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At least 37 records · Page 2

Novel laser-processed CsI:Tl detector for SPECT

Purpose: The aim of this work is to demonstrate the feasibility of a novel technique for fabrication of high spatial resolution CsI:Tl scintillation detectors for single photon emission computed tomography systems. Methods: The scintillators are fabricated using laser-induced optical barriers technique to create optical microstructures (or optical barriers) inside the CsI:Tl crystal bulk. The laser-processed CsI:Tl crystals are 3, 5, and 10 mm in thickness. In this work, the authors focus on the simplest pattern of optical barriers in that the barriers are created in the crystal bulk to form pixel-like patterns resembling mechanically pixelated scintillators. The monolithic CsI:Tl scintillator samples are fabricated with optical barrier patterns with 1.0 × 1.0 mm{sup 2} and 0.625 × 0.625 mm{sup 2} pixels. Experiments were conducted to characterize the fabricated arrays in terms of pixel separation and energy resolution. A 4 × 4 array of multipixel photon counter was used to collect the scintillation light in all the experiments. Results: The process yield for fabricating the CsI:Tl arrays is 100% with processing time under 50 min. From the flood maps of the fabricated detectors exposed to 122 keV gammas, peak-to-valley (P/V) ratios of greater than 2.3 are calculated. The P/V values suggest that regardless of the crystal thickness, the pixels can be resolved. Conclusions: The results suggest that optical barriers can be considered as a robust alternative to mechanically pixelated arrays and can provide high spatial resolution while maintaining the sensitivity in a high-throughput and cost-effective manner.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Quantum efficiencies of imaging detectors with alkali halide photocathodes. I - Microchannel plates with separate and integral CsI photocathodes

Measurements and comparisons have been made of the quantum efficiencies of microchannel plate (MCP) detectors in the far-UV (below 2000-A) wavelength range using CsI photocathodes (a) deposited on the front surfaces of microchannel plates and (b) deposited on solid substrates as opaque photocathodes with the resulting photoelectrons input to microchannel plates. The efficiences were measured in both pulse-counting and photodiode modes of operation. Typical efficiencies are about 15 percent at 1216 A for a CsI-coated MCP compared with 65 percent for an opaque CsI photocathode MCP detector. Special processing has yielded an efficiency as high as 20 percent for a CsI-coated MCP. This may possibly be further improved by optimization of the tilt angle of the MCP channels relative to the front face of the MCP and incident radiation. However, at present there still remains a factor of at least 3 quantum efficiency advantage in the separate opaque CsI photocathode configuration.

Carruthers, George R.↗

A spaceborne optical interferometer: The JPL CSI mission focus

The JPL Control Structure Interaction (CSI) program is part of the larger NASA-wide CSI program. Within this larger context, the JPL CSI program will emphasize technology for systems that demand micron or sub-micron level control, so-called Micro-Precision Controlled Structures (u-PCS). The development of such technology will make it practical to fly missions with large optical or large precision antenna systems. In keeping with the focused nature of the desired technology, the JPL approach is to identify a focus mission, develop the focus mission CSI system design to a preliminary level, and then use this design to drive out requirements for CSI technology development in the design and analysis, ground test bed, and flight experiment areas.

Laskin, R. A.↗

CSI compensation for reduced-order model based control of a flexible robot manipulator

In controller design for flexible structures, certain system modes are extremely important for the overall performance of the structure. A reduced-order model (ROM) based control focuses on these modes, providing a viable, active control algorithm for large systems. Unfortunately, unmodeled structure dynamics can interact with the ROM controller (CSI) and cause crippling deterioration of system performance, possibly to the point that system stability is lost. A residual model filter (RMF) eliminates one channel of control structure interaction (CSI), while adding only a simple, second-order filter to the control loop. Thus, the ROM controller can be designed independently, based strictly on performance criteria, and residual mode filters can then be selected to compensate for CSI. A flexible robot manipulator is used for preliminary experimentation with the ROM/RMF design methodology. Since the controller was to be implemented both with, and without compensation for CSI, the ROM control gains are carefully chosen such that closed loop stability is never compromised. In this way, RMF effectiveness is easily evaluated in terms of the improvement in system performance resulting from CSI compensation.

Reisenauer, Brian T.↗

Feasibility of using a smallsat for a dedicated on-orbit CSI laboratory

Control-Structure Integration (CSI) technology will be needed for the success of many future space missions, however, this technology will not be seriously considered for use by program managers if it is not first demonstrated in space. This paper will represent the results of a study that addressed the feasibility of orbiting a relatively low-cost CSI laboratory available to government, industry, and academic guest investigators by using the QuickStar bus, a flight-proven smallsat, launched as a secondary payload aboard a Delta II launch vehicle. This study developed a representative CSI experiment payload, which included a structural test article, sensors, actuators, and disturbances sources, to be integrated into the bus. The resulting concept for a CSI orbital lab was evaluated based on how well the concept satisfied generally accepted CSI flight-test objectives, and its cost and reliability.

