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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 37 records · Page 2
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

The gallium solar neutrino capture cross section revisited

Solar neutrino flux constraints from the legacy GALLEX/GNO and SAGE experiments continue to influence contemporary global analyses of neutrino properties. The constraints depend on the neutrino absorption cross sections for various solar sources. Following recent work updating the 51 Cr and 37 Ar neutrino source cross sections, we reevaluate the 71 Ga solar neutrino cross sections, focusing on contributions from transitions to 71 Ge excited states, but also revising the ground-state transition to take into account new 71 Ge electron-capture lifetime measurements and various theory corrections. The excited-state contributions have been traditionally taken from forward-angle (𝑝, 𝑛) cross sections. Here we correct this procedure for the ≈ 10%–20% tensor operator contribution that alters the relationship between Gamow-Teller and (𝑝, 𝑛) transition strengths. Using state-of-the-art nuclear shell-model calculations to evaluate this correction, we find that it lowers the 8 B and hep neutrino cross sections. However, the addition of other corrections, including contributions from near-threshold continuum states that radiatively decay, leads to an overall increase in the 8 B and hep cross sections of ≈ 10% relative to the values recommended by Bahcall. Uncertainties are propagated using Monte Carlo simulations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

A kinetic line-driven radiation operator and its application to Gyrokinetics

A velocity dependent, kinetic model for line radiation is developed for continuum kinetic codes. It has been implemented in the full-f gyrokinetic code Gkeyll. The total radiation for a charge state is modeled as an advection in velocity space with a form of $\nabla_v \cdot(v\nu(v)f(v))$, guaranteeing particle conservation. The velocity dependence (in the form of an effective frequency $\nu(v)$) is found through fitting the energy loss of the operator, i.e. the second velocity moment, to the radiation data in the OpenADAS database. Therefore, each individual transition does not need to be evaluated every time step, significantly reducing the computational cost of including line radiation in a kinetic model. The dependence on velocity instead of the usual, temperature, allows the radiation to be computed from non-Maxwellian electron distribution functions: We benchmark the model against a collisional radiative model using isotropic non-Maxwellian distribution functions. A velocity dependent model of radiation can more accurately describe the radiation in the more kinetic regimes expected in reactor-scale devices. The velocity dependence qualitatively captures the quantum mechanical need for a minimum velocity before any radiation occurs.

kinetic↗
DOE OSTI2022

The High-Frequency Signature of Slow and Fast Laboratory Earthquakes

Tectonic faults fail through a spectrum of slip modes, ranging from slow aseismic creep to rapid slip during earthquakes. Understanding the seismic radiation emitted during these slip modes is key for advancing earthquake science and earthquake hazard assessment. In this work, we use laboratory friction experiments instrumented with ultrasonic sensors to document the seismic radiation properties of slow and fast laboratory earthquakes. Stick-slip experiments were conducted at a constant loading rate of 8 μm/s and the normal stress was systematically increased from 7 to 15 MPa. We produced a full spectrum of slip modes by modulating the loading stiffness in tandem with the fault zone normal stress. Acoustic emission data were recorded continuously at 5 MHz. We demonstrate that the full continuum of slip modes radiate measurable high-frequency energy between 100 and 500 kHz, including the slowest events that have peak fault slip rates <100 μm/s. The peak amplitude of the high-frequency time-domain signals scales systematically with fault slip velocity. Stable sliding experiments further support the connection between fault slip rate and high-frequency radiation. Experiments demonstrate that the origin of the high-frequency energy is fundamentally linked to changes in fault slip rate, shear strain, and breaking of contact junctions within the fault gouge. Our results suggest that having measurements close to the fault zone may be key for documenting seismic radiation properties and fully understanding the connection between different slip modes.

