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Inverse atmospheric radiative transfer problems - A nonlinear minimization search method of solution

The paper studies the inversion of the radiative transfer equation describing the interaction of electromagnetic radiation with atmospheric aerosols. The interaction can be considered as the propagation in the aerosol medium of two light beams: the direct beam in the line-of-sight attenuated by absorption and scattering, and the diffuse beam arising from scattering into the viewing direction, which propagates more or less in random fashion. The latter beam has single scattering and multiple scattering contributions. In the former case and for single scattering, the problem is reducible to first-kind Fredholm equations, while for multiple scattering it is necessary to invert partial integrodifferential equations. A nonlinear minimization search method, applicable to the solution of both types of problems has been developed, and is applied here to the problem of monitoring aerosol pollution, namely the complex refractive index and size distribution of aerosol particles.

Fymat, A. L.↗

Why Does Atmospheric Radiative Heating Weaken Midlatitude Cyclones?

Abstract Recent work has indicated that atmospheric radiative heating reduces the kinetic energy of large‐scale eddies in the midlatitudes. However, a physical mechanism that connects radiation to the midlatitude eddy kinetic energy is still uncertain. Using a high‐resolution general circulation model we perform an experiment in which the radiative cooling profile at each model time step is overwritten with the climatological mean, computed from a control simulation. This approach separates the mean and transient effects of radiative heating on the extratropical circulation. We find that, when radiative heating is fixed, the globally‐averaged eddy kinetic energy is enhanced by ∼6%. We show that thermal radiation dampens temperature anomalies near the surface and tropopause in low‐pressure systems, destroying eddy available potential energy and eddy kinetic energy. We identify this as a possible mechanism by which atmospheric radiative heating weakens midlatitude cyclones.

Mischell, Eric↗

The Role of DYNAMO in Situ Observations in Improving NASA Ceres-like Daily Surface and Atmospheric Radiative Flux Estimates

The daily surface and atmospheric radiative fluxes from NASA Clouds and the Earths RadiantEnergy System (CERES) Synoptic 1 degree (SYN1deg) Ed3A are among the most widely used data to studycloud-radiative feedback. The CERES SYN1deg data are based on Fu-Liou radiative transfer computations thatuse specific humidity (Q) and air temperature (T) from NASA Global Modeling and Assimilation Office (GMAO)reanalyses as inputs and are therefore subject to the quality of those fields. This study uses in situ Q and Tobservations collected during the Dynamics of the Madden-Julian Oscillation (DYNAMO) field campaign toaugment the input stream used in the NASA GMAO reanalysis and assess the impact on the CERES dailysurface and atmospheric longwave estimates. The results show that the assimilation of DYNAMOobservations considerably improves the vertical profiles of analyzed Q and T over and near DYNAMO stationsby moistening and warming the lower troposphere and upper troposphere and drying and cooling themid-upper troposphere. As a result of these changes in Q and T, the computed CERES daily surface downwardlongwave flux increases by about 5 W m(exp -2), due mainly to the warming and moistening in the lowertroposphere; the computed daily top-of-atmosphere (TOA) outgoing longwave radiation increases by2-3 W m(exp -2) during dry periods only. Correspondingly, the estimated local atmospheric longwave radiativecooling enhances by about 5 W m(exp -2) (7-8 W m(exp -2)) during wet (dry) periods. These changes reduce the bias inthe CERES SYN1deg-like daily longwave estimates at both the TOA and surface and represent animprovement over the DYNAMO region.

