.

Bounds on Heavy Axions with an X-Ray Free Electron Laser

We present new exclusion bounds obtained at the European X-Ray Free Electron Laser facility (EuXFEL) on axionlike particles in the mass range 10 -3 eV ≲ m a ≲ 10 4 eV. Our experiment exploits the Primakoff effect via which photons can, in the presence of a strong external electric field, decay into axions, which then convert back into photons after passing through an opaque wall. While similar searches have been performed previously at a third-generation synchrotron [Yamaji et al., Phys. Lett. B 782, 523 (2018)], our work demonstrates improved sensitivity, exploiting the higher brightness of x-rays at EuXFEL.

47 OTHER INSTRUMENTATION

“Beam à la carte”: Laser heater shaping for attosecond pulses in a multiplexed x-ray free-electron laser

Electron beam shaping allows the control of the temporal properties of x-ray free-electron laser pulses from femtosecond to attosecond timescales. Here, we demonstrate the use of a laser heater to shape electron bunches and enable the generation of attosecond x-ray pulses. We demonstrate that this method can be applied in a selective way, shaping a targeted subset of bunches while leaving the remaining bunches unchanged. This experiment enables the delivery of shaped x-ray pulses to multiple undulator beamlines, with pulse properties tailored to specialized scientific applications.

43 PARTICLE ACCELERATORS

ExaFEL: extreme-scale real-time data processing for X-ray free electron laser science

ExaFEL is an HPC-capable X-ray Free Electron Laser (XFEL) data analysis software suite for both Serial Femtosecond Crystallography (SFX) and Single Particle Imaging (SPI) developed in collaboration with the Linac Coherent Lightsource (LCLS), Lawrence Berkeley National Laboratory (LBNL) and Los Alamos National Laboratory. ExaFEL supports real-time data analysis via a cross-facility workflow spanning LCLS and HPC centers such as NERSC and OLCF. Our work therefore constitutes initial path-finding for the US Department of Energy's (DOE) Integrated Research Infrastructure (IRI) program. We present the ExaFEL team's 7 years of experience in developing real-time XFEL data analysis software for the DOE's exascale supercomputers. We present our experiences and lessons learned with the Perlmutter and Frontier supercomputers. Furthermore we outline essential data center services (and the implications for institutional policy) required for real-time data analysis. Finally we summarize our software and performance engineering approaches and our experiences with NERSC's Perlmutter and OLCF's Frontier systems. This work is intended to be a practical blueprint for similar efforts in integrating exascale compute resources into other cross-facility workflows.

59 BASIC BIOLOGICAL SCIENCES

Quantum/classical mode evolution in free electron laser oscillators

The problem of oscillator evolution and mode competition in free electron lasers is studied. Relativistic quantum field theory is used to calculate electron wave functions, the angular distribution of spontaneous emission, and the transition rates for stimulated emission and absorption in each mode. The photon rate equation for the weakfield regime is presented. This rate equation is applied to oscillator evolution with a conventional undulator, a two-stage optical klystron, and a tapered undulator. The effects of noise are briefly discussed.

Bosco, P.

Effects of introducing a gas into the free-electron laser

The introduction of a gas into the wiggler section of a free electron laser (FEL) alters the phase velocity of the electromagnetic wave, and so changes the synchronism condition relating wavelength to wiggler parameters and beam energy. This provides a means for tuning the frequency of an oscillator, with the addition of 200 torr of hydrogen gas, the wavelength of a FEL operating in the near infrared without gas was reduced by 0.73 microns. The plasma generated from ionization of the hydrogen molecules by collisions with the electron beam diminished the oscillator gain, but this effect was eliminated by the addition of less than 0.1 percent of an electron attachment gas. Gain is also reduced by multiple scattering of the beam electrons, but this effect is not severe for a 1-m wiggler length. When hydrogen is used, a FEL with fixed wiggler parameters and electron energy can be tuned from the near infrared to about 1200 A, and, with helium, the wavelength can be reduced to 600 A.

Pantell, R. H.

Beam dynamics in a storage ring with a free-electron laser

In this paper, we study the dynamics of the electron beam in a diffraction limited storage ring with a high-gain free-electron laser. We present in detail the design, including lattice, dynamic aperture, intrabeam scattering, and coherent synchrotron radiation. The simulation of the electron storage ring combined with the free-electron laser is carried out until the electron beam reaches its equilibrium. We find that the initial exponential radiation power is reduced approximately to linear with respect to the undulator length due to the large increase of the energy spread from the free-electron laser.

