Dendrite corrosion of 316L stainless steel weld joint in NaCl–MgCl2 molten salt loop
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The gravitational pressure in many astrophysical objects exceeds one gigabar (one billion atmospheres), creating extreme conditions where the distance between nuclei approaches the size of the K shell. This close proximity modifies these tightly bound states and, above a certain pressure, drives them into a delocalized state. Both processes substantially affect the equation of state and radiation transport and, therefore, the structure and evolution of these objects. Still, our understanding of this transition is far from satisfactory and experimental data are sparse. Here, in this work, we report on experiments that create and diagnose matter at pressures exceeding three gigabars at the National Ignition Facility where 184 laser beams imploded a beryllium shell. Bright X-ray flashes enable precision radiography and X-ray Thomson scattering that reveal both the macroscopic conditions and the microscopic states. The data show clear signs of quantum-degenerate electrons in states reaching 30 times compression, and a temperature of around two million kelvins. At the most extreme conditions, we observe strongly reduced elastic scattering, which mainly originates from K-shell electrons. We attribute this reduction to the onset of delocalization of the remaining K-shell electron. With this interpretation, the ion charge inferred from the scattering data agrees well with ab initio simulations, but it is significantly higher than widely used analytical models predict.
Intense x-ray pulses can cause the non-thermal structural transformation of diamond. At the SACLA XFEL facility, pump x-ray pulses triggered this phase transition, and probe x-ray pulses produced diffraction patterns. Time delays were observed from 0 to 250 fs, and the x-ray dose varied from 0.9 to 8.0 eV/atom. The intensity of the (111), (220), and (311) diffraction peaks decreased with time, indicating a disordering of the crystal lattice. From a Debye–Waller analysis, the rms atomic displacements perpendicular to the (111) planes were observed to be significantly larger than those perpendicular to the (220) or (311) planes. At a long time delay of 33 ms, graphite (002) diffraction indicates that graphitization did occur above a threshold dose of 1.2 eV/atom. These experimental results are in qualitative agreement with XTANT+ simulations using a hybrid model based on density-functional tight-binding molecular dynamics.
We have developed an experimental platform at the National Ignition Facility that employs colliding planar shocks to produce warm dense matter with uniform conditions and enable high-precision equation of state measurements. The platform uses simultaneous x-ray Thomson scattering and x-ray radiography to measure the density, electron temperature, and ionization state in warm dense matter. The experimental platform is designed to create a large volume of uniform plasma (approximately 700×700×150μm 3 ) at pressures approaching 100 Mbar and minimize the distribution of plasma conditions in the x-ray scattering volume, significantly improving the precision of the measurements. Here, in this study, we present the experimental design of the platform and compare hydrodynamic simulations to x-ray radiography data from initial experiments studying hydrocarbons, producing uniform densities within ±25% of the average probed condition. We show that the platform creates a homogeneous plasma that can be characterized using x-ray Thomson scattering. Thus, the new platform enables accurate measurements of plasma conditions necessary to test models for the equation of state and ionization potential depression in the warm dense matter regime.
Understanding the behavior of polymer foams at high energy density conditions is crucial to advance inertial fusion energy research. Here, we present a new experimental platform designed to measure the thermodynamic state of these materials at megabar pressures. At the Matter in Extreme Conditions Endstation of the Linac Coherent Light Source, we heat samples using an optical, high-intensity, femtosecond laser and dynamically probe them with ultra-short, coherent x-ray pulses of high peak brightness. We perform x-ray Thomson scattering measurements in forward and backward scattering geometries to capture both collective and non-collective electron behavior in the sample. Simultaneously, x-ray fluorescence spectroscopy is used to measure the emission from a mid-Z dopant, providing complementary information on the plasma conditions. By combining these techniques, we obtain temporally resolved temperature measurements of the transient warm dense matter states. Our initial experiments designed to benchmark the platform with carbon samples yielded data resolving the ultrafast response to laser heating with sub-picosecond resolution, measuring plasma temperatures exceeding 50 eV. These findings lay the foundation for precision studies of the dynamic evolution of laser-heated polymer foams.
Abstract This work presents first insights into the dynamics of free-surface release clouds from dynamically compressed polystyrene and pyrolytic graphite at pressures up to 200 GPa, where they transform into diamond or lonsdaleite, respectively. These ejecta clouds are released into either vacuum or various types of catcher systems, and are monitored with high-speed recordings (frame rates up to 10 MHz). Molecular dynamics simulations are used to give insights to the rate of diamond preservation throughout the free expansion and the catcher impact process, highlighting the challenges of diamond retrieval. Raman spectroscopy data show graphitic signatures on a catcher plate confirming that the shock-compressed PS is transformed. First electron microscopy analyses of solid catcher plates yield an outstanding number of different spherical-like objects in the size range between ten(s) up to hundreds of nanometres, which are one type of two potential diamond candidates identified. The origin of some objects can unambiguously be assigned, while the history of others remains speculative.
