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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Closure Report for the Project Shoal Area: Subsurface Corrective Action Unit 447 Shoal,Nevada, Site

The U.S. Department of Energy (DOE) Office of Legacy Management (LM) has prepared this Closure Report for subsurface Corrective Action Unit (CAU) 447 at the Shoal, Nevada, Site, which was formerly called the Project Shoal Area. The Shoal site was the location of an underground nuclear test in 1963 that resulted in residual radionuclide contamination at the detonation depth of 1211 feet (ft) (DOE 2015a). The environmental restoration process and Corrective Action strategy are conducted in accordance with the Federal Facility Agreement and Consent Order (FFACO) (FFACO 1996, as amended) and all applicable Nevada Division of Environmental Protection (NDEP) statues and regulations. Responsibility for the environmental site restoration was transferred from the DOE, National Nuclear Security Administration, Nevada Field Office, to LM on October 1, 2006. The Shoal site is south of U.S. Highway 50, approximately 30 miles southeast of Fallon, in Churchill County, Nevada (Figure 1). The site was selected for underground nuclear testing in 1961, as part of the Vela Uniform Program. Vela was a research and development program directed toward locating, detecting, and identifying underground and high-altitude nuclear detonations. The Vela Uniform program was specific to underground detonations (AEC 1964). The objective of Project Shoal was to detonate a nuclear device underground in an active seismic area to improve the United States’ ability to detect, identify, and locate underground nuclear detonations. The underground nuclear test at Shoal was a joint effort between the U.S. Department of Defense (DOD) and the U.S. Atomic Energy Commission (AEC), which was the predecessor agency to DOE. Figure 1 is a map showing the site location.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
NASA NTRS1985

Enrichments for phototrophic bacteria and characterization by morphology and pigment analysis

The purpose of this investigation was to examine several sulfide containing environments for the presence of phototrophic bacteria and to obtain enriched cultures of some of the bacteria present. The field sites were Alum Rock State Park, the Palo Alto salt marsh, the bay area salt ponds, and Big Soda Lake (near Fallon, Nevada). Bacteria from these sites were characterized by microscopic examination, measurement of in vitro absorption spectra, and analysis of carotenoid pigments. Field observations at one of the bay area salt ponds, in which the salt concentration was saturating (about 30 percent NaCl) and the sediments along the shore of the pond covered with a gypsum crust, revealed a layer of purple photosynthetic bacteria under a green layer in the gypsum crust. Samples of this gypsum crust were taken to the laboratory to measure light transmission through the crust and to try to identify the purple photosynthetic bacteria present in this extremely saline environment.

Brune, D.↗
DOE OSTI2018

Terminating states in the positive-parity structures of As67

The energy levels and γ-ray decay scheme of the positive-parity states in the Tz=12 nucleus 67As have been studied by using the 40Ca(36Ar,2αp)67As reaction at a beam energy of 145 MeV. Two new band structures have been identified which can be connected to the previously known levels. The results for these bands are compared with configuration-dependent cranked Nilsson–Strutinsky calculations. The good level of agreement between theory and experiment suggests that these structures can be interpreted in terms of configurations that involve three g92 particles and that both possess noncollective terminating states.

59 ≤ A ≤ 89↗
DOE OSTI2021

Configuration mixing in 28 Mg and the 26 Mg (t,p) 28 Mg reaction

We have studied the 26 Mg(t,p) 28 Mg reaction. The nucleus 28 Mg lies between 24 Mg and 32 Mg, the latter of which is central to the “island of inversion” characterized by low-lying neutron fp-shell configurations. The present results show that the second-excited 0 + state in 28 Mg contains large fp-shell occupation for the neutrons. The experiment was performed in inverse kinematics using the HELIcal Orbit Spectrometer (HELIOS) at Argonne National Laboratory. Shell-model calculations using the SDPF-MU interaction yielded level energies and two-neutron transfer amplitudes that were used in one-step distorted-wave Furthermore, born approximation calculations to provide theoretical predictions of the proton angular distributions. In many, but not all cases, the data were in good agreement with theoretical predictions.

