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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Attosecond inner-shell lasing at ångström wavelengths

Since the invention of the laser, nonlinear effects such as filamentation, Rabi cycling and collective emission have been explored in the optical regime, leading to a wide range of scientific and industrial applications. X-ray free-electron lasers (XFELs) have extended many optical techniques to X-rays for their advantages of ångström-scale spatial resolution and elemental specificity. An example is XFEL-driven inner-shell Kα 1 (2p 3/2 → 1s 1/2 ) X-ray lasing in elements ranging from neon to copper, which has been used for nonlinear spectroscopy and development of new X-ray laser sources. Here, in this study, we show that strong lasing effects similar to those in the optical regime can occur at 1.5–2.1 Å wavelengths during high-intensity (>10 19 W cm −2 ) XFEL-driven Kα 1 lasing of copper and manganese. Depending on the temporal XFEL pump pulse substructure, the resulting X-ray pulses (about 10 6 −10 8 photons) can exhibit strong spatial inhomogeneities and spectral splitting, inhomogeneities and broadening. Three-dimensional Maxwell–Bloch calculations show that the observed spatial inhomogeneities result from X-ray filamentation and that the broad spectral features are driven by sub-femtosecond Rabi cycling. Our simulations indicate that these X-ray pulses can have pulse lengths of less than 100 attoseconds and coherence properties that provide opportunities for quantum X-ray optics applications.

47 OTHER INSTRUMENTATION↗
DOE OSTI2025

Laser-driven ultrafast transmission electron microscopy

Recent advances in lasers and electron optics technology have allowed transmission electron microscopes to achieve high spatial and temporal resolution, making them capable of tracking atoms, charges and spin motions down to the attosecond and nanometre scales. This Primer discusses the most common and practical experimental implementation of time-resolved transmission electron microscopy and the stroboscopic mode for evaluating ultrafast reversible dynamics. An in-depth discussion of photo-induced near-field electron microscopy, a technique unique to laser-assisted electron microscopy, is also provided, covering its prospective applications in the study of coherent phenomena in quantum materials. The experimental strategies and limitations in investigating the structural dynamics of materials and nanostructures by imaging, diffraction and spectroscopy are also described in detail, with a direct comparison with more conventional and established techniques. Here, we provide key information for new researchers who intend to use ultrafast transmission electron microscopy to address new challenges in specific materials science, condensed matter and nanophotonics.

Transmission electron microscopy↗
DOE OSTI2021

Electron choreography at the attosecond time scale

Abstract In this work, we report on coherent control of electron dynamics in atoms via attosecond pulse-shaping. We show that the photoelectron emission from argon gas produced by absorption of an attosecond pulse train (APT) made of odd and even harmonics can be manipulated along the direction of polarization of the light by tuning the spectral components (amplitude and phase) of the pulse. In addition, we show that APTs produced with a two-color (400- plus 800 nm) femtosecond driving field exhibit high temporal tunability, which is optimized for an intensity ratio between the two colors in the range of 0.1 to 5%.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS2007

Mobile CARS - IRS Instrument for Simultaneous Spectroscopic Measurement of Multiple Properties in Gaseous Flows

This paper describes a measurement system based on the dual-pump coherent anti-Stokes Raman spectroscopy (CARS) and interferometric Rayleigh scattering (IRS) methods. The IRS measurement is performed simultaneously with the CARS measurement using a common green laser beam as a narrow-band light source. The mobile CARS-IRS instrument is designed for the use both in laboratories as well as in ground-based combustion test facilities. Furthermore, it is designed to be easily transported between laboratory and test facility. It performs single-point spatially and temporally resolved simultaneous measurements of temperature, species mole fraction of N2, O2, and H2, and two-components of velocity. A mobile laser system can be placed inside or outside the test facility, while a beam receiving and monitoring system is placed near the measurement location. Measurements in a laboratory small-scale Mach 1.6 H2-air combustion-heated supersonic jet were performed to test the capability of the system. Final setup and pretests of a larger scale reacting jet are ongoing at NASA Langley Research Center s Direct Connect Supersonic Combustor Test Facility (DCSCTF).

