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At least 343 records · Page 19

All sources NASA NTRS DOE OSTI

DOE OSTI2023

Prediction on X-ray output of free electron laser based on artificial neural networks

Abstract Knowledge of x-ray free electron lasers’ (XFELs) pulse characteristics delivered to a sample is crucial for ensuring high-quality x-rays for scientific experiments. XFELs’ self-amplified spontaneous emission process causes spatial and spectral variations in x-ray pulses entering a sample, which leads to measurement uncertainties for experiments relying on multiple XFEL pulses. Accurate in-situ measurements of x-ray wavefront and energy spectrum incident upon a sample poses challenges. Here we address this by developing a virtual diagnostics framework using an artificial neural network (ANN) to predict x-ray photon beam properties from electron beam properties. We recorded XFEL electron parameters while adjusting the accelerator’s configurations and measured the resulting x-ray wavefront and energy spectrum shot-to-shot. Training the ANN with this data enables effective prediction of single-shot or average x-ray beam output based on XFEL undulator and electron parameters. This demonstrates the potential of utilizing ANNs for virtual diagnostics linking XFEL electron and photon beam properties.

47 OTHER INSTRUMENTATION↗

NASA NTRS1981

Theoretical quasar emission line ratios. IV - General asymptotic escape probabilities and the effects of linear Stark broadening

Established techniques permitting the evaluation of exact asymptotic forms of photon escape probabilities for a wide range of absorption coefficient profile types are used for QSO radiative transfer effect studies, and it is shown that the exact formulae are easily evaluated. It is found that some of the commonly used expressions overestimate the true value by a factor of about two, and a computationally expedient approximate expression is derived for the asymptotic form of the photon escape probability when linear Stark broadening contributes to the line absorption coefficient profile in hydrogenic lines. Attention is given to Lyman-alpha, for the case in which partial redistribution, over the linear Stark component of the line absorption coefficient profile, dominates single-flight photon escape.

Puetter, R. C.↗

NASA NTRS2000

Continued RXTE Observations of Three Blazars

This project continued (during Cycle 3 of the RXTE mission) weekly observations of the quasars PKS 1510-089 and 3C 454.3 and the BL Lac object OJ 287. The data were analyzed by the PI and his graduate student. In the middle of Cycle 3, the PI changed the mode of observation of 3C 454.3, based on a report from another astronomer that observations with the Rosat satellite had found a strong confusing X-ray source about 45 arcmin away. The RXTE observations, in which the flux was measured while pointing directly at 3C 454.3 and then 15' from 3C 454.3, in the direction away from the confusing source. The flux decreased considerably, and so it appears that nearly all the X-ray flux measured by RXTE comes from the confusing source rather than the quasar. OJ 287 was detected only at one epoch of the Cycle 3 observations. This corresponded to a particularly quiet period for this source, when its flux at other wavebands was also low. From the single epoch of detection, no conclusions can be drawn concerning the general nature of the X-ray emission from this object. In contrast to the other two sources, the results of the observations of PKS 1510-089, when combined with data from cycles 3 and 4, are very interesting. The RXTE (2.4-20 keV) abd 14.5 GHz University of Michigan Radio Astronomy Observatory (UMRAO) light curves through the end of RXTE Cycle 4 are shown for PKS 1510-089. Visual inspection reveals an obvious correlation between the X-ray and 14.5 GHz light curves. While this is as expected in the SSC model in a source with simultaneous mm-wave (the photons thought to be scattered to X-ray energies) and cm-wave variations, the X-ray spectrum is flat ("energy" spectral index alpha = 0.2-0.5, where F (sub v) proportional to v (sup - alpha)) compared with the mm-wave synchrotron spectrum (alpha approximately equal to 0.8). The PI is currently engaged in theoretical work to determine whether this is possible for an SSC model.