58 GEOSCIENCES↗
DOE OSTI2021

Evolution of microstructures in radiation fields using a coupled binary-collision Monte Carlo phase field approach

The simulation of radiation effects in materials broadly falls into two categories. At short time and length scales lies the modeling of primary radiation damage, such as point defect creation, energy deposition, and ballistic mixing. This is followed by the modeling at longer time scales of thermally activated microstructure evolution and defect reactions, such as recombination, clustering, and coarsening. The binary collision Monte Carlo method is an established, numerically efficient method for the computation of primary radiation damage. Conversely, the phase field method is a state of the art method for microstructure evolution on longer time and length scales. Here we present a concurrent coupling of these two methods, overcoming the difference between the discrete object Monte Carlo paradigm for primary radiation damage and the continuum field variable approach for microstructure evolution. The coupling is bidirectional, in which the microstructure evolution in the MOOSE finite element frame- work provides the spatial scattering data set for the charged particle trans- port and receives point defect, mass transport, and heat source terms from the simulated collision cascades that contribute to the field variable evolution. The concurrent coupling scheme is implemented in the code Magpie and demonstrated by investigating patterning for a model irradiated immiscible binary alloy. The results from the coupled binary collision Monte Carlo/phase field simulations reproduce the results of analytical models for phase separation, phase mixing, and patterning, supporting the approach and indicating its utility for modeling real materials systems.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Climate-Relevant Gas Absorption Properties from AWARE and Other ARM Spectral Measurements (Final Report)

The objective of this project has been to use measurements from the Atmospheric Emitted Radiance Interferometer (AERI) deployed at ARM sites to improve our knowledge of uncertain infrared spectroscopic parameters of importance to climate, remote sensing, and data assimilation. A primary focus has been the water vapor continuum in the infrared atmospheric window. Radiation codes used to predict climate and weather base their representation of the water vapor continuum in this window on the MT_CKD model, but in this spectral region the MT_CKD water vapor continuum absorption coefficients were derived almost two decades ago by an analysis of AERI measurements for conditions with a limited range of precipitable water vapor (PWV) and temperature values, leading to uncertainty in the derived coefficients. This project has included a new, comprehensive analysis of all aspects of the water vapor continuum in the atmospheric window -- the self continuum, the foreign continuum, and the self continuum temperature dependence, all resolved spectrally. Having a wide range of PWV amounts and temperatures from deployments of the ARM Mobile Facility for GoAmazon as well as the more than a decade of AERI measurements at SGP has provided an appropriate foundation for such a comprehensive analysis.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Terahertz bound state in the continuum in dielectric membrane metasurfaces

Mie-resonant metasurfaces composed of subwavelength dielectric resonators enable an efficient route for electromagnetic wave manipulation. Among these manipulations, a localized mode with a high-quality factor coexisting with a continuous spectrum of radiating waves termed bound state in the continuum (BIC) can arouse many exotic applications in photonics. Here, we demonstrate the terahertz BIC in a dielectric membrane metasurface and analyze its resonant nature based on Mie-resonant multipoles and vector spherical harmonics. The intrinsic splitting of the resonances under oblique incidence is also explored, in which the conversion of multipole radiation patterns versus the oblique angle will drive the resonances from BIC to leaky modes or vice versa. Both Γ and off-Γ point BICs could be identified as the superposition cancellation of vector spherical harmonics for both p-wave and s-wave. Our research not only provides a novel perspective for exploring the essence of BIC metasurfaces in the terahertz regime, but also points new opportunities for achieving terahertz BIC metasurfaces with ultra-high quality factors.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Autoionizing Polaritons in Attosecond Atomic Ionization

Light-induced states and Autler-Townes splitting of laser-coupled states are common features in the photoionization spectra of laser-dressed atoms. The entangled light-matter character of metastable Autler-Townes multiplets, which makes them autoionizing polaritons, however, is still largely unexplored. We employ attosecond transient-absorption spectroscopy in argon to study the formation of polariton multiplets between the 3s –1 4p and several light-induced states. We measure a controllable stabilization of the polaritons against ionization, in excellent agreement with ab initio theory. Using an extension of the Jaynes-Cummings model to autoionizing states, we show that this stabilization is due to the destructive interference between the Auger decay and the radiative ionization of the polaritonic components. Furthermore, these results give new insights into the optical control of electronic structure in the continuum and unlock the door to applications of radiative stabilization in metastable polyelectronic systems.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2024

Constraints on the origin of the radio synchrotron background via angular correlations