Bivolaru, Daniel↗
NASA NTRS2016

Electromagnetic Basis of Metabolism and Heredity

Living organisms control their cellular biological clocks to maintain functional oscillation of the redox cycle, also called the "metabolic cycle" or "respiratory cycle". Organization of cellular processes requires parallel processing on a synchronized time-base. These clocks coordinate the timing of all biochemical processes in the cell, including energy production, DNA replication, and RNA transcription. When this universal time keeping function is perturbed by exogenous induction of reactive oxygen species (ROS), the rate of metabolism changes. This causes oxidative stress, aging and mutations. Therefore, good temporal coordination of the redox cycle not only actively prevents chemical conflict between the reductive and oxidative partial reactions; it also maintains genome integrity and lifespan. Moreover, this universal biochemical rhythm can be disrupted by ROS induction in vivo. This in turn can be achieved by blocking the electron transport chain either endogenously or exogenously by various metabolites, e.g. hydrogen sulfide (H2S), highly diffusible drugs, and carbon monoxide (CO). Alternatively, the electron transport in vivo can be attenuated via a coherent or interfering transfer of energy from exogenous ultralow frequency (ULF) and extremely low frequency (ELF) electromagnetic (EM) fields, suggesting that-on Earth-such ambient fields are an omnipresent (and probably crucially important) factor for the time-setting basis of universal biochemical reactions in living cells. Our work demonstrated previously un-described evidence for quantum effects in biology by electromagnetic coupling below thermal noise at the universal electron transport chain (ETC) in vivo.

Electromagnetic↗
DOE OSTI2024

Modeling phonon-mediated quasiparticle poisoning in superconducting qubit arrays

Correlated errors caused by ionizing radiation impacting superconducting qubit chips are problematic for quantum error correction. Such impacts generate quasiparticle (QP) excitations in the qubit electrodes, which temporarily reduce qubit coherence significantly. The many energetic phonons produced by a particle impact travel efficiently throughout the device substrate and generate quasiparticles with high probability, thus causing errors on a large fraction of the qubits in an array simultaneously. Here, we describe a comprehensive strategy for the numerical simulation of the phonon and quasiparticle dynamics in the aftermath of an impact. We compare the simulations with experimental measurements of phonon-mediated QP poisoning and demonstrate that our modeling captures the spatial and temporal footprint of the QP poisoning for various configurations of phonon downconversion structures. We thus present a path forward for the operation of superconducting quantum processors in the presence of ionizing radiation.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1980

Coherent Anti-stokes Raman Spectroscopy (CARS) of gun propellant flames

Temperature measurements were made in a slightly fuel rich, premixed propane/air reference flame and nitrate ester propellant flames burning in air at atmospheric pressure using coherent anti-stokes raman scattering (CARS). Both single and multiple pulse VARS spectra of nitrogen in the reference flame were in good agreement with calculated and reported values. Single pulse CARS nitrogen spectra obtained in the propellant flames were analyzed to give temperatures consistent with values calculated using the NASA-Lewis thermochemical calculation. Comparison of a 0.1 second separated sequence of single pulse CARS spectra indicate turbulent air mixing in these propellant flames. The CARS spectral results demonstrate that temporal and spatially resolved temperature measurements could be determined in transient, turbulent flames.

Mcilwain, M. E.↗
DOE OSTI2021

Influence of inhomogeneous stochasticity on the falsifiability of mean-field theories and examples from accretion disc modelling

ABSTRACT Despite spatial and temporal fluctuations in turbulent astrophysical systems, mean-field theories can be used to describe their secular evolution. However, observations taken over time scales much shorter than dynamical time scales capture a system in a single state of its turbulence ensemble. Comparing with mean-field theory can falsify the latter only if the theory is additionally supplied with a quantified precision. The central limit theorem provides appropriate estimates to the precision only when fluctuations contribute linearly to an observable and with constant coherent scales. Here, we introduce an error propagation formula that relaxes both limitations, allowing for non-linear functional forms of observables and inhomogeneous coherent scales and amplitudes of fluctuations. The method is exemplified in the context of accretion disc theories, where inhomogeneous fluctuations in the surface temperature are propagated to the disc emission spectrum – the latter being a non-linear and non-local function of the former. The derived precision depends non-monotonically on emission frequency. Using the same method, we investigate how binned spectral fluctuations in telescope data change with the spectral resolving power. We discuss the broader implications for falsifiability of a mean-field theory.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1988

