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NASA NTRS1992

A Segmented Ion-Propulsion Engine

New design approach for high-power (100-kW class or greater) ion engines conceptually divides single engine into combination of smaller discharge chambers integrated to operate as single large engine. Analogous to multicylinder automobile engine, benefits include reduction in required accelerator system span-to-gap ratio for large-area engines, reduction in required hollow-cathode emission current, mitigation of plasma-uniformity problem, increased tolerance to accelerator system faults, and reduction in vacuum-system pumping speed.

Brophy, John R.↗

NASA NTRS2016

Health and Climate Impacts of Ocean-Going Vessels in East Asia

East Asia has the most rapidly growing shipping emissions of both CO2 and traditional air pollutants, but the least in-depth analysis. Full evaluation of all pollutants is needed to assess the impacts of shipping emissions. Here, using an advanced method based on detailed dynamic ship activity data, we show that shipping emissions in East Asia accounted for 16% of global shipping CO2 in 2013, compared to only 4-7% in 2002-2005. Increased emissions lead to large adverse health impacts, with 14,500-37,500 premature deaths per year. Global mean radiative forcing from East Asian shipping is initially negative, but would become positive after approximately eight years for constant current emissions. As a large fraction of vessels are registered elsewhere, joint efforts are necessary to reduce emissions and mitigate the climate and health impacts of shipping in the region.

climate change impacts↗

NASA NTRS2016

Foreground Bias from Parametric Models of Far-IR Dust Emission

We use simple toy models of far-IR dust emission to estimate the accuracy to which the polarization of the cosmic microwave background can be recovered using multi-frequency fits, if the parametric form chosen for the fitted dust model differs from the actual dust emission. Commonly used approximations to the far-IR dust spectrum yield CMB residuals comparable to or larger than the sensitivities expected for the next generation of CMB missions, despite fitting the combined CMB plus foreground emission to precision 0.1 percent or better. The Rayleigh-Jeans approximation to the dust spectrum biases the fitted dust spectral index by (Delta)(Beta)(sub d) = 0.2 and the inflationary B-mode amplitude by (Delta)(r) = 0.03. Fitting the dust to a modified blackbody at a single temperature biases the best-fit CMB by (Delta)(r) greater than 0.003 if the true dust spectrum contains multiple temperature components. A 13-parameter model fitting two temperature components reduces this bias by an order of magnitude if the true dust spectrum is in fact a simple superposition of emission at different temperatures, but fails at the level (Delta)(r) = 0.006 for dust whose spectral index varies with frequency. Restricting the observing frequencies to a narrow region near the foreground minimum reduces these biases for some dust spectra but can increase the bias for others. Data at THz frequencies surrounding the peak of the dust emission can mitigate these biases while providing a direct determination of the dust temperature profile.

cosmic microwave background↗

NASA NTRS2022

Gulf of Mexico Health & Air Quality Ii: Mapping Methane Emission Plumes Using Sunglint-Configured Imagery for Monitoring Offshore Oil and Gas Activity

Offshore oil and gas production in the United States is a major source of anthropogenic greenhouse gas emissions and accounts for nearly 30% of global oil and gas production. Methane venting and flaring are primary contributors to offshore emissions, and monitoring these activities is crucial for mitigating greenhouse gas emissions. Limited ground truthing and intermittent offshore satellite revisits make monitoring venting and flaring challenging. The Bureau of Ocean Energy Management (BOEM) and the Bureau of Safety and Environmental Enforcement (BSEE) oversee offshore oil and gas activity but rely primarily on operator-reported data. The non-profit organization SkyTruth monitors natural resources like methane and identifies sources of fugitive emissions. By combining BOEM and BSEE’s operational data along with observations from Sentinel-2 Multispectral Instrument (MSI), Landsat 8 Operational Land Imager (OLI) and Landsat 9 OLI-2, and PRecursore IperSpettrale della Missione Applicativa (PRISMA), the team further identified ultra-emitter point sources in the Gulf of Mexico using sunglint-configured imagery. We quantified these plume emission rates using the methodology from Varon et al. (2020). The team found three plumes in the Gulf of Mexico occurring between 2020 and 2022 using Sentinel-2 MSI and Landsat 9 OLI-2 imagery, in addition to the single plume identified by the Gulf of Mexico Health & Air Quality I team, and successfully quantified three plumes. Our statistical retrieval of three PRISMA images tasked over areas of interest yielded no methane plumes, despite a successful test of a known plume in Assam, India. These analyses serve as a proof of concept for the utility of remote sensing for methane emission monitoring offshore, which can complement regulator emission inventories and validate self-reported operator records.