DYNAMO↗

Preliminary design for Arctic atmospheric radiative transfer experiments

If current plans are realized, within the next few years, an extraordinary set of coordinated research efforts focusing on energy flows in the Arctic will be implemented. All are motivated by the prospect of global climate change. SHEBA (Surface Energy Budget of the Arctic Ocean), led by the National Science Foundation (NSF) and the Office of Naval Research (ONR), involves instrumenting an ice camp in the perennial Arctic ice pack, and taking data for 12-18 months. The ARM (Atmospheric Radiation Measurement) North Slope of Alaska and Adjacent Arctic Ocean (NSA/AAO) Cloud and Radiation Testbed (CART) focuses on atmospheric radiative transport, especially in the presence of clouds. The NSA/AAO CART involves instrumenting a sizeable area on the North Slope of Alaska and adjacent waters in the vicinity of Barrow, and acquiring data over a period of about 10 years. FIRE (First ISCCP (International Satellite Cloud Climatology Program) Regional Experiment) Phase 3 is a program led by the National Aeronautics and Space Administration (NASA) which focuses on Arctic clouds, and which is coordinated with SHEBA and ARM. FIRE has historically emphasized data from airborne and satellite platforms. All three program anticipate initiating Arctic data acquisition during spring, 1997. In light of his historic opportunity, the authors discuss a strawman atmospheric radiative transfer experimental plan that identifies which features of the radiative transport models they think should be tested, what experimental data are required for each type of test, the platforms and instrumentation necessary to acquire those data, and in general terms, how the experiments could be conducted. Aspects of the plan are applicable to all three programs.

Zak, B. D.↗

Performance and Reliability Assessment of the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) Data Advisor (ADA)

The Atmospheric Radiation Measurement (ARM) User Facility provides one of the world's largest openly accessible repositories of atmospheric observations through the ARM Data Discovery platform. Although the repository contains more than three decades of measurements collected from permanent observatories, mobile facilities, aircraft campaigns, and field experiments, identifying appropriate datasets can be challenging, particularly for new users unfamiliar with ARM instrumentation and datastream organization. To improve data accessibility, the ARM Data Center developed the ARM Data Advisor (ADA), an artificial intelligence-powered assistant designed to facilitate scientific data discovery, dataset interpretation, and user guidance. This report evaluates ADA's performance as a domain-specific scientific assistant using realistic atmospheric science workflows. The evaluation examines five key capabilities: data retrieval and curation efficiency, hallucination resistance, scientific reasoning, response to ambiguous queries, and content retention and session continuity. Representative prompts were developed to simulate typical interactions between researchers and the ARM Data Discovery platform, and ADA's responses were assessed for retrieval completeness, scientific accuracy, consistency, and practical usefulness. In these representative tests, ADA reduced the complexity of discovering and accessing ARM datasets by recommending appropriate datastreams, explaining instrumentation, interpreting metadata, and assisting with data processing workflows. ADA also exhibits strong domain knowledge of atmospheric science terminology and generally resists hallucination by acknowledging unavailable datasets and requesting clarification when appropriate. Overall, the results indicate that ADA represents a promising advancement in scientific data discovery within the ARM User Facility and has considerable potential to improve researcher productivity, particularly for new users and interdisciplinary scientists seeking efficient access to ARM observations.

Salvador, Christian [ORNL] (ORCID:0000000283287777↗

Atmospheric Radiation Measurement (ARM)/CART site

The DOE's Atmospheric Radiation Measurement (ARM) goals are as follows: (1) to provide an experimental test bed for improving the treatment of radiative transfer in global climate models (GCM's) under all kinds of cloud cover; and (2) to improve the parameterization and modeling of cloud formation, maintenance, dissipation, and related processes in GCM's. The scientific requirements which are most critical to the objectives of ARM are discussed.