Plasma instabilities stimulated by HF transmitters in space

Diffuse incoherent signal returns are often observed on Alouette and ISIS topside ionograms in addition to coherent echoes of electromagnetic and electrostatic waves. These diffuse signals, which at times can be the dominant features on topside ionograms, have been attributed to sounder-induced temperature anisotropies which drive the Harris instability. Previous theoretical investigations were based on the electrostatic approximation to the dispersion equation. The present paper will present calculations indicating that when the electromagnetic terms are retained in the dispersion equation and when the sounder-stimulated perpendicular electron temperature approaches 1 keV, then the whistler mode can have a temporal growth rate larger than the electrostatic electron cyclotron harmonic wave mode central to the diffuse resonance problem. Present sounders lack the power and antenna lengths to generate whistler mode waves in this manner. In addition, such waves would have large group velocities and would quickly leave the vicinity of the sounder. Experiments to investigate the wave growth, propagation, and damping of such stimulated waves are planned for the 1990s using a highly flexible sounder on the Space Shuttle and a receiver on a subsatellite.

Benson, Robert F.↗
NASA NTRS2022

Study of the Mass-loss Rate from the Sun

We investigate the temporal evolution of the yearly total mass-loss rate (YTMLR) from the Sun through coronal mass ejections (CMEs) over solar cycles 23 and 24. The mass determination of CMEs can be subject to significant uncertainty. To minimize this problem, we have used extensive statistical analysis. For this purpose, we employed data included in the Coordinated Data Analysis Workshop (CDAW) catalog. We estimated the contributions to mass loss from the Sun from different subsamples of CMEs (selected on the basis of their masses, angular widths, and position angles). The temporal variations of the YTMLR were compared to those of the sunspot number (SSN), X-ray flare flux, and the Disturbance Storm Time (Dst) index. We show that the CME mass included in the CDAW catalog reflects with high accuracy the actual mass-loss rate from the Sun through CMEs. Additionally, it is shown that the CME mass distribution in the log-lin representation reflects the Gaussian distribution very well. This means that the CMEs included in the CDAW catalog form one coherent population of ejections that have been correctly identified. Unlike the CME occurrence rate, it turns out that the YTMLR is a very good indicator of solar activity (e.g., SSN) and space weather (e.g., Dst index) consequences. These results are very important, since the YTMLR, unlike the mass loss through solar wind, significantly depends on solar cycles.

the sun↗
DOE OSTI2021

Attosecond Intramolecular Scattering and Vibronic Delays

We study the temporal and vibrational signature of the universal nuclear recoil associated with the electron emission and intramolecular scattering that accompanies the photoelectric effect. We illustrate these phenomena in the photoionization of the CO molecule from the C-1s orbital using an analytical model that reproduces the entangled character of the nuclear and electronic motion in this process. We show that the photoelectron emission delay can be decomposed into its localization and resonant-confinement components. Photoionization by a broadband x-ray pulse results in a coherent vibrational ionic state delayed compared to the classical sudden-photoemission limit.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS2019

MODIS Aqua Reflective Solar Bands Calibration for NASA's R2018 Ocean Color Products

Remote sensing ocean color products have stringent requirements on radiometric calibration stability. To address a calibration deficiency in MODIS Aqua in recent years, the NASA Ocean Biological Processing Group (OBPG) developed a new calibration for the reflective solar bands. Prior to the reprocessing of NASA's ocean color products for 2018 (R2018), the OBPG MODIS products had been based on calibration provided by the MODIS Calibration Support Team (MCST). Several modifications were made to the MCST calibration approach to improve the calibration accuracy for ocean color products. These include: 1) apply 936nm detector normalization to solar diffuser stability monitor (SDSM) data to reduce coherent noise; 2) modeling solar diffuser (SD) degradation wavelength dependency to determine SD degradation in near-infrared and shortwave infrared wavelength; 3) detector gains are computed using SD screen-closed data to better match ocean radiance levels in all bands; 4) a simple atmospheric correction is performed to reduce bidirectional reflectance distribution function (BRDF) effects in desert trends; 5) modulated relative spectral response (RSR) impact on ocean data is estimated and used to adjust the calibration coefficients. 6) smoothing is used to characterize the temporal change in calibration, and response versus scan angle (RVS) changes are characterized using 2nd order polynomials to improve spatial/temporal calibration stability. Relative to the previous R2014 ocean color products, the R2018 calibration removed the suspect late-mission global trends in blue-band water-leaving reflectance, and some anomalously large short-term variability (spikes) in the temporal trend of chlorophyll concentration. This paper will describe the OBPG calibration with a focus on the differences between the MCST and OBPG approaches.