ABSTRACT The origin of the radio synchrotron background (RSB) is currently unknown. Its understanding might have profound implications in fundamental physics or might reveal a new class of radio emitters. In this work, we consider the scenario in which the RSB is due to extragalactic radio sources and measure the angular cross-correlation of Low-Frequency Array (LOFAR) images of the diffuse radio sky with matter tracers at different redshifts, provided by galaxy catalogues and cosmic microwave background lensing. We compare these measured cross-correlations to those expected for models of RSB sources. We find that low-redshift populations of discrete sources are excluded by the data, while higher redshift explanations are compatible with available observations. We also conclude that at least 20 per cent of the RSB surface brightness level must originate from populations tracing the large-scale distribution of matter in the Universe, indicating that at least this fraction of the RSB is of extragalactic origin. Future measurements of the correlation between the RSB and tracers of high-redshift sources will be crucial to constraining the source population of the RSB.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Magnetic Misalignment of Interstellar Dust Filaments

We present evidence for scale-independent misalignment of interstellar dust filaments and magnetic fields. We estimate the misalignment by comparing millimeter-wave dust-polarization measurements from Planck with filamentary structures identified in neutral-hydrogen (H I ) measurements from H I 4PI. We find that the misalignment angle displays a scale independence (harmonic coherence) for features larger than the H I 4PI beamwidth (16$\acute{.}$2). We additionally find a spatial coherence on angular scales of ${ \mathcal O }(1^\circ )$. We present several misalignment estimators formed from the auto- and cross-spectra of dust-polarization and H I -based maps, and we also introduce a map-space estimator. Applied to large regions of the high-Galactic-latitude sky, we find a global misalignment angle of ~2°, which is robust to a variety of masking choices. By dividing the sky into small regions, we show that the misalignment angle correlates with the parity-violating TB cross-spectrum measured in the Planck dust maps. The misalignment paradigm also predicts a dust EB signal, which is of relevance in the search for cosmic birefringence but as yet undetected; the measurements of EB are noisier than those of TB, and our correlations of EB with misalignment angle are found to be weaker and less robust to masking choices. We also introduce an H I -based dust-polarization template constructed from the Hessian matrix of the H I intensity, which is found to correlate more strongly than previous templates with Planck dust B modes.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

A Continuum Dislocation Dynamics Crystal Plasticity Approach to Irradiated Body-Centered Cubic α-Iron

Radiation-induced embrittlement of reactor pressure vessel (RPV) steels can potentially limit the operating life of nuclear power plants. Over extended exposure to radiation doses, these body-centered cubic (BCC) irons demonstrate irradiation damage. Here, we present a continuum dislocation density (CDD) crystal plasticity model to capture the interaction among dislocations and self-interstitial atom (SIA) loops in α-iron. We demonstrate the importance of modeling cross slip using a combined stochastic Monte Carlo approach and the role of slip system strength anisotropy in capturing stochastic cross slip interactions. Through these captured interactions, the CDD crystal plasticity model can capture both the stress response and the physical evolution of dislocations on different slip system planes. Single-crystal verification experiments are used to calibrate the CDD crystal plasticity model, and a set of simplified polycrystalline simulations demonstrates the model’s ability to capture the stress response from tensile experiments on α-iron.

36 MATERIALS SCIENCE↗
DOE OSTI2024

A More Transparent Infrared Window

The infrared window region (780–1,250 cm –1 , 12.8 to 8.0 μm) is of great importance to Earth's climate due to its high transparency and thermal energy. We present here a new investigation of the transparency of this spectral region based on observations by interferometers of downwelling surface radiance at two DOE Atmospheric Radiation Measurement program sites. We focus on the dominant source of absorption in this region, the water vapor continuum, and derive updated values of spectral absorption coefficients for both the self and foreign continua. Our results show that the self continuum is too strong in the previous version of Mlawer-Tobin_Clough-Kneizys-Davies (MT_CKD) water vapor continuum model, a result that is consistent with other recent analyses, while the foreign continuum is too weak in MT_CKD. In general, the weaker self continuum derived in this study results in an overall increase in atmospheric transparency in the window, although in atmospheres with low amounts of water vapor the transparency may slightly decrease due to the increase in foreign continuum absorption. These continuum changes lead to a significant decrease in downwelling longwave flux at the surface for moist atmospheres and a modest increase in outgoing longwave radiation. The increased fraction of surface-leaving radiation that escapes to space leads to a notable increase (~5–10%) in climate feedback, implying that climate simulations that use the new infrared window continuum will show somewhat less warming than before. This study also points out the possibly important role that aerosol absorption may play in the longwave radiative budget.

