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DOE OSTI2024

Performance of the Fermilab Linac Injector

The Fermilab Linac injection line consists of a 35 keV magnetron-type H- ion source, two-solenoid Low Energy Beam Transport (LEBT), 201 MHz 4-rod 750 keV Radio Frequency Quadrupole (RFQ), and a Medium Energy Transport (MEBT) containing 4 quadrupoles and a bunching cavity. The injector delivers 25 mA, 48 s pulses to drift-tube Linac at a repetition rate of 15Hz. The transmission efficiency has been lower than expected since commissioning. Recent beam current measurements suggest that the beam is primarily lost upstream of the RFQ exit. Numerical simulations indicate that ions passing through the non-linear field region of the solenoids could produce a beam with an increased emittance resulting in up to 50 % of the LEBT beam current failing to meet the RFQ acceptance. An aperture restriction was installed upstream of the first solenoid to remove these ions. This report describes the results of measurements and simulations as well as the LEBT tuning.

Jones, Daniel C.↗

DOE OSTI2024

Performance of the Fermilab Linac Injector

Jones, Daniel C.↗

DOE OSTI2024

Performance of the Fermilab Linac Injector

The Fermilab Linac injection line consists of a 35 keV magnetron-type H\textsuperscript{-} ion source, two-solenoid Low Energy Beam Transport (LEBT), 201 MHz 4-rod 750 keV Radio Frequency Quadrupole (RFQ), and a Medium Energy Transport (MEBT) containing 4 quadrupoles and a bunching cavity. The injector delivers 25 mA, 48 µs pulses to the drift-tube Linac at a repetition rate of 15Hz. The transmission efficiency of the injector has been lower than expected since commissioning. Recent beam current measurements suggest that the beam is primarily lost upstream of the RFQ exit. Numerical simulations indicate that ions passing through the non-linear field region of the solenoids could produce a beam with an increased emittance resulting in up to 50\% of the LEBT beam current failing to meet the RFQ acceptance. An aperture restriction was installed upstream of the first solenoid to remove these ions. This report describes the results of measurements and simulations as well as the LEBT tuning.

43 PARTICLE ACCELERATORS↗

DOE OSTI2025

Stability and Viability of Off-Axis Photoemission Geometries in 4D Ultrafast Electron Microscopy

Femtosecond (fs) laser-based 4D ultrafast electron microscopy (UEM) commonly makes use of photoelectron emission from a source material in the electron gun region of an otherwise conventional TEM. For TEMs equipped with thermionic guns, the source material is often LaB 6 , the same as used for thermionic operation. Here, such thermionic-based UEMs have proven useful for applications requiring large electron fluxes (i.e., high beam currents) often at the expense of beam coherence and brightness, which is especially important for single-shot nanosecond applications. Importantly, for fs-based UEMs, beam currents can be controlled over a broad range of parameter space through the properties of the fs laser and the photon pulses produced therefrom.

Willis, Simon A. [University of Minnesota, Minneap↗

DOE OSTI2026

Non-Intrusive Load Monitoring of EBW Processes A Second Study [Slides]

The Objective is to Determine if induced off-nominal welding disturbances: (1) Beam arc out (weld on high vapor pressure aluminum plate); (2) Pulsed beam voltage; (3) Pulsed beam current; and (4) Pulsed beam focus current can be observed in the input power to the high-voltage cabinet powering the EB gun, ie Non-Instrusive Load Monitoring (NILM).

36 MATERIALS SCIENCE↗

DOE OSTI2024

Cross-sections for 43 Sc, 44 m Sc, and 44 g Sc from two heavy ion reactions

Two different heavy ion reactions were used to produce 43 Sc (t$_{\frac12}$ = 3.891 h), 44g Sc (t$_{\frac12}$ = 4.042 h), and 44m Sc (t$_{\frac12}$ = 58.61 h) among other stable or long-lived chemically separable products. Production cross sections for 19 F + 27 Al and the reverse kinematic reaction 35 Cl + nat B were measured using an MC-SNICS ion source and the Notre Dame FN Tandem Accelerator. 19 F beams from 35 to 60 MeV were produced with beam currents between 40–80 pnA and 35 Cl beams were produced at six entrance energies with comparable beam currents. This work reports nuclear reaction cross sections 27 Al ( 19 F, x) 43 Sc, 27 Al ( 19 F, pn) 44g Sc, and 27 Al ( 19 F, pn) 44m Sc at six energies between 35 and 60 MeV lab energy. Cross sections within the same energy range were measured for 27 Al ( 19 F, 3pn) 42 K and 27 Al ( 19 F, 3p) 43 K. Comparative measurements were performed for the same compound nucleus produced from nat B( 35 Cl, x) 43 Sc, nat B( 35 Cl, pn) 44g Sc, and nat B( 35 Cl, pn) 44m Sc. The measured thin target cross sections show an overestimation by several statistical models for the scandium radioisotopes. This is corroborated by the measured thick target production rates for both entrance channels. This may be due to angular momentum effects of a heavy ion entrance channel compared to light-ion production, but additional work is required to understand this discrepancy. Finally, these measurements demonstrate that the medically useful 43 Sc, 44g Sc, and 44m Sc radioisotopes can be free of the long-lived contaminant 46 Sc without the use of enriched targets, using heavy ion beams and robust target materials.