sunglint↗

NASA NTRS2017

Forest Carbon Emissions from Cropland Expansion in the Brazilian Cerrado Biome

Land use, land use change, and forestry accounted for two-thirds of Brazil's greenhouse gas emissions profile in 2005. Amazon deforestation has declined by more than 80% over the past decade, yet Brazil's forests extend beyond the Amazon biome. Rapid expansion of cropland in the neighboring Cerrado biome has the potential to undermine climate mitigation efforts if emissions from dry forest and woodland conversion negate some of the benefits of avoided Amazon deforestation. Here, we used satellite data on cropland expansion, forest cover, and vegetation carbon stocks to estimate annual gross forest carbon emissions from cropland expansion in the Cerrado biome. Nearly half of the Cerrado met Brazil's definition of forest cover in 2000 (greater than or equal to 0.5 ha with greater than or equal to 10% canopy cover). In areas of established crop production, conversion of both forest and non-forest Cerrado formations for cropland declined during 2003-2013. However, forest carbon emissions from cropland expansion increased over the past decade in Matopiba, a new frontier of agricultural production that includes portions of Maranhao, Tocantins, Piau, and Bahia states. Gross carbon emissions from cropland expansion in the Cerrado averaged 16.28 Tg C yr (exp -1) between 2003 and 2013, with forest-to-cropland conversion accounting for 29% of emissions. The fraction of forest carbon emissions from Matopiba was much higher; between 2010-2013, large-scale cropland conversion in Matopiba contributed 45% of total Cerrado forest carbon emissions. Carbon emissions from Cerrado-tocropland transitions offset 5-7% of the avoided emissions from reduced Amazon deforestation rates during 2011-2013. Comprehensive national estimates of forest carbon fluxes, including all biomes, are critical to detect cross-biome leakage within countries and achieve climate mitigation targets to reduce emissions from land use, land use change, and forestry.

remote sensing↗

NASA NTRS2024

X-57 Maxwell High Lift Motor Controller Electromagnetic Interference Test Results

During research and development for NASA’s X-57 Maxwell all-electric aircraft project, the efficiency and power density requirements of its electric propulsion subsystem components were met, but aspects of integrating its powertrain subsystems proved problematic. Electromagnetic interference (EMI) from the cruise motor controller (CMC) was a significant challenge for the project. This problem was exacerbated by the lack of EMI requirements imposed on subsystem powertrain components. This report presents the results of EMI testing of the X-57 high lift motor controller (HLMC) at the NASA Glenn Research Center’s EMI Laboratory. For reference, the conducted emissions are compared to DO–160G and MIL–STD–61G conducted emissions limits. After the EMI test, mitigation of the conducted emissions using lightweight EMI chokes produced at NASA Glenn was evaluated using the Fast Fourier Transform (FFT) capability of an oscilloscope in the hardware development laboratory. This process can contribute to the rapid prototyping of electric powertrain components and EMI filters and improve the likelihood of successful EMI qualification at the component and system levels.