Pennell, Bill↗

Validation of the Archived CERES Surface and Atmosphere Radiation Budget (SARB) at SGP

The CERES Surface and Atmosphere Radiation Budget (SARB) product (Charlock et al, 2002) includes the vertical profile of broadband SW, broadband LW, and 8-12 micron window (WN) fluxes; upwelling and downwelling at TOA, 70 hPa, 200 hPa, 500 hPa, and the surface; and for all-sky and clear-sky conditions. We test the archived CERES TRMM record of SARB for January-August 1998 and focus on discrepancies with ground-based measurements at SGP. The CERES SARB is generated by a highly modified Fu-Liou radiative transfer code (Fu and Liou, 1993). The most critical inputs for this application are cloud optical properties (fractional area, optical depth, particle size and phase, height of top, and estimate of geometrical thickness Minnis et al., 2002) from the narrowband VIRS imager. Numerous VIRS pixels (approx. 2km resolution at nadir) are matched to each of the large (approx. 20km) CERES broadband footprints (Wielicki et al, 1996). Other inputs include temperature and humidity from ECMWF (Rabier et al, 1998) , NCEP ozone profiles from SBUV and TOVS (Yang et al, 2001), aerosol optical thickness (AOT) from the Model for Atmospheric Transport and Chemistry (MATCH) aerosol assimilation (Collins et al., 2001) or alternately from the VIRS imager (Ignatov and Stowe, 2000). VIRS AOT is available for clear and partly cloudy ocean footprints during daylight; and only when viewing geometry renders a contribution from sunglint as unlikely. For other footprints, AOT is taken from MATCH. AOT is apportioned into fractions of dust (Tegan and Lacis, 1996), sea salt, sulfate, dust, soluble organic, insoluble organic, and soot (Hess et al., 1996) using the 6-hourly MATCH output. Tuned fluxes are retrieved by adjusting inputs to nudge computed TOA fluxes toward CERES observations (Rose et al, 1997). In clear conditions, the fields of humidity, surface skin temperature, surface albedo and AOT are adjusted to produce a closer match of computed and observed fluxes at TOA. When CERES footprints have clouds, the cloud optical thickness, fractional area within the footprint, and temperature of cloud top are adjusted by the tuning algorithm. Both tuned and untuned fluxes are archived, as are the respective adjustments to any parameters at the surface or within the atmosphere.

Charlock, Thomas P.↗

The Skylab concentrated atmospheric radiation project

The Skylab field phase in June, August and September of 1973 for the Skylab concentrated atmospheric radiation project provided an opportunity to conduct infrared and solar observations and subsequent calculations beneath the orbiting space vehicle during EREP overpasses. Infrared and solar transmission and absorption properties observed within the atmosphere were compared with EREP experiments, notably the S-191 and S-192. These same observations were later employed in the development and comparison of various atmospheric infrared and solar radiative transfer approximations. Solar radiation observations and calculations in the scattering atmosphere included the 0.4 to 1.1 microns spectral range while infrared observations and calculations covered the spectral band and portions thereof within the 5.0 to 40.0 microns region. Principal conclusions drawn from the solar radiation research and the infrared radiation research are discussed.

Kuhn, P. M.↗

The Atmospheric Radiation Measurement Program May 2003 Intensive Operations Period Examining Aerosol Properties and Radiative Influences: Preface to Special Section

Atmospheric aerosols influence climate by scattering and absorbing radiation in clear air (direct effects) and by serving as cloud condensation nuclei, modifying the microphysical properties of clouds, influencing radiation and precipitation development (indirect effects). Much of present uncertainty in forcing of climate change is due to uncertainty in the relations between aerosol microphysical and optical properties and their radiative influences (direct effects) and between microphysical properties and their ability to serve as cloud condensation nuclei at given supersaturations (indirect effects). This paper introduces a special section that reports on a field campaign conducted at the Department of Energy Atmospheric Radiation Measurement site in North Central Oklahoma in May, 2003, examining these relations using in situ airborne measurements and surface-, airborne-, and space-based remote sensing.