calibration↗
NASA NTRS1992

Analysis of space geodetic measurements for studying the dynamics of the solid Earth

During the last decade, there has been an unprecedented improvement in both the accuracy and the temporal resolution of Earth rotation measurements. Determination of the position of the Earth's rotation axis both in inertial space and with respect to the crust with accuracies of about 0.3 milliarcseconds (mas) are now routine. In recent years, there has been an emphasis on the determination of short-period (daily and less) variations in Earth rotation. Two space based geodetic systems, very long baseline interferometry (VLBI) and the global positioning system (GPS) have proved to be very successful in this endeavor. Results for the tidally coherent part of the subdaily Earth rotation variations determined from the analysis of VLBI data are discussed. The magnitude of other subdaily variations are also considered.

Herring, Thomas A.↗
DOE OSTI2024

High-energy, low-jitter, narrowband ps probe laser for kHz-rate fs/ps coherent anti-Stokes Raman scattering

Hybrid fs/ps coherent anti-Stokes Raman scattering (CARS) thermometry often utilizes ps probe pulses derived from pulse shaping or spectrally filtering the primary laser source or by synchronization with a low repetition rate external laser. This results in limited energy, spectral resolution, and/or repetition rate of the ps probe. In this work, a master-oscillator power-amplifier (MOPA) laser was synchronized to the oscillator of a Ti:sapphire regenerative amplifier to achieve high-energy (600 µJ), narrowband (58 ps) probe pulses at kHz repetition rates. Furthermore, temporal filtering allows the pulse characteristics to be adjusted for each application. At 25 Torr, relevant to high-speed flows, the kHz-rate MOPA system generated signal-to-noise ratios 3× higher in nitrogen and had improved precision relative to a 10 ps probe derived from spectral filtering and the power-amplifier. The MOPA system also enabled single-shot ro-vibrational hybrid fs/ps CARS thermometry in 650 K heated air.

47 OTHER INSTRUMENTATION↗
NASA NTRS1993

Diurnal and Semidiurnal Variations in Earth Rotation

During the last decade there has been an unprecedented improvement in both the accuracy, the temporal resolution of Earth's rotation measurements. Determination of the position of the Earth's rotation axis both in inertial space and with respect to the crust with accuracies of about 0.3 milliarcseconds (mas) are now routine. In recent years, there has been and emphasis on the determination of short-period (daily and less) variations in Earth rotation. Two space based geodetic systems, very long baseline interferometry (VLBI) and the global positioning system (GPS) have proved to be very successful in this endeavor. Results for the tidally coherent part of the subdaily Earth rotation variations determined from the analysis of VLBI data are discussed. The magnitude of other subdaily variations are also considered.

Herring, T.↗
DOE OSTI2021

Ionizing photon interactions modulate the optical properties of crystals with femtosecond scale temporal resolution