07 ISOTOPE AND RADIATION SOURCES↗

DOE OSTI2025

Spallation Neutron Source Proton Power Upgrade (PPU) Project: Lessons Learned for CD-4

The SNS PPU project goals were to design, build, install and test the equipment necessary to double the accelerator power from 1.4 MW to 2.8 MW and to deliver a 2.0 MW qualified target. PPU also included the provision of a stub-out in the SNS accumulator-ring-to-target tunnel to facilitate a rapid connection to a new proton beamline for the Second Target Station (STS) project. The power capability was doubled by increasing the proton beam energy by 33% and the peak beam current by 50%, relative to pre-PPU accelerator performance. The project also included modifications to some buildings and services. The PPU project accomplished the energy upgrade by fabricating and installing new superconducting radiofrequency (RF) cryomodules, with supporting RF equipment, in the existing linac tunnel and klystron gallery, respectively. The High Voltage Converter Modulators (HVCM) and klystrons for some of the existing installed RF equipment were upgraded to handle the higher beam current. The increased beam power of 2 MW on the First Target Station (FTS) was enabled by the addition of a new high-volume gas injection system for pressure pulse and cavitation mitigation in the mercury target and a redesigned mercury target vessel.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Documentation of Air Emissions Source Term for Radionuclide NESHAP Compliance: TA-53 Building 0984 Isotope Production Facility

This paper will document the air emissions source term for the TA-53 Building 0984 Isotope Production Facility (IPF). The facility has historically been managed as a minor source under Radionuclide NESHAP regulations, but began using a wider variety of irradiation targets and a higher beam current. To support expanded generation of actinium-225 for medical diagnostic and therapeutic uses, IPF is now irradiating thorium targets and the beam current is planned to increase from 250 microamperes up to 600 microamperes. These changes merit a review of the anticipated source term under the new proposed operational conditions. The end result of the review indicates the main stack (Exhaust Stack ES-1) needs to be managed as a major source with continuous emissions monitoring. No additional advance notifications or permitting is required as a result of these operational changes.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2026

Measurement of the LCLS-II dark current using the LDMX Trigger Scintillator Prototype

The Light Dark Matter eXperiment (LDMX) is a proposed fixed-target missing momentum search for sub-GeV thermal relic dark matter. LDMX aims to probe thermal dark matter targets with 1016 electrons on target. Such an approach requires a high-repetition rate, low-current beam, with an average of one electron on target per event. These requirements are well-suited to the DArk Sector Experiments at LCLS-II (DASEL) facility, which will take advantage of the unused RF buckets between LCLS-II bunches to produce a well-defined low-current beam with a 26.9 ns bunch spacing. This document describes the results of a measurement of dark current in the Sector 30 transfer line (S30XL) of the LCLS-II beam, using a prototype of the LDMX trigger scintillator (TS) subsystem.

Berzin, Elizabeth [SLAC]↗

DOE OSTI2025

Deuteron-induced reactions on natural Zr from threshold to 50 MeV: production of 86g Y

Two stacks of thin Zr foils were irradiated with 30 and 50 MeV deuterons, respectively, using the Lawrence Berkeley National Laboratory 88-Inch Cyclotron, and 19 excitation functions for nat Zr(d,x) reactions were measured over a beam energy range of 6.3–47.64 MeV, where the independent cross sections for nat Zr(d,x) 88 Nb and nat Zr(d,x) 86m,g Y were measured for the first time. The well-characterized nat Fe(d,x) 56 Co, nat Ni(d,x) 56 Co, nat Ni(d,x) 58 Co, nat Ni(d,x) 61 Cu, nat Ti(d,x) 46 Sc and nat Ti(d,x) 48 V monitor reactions were used to determine the deuteron beam current throughout the stacks. All cross sections were determined using High Purity Germanium (HPGe) detector γ-ray spectroscopy. A variance minimization technique was employed to simultaneously constrain the deuteron beam currents with multiple monitor reactions, thus reducing systematic uncertainties. An additional 16 channels are reported for reactions on the nickel, titanium, and iron monitor foils, leading to a total of 35 excitation functions, with seven reaction channels reported for the first time in this work. The measured excitation functions are compared to calculations provided by the reaction modeling codes TALYS – 2.0, ALICE – 2020, CoH – 3.5.3 and EMPIRE – 3.2.3, as well as the TENDL – 2023 data library. The degree of agreement between theory and experiments is discussed. The possible production of the important PET radionuclide 86g Y via the nat Zr(d,x) route was critically examined. The physical yields for nat Zr(d,x) 86 Y and other yttrium isotopes produced were calculated and compared to other production pathways. Due to high-level of associated radionuclide impurities, this route cannot deliver 86g Y suitable for medical applications.