Ferrare, Richard↗

Radiative Flux Measurements from ARISE: A Comparison with CERES Top-of-Atmosphere Radiative Fluxes

Uncertainty in top-of-atmosphere (TOA) radiation fluxes observations are larger in the Arctic than in other regions. These uncertainties are due to the low sun angles and the highly reflective, anisotropic, and heterogeneous surface conditions. Quantifying, attributing, and reducing Arctic TOA radiative flux uncertainty enables a better understanding of the rapidly changing Arctic. To advance this goal, we compare the Cloud and Earth’s Radiant Energy System (CERES) TOA radiative fluxes with Arctic Radiation-IceBridge Sea and Ice Experiment (ARISE) campaign measurements collected in September 2014. We compare CERES TOA and aircraft radiative flux measurements using two complementary approaches: grid box average fluxes and instantaneously matched footprints. The grid box mean flux comparison indicates an agreement between CERES and aircraft measurements within 2 uncertainty (calibration and inversion) in the longwave for all five grid boxes and for four-of-five grid boxes in the shortwave; shortwave and longwave mean differences are -7.9 and +2.3 Wm‑2, respectively. The comparison of 36 instantaneously matched footprints with aircraft measurements reveals mean differences of -10.5 and 0.4 Wm‑2 in the shortwave and longwave, respectively. To further explore the persistent negative difference in the shortwave, we further quantify the effects of temporal and spatial sampling differences, angular distribution models, and scene identification to CERES-aircraft differences. Our analysis indicates that sampling differences (including scene evolution) account for an additional 1.8 and 1.7% uncertainty in the shortwave and longwave, respectively and indicates no bias. After accounting for this sampling uncertainty, all CERES-aircraft grid box mean fluxes agree within 2 uncertainty. Scene identification errors due to sea ice concentration data set differences exhibit no bias in the shortwave flux difference and indicate the possibility of substantial differences in the CERES fluxes in specific cases with large spatial heterogeneity. Considering the instantaneously matched footprints, we find that the angular distribution models account may account for up to ‑7.3 Wm-2 of the persistent CERES-aircraft shortwave flux difference due to systematic differences in the anisotropy for sea ice partly cloudy scenes. Additional analysis using a special scan model with the CERES FM2 instrument suggests a significant view zenith angle dependence of the CERES fluxes for sea ice partly cloudy scenes where shortwave fluxes systematically decrease with increasing view zenith angle; no dependence is found for other scene types. We conclude that (1) spatial heterogeneity and scene temporal evolution substantially limit our ability to use aircraft measurements to place strong constraints on CERES TOA fluxes and (2) that the representation of anisotropy in sea ice partly cloudy scenes is a significant factor contributing to the persistent negative CERES-aircraft shortwave flux difference in this comparison and require additional data to analysis fully quantify the potential bias.

Patrick C Taylor↗

Introduction to the Theory of Atmospheric Radiative Transfer

The fundamental physical and mathematical principles governing the transmission of radiation through the atmosphere are presented, with emphasis on the scattering of visible and near-IR radiation. The classical two-stream, thin-atmosphere, and Eddington approximations, along with some of their offspring, are developed in detail, along with the discrete ordinates method of Chandrasekhar. The adding and doubling methods are discussed from basic principles, and references for further reading are suggested.

Buglia, J. J.↗

Technical Report Series on Global Modeling and Data Assimilation: A Coupled Ocean-Atmosphere Radiative Model for Global Ocean Biogeochemical Models - Volume 22

An ocean-atmosphere radiative model (OARM) evaluates irradiance availability and quality in the water column to support phytoplankton growth and drive ocean thermodynamics. An atmospheric component incorporates spectral and directional effects of clear and cloudy skies as a function of atmospheric optical constituents, and spectral reflectance across the air-sea interface. An oceanic component evaluates the propagation of spectral and directional irradiance through the water column as a function of water, five phytoplankton groups, and chromophoric dissolved organic matter. It tracks the direct and diffuse streams from the atmospheric component, and a third stream, upwelling diffuse irradiance. The atmospheric component of OARM was compared to data sources at the ocean surface with a coefficient of determination (r2) of 0.97 and a root mean square of 12.1%.