In this work, we continue our study of a new method for the detection of ionizing radiation with the potential for a dramatic improvement in coincidence time resolution (CTR) for time-of-flight positron emission tomography (ToF-PET) using the modulation of a material's optical properties instead of the scintillation mechanism. Our previous work has shown that for non-scintillation materials such as bismuth silicon oxide (BSO) and cadmium telluride (CdTe), their refractive index can be modulated by annihilation photon interactions. Additionally, the ultrafast nature of this process however remains unexplored. The ionizing radiation-induced charge carriers alter the local band structure in these materials, thus changing the complex refractive index. This mechanism is routinely used at the linac coherent light source (LCLS) facility of the SLAC National Accelerator Laboratory to measure x-ray pulse arrival times with femtosecond scale resolution for photon energies between 0.5 and 10 keV. The method described here follows that example by using a frequency chirped visible continuum pulse to provide a monotonic wavelength-to-time mapping by which one can measure the time-dependent refractive index modulation. In addition, we describe an interference-based measurement setup that allows for significantly improved sensitivity while preserving a timing precision of approximately 10 fs (σ) when measuring the arrival time of below 10 keV x-ray pulses with yttrium aluminum garnet (YAG) crystal. The method is presented in the context of ToF-PET application with further discussions on the potential CTR achievable if a similar detection concept is adopted for detecting 511 keV photons. Semi-empirical analysis indicates that the predicted CTR achievable is on the order of 1 ps (FWHM).

59 BASIC BIOLOGICAL SCIENCES↗
NASA NTRS2003

Observed and Modeled Trends in Southern Ocean Sea Ice

Conceptual models and global climate model (GCM) simulations have both indicated the likelihood of an enhanced sensitivity to climate change in the polar regions, derived from the positive feedbacks brought about by the polar abundance of snow and ice surfaces. Some models further indicate that the changes in the polar regions can have a significant impact globally. For instance, 37% of the temperature sensitivity to a doubling of atmospheric CO2 in simulations with the GCM of the Goddard Institute for Space Studies (GISS) is attributable exclusively to inclusion of sea ice variations in the model calculations. Both sea ice thickness and sea ice extent decrease markedly in the doubled CO, case, thereby allowing the ice feedbacks to occur. Stand-alone sea ice models have shown Southern Ocean hemispherically averaged winter ice-edge retreats of 1.4 deg latitude for each 1 K increase in atmospheric temperatures. Observations, however, show a much more varied Southern Ocean ice cover, both spatially and temporally, than many of the modeled expectations. In fact, the satellite passive-microwave record of Southern Ocean sea ice since late 1978 has revealed overall increases rather than decreases in ice extents, with ice extent trends on the order of 11,000 sq km/year. When broken down spatially, the positive trends are strongest in the Ross Sea, while the trends are negative in the Bellingshausen/Amundsen Seas. Greater spatial detail can be obtained by examining trends in the length of the sea ice season, and those trends show a coherent picture of shortening sea ice seasons throughout almost the entire Bellingshausen and Amundsen Seas to the west of the Antarctic Peninsula and in the far western Weddell Sea immediately to the east of the Peninsula, with lengthening sea ice seasons around much of the rest of the continent. This pattern corresponds well with the spatial pattern of temperature trends, as the Peninsula region is the one region in the Antarctic with a strong record of temperature increases. Still, although the patterns of the temperature and ice changes match fairly well, there is a substantial ways to go before these patterns are understood (and can be modeled) in the full context of global change.

Parkinson, Claire L.↗
NASA NTRS2009

Discovery of a 115 Day Orbital Period in the Ultraluminous X-ray Source NGC 5408 X-1

We report the detection of a 115 day periodicity in SWIFT/XRT monitoring data from the ultraluminous X-ray source (ULX) NGC 5408 X-1. Our o ngoing campaign samples its X-ray flux approximately twice weekly and has now achieved a temporal baseline of ti 485 days. Periodogram ana lysis reveals a significant periodicity with a period of 115.5 +/- 4 days. The modulation is detected with a significance of 3.2 x 10(exp -4) . The fractional modulation amplitude decreases with increasing e nergy, ranging from 0.13 +/- 0.02 above 1 keV to 0.24 +/- 0.02 below 1 keV. The shape of the profile evolves as well, becoming less sharply peaked at higher energies. The periodogram analysis is consistent wi th a periodic process, however, continued monitoring is required to c onfirm the coherent nature of the modulation. Spectral analysis indic ates that NGC 5408 X-1 can reach 0.3 - 10 keV luminosities of approxi mately 2 x 10 40 ergs/s . We suggest that, like the 62 day period of the ULX in M82 (X41.4-1-60), the periodicity detected in NGC 5408 X-1 represents the orbital period of the black hole binary containing the ULX. If this is true then the secondary can only be a giant or super giant star.

Strohmayer, Tod E.↗