43 PARTICLE ACCELERATORS

A Flat Analyzer Polycapillary Spectrometer for X-ray Absorption Spectroscopy of Dilute Transition Metals at X-ray-Free Electron Lasers

X-ray absorption spectroscopy (XAS) coupled with highly intense pulses from an X-ray-free electron laser (XFEL) can be used to track ultrafast chemical dynamics. Nonetheless, measurements for dilute samples (≤1 mM) have been exceptionally challenging, as scattering background signals dominate over the sample’s X-ray fluorescence. We show that femtosecond time-resolved XAS measurements of sub-millimolar transition metal solutions are now possible at the Linac Coherent Light Source (LCLS) using a high-throughput polycapillary XAS spectrometer, designed, developed, and commissioned at LCLS and the Stanford Synchrotron Radiation Lightsource (SSRL). The instrument integrates three polycapillary optics that collect and collimate X-ray fluorescence emitted from the interaction point with a high solid angle. X-ray collimated fluorescence is then selectively diffracted by coupled graphite analyzer crystals. As a result, the contribution of scattered photons is suppressed. Experiments at the Pt L 3 -edge on 0.1 mM aqueous K 2 PtCl 6 (delivered via a 100 μm liquid jet) were successfully performed in the laser pump X-ray probe configuration at the LCLS XCS and XPP instruments. We report the transient spectra of hexachloroplatinate within the first 10 ps after a 266 nm photoexcitation. We observed a short-lived reduced intermediate (≈2 ps). The polycapillary X-ray spectrometer at LCLS now enables the efficient study of the dynamics of ultradilute transition metals in solution. This capability opens the door to investigating plasmonic systems, photocatalysts, enzymes, and other scarce and dilute samples.

LCLS

Free electron lasers driven by linear induction accelerators: High power radiation sources

The technology of Free Electron Lasers (FELs) and linear induction accelerators (LIAs) is addressed by outlining the following topics: fundamentals of FELs; basic concepts of linear induction accelerators; the Electron Laser Facility (a microwave FEL); PALADIN (an infrared FEL); magnetic switching; IMP; and future directions (relativistic klystrons). This presentation is represented by viewgraphs only.

Orzechowski, T. J.

Over 8 hours of continuous operation of a free-electron laser driven by a laser-plasma accelerator

Since the emergence of laser-plasma accelerators (LPAs), substantial work has been dedicated to using LPAs to drive free-electron lasers (FELs) for a broad range of applications. Despite recent breakthroughs, which have proven the fundamental feasibility of operating FELs with an LPA source, stable FEL operation over multiple hours without operator input had yet to be achieved. In this work, we report significant improvements to the stability of a hundred terawatt laser system, resulting in successful demonstration of reliable, long-term operation of an LPA-driven FEL in the self-amplified spontaneous emission (SASE) regime at 420 nm. The LPA source delivered 100 MeV electron beams at 1 Hz with high stability over more than 10 h, enabling over 8 h of continuous FEL operation without operator input. The acquired data were subsequently used to investigate correlations between the measured undulator radiation and parameters of the drive laser, plasma source, and electron beam. The revealed connections between LPA and FEL performance gave important additional insights into ways to further improve and stabilize the system, thus demonstrating the capability of our setup to serve as a powerful platform for future studies of LPA-driven FEL operation. The one-of-a-kind integration of multiple stabilization concepts onto the LPA facility discussed in this manuscript yielded significant accelerator and light source improvements (with residual correlations suggesting even more is possible), which will positively impact LPA applications at large.

Kohrell, Finn [Lawrence Berkeley National Laborato

Gain-enhanced free-electron laser with an electromagnetic pump field

The feasibility of enhancing the gain for the free electron laser (FEL) with an electromagnetic (EM) pump field has been considered. The enhancement is provided by reacceleration of the electrons in the interaction region by means of a static, axial electric field. A FEL utilizing a low energy electron beam and a wiggler magnet with a periodicity on the order of 1 cm would produce far infared (FIR) radiation with wavelengths on the order of a few hundred microns. The use of the FIR radiation as the pump field in a two-stage FEL is envisioned to obtain visible radiation with a low energy electron beam. A summary is provided regarding the theory and equations of motion for the EM-pumped FEL. The derived relations are applied to the second stage of such a two-stage FEL. The obtained equations have been incorporated into a computer code which has been used to calculate laser gain and energy conversion efficiency.