Bicos, A. S.↗

The luminescence characteristics of CsI(Na) crystal under {alpha} and X/{gamma} excitation

In this paper, we study the effective decay time characteristic of CsI(Na) crystal under {sup 239}Pu alpha particle and {sup 137}Cs gamma-ray excitation using a single photon counting decay time measurement system. The measurement system employs a silicon optical fiber to couple and transit single photon. The slow decay time component of CsI(Na) crystal is 460-550 ns. We observe a 15 ns fast decay component under alpha particle excitation. In addition, we find that the primary stage of the falling edge in the decay time curve is non-exponential and drops rapidly when CsI(Na) crystal is excited by {sup 239}Pu alpha particles. Since the high density of self-trapped-excitons (STEs) is produced in alpha particle excitation process, we propose that the fast falling edge is corresponding to the quenching process of STEs which transit with non-radiation in the case of high excitation density. To prove this proposal, we excited the CsI(Na) crystal with sub-nanosecond intensive pulsed X-ray radiation. Our X-ray impinging results show that the fast falling edge also exists under low energy (average 100 keV) bremsstrahlung X-ray excitation.

36 MATERIALS SCIENCE↗

Thorium-doped CsI: Implications for the thorium nuclear clock transition

For 229m Th isomer nucleus with an anomalously low nuclear excitation energy, E$\star$ (currently accepted value of 7.8 ± 0.5 eV), the bound internal conversion (BIC) decay process is caused by the excitation of a valence electron that is sensitive to the electronic structure of the atomic-sized neighborhood. For this, we analyze an experiment where an impacting Th ion is neutralized by a negatively charged ion-receiving cesium iodide (CsI) surface, to obtain the minimal nuclear excitation energy E$\star\atop{min}$ necessary for BIC promotion of a Th-impurity valence electron in a CsI matrix. We analyze two cases: CsI with Th deposited into the bulk and with Th deposited on the CsI surface. In the bulk we consider band gap effects while on the surface we consider the work function. The energy to pull the electron to the surface is 1.5 – 2.2 eV depending on the surface plane, while to promote to the conduction band in the bulk it is 1.5 eV. Therefore we conclude that the Th-surface interaction can significantly reduce the lower E$\star$ bound of 6.3 eV, as estimated from the direct observation of the Th-clock transition [von der Wense et al., Nature (London) 533, 47 (2016)]. We suggest coating the multichannel plate with differing materials leading to different Th-impurity gaps and work functions can further narrow the E$\star$ uncertainty interval.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Comprehensive Comparative Analysis: VSI-based vs. CSI-based Motor Drive Systems with Sinusoidal Output Voltage

The emergence of wide-bandgap (WBG) power devices opens opportunities for current source inverters (CSIs) to provide a promising alternative drive configuration for motor drive applications. The sinusoidal output voltage of CSI offers significant advantages for numerous motor drive applications, including reducing the risks associated with motor terminal overvoltages and bearing discharge currents. This paper compares the performance of CSIs and voltage source inverters (VSIs) with the same performance capabilities. More specifically, sine filters are added to the VSI output terminals to match the CSI performance, and a front-end boost converter is added to the VSI to match the CSI’s voltage-boost capability. The results show that the CSI active components require 48% less volume than the VSI, combined with other performance advantages that make it an appealing candidate for some future motor drive applications.

current source inverter, motor drive system, passi↗

Alternative Vector PWM for CSI Common-Mode Voltage Reduction During Voltage-Boost Operation with Low Modulation Index

This paper proposes a new pulse-width modulation (PWM) scheme named alternative vector PWM (AVM) algorithm that reduces the common-mode voltage (vCM) generated by a 3-phase current source inverter (CSI) during operation within a portion of its voltage-boost regime when the CSI’s modulation index is below 1/3–√(=0.5774). Three different active current vector pairs (one conventional pair with adjacent active current vectors and two proposed pairs with non-adjacent active current vectors) are used to reduce vCM based on the CSI’s output voltage conditions. Experimental results confirm significant reductions in major vCM spectral components by up to approx. 85% between the 3rd harmonic of the fundamental frequency and the CSI’s PWM frequency, validating the advantages of the proposed AVM algorithm over the conventional PWM.

42 ENGINEERING↗

Control technology overview in CSI

A brief control technology overview is given in Control Structures Interaction (CSI) by illustrating that many future NASA mission present significant challenges as represented by missions having a significantly increased number of important system states which may require control and by identifying key CSI technology needs. The JPL CSI related technology developments are discussed to illustrate that some of the identified control needs are being pursued. Since experimental confirmation of the assumptions inherent in the CSI technology is critically important to establishing its readiness for space program applications, the areas of ground and flight validation require high priority.