The ICARUS liquid argon time projection chamber (LArTPC) neutrino detector has been taking physics data since 2022 as part of the Short-Baseline Neutrino (SBN) Program. This paper details the equalization of the response to charge in the ICARUS time projection chamber (TPC), as well as data-driven tuning of the simulation of ionization charge signals and electronics noise. The equalization procedure removes non-uniformities in the ICARUS TPC response to charge in space and time. This work leverages the copious number of cosmic ray muons available to ICARUS at the surface. The ionization signal shape simulation applies a novel procedure that tunes the simulation to match what is measured in data. The end result of the equalization procedure and simulation tuning allows for a comparison of charge measurements in ICARUS between Monte Carlo simulation and data, showing good performance with minimal residual bias between the two.
This paper reports on a measurement of electron-ion recombination in liquid argon in the ICARUS liquid argon time projection chamber (LArTPC). A clear dependence of recombination on the angle of the ionizing particle track relative to the drift electric field is observed. An ellipsoid modified box (EMB) model of recombination describes the data across all measured angles. These measurements are used for the calorimetric energy scale calibration of the ICARUS TPC, which is also presented. The impact of the EMB model is studied on calorimetric particle identification, as well as muon and proton energy measurements. Accounting for the angular dependence in EMB recombination improves the accuracy and precision of these measurements.
The ICARUS liquid argon TPC detector is taking data on the Booster (BNB) and Main Injector (NuMI) Neutrino beam lines at Fermilab with a trigger system based on the scintillation light produced by charged particles in coincidence with the proton beam extraction from the accelerators. The architecture and the deployment of the trigger system in the first two runs for physics are presented, as well as the triggered event rates. The event recognition efficiency has been evaluated as a function of the deposited energy and the position of cosmic muons stopping inside the detector.
This paper describes the cryogenic and purification systems of the ICARUS T600 detector in its present implementation at the Fermi National Laboratory, Illinois, U.S.A. The ICARUS T600 detector is made of four large Time Projection Chambers, installed in two separate containers of about 275 m 3 each. The detector uses liquid argon both as target and as active medium. For the correct operation of the detector, the liquid argon must be kept in very stable thermal conditions and the contamination of electronegative impurities must be consistently kept at the level of small fractions of parts per billion. The detector was previously operated in Italy, at the INFN Gran Sasso Underground Laboratory (LNGS), in a three-year run on the CERN to LNGS Long Baseline Neutrino Beam. For its operation on the Booster and NuMI neutrino beams at Fermilab, for the search of sterile neutrinos and measurements of neutrino-argon cross sections, the detector was moved from Gran Sasso to CERN for the upgrades required for operation at shallow depth with high intensity neutrino beams. The liquid argon containers, the thermal insulation and all the cryogenic equipment have been completely re-designed and rebuilt, following the schemes of the previous installation in Gran Sasso. The detector and all the equipment have been transported to Fermilab, where they have been installed, tested and recently put into operation. The work described in this paper has been conducted as a joint responsibility of CERN and Fermilab with the supervision provided by the ICARUS Collaboration. Design, installation, testing, commissioning and operation are the result of a common effort of CERN, Fermilab and INFN groups.
This paper presents the first neutrino cross-section measurement from the ICARUS detector at Fermilab, using Neutrinos at the Main Injector (NuMI) beam data collected from two beam operation periods corresponding to 2.5 × 10 20 protons-on-target in neutrino beam mode. The signal is defined by events with no pions produced in the final state, a topology dominated by charged-current quasielasticlike signatures. The measurement is reported as flux-averaged differential cross sections as functions of kinematic variables that provide sensitivity to the complex nuclear effects that often dominate the systematic uncertainty budgets of neutrino oscillation measurements. Specifically, this work reports cross sections in two angular variables—the angle of the outgoing lepton and the opening angle between the lepton and leading proton—and two variables characterizing the kinematic imbalance between the muon and proton in the plane transverse to the incoming neutrino. These results are compared against predictions from a variety of neutrino event generators, with p values calculated between the extracted cross sections and each prediction. Overall, the predictions agree with the data; however, the current budget of uncertainties does not yet provide sufficient discriminating power to favor a specific model.