Gregg, Watson W.↗

The Skylab concentrated atmospheric radiation project - An overview

An overview is presented of the Skylab Concentrated Atmospheric Radiation Project (SCARP), which was conducted to determine the accuracy and applicability of different models of radiation transfer through air masses of differing characteristics including varying amounts of wet and dry aerosols. Sites surveyed included onshore and offshore areas in the vicinity of Houston, Texas, the White Sands Missile Range in New Mexico, and Phoenix, Arizona, which provided a variety of warm, hot, dry, wet, clean, and dirty atmospheres. A typical exercise is described, and problems encountered during the experiment are discussed. It is noted that ten models of atmospheric scattering were utilized and that available data is being compared with the models.

Whitehead, V. S.↗

Cloud Droplet Size and Liquid Water Path Retrievals From Zenith Radiance Measurements: Examples From the Atmospheric Radiation Measurement Program and the Aerosol Robotic Network

The ground-based Atmospheric Radiation Measurement Program (ARM) and NASA Aerosol Robotic Network (AERONET) routinely monitor clouds using zenith radiances at visible and near-infrared wavelengths. Using the transmittance calculated from such measurements, we have developed a new retrieval method for cloud effective droplet size and conducted extensive tests for non-precipitating liquid water clouds. The underlying principle is to combine a water-absorbing wavelength (i.e. 1640 nm) with a nonwater-absorbing wavelength for acquiring information on cloud droplet size and optical depth. For simulated stratocumulus clouds with liquid water path less than 300 g/sq m and horizontal resolution of 201m, the retrieval method underestimates the mean effective radius by 0.8 m, with a root-mean-squared error of 1.7 m and a relative deviation of 13 %. For actual observations with a liquid water path less than 450 gm.2 at the ARM Oklahoma site during 2007-2008, our 1.5 min-averaged retrievals are generally larger by around 1 m than those from combined ground-based cloud radar and microwave radiometer at a 5min temporal resolution. We also compared our retrievals to those from combined shortwave flux and microwave observations for relatively homogeneous clouds, showing that the bias between these two retrieval sets is negligible, but the error of 2.6 m and the relative deviation of 22% are larger than those found in our simulation case. Finally, the transmittance-based cloud effective droplet radii agree to better than 11% with satellite observations and have a negative bias of 1 m. Overall, the retrieval method provides reasonable cloud effective radius estimates, which can enhance the cloud products of both ARM and AERONET.

Chiu, J. C.↗

The Performance of Current Atmospheric Radiation Codes in Phase I of CIRC

The Continual Intercomparison of Radiation Codes (CIRC) is intended as an evolving and regularly updated reference source for evaluation of radiative transfer (RT) codes used in Global Climate Models and other atmospheric applications. In our presentation we will discuss our evaluation of the performance of 13 shortwave and 11 longwave RT codes that participated in Phase I of CIRC. CIRC differs from previous intercomparisons in that it relies on an observationally validated catalogue of cases. The seven CIRC Phase I baseline cases, five cloud-free, and two with overcast liquid clouds, are built around observations by the Atmospheric Radiation Measurements (ARM) program that satisfy the goals .of Phase I, namely to examine RT model performance in realistic, yet not overly complex, atmospheric conditions. Besides the seven baseline cases, additional idealized "subcases" are also examined to facilitate interpretation of model errors. We will quantify individual model performance with respect to reference line-by-line calculations, and will also highlight RT code behavior for conditions of doubled CO2 , aspects of utilizing a spectral specification of surface albedo, and the impact of the inclusion of scattering in the thermal infrared. Our analysis suggests that RT codes should work towards improving their calculation of diffuse shortwave flux, shortwave absorption, treatment of spectral surface albedo, and shortwave CO2 forcing. Despite practical difficulties in comparing our results to previous results by the Intercomparison of Radiation Codes in Climate Models (ICRCCM) conducted about 20 years ago, it appears that the current generation of RT codes do indeed perform better than the codes of the ICRCCM era. By enhancing the range of conditions under which participating codes are tested, future CIRC phases will hopefully allow even more rigorous examination of RT code performance.

Oreopoulos, L.↗