58 GEOSCIENCES↗
DOE OSTI2024

Data/code for Mlawer et al. 2024 (A more transparent infrared window)

The infrared window region (780–1,250 cm –1 , 12.8 to 8.0 μm) is of great importance to Earth's climate due to its high transparency and thermal energy. We present here a new investigation of the transparency of this spectral region based on observations by interferometers of downwelling surface radiance at two DOE Atmospheric Radiation Measurement program sites. We focus on the dominant source of absorption in this region, the water vapor continuum, and derive updated values of spectral absorption coefficients for both the self and foreign continua. Our results show that the self continuum is too strong in the previous version of Mlawer-Tobin_Clough-Kneizys-Davies (MT_CKD) water vapor continuum model, a result that is consistent with other recent analyses, while the foreign continuum is too weak in MT_CKD. In general, the weaker self continuum derived in this study results in an overall increase in atmospheric transparency in the window, although in atmospheres with low amounts of water vapor the transparency may slightly decrease due to the increase in foreign continuum absorption. These continuum changes lead to a significant decrease in downwelling longwave flux at the surface for moist atmospheres and a modest increase in outgoing longwave radiation. The increased fraction of surface-leaving radiation that escapes to space leads to a notable increase (~5–10%) in climate feedback, implying that climate simulations that use the new infrared window continuum will show somewhat less warming than before. This study also points out the possibly important role that aerosol absorption may play in the longwave radiative budget.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Enhancing photonic systems using topology and non-Hermiticity

The broad goal of this project was to develop new analytical and numerical insights for how important photonic processes can be improved using recently discovered principles in topological and non-Hermitian physics. In particular, there are two recent discoveries that we aimed to harness to achieve this goal. First, it was discovered in condensed matter physics that crystalline symmetries can protect low-dimensional topologically protected states in lattices without the need for breaking time-reversal symmetry. These so-called ‘higher-order’ topological systems represent an important development for photonic systems, where it is very difficult to break time-reversal symmetry, and which had been previously thought necessary to realize topological phenomena. Second, the last decade has seen a significant amount of interest in phenomena which are unique to non-Hermitian systems, i.e., systems which do not conserve energy. For example, spatially patterned gain and loss can be used to realize exceptional points, which are degeneracies in a system’s spectrum where the system becomes defective, while the existence of radiative losses also enables a new route to confinement through bound states in the continuum. For such non-Hermitian phenomena, photonics again represents a critical platform, as photonic systems naturally lose light to their radiative environments, making them generally non-Hermitian, and it is also possible to incorporate additional gain or loss. Based on these broad principles, we pursued a range of projects to harness bound states in the continuum in a variety of different systems and architectures, develop real-space methods for classifying topological systems to yield better photonic design principles, and a novel Brillouin-based fiber laser for sensing strain.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2023

Quantum-Path-Resolved Attosecond High-Harmonic Spectroscopy

Strong-field ionization of molecules releases electrons which can be accelerated and driven back to recombine with their parent ion, emitting high-order harmonics. This ionization also initiates attosecond electronic and vibrational dynamics in the ion, evolving during the electron travel in the continuum. Revealing this subcycle dynamics from the emitted radiation usually requires advanced theoretical modeling. Here we show that this can be avoided by resolving the emission from two families of electronic quantum paths in the generation process. The corresponding electrons have the same kinetic energy, and thus the same structural sensitivity, but differ by the travel time between ionization and recombination-the pump-probe delay in this attosecond self-probing scheme. We measure the harmonic amplitude and phase in aligned CO 2 and N 2 molecules and observe a strong influence of laser-induced dynamics on two characteristic spectroscopic features: a shape resonance and multichannel interference. This quantum-path-resolved spectroscopy thus opens wide prospects for the investigation of ultrafast ionic dynamics, such as charge migration.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2024