20 ≤ A ≤ 38↗
DOE OSTI2018

Examination of the low-energy enhancement of the γ -ray strength function of Fe 56

A model-independent technique was used to determine the gamma-ray strength function (gamma SF) of Fe-56 down to gamma-ray energies less than 1 MeV for the first time with GRETINA using the (p, p') reaction at 16MeV. No difference was observed in the energy dependence of the gamma SF built on 2(+) and 4(+) final states, supporting the Brink hypothesis. In addition, angular distribution and polarization measurements were performed. The angular distributions are consistent with dipole radiation. The polarization results show a small bias towards magnetic character in the region of the enhancement.

Jones, M. D.↗
DOE OSTI2018

Intruder configurations of excited states in the neutron-rich isotopes P 33 and P 34

Here, excited states in the neutron-rich isotopes P 33 and P 34 were populated by the O 18 + O 18 fusion-evaporation reaction at E lab = 24 MeV. The Gammasphere array was used along with the Microball particle detector array to detect γ transitions in coincidence with the charged particles emitted from the compound nucleus S 36 . The use of Microball enabled the selection of the proton emission channel. It also helped in determining the exact position and energy of the emitted proton; this was later employed in kinematic Doppler corrections. 16 new transitions and 13 new states were observed in P 33 and 21 γ rays and 20 energy levels were observed in P 34 for the first time. The nearly 4 π geometry of Gammasphere allowed the measurement of γ -ray angular distributions leading to spin assignments for many states. The experimental observations for both isotopes were interpreted with the help of shell-model calculations using the (0+1) ℏ ω PSDPF interaction. The calculations accounted for both the 0p-0h and 1p-1h states reasonably well and indicated that 2p-2h excitations might dominate the higher-spin configurations in both P 33 and P 34 .

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

First Spectroscopy of the Near Drip-line Nucleus Mg 40

One of the most exotic light neutron-rich nuclei currently accessible for experimental study is 40 Mg , which lies at the intersection of the nucleon magic number N=28 and the neutron drip line. Low-lying excited states of 40 Mg have been studied for the first time following a one-proton removal reaction from 41 Al, performed at the Radioactive Isotope Beam Factory of RIKEN Nishina Center with the DALI2 γ-ray array and the ZeroDegree spectrometer. Two γ-ray transitions were observed, suggesting an excitation spectrum that shows unexpected properties as compared to both the systematics along the Z=12, N ≥ 20 Mg isotopes and available state-of-the-art theoretical model predictions. A possible explanation for the observed structure involves weak-binding effects in the low-lying excitation spectrum.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

The Impact of Device Polarity on the Performance of Polymer–Fullerene Solar Cells

Abstract Diketopyrrolopyrrole (DPP)‐conjugated polymers are a versatile class of semiconductors for application in organic solar cells because of their tunable optoelectronic properties. A record power conversion efficiency (PCE) of 9.4% was recently achieved for DPP polymers, but further improvements are required to reach true efficiency limits. Using five DPP polymers with different chemical structures and molecular weights, the device performance of polymer:fullerene solar cells is systematically optimized by considering device polarity, morphology, and light absorption. The polymer solubility is found to have a significant effect on the optimal device polarity. Soluble polymers show a 10–25% increase in PCE in inverted device configurations, while the device performance is independent of device polarity for less soluble DPP derivatives. The difference seems related to the polymer to fullerene weight ratio at the ZnO interface in inverted devices, which is higher for more soluble DPP polymers. Optimization of the nature of the cosolvent to narrow the fibril width of polymers in the blends toward the exciton diffusion length enhances charge generation. Additionally, the use of a retroreflective foil increases absorption of light. Combined, the effects afford a PCE of 9.6%, among the highest for DPP‐based polymer solar cells.