Silicon carbide↗

NASA NTRS2010

Recent Stirling Conversion Technology Developments and Operational Measurements at NASA Glenn Research Center

In support of the Advanced Stirling Radioisotope Generator (ASRG) project and other potential applications, NASA Glenn Research Center (GRC) has initiated convertor technology development efforts in the areas of acoustic emission, electromagnetic field mitigation, thermoacoustic Stirling conversion, and multiple-cylinder alpha arrangements of Stirling machines. The acoustic emission measurement effort was developed as a health monitoring metric for several Stirling convertors undergoing life testing. While accelerometers have been used in the past to monitor dynamic signature, the acoustic sensors were chosen to monitor cycle events, such gas bearing operation. Several electromagnetic interference (EMI) experiments were performed on a pair of Advanced Stirling Convertors (ASC). These tests demonstrated that a simple bucking coil was capable of reducing the alternating current (ac) magnetic field below the ASRG system specification. The thermoacoustic Stirling concept eliminates the displacer typically found in Stirling machines by making use of the pressure oscillations of a traveling acoustic wave. A 100 W-class thermoacoustic Stirling prototype manufactured by Northrop Grumman Space and Technology was received and tested. Another thermoacoustic prototype designed and fabricated by Sunpower, Inc., will be tested in the near future. A four cylinder free piston alpha prototype convertor was received from Sunpower, Inc. and has been tested at GRC. This hardware was used as a proof of concept to validate thermodynamic models and demonstrate stable operation of multiple-cylinder free-piston Stirling conversion. This paper will discuss each of these activities and the results they produced.

Oriti, Salvatore M.↗

NASA NTRSDate not supplied

MISTRAL: Concept and Analysis of Persistent Airborne Localization of GHG Emissions

In this study, we propose a concept for localizing and mitigating greenhouse gases and other emissions from areas of various sizes, using a multiscale, airborne localization fleet, supported by information from satellites. Our objective is a rapidly implementable capability for the reduction of atmospheric methane by empowering the communities in proximity to emissions to actively contribute to methane mitigation via fleet operations by local governments, first responders, and individuals . Fully autonomous operations are economically desirable and technically feasible now. However, the development of regulations for autonomous operations is in early stages. Since rapid impact is critical to reducing emissions, the concept starts with remotely controlled vehicles. As regulations for autonomous operations reach maturity, the concept can be easily transitioned from the remotely piloted to autonomous mode. We report on a preliminary system analysis of the concept. Localization of methane emissions from the Permian Basin oil and gas production site serves as the design reference mission; however, the airborne concept is applicable to a broad range of use cases, and we describe several in this analysis. We consider leveraging satellite and ground-based resources within the airborne concept of operations. The study analyses uninhabited aerial system localization operations under the most conservative assumptions on resources and available information. Even under these assumptions, the concept is shown to be viable for local community operations.

airborne methane localization↗

NASA NTRS2021

Reductions in NO2 Burden Over North Equatorial Africa from Decline in Biomass Burning in Spite of Growing Fossil Fuel Use, 2005 to 2017

Socioeconomic development in low- and middle-income countries has been accompanied by increased emissions of air pollutants, such as nitrogen oxides [NOx: nitrogen dioxide (NO2) + nitric oxide (NO)], which affect human health. In sub-Saharan Africa, fossil fuel combustion has nearly doubled since 2000. At the same time, landscape biomass burning—another important NOx source—has declined in north equatorial Africa, attributed to changes in climate and anthropogenic fire management. Here, we use satellite observations of tropospheric NO2 vertical column densities (VCDs) and burned area to identify NO2 trends and drivers over Africa. Across the northern ecosystems where biomass burning occurs—home to hundreds of millions of people—mean annual tropospheric NO2 VCDs decreased by 4.5% from 2005 through 2017 during the dry season of November through February. Reductions in burned area explained the majority of variation in NO2 VCDs, though changes in fossil fuel emissions also explained some variation. Over Africa’s biomass burning regions, raising mean GDP density (USD·km−2) above its lowest levels is associated with lower NO2 VCDs during the dry season, suggesting that economic development mitigates net NO2 emissions during these highly polluted months. In contrast to the traditional notion that socioeconomic development increases air pollutant concentrations in low- and middle-income nations, our results suggest that countries in Africa’s northern biomass-burning region are following a different pathway during the fire season, resulting in potential air quality benefits. However, these benefits may be lost with increasing fossil fuel use and are absent during the rainy season.