BOSS quasar outflows traced by C iv

ABSTRACT We investigate possible factors that drive fast quasar outflows using a sample of 39 249 quasars at median redshift 〈z〉 ≈ 2.17. Unique to this study, the quasar redshifts are re-measured based on the Mg ii emission line, and explore unprecedented outflow velocities (>6000 km s−1), while maintaining statistical significance. We measure reliable C iv blueshifts for 1178 quasars with velocities >2500 km s−1. From those, 255(13) quasars have blueshifts above 4000(6000) km s−1, with the highest C iv velocity ≈7000 km s−1. Several correlations are observed, where higher C iv blueshifts in general are in quasars with broader, weaker C iv emission profiles, weak He ii emission, larger Eddington ratios, and bluer ultraviolet (UV) continuum slope across the rest-frame UV to near-infrared. Analysis reveals two primary factors contributing to faster outflows: higher Eddington ratios, and softer far-UV continuum (hν >24.6 eV). We find supporting evidence that radiative line driving may generate extreme outflow velocities, influenced by multiple factors as suggested by the aforementioned correlations. This evidence highlights the importance of considering a multidimensional parameter space in future studies when analyzing large C iv blueshifts to determine the fundamental causes of outflows.

Gillette, Jarred (ORCID:0000000185284839)↗
DOE OSTI2021

Interstellar Extinction, Polarization, and Grain Alignment in the Sh 2-185 (IC 59 and IC 63) Region

Optical and infrared continuum polarization from the interstellar medium is driven by radiative processes aligning the grains with the magnetic field. While a quantitative, predictive theory of radiative alignment torques (RATs) exists and has been extensively tested, several parameters of the theory remain to be fully constrained. In a recent paper, Medan & Andersson showed that the polarization efficiency (and therefore grain alignment efficiency) at different locations in the wall of the Local Bubble (LB) could be modeled as proportional to the integrated light intensity from the surrounding stars and OB associations. Here we probe that relationship at high radiation field intensities by studying the extinction and polarization in the two reflection nebulae IC 59 and IC 63 in the Sh 2-185 H ii region, illuminated by the B0 IV star γ Cassiopeia. We combine archival visual polarimetry with new seven-band photometry in the Vilnius system, to derive the polarization efficiency from the material. We find that the same linear relationship seen in the LB wall also applies to the Sh 2-185 region, strengthening the conclusion from the earlier study.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Characterizing leaf-scale fluorescence with spectral invariants

Sun-induced chlorophyll fluorescence (SIF) is increasingly recognized as a non-destructive probe for tracking terrestrial photosynthesis. Emerging developments in spectral invariants theory provide an innovative and efficient approach for representing SIF radiative transfer processes at the canopy scale. However, modeling leaf-scale fluorescence based on the spectral invariants properties (SIP) remains underexplored. In this study, the spectral invariants theory is employed for the first time to model the leaf-scale total, backward and forward fluorescence (leaf-SIP SIF). The leaf-SIP SIF model separates the leaf-scale radiative transfer process into two distinct components: the wavelength-dependent one associated with leaf biochemical properties, and the wavelength-independent component linked to leaf structural characteristics. The leaf structure-related effects are characterized by two spectrally invariant parameters: the photon recollision probability (p) and the scattering asymmetry parameter (q), which are parameterized using the directly measurable leaf dry matter. Evaluation against field measurements shows that the proposed leaf-SIP SIF model has a good performance, with coefficient of determination (R 2 ) of 0.89, 0.89, 0.90 and root mean squared errors (RMSE) of 1.28, 0.69, 0.74 Wm -2 µm -1 sr -1 , respectively for the total, backward, and forward fluorescence (660–800 nm). The leaf-SIP SIF model with a more concise formulation demonstrates comparable performance with the widely used Fluspect model. Further, the leaf-SIP SIF model provides a simple and efficient approach for simulating leaf-scale fluorescence, with the potential to be integrated into a unified SIP-based model framework for simulating the radiative transfer processes across the soil-leaf-canopy-atmosphere continuum.

59 BASIC BIOLOGICAL SCIENCES↗