Li, Mengmeng↗
DOE OSTI2020

Precise Control of Phase Separation Enables 12% Efficiency in All Small Molecule Solar Cells

Abstract Compared to conjugated polymers, small‐molecule organic semiconductors present negligible batch‐to‐batch variations, but presently provide comparatively low power conversion efficiencies (PCEs) in small‐molecular organic solar cells (SM‐OSCs), mainly due to suboptimal nanomorphology. Achieving precise control of the nanomorphology remains challenging. Here, two new small‐molecular donors H13 and H14 , created by fluorine and chlorine substitution of the original donor molecule H11 , are presented that exhibit a similar or higher degree of crystallinity/aggregation and improved open‐circuit voltage with IDIC‐4F as acceptor. Due to kinetic and thermodynamic reasons, H13 ‐based blend films possess relatively unfavorable molecular packing and morphology. In contrast, annealed H14 ‐based blends exhibit favorable characteristics, i.e., the highest degree of aggregation with the smallest paracrystalline π–π distortions and a nanomorphology with relatively pure domains, all of which enable generating and collecting charges more efficiently. As a result, blends with H13 give a similar PCE (10.3%) as those made with H11 (10.4%), while annealed H14 ‐based SM‐OSCs have a significantly higher PCE (12.1%). Presently this represents the highest efficiency for SM‐OSCs using IDIC‐4F as acceptor. The results demonstrate that precise control of phase separation can be achieved by fine‐tuning the molecular structure and film formation conditions, improving PCE and providing guidance for morphology design.

Bin, Haijun↗
DOE OSTI2018

Improving Automation Transparency: Addressing Some of Machine Learning’s Unique Challenges

Abstract. A variety of factors can affect one’s reliance on an automated aid. Some of these factors include one’s per-ception of the system’s trustworthiness, such as perceived reliability of the system or one’s ability to understand the system’s underlying reasoning. A mismatch between the operator’s perception and the true capabilities and charac-teristics of the system can lead to inappropriate reliance on the tool. This improper use of the system can manifest as either underutilization of the technology or complacency resulting from over-trusting the system. Increasing an au-tomated tool’s transparency is one approach that enables the operator to more appropriately rely on the technology. Transparent automated systems provide additional infor-mation that allows the user to see the system’s intent and understand its underlying processes and capabilities. Sev-eral researchers have developed frameworks to support the design of more transparent automation. However, these frameworks may not fully consider the particular challeng-es to transparency design introduced by automation that leverages machine learning. Like all automation, these systems can benefit from transparency. However, artificial intelligence poses new challenges that must be considered when designing for transparency. Unique considerations must be made in terms of the type, and amount or level of transparency information conveyed to the user.

Transparency, Machine Learning, Automation↗
DOE OSTI2018

In-situ synchrotron X-ray study of microstructural evolution during creep deformation in Grade 91 steel

Here, creep deformation mechanism of Grade 91 steel at 650 °C was investigated in-situ via wide-angle X-ray scattering (WAXS). WAXS peak broadening and a modified Williamson-Hall analysis provided information on evolution of dislocation densities in the primary α–Fe phase, while WAXS peak shifts provided lattice strains in the α–Fe matrix, M 23 C 6 and MX precipitates. Load transfer was not evident during in-situ creep deformation, suggesting that precipitates did not significantly strengthen the matrix during creep deformation. Peak broadening results illustrated an increase in average dislocation density during primary stage creep. After onset of secondary creep, there was a decrease in dislocation density, attributed to annihilation and re-ordering of dislocations in the subgrain structure, followed by a relatively constant average dislocation density with increasing strain.