Dahlgren, J. B.↗

The Langley Research Center CSI phase-0 evolutionary model testbed-design and experimental results

A testbed for the development of Controls Structures Interaction (CSI) technology is described. The design philosophy, capabilities, and early experimental results are presented to introduce some of the ongoing CSI research at NASA-Langley. The testbed, referred to as the Phase 0 version of the CSI Evolutionary model (CEM), is the first stage of model complexity designed to show the benefits of CSI technology and to identify weaknesses in current capabilities. Early closed loop test results have shown non-model based controllers can provide an order of magnitude increase in damping in the first few flexible vibration modes. Model based controllers for higher performance will need to be robust to model uncertainty as verified by System ID tests. Data are presented that show finite element model predictions of frequency differ from those obtained from tests. Plans are also presented for evolution of the CEM to study integrated controller and structure design as well as multiple payload dynamics.

Belvin, W. K.↗

Yield, variance and spatial distribution of electron–hole pairs in CsI

A Monte Carlo (MC) method previously developed has been applied to simulate the interaction of photons, with energies ranging from 50 eV to ~ 1 MeV, with CsI and the subsequent electron cascades. The MC model has been employed to compute nano-scale spatial distributions of electron-hole pairs and important intrinsic properties, including W, the mean energy per electron-hole pair, and the Fano factor, F. W exhibits discontinuities at the shell edges that follow the photoionization cross sections and decreases with increasing photon energy (from ~19 to 15 eV), with an asymptotic value of 15.2 eV at high energy. This decrease may contribute the initial rise in relative light yield with incident energy observed experimentally for CsI, thus suggesting that nonlinearity may be associated with intrinsic properties of the material at low energies. F is calculated to increase with increasing energy and has an asymptotic value of 0.28. A significant number of electron-hole pairs are produced through the different ionization channels of core shells and corresponding relaxation processes, which may explain why F is larger for CsI than for Si or Ge. Finally, the calculated spatial distributions show that the electron-hole pairs are primarily distributed along fast electron tracks. These spatial distributions constitute important input for large-scale simulations of electron-hole pair transport.

CsI.↗

CsI-Antisolvent Adduct Formation in All-Inorganic Metal Halide Perovskites

The excellent optoelectronic properties shown by hybrid organic/inorganic metal halide perovskites are all predicated on precisely controlling the exact nucleation and crystallization dynamics that occur during film formation. In general, high-performance thin films are obtained by a method commonly called solvent engineering (or antisolvent quench) processing. The solvent engineering method removes excess solvent, but importantly leaves behind solvent that forms chemical adducts with the lead-halide precursor salts. These adduct-based precursor phases control nucleation and the growth of the polycrystalline domains. There has not yet been a comprehensive study comparing the various antisolvents used in different perovskite compositions containing cesium. In addition, there have been no reports of solvent engineering for high efficiency in all-inorganic perovskites such as CsPbI 3 . In this work, inorganic perovskite composition CsPbI 3 is specifically targeted and unique adducts formed between CsI and precursor solvents and antisolvents are found that have not been observed for other A-site cation salts. These CsI adducts control nucleation more so than the PbI 2 -dimethyl sulfoxide (DMSO) adduct and demonstrate how the A-site plays a significant role in crystallization. The use of methyl acetate (MeOAc) in this solvent engineering approach dictates crystallization through the formation of a CsI-MeOAc adduct and results in solar cells with a power conversion efficiency of 14.4%.

14 SOLAR ENERGY↗

Development of low background CsI(Tl) and NaI(Tl) crystals for WIMP search

We have developed low background CsI(Tl) and NaI(Tl) crystals to search for weakly interacting massive particles as well as to verify the origin of the annual modulation signal observed by the DAMA/LIBRA experiment. Extensive studies about the contamination mechanisim of {sup 137}Cs in CsI powder lead to the growth of ultra-low-background CsI(Tl) crystals. Similar approaches for NaI(Tl) crystals have been applied to reduce internal backgrounds to less than 0.5 counts/kg/day/keV. Status and understanding of backgrounds and background reduction in NaI(Tl) crystals will be discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Quality Assurance on Undoped CsI Crystals for the Mu2e Experiment

The Mu2e experiment is constructing a calorimeter consisting of 1,348 undoped CsI crystals in two disks. Each crystal has a dimension of 34 x 34 x 200 mm 3 , and is readout by a large area silicon PMT array. A series of technical specifications was defined according to physics requirements. Preproduction CsI crystals were procured from three firms: Amcrys, Saint-Gobain and Shanghai Institute of Ceramics. We report the quality assurance on crystal's scintillation properties and their radiation hardness against ionization dose and neutrons. With a fast decay time of 30 ns and a light output of more than 100 p.e./MeV measured with a bi-alkali PMT, undoped CsI crystals provide a cost-effective solution for the Mu2e experiment.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Light output measurements and computational models of microcolumnar CsI scintillators for x-ray imaging