Hiddleston, H. R.

The effect of space charge fields due to finite length electron beams in the free-electron laser

The space charge electric field of a finite length electron beam in the free electron laser amplifier with a tapered wiggler is analyzed. In the free drift region between the accelerator and laser, expressions for the increase of energy spread due to the self field are presented. In the FEL interaction region, the general conditions on the importance of the self electric field in the equations of motion is obtained. A numerical example of the FEL experiment at 10.6 microns is given.

Tang, C.-M.

First high peak and average power single-pass THz free-electron laser in operation

We report on the operation of the first high peak and average power single-pass terahertz free-electron laser (THz FEL) based on a high-brightness photoinjector for developing a THz source for pump-probe experiments at advanced x-ray FELs (XFELs). Electron beams with 17 MeV/c momentum and charge up to 2.4 nC were used to generate narrow-band 3 THz radiation with pulse energies of more than 0.1 mJ. The novelty of the realized method is that the undulator radiation by electron beams is much longer than the radiation wavelength, with FEL starting from coherent beam contribution rather than shot noise. This proved to be not a simple scaling of the XFEL mechanism due to the significant role of the bunching factor in the considered case.

47 OTHER INSTRUMENTATION

A high repetition rate millimeter wavelength accelerator for an X-ray free-electron laser

A compact collinear wakefield accelerator has been designed for an X-ray free-electron laser capable of operating at a pulse repetition rate in the tens of kilohertz. The maximum achievable accelerating gradient has been determined, with its limitation linked to beam breakup instability. The fabrication techniques for the principal components of the accelerator including wakefield generation, couplers for excess power extraction and diagnostics, focusing quadrupoles, and a novel undulator have been discussed. Results from various laboratory and beam-based tests on these components have been compared to their original design specifications and demonstrated very good agreement. A preliminary design for the XFEL has been presented, featuring a novel small-period, force-neutral, adjustable-phase undulator.

26 undulator

Whistler Chorus Amplification in the Magnetosphere: The Nonlinear Free‐Electron Laser Model and the Ginzburg‐Landau Equation

We present a novel nonlinear model for whistler-mode chorus amplification based on the free-electron laser (FEL) mechanism. First, we derive the nonlinear collective variable equations for the whistler-electron interaction. Consistent with in situ satellite observations, these equations predict that a small seed wave can undergo exponential growth, reaching a peak of a few hundred picoteslas after a few milliseconds, followed by millisecond timescale amplitude modulations. Next, we show that when one accounts for multiple wave frequencies and wave spatial variations, the amplitude and phase of the whistler wave can be described by the Ginzburg-Landau equation (GLE), providing a framework for the investigation of solitary wave behavior of chorus modes. These findings enhance our understanding of wave-particle interactions and space weather in the Van Allen radiation belts, deepen the connection between whistler-electron dynamics and FELs, and reveal a novel connection between whistler-mode chorus and the GLE.

Ginsburg-Landau equation

The nonlinear wave equation for higher harmonics in free-electron lasers

The nonlinear wave equation and self-consistent pendulum equation are generalized to describe free-electron laser operation in higher harmonics; this can significantly extend their tunable range to shorter wavelengths. The dynamics of the laser field's amplitude and phase are explored for a wide range of parameters using families of normalized gain curves applicable to both the fundamental and harmonics. The electron phase-space displays the fundamental physics driving the wave, and this picture is used to distinguish between the effects of high gain and Coulomb forces.

Colson, W. B.

The free-electron laser - Maxwell's equations driven by single-particle currents

It is shown that if single particle currents are coupled to Maxwell's equations, the resulting set of self-consistent nonlinear equations describes the evolution of the electron beam and the amplitude and phase of the free-electron-laser field. The formulation is based on the slowly varying amplitude and phase approximation, and the distinction between microscopic and macroscopic scales, which distinguishes the microscopic bunching from the macroscopic pulse propagation. The capabilities of this new theoretical approach become apparent when its predictions for the ultrashort pulse free-electron laser are compared to experimental data; the optical pulse evolution, determined simply and accurately, agrees well with observations.

Colson, W. B.