air pollution↗

NASA NTRS2007

Lunar Dust Charging by Photoelectric Emissions

The lunar surface is covered with a thick layer of sub-micron/micron size dust grains formed by meteoritic impact over billions of years. The fine dust grains are levitated and transported on the lunar surface, as indicated by the transient dust clouds observed over the lunar horizon during the Apollo 17 mission. Theoretical models suggest that the dust grains on the lunar surface are charged by the solar UV radiation as well as the solar wind. Even without any physical activity, the dust grains are levitated by electrostatic fields and transported away from the surface in the near vacuum environment of the Moon. The current dust charging and levitation models, however, do not fully explain the observed phenomena. Since the abundance of dust on the Moon s surface with its observed adhesive characteristics has the potential of severe impact on human habitat and operations and lifetime of a variety of equipment, it is necessary to investigate the charging properties and the lunar dust phenomena in order to develop appropriate mitigating strategies. Photoelectric emission induced by the solar UV radiation with photon energies higher than the work function of the grain materials is recognized to be the dominant process for charging of the lunar dust, and requires measurements of the photoelectric yields to determine the charging and equilibrium potentials of individual dust grains. In this paper, we present the first laboratory measurements of the photoelectric efficiencies and yields of individual sub-micron/micron size dust grains selected from sample returns of Apollo 17, and Luna 24 missions, as well as similar size dust grains from the JSC-1 simulants. The measurements were made on a laboratory facility based on an electrodynamic balance that permits a variety of experiments to be conducted on individual sub-micron/micron size dust grains in simulated space environments. The photoelectric emission measurements indicate grain size dependence with the yield increasing by an order of magnitude for grains of sub-micron to several micron size radii, at which it reaches asymptotic values. The yield for large size grains is found to be more than an order of magnitude higher than the bulk measurements on lunar fines reported in the literature.

Abbas, M. M.↗

NASA NTRS2007

Lunar Dust Charging by Photoelectric Emissions

The lunar surface is covered with a thick layer of sub-micron/micron size dust grains formed by meteoritic impact over billions of years. The fine dust grains are levitated and transported on the lunar surface, as indicated by the transient dust clouds observed over the lunar horizon during the Apollo 17 mission. Theoretical models suggest that the dust grains on the lunar surface are charged by the solar ultraviolet (UV) radiation as well as the solar wind. Even without any physical activity, the dust grains are levitated by electrostatic fields and transported away from the surface in the near vacuum environment of the Moon. The current dust charging and levitation models, however, do not fully explain the observed phenomena. Since the abundance of dust on the Moon's surface with its observed adhesive characteristics has the potential of severe impact on human habitat and operations and lifetime of a variety of equipment, it is necessary to investigate the charging properties and the lunar dust phenomena in order to develop appropriate mitigating strategies. Photoelectric emission induced by the solar UV radiation with photon energies higher than the work function (WF) of the grain materials is recognized to be the dominant process for charging of the lunar dust, and requires measurements of the photoelectric yields to determine the charging and equilibrium potentials of individual dust grains. In this paper, we present the first laboratory measurements of the photoelectric efficiencies and yields of individual sub-micron/micron size dust grains selected from sample returns of Apollo 17 and Luna-24 missions as well as similar size dust grains from the JSC-1 simulants. The measurements were made on a laboratory facility based on an electrodynamic balance that permits a variety of experiments to be conducted on individual sub-micron/micron size dust grains in simulated space environments. The photoelectric emission measurements indicate grain size dependence with the yield increasing by an order of magnitude for grains of sub-micron to several micron size radii, at which it reaches asymptotic values. The yield for large size grains is found to be more than an order of magnitude higher than the bulk measurements on lunar fines reported in the literature.