Purpose: The authors report on measurements of light output and spatial resolution of microcolumnar CsI:Tl scintillator detectors for x-ray imaging. In addition, the authors discuss the results of simulations aimed at analyzing the results of synchrotron and sealed-source exposures with respect to the contributions of light transport to the total light output. Methods: The authors measured light output from a 490-μm CsI:Tl scintillator screen using two setups. First, the authors used a photomultiplier tube (PMT) to measure the response of the scintillator to sealed-source exposures. Second, the authors performed imaging experiments with a 27-keV monoenergetic synchrotron beam and a slit to calculate the total signal generated in terms of optical photons per keV. The results of both methods are compared to simulations obtained with hybridMANTIS, a coupled x-ray, electron, and optical photon Monte Carlo transport package. The authors report line response (LR) and light output for a range of linear absorption coefficients and describe a model that fits at the same time the light output and the blur measurements. Comparing the experimental results with the simulations, the authors obtained an estimate of the absorption coefficient for the model that provides good agreement with the experimentally measured LR. Finally, the authors report light output simulation results and their dependence on scintillator thickness and reflectivity of the backing surface. Results: The slit images from the synchrotron were analyzed to obtain a total light output of 48 keV{sup −1} while measurements using the fast PMT instrument setup and sealed-sources reported a light output of 28 keV{sup −1}. The authors attribute the difference in light output estimates between the two methods to the difference in time constants between the camera and PMT measurements. Simulation structures were designed to match the light output measured with the camera while providing good agreement with the measured LR resulting in a bulk absorption coefficient of 5 × 10{sup −5} μm{sup −1}. Conclusions: The combination of experimental measurements for microcolumnar CsI:Tl scintillators using sealed-sources and synchrotron exposures with results obtained via simulation suggests that the time course of the emission might play a role in experimental estimates. The procedure yielded an experimentally derived linear absorption coefficient for microcolumnar Cs:Tl of 5 × 10{sup −5} μm{sup −1}. To the author’s knowledge, this is the first time this parameter has been validated against experimental observations. The measurements also offer insight into the relative role of optical transport on the effective optical yield of the scintillator with microcolumnar structure.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

SU-E-T-524: In-Vivo Diode Dosimetry Proton Therapy Range Verification Validation Study for Pediatric CSI

Purpose: With the aim of reducing acute esophageal radiation toxicity in pediatric patients receiving craniospinal irradiation (CSI), we investigated the implementation of an in-vivo, adaptive proton therapy range verification methodology. Simulation experiments and in-phantom measurements were conducted to validate the range verification technique for this clinical application. Methods: A silicon diode array system has been developed and experimentally tested in phantom for passively scattered proton beam range verification for a prostate treatment case by correlating properties of the detector signal to the water equivalent path length (WEPL). We propose to extend the methodology to verify range distal to the vertebral body for pediatric CSI cases by placing this small volume dosimeter in the esophagus of the anesthetized patient immediately prior to treatment. A set of calibration measurements was performed to establish a time signal to WEPL fit for a “scout” beam in a solid water phantom. Measurements are compared against Monte Carlo simulation in GEANT4 using the Tool for Particle Simulation (TOPAS). Results: Measurements with the diode array in a spread out Bragg peak of 14 cm modulation width and 15 cm range (177 MeV passively scattered beam) in solid water were successfully validated against proton fluence rate simulations in TOPAS. The resulting calibration curve allows for a sensitivity analysis of detector system response with dose rate in simulation and with individual diode position through simulation on patient CT data. Conclusion: Feasibility has been shown for the application of this range verification methodology to pediatric CSI. An in-vivo measurement to determine the WEPL to the inner surface of the esophagus will allow for personalized adjustment of the treatment plan to ensure sparing of the esophagus while confirming target coverage. A Toltz acknowledges partial support by the CREATE Medical Physics Research Training Network grant of the Natural Sciences and Engineering Research Council (Grant number: 432290)

60 APPLIED LIFE SCIENCES↗

Photoemission from CsI - Calculation.

Calculations of optical and photoemission spectra for CsI based on first-order allowed transitions between Bloch-wave states are discussed. The calculations, utilizing energy-band data for CsI published by Onodera (1968), were performed by computer sampling of regions in the Brillouin zone. The photoelectric spectra of CsI, calculated on the basis of an interpolated band scheme, display features which are in general agreement with the experimentally determined photoelectric energy distribution curves.

Distefano, T. H.↗