We present the use of x-ray fluorescence spectroscopy (XFS) to a sensitive temperature diagnostic in shocked foams at temperatures of 30–75 eV. Cobalt-doped foams were shock compressed using a planar drive at the OMEGA laser facility and photo-pumped with a Zn He𝛼 x-ray source. Analysis of the resulting cobalt 𝐾𝛽 x-ray fluorescence spectra using collisional radiative codes allows the temperature to be determined in the shocked foams. Furthermore, this method provides a sensitive and robust technique to determine temperatures in high-energy-density physics experiments in the tens of electronvolts temperature range. In these experiments, we find that radiation hydrodynamic simulations predict a lower temperature in the shocked foams compared to analysis of the XFS data using collisional radiative models. Although additional experiments with an independent temperature diagnostic to absolutely calibrate XFS spectra for these conditions will be required to resolve this discrepancy, these results demonstrate the excellent temperature sensitivity of XFS spectra for high-energy-density physics experiments.
We present the first measurement of the negative pion total hadronic cross section on argon in a restricted phase space, which we performed at the Liquid Argon In A Testbeam (LArIAT) experiment. All hadronic reaction channels, as well as hadronic elastic interactions with scattering angle greater than 5° are included. The pions have kinetic energies in the range 100–700 MeV and are produced by a beam of charged particles impinging on a solid target at the Fermilab test beam facility. LArIAT employs a 0.24 ton active mass liquid argon time projection chamber (LArTPC) to measure the pion hadronic interactions. For this measurement, LArIAT has developed the “thin slice method,” a new technique to measure cross sections with LArTPCs. While moderately higher, our measurement of the π - -Ar total hadronic cross section is generally in agreement with the geant4 prediction.
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We present the result of a search for inelastic boosted dark matter using the data corresponding to an exposure of 0.13 kton · year , collected by the ICARUS T-600 detector during its 2012–2013 operational period at the INFN Gran Sasso Underground National Laboratory. The benchmark boosted dark matter model features a multiparticle dark sector with a U ( 1 ) ′ gauge boson, the dark photon. The kinetic mixing of the dark photon with the Standard Model photon allows for a portal between the dark sector and the visible sector. The inelastic boosted dark matter interaction occurs when a dark matter particle inelastically scatters with an electron in the ICARUS detector, producing an outgoing, heavier dark sector state which subsequently decays back down to the dark matter particle, emitting a dark photon. The dark photon subsequently couples to a Standard Model photon through kinetic mixing. The Standard Model photon then converts to an electron-positron pair in the detector. This interaction process provides a distinct experimental signature that consists of a recoil electron from the primary interaction and an associated electron-positron pair from the secondary vertex. After analyzing 4,134 triggered events, the search results in zero observed events. Exclusion limits are set in the dark photon mass and coupling ( m X , ε ) parameter space for several selected optimal boosted dark matter mass sets and cover previously unexplored parameter space. Published by the American Physical Society 2025
We present a search for long-lived particles (LLPs), produced in kaon decays, that decay to two muons inside the ICARUS neutrino detector. This channel would be a signal of hidden sector models that can address outstanding issues in particle physics such as the strong CP problem and the microphysical origin of dark matter. The search is performed with data collected in the Neutrinos at the Main Injector (NuMI) beam at Fermilab corresponding to 2.41 × 10 20 protons-on-target. No new physics signal is observed, and we set world leading limits on heavy QCD axions, as well as for the Higgs portal scalar among dedicated searches. Limits are also presented in a model-independent way applicable to any new physics model predicting the process 𝐾 → 𝜋 + 𝑆(→ 𝜇𝜇), for a LLP 𝑆. This result is the first search for new physics performed with the ICARUS detector at Fermilab. It paves the way for the future program of LLP searches at ICARUS.
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Germline-targeting (GT) HIV vaccine strategies are predicated on deriving broadly neutralizing antibodies (bnAbs) through multiple boost immunogens. However, as the recruitment of memory B cells (MBCs) to germinal centers (GCs) is inefficient and may be derailed by serum antibody–induced epitope masking, driving further B cell receptor (BCR) modification in GC-experienced B cells after boosting poses a challenge. Using humanized immunoglobulin knockin mice, we found that GT protein trimer immunogen N332-GT5 could prime inferred-germline precursors to the V3-glycan–targeted bnAb BG18 and that B cells primed by N332-GT5 were effectively boosted by either of two novel protein immunogens designed to have minimum cross-reactivity with the off-target V1-binding responses. The delivery of the prime and boost immunogens as messenger RNA lipid nanoparticles (mRNA-LNPs) generated long-lasting GCs, somatic hypermutation, and affinity maturation and may be an effective tool in HIV vaccine development.