86gY↗

DOE OSTI2025

Numerical Analysis of High-Order Modes in SRF Resonators for Particle Accelerators

Over the past decades, superconducting technology has rapidly evolved towards high accelerating gradients and low surface resistance, making it possible to operate particle accelerators with high average beam currents and large duty factors. However, RF losses due to coherent excitation of the HOM become the limiting factor for these regimes. Unlike the cavity operating mode, which is tuned separately, the HOM parameters can significantly vary from one cavity to another due to finite mechanical tolerances during the manufacturing process. Thus, it is of utmost importance to know the HOM parameter spread in advance in order to predict unexpected cryogenic losses, overheating of beam line components and maintain stable beam dynamics. In this paper, we present a method for generating cavity geometry with an arbitrary spread of mechanical imperfections and numerically evaluating HOM statistics. Knowing the spread of HOM parameters, we calculated the probability of resonant HOM losses in SRF accelerating cavities used in CW beam current machines such as the PIP-II and LCLS-II linacs, as well as for the SRF crab-cavity for the ILC project. Finally, we present experimental results of HOM spectra measurements in hundreds of 1.3 GHz cavities installed in LCLS-II cryomodules. Studying the effects of HOM excitation results in specifications of the SRF cavity and cryomodule and can significantly impact the efficiency and reliability of the machine operation.

Lunin, Andrei [Fermilab] (ORCID:0000000290096792)↗

DOE OSTI2025

Discovery of new isotopes in the fragmentation of 82 Se and insights into their production

The production cross sections of neutron-rich nuclei for elements just above 60 Ca were measured at the Facility for Rare Isotope Beams (FRIB). Four previously unobserved isotopes ( 63 Sc, 65,66 Ti, and 68 V) were produced, separated, and identified for the first time using the Advanced Rare Isotope Separator (ARIS). One event was found to be consistent with 61 Ca . The new isotopes were created through the interaction of an 82 Se beam with a carbon target at an energy of 228 MeV/𝑢 and a primary beam current of 1.07 p⁢µ⁢A. The event-by-event particle identification of the mass number (𝐴), atomic number (𝑍), and ionic charge state (𝑞) for the reaction products was achieved by combining measurements of energy loss, time of flight, magnetic rigidity, and total kinetic energy. This successful search for new isotopes, conducted at the beginning of FRIB's third year of operation, highlights the facility's discovery potential, which will continue to grow as the beam current increases. The production cross sections were analyzed in the context of the newly developed Δ⁢𝐵⁢𝐸 systematics that provides trends in neutron-rich regions and increased sensitivity to nuclear binding, an important nuclear structure observable. Furthermore, the new systematics addresses gaps in 𝑄 𝑔 -based methods commonly used to interpret the production cross sections of light neutron-rich elements, and provides an efficient empirical approach to describe cross-section trends across isotopic chains. Good agreement with the measured data was obtained when the Δ⁢𝐵⁢𝐸 systematics and abrasion-ablation calculations were performed using the Hartree-Fock-Bogoliubov (HFB-22) mass table.

59 ≤ A ≤ 89↗

DOE OSTI2025

Evaluation of current density measurement methods for high-current, low-beta electron beams

Recent current density measurements with a low-beta electron beam (β=0.5-0.75) are strongly affected by electron scatter and Cherenkov limits. These invasive measurements are heavily influenced by the electron energy and the intercepting material properties: density, index of refraction, and atomic number. We evaluate various measurement methods, including x-ray scintillation and Cherenkov emission. To optimize the x-ray scintillation technique for this energy regime, metal foils of differing atomic number (Z) and thickness were placed upstream of a scintillation screen. We have selected Cherenkov emitters, based on a material refractive index, in order to differentiate the contributions from electron scatter and produced fluorescence, Cherenkov emission, and total internal reflection. The observed distributions for both approaches are verified through MCNP6®. Additionally, the simulations provide insight as to what physical processes dominate the measured distribution. We conclude by determining the limits and optimal measurement range for each measurement technique.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Simulation and measurement of beam-induced heating of ceramic vacuum chambers