Abbas, M. M.↗

NASA NTRS2021

Present and future aerosol impacts on Arctic climate change in the GISS-E2.1 Earth system model

The Arctic is warming 2 to 3 times faster than the global average, partly due to changes in short-lived climate forcers (SLCFs) including aerosols. In order to study the effects of atmospheric aerosols in this warming, recent past (1990–2014) and future (2015–2050) simulations have been carried out using the GISS-E2.1 Earth system model to study the aerosol burdens and their radiative and climate impacts over the Arctic (>60°N), using anthropogenic emissions from the Eclipse V6b and the Coupled Model Intercomparison Project Phase 6 (CMIP6) databases, while global annual mean greenhouse gas concentrations were prescribed and kept fixed in all simulations. Results showed that the simulations have underestimated observed surface aerosol levels, in particular black carbon (BC) and sulfate (SO2−4), by more than 50 %, with the smallest biases calculated for the atmosphere-only simulations, where winds are nudged to reanalysis data. CMIP6 simulations performed slightly better in reproducing the observed surface aerosol concentrations and climate parameters, compared to the Eclipse simulations. In addition, simulations where atmosphere and ocean are fully coupled had slightly smaller biases in aerosol levels compared to atmosphere-only simulations without nudging. Arctic BC, organic aerosol (OA), and SO2−4 burdens decrease significantly in all simulations by 10 %–60 % following the reductions of 7 %–78 % in emission projections, with the Eclipse ensemble showing larger reductions in Arctic aerosol burdens compared to the CMIP6 ensemble. For the 2030–2050 period, the Eclipse ensemble simulated a radiative forcing due to aerosol–radiation interactions (RFARI) of −0.39 ± 0.01 W/sq. m, which is −0.08 W/sq. m larger than the 1990–2010 mean forcing (−0.32 W/sq. m), of which −0.24 ± 0.01 W/sq. m was attributed to the anthropogenic aerosols. The CMIP6 ensemble simulated a RFARI of −0.35 to −0.40 W/sq. m for the same period, which is −0.01 to −0.06 W/sq. m larger than the 1990–2010 mean forcing of −0.35 W/sq. m. The scenarios with little to no mitigation (worst-case scenarios) led to very small changes in the RFARI, while scenarios with medium to large emission mitigations led to increases in the negative RFARI, mainly due to the decrease in the positive BC forcing and the decrease in the negative SO2−4 forcing. The anthropogenic aerosols accounted for −0.24 to −0.26 W/sq. m of the net RFARI in 2030–2050 period, in Eclipse and CMIP6 ensembles, respectively. Finally, all simulations showed an increase in the Arctic surface air temperatures throughout the simulation period. By 2050, surface air temperatures are projected to increase by 2.4 to 2.6 °C in the Eclipse ensemble and 1.9 to 2.6 °C in the CMIP6 ensemble, compared to the 1990–2010 mean. Overall, results show that even the scenarios with largest emission reductions leads to similar impact on the future Arctic surface air temperatures and sea-ice extent compared to scenarios with smaller emission reductions, implying reductions of greenhouse emissions are still necessary to mitigate climate change.

Aerosols↗

NASA NTRS2018

Land-Use Emissions Play a Critical Role in Land Based Mitigation for Paris Climate Targets

Scenarios that limit global warming to below 2 degrees Centigrade by 2100 assume significant land-use change to support large-scale carbon dioxide (CO2) removal from the atmosphere by afforestation/reforestation, avoided deforestation, and Biomass Energy with Carbon Capture and Storage (BECCS). The more ambitious mitigation scenarios require even greater land area for mitigation and/or earlier adoption of CO2 removal strategies. Here we show that additional land-use change to meet a 1.5 degrees Centigrade climate change target could result in net losses of carbon from the land. The effectiveness of BECCS strongly depends on several assumptions related to the choice of biomass, the fate of initial above ground biomass, and the fossil-fuel emissions offset in the energy system. Depending on these factors, carbon removed from the atmosphere through BECCS could easily be offset by losses due to land-use change. If BECCS involves replacing high-carbon content ecosystems with crops, then forest-based mitigation could be more efficient for atmospheric CO2 removal than BECCS.