36 MATERIALS SCIENCE↗
DOE OSTI2018

LUX trigger efficiency

The Large Underground Xenon experiment (LUX) searches for dark matter using a dual-phase xenon detector. LUX uses a custom-developed trigger system for event selection. Here, the trigger efficiency, which is defined as the probability that an event of interest is selected for offline analysis, is studied using raw data obtained from both electron recoil (ER) and nuclear recoil (NR) calibrations. The measured efficiency exceeds 98% at a pulse area of 90 detected photons, which is well below the WIMP analysis threshold on the S2 pulse area. The efficiency also exceeds 98% at recoil energies of 1.3 keV and above, for both ER and NR. In conclusion, the measured trigger efficiency varies between 99% and 100% over the fiducial volume of the detector.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

UCGretina geant4 simulation of the GRETINA Gamma-Ray Energy Tracking Array

UCGretina, a geant4 simulation of the GRETINA gamma-ray tracking array of highly-segmented high-purity germanium detectors is described. We have developed a model of the array, in particular of the Quad Module and the capsules, that gives good agreement between simulated and measured photopeak efficiencies over a broad range of gamma-ray energies and reproduces the shape of the measured Compton continuum. Both of these features are needed in order to accurately extract gamma-ray yields from spectra collected in in-beam gamma-ray spectroscopy measurements with beams traveling at v / c ≳0.3 at the National Superconducting Cyclotron Laboratory and the Facility for Rare Isotope Beams. In the process of developing the model, we determined that millimeter-scale layers of passive germanium surrounding the active volumes of the simulated crystals must be included in order to reproduce measured photopeak efficiencies. In conclusion, we adopted a simple model of effective passive layers and developed heuristic methods of determining passive-layer thicknesses by comparison of simulations and measurements for a single crystal and for the full array. Prospects for future development of the model are discussed.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

The polarization sensitivity of GRETINA

Compton polarimeters have played an important role in the study of nuclear structure physics, but have often been limited in their applications because of relatively low -ray detection efficiency. With the advent of -ray tracking detector arrays, which feature nearly solid angle coverage and the ability to identify the location of Compton-scattering events to within a few millimeters, this limitation can be overcome. Here we present a characterization of the performance of the Gamma Ray Energy Tracking In-beam Nuclear Array (GRETINA) as a Compton polarimeter using the 24 Mg(p,p') reaction at 2.45 MeV proton energy. We also discuss a new capability added to the simulation package UCGretina to simulate the emission of polarized photons, and compare it to the measured data. Lastly, we use these simulations to predict the performance of the Gamma Ray Energy Tracking Array (GRETA).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

E2 rotational invariants of 0$^{+}_{1}$ and 2$^{+}_{1}$ states for 106 Cd: The emergence of collective rotation

The collective structure of 106 Cd is elucidated by multi-step Coulomb excitation of a 3.849 MeV/A beam of 106 Cd on a 1.1 mg/cm 2 208 Pb target using GRETINA-CHICO2 at ATLAS. Fourteen E2 matrix elements were obtained. The nucleus 106 Cd is a prime example of emergent collectivity that possesses a simple structure: it is free of complexity caused by shape coexistence and has a small, but collectively active number of valence nucleons. This work follows in a long and currently active quest to answer the fundamental question of the origin of nuclear collectivity and deformation, notably in the cadmium isotopes. The results are discussed in terms of phenomenological models, the shell model, and Kumar-Cline sums of E2 matrix elements. The < 0$^{+}_{2}$ ||E2||2$^{+}_{1}$ > matrix element is determined for the first time, providing a total, converged measure of the electric quadrupole strength, < Q 2 >, of the first-excited 2$^{+}_{1}$ level relative to the 0$^{+}_{1}$ ground state, which does not show an increase as expected of harmonic and anharmonic vibrations. Strong evidence for triaxial shapes in weakly collective nuclei is indicated; collective vibrations are excluded. This is contrary to the only other cadmium result of this kind in 114 Cd by C. Fahlander et al., Nucl. Phys. A485, 327 (1988), which is complicated by low-lying shape coexistence near midshell.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

Intruder configurations in 29 Ne at the transition into the island of inversion: Detailed structure study of 28 Ne

Detailed γ-ray spectroscopy of the exotic neon isotope 28 Ne has been performed for the first time using the one-neutron removal reaction from 29 Ne on a liquid hydrogen target at 240 MeV/nucleon. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for 28 Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N=20 and N=28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