In this article, we summarize recent theoretical and experimental studies of the impedance and beam-induced heating of titanium-coated ceramic vacuum chambers used in the NSLS-II injection kickers. The impedance was calculated using the field matching theory assuming planar approximation and compared with the mpedanceake2 code. For the coating thickness of a few microns, we demonstrated that the beam-induced power is dissipated in the titanium coating and that the longitudinally averaged two-dimensional power density is approximated by an analytical expression, thus allowing the use of a simplified model of the power density as input for the code to simulate the temperature distribution with realistic nonuniform thickness of the Ti coating. For a few values of the NSLS-II beam current, we measured the beam-induced heating of two ceramic chambers using thermal sensors installed along the chamber and compared the measurement results with the simulations. Published by the American Physical Society 2024

36 MATERIALS SCIENCE↗

DOE OSTI2024

Proton beam dynamics in bare IOTA with intense space-charge

We are commissioning a 2.5-MeV proton beam for the Integrable Optics Test Accelerator at Fermilab, allowing experiments in the strong space-charge regime with incoherent betatron tune shifts nearing 0.5. Accurate modelling of space-charge dynamics is vital for understanding planned experiments. We compare anticipated emittance growth and beam loss in the bare IOTA configuration using transverse space-charge models in Xsuite, PyORBIT, and MADX simulation codes. Our findings reveal agreement within a factor of 2 in core phase-space density predictions up to 100 synchrotron periods at moderate beam currents, while tail distributions and beam loss show significant differences.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Proton Beam Dynamics in Bare IOTA with Intense Space-Charge

We are commissioning a 2.5~MeV proton beam for the Integrable Optics Test Accelerator at Fermilab, allowing experiments in the strong space-charge regime with incoherent betatron tune shifts nearing 0.5. Accurate modelling of space-charge dynamics is vital for understanding planned experiments. We compare anticipated emittance growth and beam loss in the bare IOTA configuration using transverse space-charge models in Xsuite, PyORBIT, and MAD-X simulation codes. Our findings reveal agreement within 30\% in core phase-space density predictions up to 100~synchrotron periods at moderate beam currents, while tail distributions and beam loss show significant differences.

43 PARTICLE ACCELERATORS↗

DOE OSTI2024

Beam Loss Assessment Through Use of Photomultiplier Tubes

Modern accelerators aim to deliver maximal beam current at stable energy with minimal beam loss. Environmental changes, among other factors, can result in increased beam loss and decreased beam throughput, prompting daily retuning of the accelerator. The compact nature of the oldest part of the linear accelerator limits the available beam instrumentation, making beam loss assessment and tuning difficult. Thus, additional devices for beam loss monitoring must be considered. Photomultiplier tube-based beam loss monitors (BLMs) were installed along the Fermilab drift tube Linac to assess beam loss. Due to noise, the data from the installed photomultiplier tubes was difficult to assess. After noise reduction and signal analysis, it was found that the signals produced by the photomultiplier tubes in response to beam loss were consistent for a given configuration and therefore a reasonable measure of beam loss. This project lays groundwork for future work in beam loss assessment using photomultiplier tubes, with the automation of the process developed in this project being the next step in this effort.

Waggoner, Alexander↗

DOE OSTI2025

Influence of Photoemission Geometry on Timing and Efficiency in 4D Ultrafast Electron Microscopy

Broader adoption of 4D ultrafast electron microscopy (UEM) for the study of chemical, materials, and quantum systems is being driven by development of new instruments as well as continuous improvement and characterization of existing technologies. Perhaps owing to the still-high barrier to entry, the full range of capabilities of laser-driven 4D UEM instruments has yet to be established, particularly when operated at extremely low beam currents (~fA). Accordingly, with an eye on beam stability, we have conducted particle tracing simulations of unconventional off-axis photoemission geometries in a UEM equipped with a thermionic-emission gun. Specifically, we have explored the impact of experimentally adjustable parameters on the time-of-flight (TOF), the collection efficiency (CE), and the temporal width of ultrashort photoelectron packets. The adjustable parameters include the Wehnelt aperture diameter (DW), the cathode set-back position (Ztip), and the position of the femtosecond laser on the Wehnelt aperture surface relative to the optic axis (Rphoto). Notable findings include significant sensitivity of TOF to DW and Ztip, as well as non-intuitive responses of CE and temporal width to varying Rphoto. As a means to improve accessibility, practical implications and recommendations are emphasized wherever possible.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