Harper, Anna B.↗

NASA NTRS2005

National Aeronautics and Space Administration (NASA) Earth Science Research for Energy Management: Overview of Energy Issues and an Assessment of the Potential for Application of NASA Earth Science Research - Part 1

Effective management of energy resources is critical for the U.S. economy, the environment, and, more broadly, for sustainable development and alleviating poverty worldwide. The scope of energy management is broad, ranging from energy production and end use to emissions monitoring and mitigation and long-term planning. Given the extensive NASA Earth science research on energy and related weather and climate-related parameters, and rapidly advancing energy technologies and applications, there is great potential for increased application of NASA Earth science research to selected energy management issues and decision support tools. The NASA Energy Management Program Element is already involved in a number of projects applying NASA Earth science research to energy management issues, with a focus on solar and wind renewable energy and developing interests in energy modeling, short-term load forecasting, energy efficient building design, and biomass production.

Atmospheric models↗

NASA NTRS2006

Laboratory Measurements of Optical and Physical Properties of Individual Lunar Dust Grains

The lunar surface is covered with a thick layer of sub-micron/micron size dust grains formed by meteoritic impact over billions of years. The fine dust grains are levitated and transported on the lunar surface, and transient dust clouds over the lunar horizon were observed by experiments during the Apollo 17 mission. Theoretical models suggest that the dust grains on the lunar surface are charged by the solar UV radiation as well as the solar wind. Even without any physical activity, the dust grains are levitated by electrostatic fields and transported away from the surface in the near vacuum environment of the Moon. The current dust charging and levitation models, however, do not fully explain the observed phenomena. Since the abundance of dust on the Moon's surface with its observed adhesive characteristics has the potential of severe impact on human habitat and operations and lifetime of a variety of equipment, it is necessary to investigate the charging properties and the lunar dust phenomena in order to develop appropriate mitigating strategies. Photoelectric emission induced by the solar UV radiation with photon energies higher than the work function of the grain materials is recognized to be the dominant process for charging of the lunar dust, and requires measurements of the photoelectric yields to determine the charging and equilibrium potentials of individual dust grains. In this paper, we present the first laboratory measurements of the photoelectric yields of individual sub-micron/micron size dust grains selected from sample returns of Apollo 17, and Luna 24 missions, as well as similar size dust grains from the JSC-1 simulants. The experimental results were obtained on a laboratory facility based on an electrodynamic balance that permits a variety of experiments to be conducted on individual sub-micron/micron size dust grains in simulated space environments. The photoelectric emission measurements indicate grain size dependence with the yield increasing by an order of magnitude for grains of radii sub-micron size to several micron radii, at which it reaches asymptotic values. The yield for large size grains is found to be more than an order of magnitude higher than the bulk measurements on lunar fines reported in the literature.

Abbas, M. M.↗

NASA NTRSDate not supplied

Development of Thermostable Carbonic Anhydrases Using Structure-Guided Recombination for Use in CO2 Removal Systems on Spacecraft

Carbon capture and storage has been a research area of great interest in recent years as a method for mitigation of CO2 emissions, due to the effects of climate change. The development of technologies for the efficient capture of CO2 are also of great interest for human spaceflight applications. One of the most promising technologies in this area is CO2 scrubbing using liquid amines, unfortunately, liquid amines with low heats of desorption tend to have slow CO2 binding kinetics. One potential solution to this problem is to use the enzyme carbonic anhydrase (CA) to enhance the kinetics of CO2 binding to liquid amines, allowing the overall process to be more energy efficient. Interest in using carbonic anhydrase as a biocatalyst has led to a number of efforts to improve the thermostability and solvent tolerance of several distinct carbonic anhydrase enzymes. In the work described here, we screened through a diverse set of natural carbonic anhydrases to identify candidates for protein engineering aimed at increased stability and activity in various liquid amines. We then used SCHEMA structure-guided recombination to develop a set of chimeric carbonic anhydrases with high thermostability and activity. These chimeras were used as the starting points for further protein engineering work targeting activity in liquid amine systems. Our ultimate goal is to test the engineered enzymes in a liquid amine system for cabin air revitalization on ISS or other spacecraft.