Marscher, Alan P.↗

DOE OSTI2021

Observation of biexciton emission from single semiconductor nanoplatelets

Quasi-two-dimensional semiconductor nanoplatelets (NPLs) are intriguing systems for studying the influence of Auger recombination processes on the multiexciton emission efficiencies in the weak in-plane confinement regime. We investigate CdSe/CdS core/shell NPLs using cryogenic temperature single particle spectroscopy and observe bright biexciton emission at high excitation powers. The average binding energy of the biexcitons is determined to be 16.5 meV. The observed switching between the biexciton and trion states indicates charging-decharging dynamics of the NPLs mediated by the Auger ionization process. These findings are highly relevant for harvesting efficient biexciton emission for energy, lighting, and quantum applications.

36 MATERIALS SCIENCE↗

DOE OSTI2025

High-energy X-ray radiography with apodized petawatt laser beams

We have produced laser wakefield-accelerated electron beams with energies of 2 GeV in Target Area 1 of the ZEUS facility. These electron beams oscillate in the accelerating structure that is produced in the wake of an ultrashort laser pulse (25 fs). These ’betatron’ oscillations result in the emission of a collimated (4 mrad divergence) beam of high-energy X-ray/gamma photons (on the order of several hundred keV). In this work, we demonstrate the capabilities of the ZEUS laser system by showing that apodizing the laser beam in the near field allows for the production of high-quality betatron X-rays for radiography purposes. This demonstrates that a high-power, large-aperture laser beam could be split into multiple parts to drive betatron X-ray sources from multiple angles or temporal delays into a High Energy Density (HED) target to be probed, enabling pump-probe measurements at multiple temporal delays or tomography on a single shot.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1986

Observation of a strong gamma-ray burst on the Spacelab 2 mission

The observation of MeV gamma radiation from a burst on August 5, 1985 is reported. The burst was dominated by a single peak about 2 s wide, with softer, lower-level emission lasting about 20 s anywhere in the burst in any energy range. In the energy range from about 560 keV to about 10 MeV, the burst peaked about 0.3 s before the peak at lower energies. Radiation in the 10-16 MeV energy range was detected about 3 s before the lower-energy radiation, with roughly the same pulse width. This radiation was not detected during the main part of the burst. The energy of this burst in the range above 1 MeV was a significant fraction of the total burst energy, confirming earlier SMM results. If the appearance of high-energy photons prior to those at low energies is a ubiquitous feature of bursts or a class of bursts, current theoretical models may require considerable revision.

Fishman, G. J.↗

DOE OSTI2023

Chapter 14: Surface plasmon resonance enhanced artificial photosynthesis of chemical fuels for energy storage

Nanostructured noble metals such as Au, Ag, and Cu have interesting optical properties because of the oscillation motions of their surface electrons upon strong coupling with light under resonance conditions. This resonant oscillation motion of conduction electrons refers to surface plasmon resonance (SPR) and localized SPR (LSPR) when localized near the surface of a nanoparticle. The extinction spectrum of a solution of plasmonic nanoparticles has tunable wavelength responses from UV to NIR due to strong light scattering and absorption which are highly sensitive to the permittivity of the nanoparticles, their sizes and shapes, and chemical environment. Strong light scattering due to the LSPR of plasmonic nanoparticles creates a strong localized and far-field intensity capable of enhancing light absorption characteristics of a chromophore near a plasmonic surface. Engineering the chromophores’ radiative decay dynamics can be done by 1) increasing its radiative decay rate to increase its photoluminescence intensity and 2) increasing its nonradiative decay rates associated to direct charge transfer to the metal surface. Such interesting photophysical properties of a chromophore can be extended to other light-absorbing materials such as semiconductor thin films and nanostructures. This plasmonic effect on the photophysics of a light-absorbing material can be theoretically and experimentally validated. The phenomenon has also been applied to advanced optoelectronic devices such as organic light-emitting diodes (OLED)1 and organic photovoltaics (OPV).2-4 The local field created by the SPR can provide an intense EM field to enhance photoluminescence emission of an organic chromophore5-8 and Raman scattering of an organic molecule, and single-molecule Raman9-10 can be detected on specially designed LSPR substrate. (Figure 1 on SPR for energy) Recent studies suggest that LSPR can be incorporated in light-harvesting and conversion systems to increase energy conversion in a solar cell and photoelectrochemical cell and chemical transformations of CO2 to chemical fuels.11-12 Plasmonic active metals naturally exhibit catalytic activities for electrochemical fuel conversion that can be enhanced by engineering their structures to form unique catalytic structures such as symmetry-broken Au-Cu Janus nanocrystals.13 These studies are critical to addressing the global challenges of energy14-15 and CO2 emission from nonrenewable sources such as coal, petroleum, and natural gas.16-17 Electrochemical systems comprised of unique photonic structures and functions that enable efficient and affordable energy harvesting/conversion/storage are highly desired for providing safe and environment-friendly energy sources. This chapter reviews our recent work of LSPR enabled photoelectrochemical water splitting and recent advances in LSPR-enabled CO2 reduction and photochemical reactions reported in the literature. Scientific and technical challenges of applying LSPR to enhance these energy conversion and storage systems are discussed at the conclusion of this chapter.