Life Support, Carbon dioxide, Carbonic anhydrase, ↗

NASA NTRS2019

State of the science in reconciling top‐down and bottom‐up approaches for terrestrial CO2 budget

Robust estimates of CO2 budget, CO2 exchanged between the atmosphere and terrestrial biosphere, are necessary to better understand the role of the terrestrial biosphere in mitigating anthropogenic CO2 emissions. Over the past decade, this field of research has advanced through understanding of the differences and similarities of two fundamentally different approaches: “top‐down” atmospheric inversions and “bottom‐up” biosphere models. Since the first studies were undertaken, these approaches have shown an increasing level of agreement, but disagreements in some regions still persist, in part because they do not estimate the same quantity of atmosphere–biosphere CO2 exchange. Here, we conducted a thorough comparison of CO2 budgets at multiple scales and from multiple methods to assess the current state of the science in estimating CO2 budgets. Our set of atmospheric inversions and biosphere models, which were adjusted for a consistent flux definition, showed a high level of agreement for global and hemispheric CO2 budgets in the 2000s. Regionally, improved agreement in CO2 budgets was notable for North America and Southeast Asia. However, large gaps between the two methods remained in East Asia and South America. In other regions, Europe, boreal Asia, Africa, South Asia, and Oceania, it was difficult to determine whether those regions act as a net sink or source because of the large spread in estimates from atmospheric inversions. These results highlight two research directions to improve the robustness of CO2 budgets: (a) to increase representation of processes in biosphere models that could contribute to fill the budget gaps, such as forest regrowth and forest degradation; and (b) to reduce sink–source compensation between regions (dipoles) in atmospheric inversion so that their estimates become more comparable. Advancements on both research areas will increase the level of agreement between the top‐down and bottom‐up approaches and yield more robust knowledge of regional CO2 budgets.

atmospheric inversion↗

NASA NTRSDate not supplied

Quantifying the benefits of improved satellite remote-sensing observations for inverse modeling of NOx and NMVOC emissions

This study aims to demonstrate the benefits of using novel high spatiotemporal retrieval products from newer satellites for top-down emission estimates of nitrogen oxides (NO x ) and non-methane volatile organic compounds (NMVOCs) for the summer of 2019 over the contiguous United States. Recent satellite retrievals have not only advanced spatiotemporal resolution but also greatly reduced error and uncertainty due to reduced noise in the retrievals compared to spaceborne sensors launched in the past. We applied inverse modeling techniques using tropospheric nitrogen dioxide (NO 2 ) and formaldehyde (H-CHO) column retrieval products from the Ozone Monitoring Instrument (OMI) and TROPOspheric Monitoring Instrument (TROPOMI) in conjunction with the Weather Research Forecast and Community Multiscale Air Quality Modeling system (WRF-CMAQ). In order to provide a better representation of background chemical composition and avoid misalignment of emission adjustment, we applied monthly scaling factors for ozone (O 3 ) and CO boundary concentrations in addition to the inclusion of lightning and aviation emissions. Satellite-constrained NO x and NMVOCs posterior emissions showed a mitigated discrepancy between observed and modeled columns. The improvement in the model performance was greater when using TROPOMI, primarily benefiting from reduced errors/biases of the satellite retrievals that enabled us to explore corresponding changes in O 3 concentrations and production sensitivity regimes using the ratio of H-CHO and NO 2 .

remote sensing↗