Pan, Shanlin↗

DOE OSTI2020

Effect of Many Modes on Self-Polarization and Photochemical Suppression in Cavities

The standard description of cavity-modified molecular reactions typically involves a single (resonant) mode, while in reality the quantum cavity supports a range of photon modes. In this work we demonstrate that as more photon modes are accounted for, physico-chemical phenomena can dramatically change, as illustrated by the cavity-induced suppression of the important and ubiquitous process of proton-coupled electron-transfer. Using a multi-trajectory Ehrenfest treatment for the photonmodes, we find that self-polarization effects become essential, and we introduce the concept of selfpolarization- modified Born-Oppenheimer surfaces as a new construct to analyze dynamics. As the number of cavity photon modes increases, the increasing deviation of these surfaces from the cavityfree Born-Oppenheimer surfaces, together with the interplay between photon emission and absorption inside the widening bands of these surfaces, leads to enhanced suppression. The present findings are general and will have implications for the description and control of cavity-driven physical processes of molecules, nanostructures and solids embedded in cavities.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2020

Integrated Data Analysis to Improve Te and Zeff Measurement on NSTX-U

The multi-energy soft x-ray (ME-SXR) camera is a new concept for a fusion plasma diagnostic based on a pixelated detector with adjustable photon cutoff thresholds. It is a single, compact, solid-state detector which combines spatial and spectral sensitivity and can be configured remotely at run time, making it ideal for a fusion environment. The detector can be configured for application to a wide range of physics problems including impurity transport, electron temperature profiles, and non-thermal effects. The detector has been installed on the Madison Symmetric Torus (MST) as part of a collaboration between Princeton Plasma Physics Laboratory and the University of Wisconsin–Madison to develop the technology and analysis techniques. A full diagnostic forward model of the ME-SXR diagnostic has been developed to enable analysis of the raw photon count data. This model incorporates the atomic physics underlying the plasma emission, diagnostic geometry, and detector response characteristics. Employing this model, a Bayesian analysis approach is used to extract electron temperature from the raw data. This analysis approach uses all available information, clearly quantifies prior information, and handles uncertainties transparently. The ME-SXR camera is being used to study the 3D (helical, stellarator-like) state that forms in the MST device. This helical core structure has improved energy confinement. The transition to the helical state is accompanied by a rise in electron temperature in the central part of the helical structure, but then this enhancement fluctuates. The characteristics of this fluctuation are being compared to a magneto-hydrodynamics model.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2023

VERITAS Discovery of Very High Energy Gamma-Ray Emission from S3 1227+25 and Multiwavelength Observations

We report the detection of very high energy gamma-ray emission from the blazar S3 1227+25 (VER J1230+253) with the Very Energetic Radiation Imaging Telescope Array System (VERITAS). VERITAS observations of the source were triggered by the detection of a hard-spectrum GeV flare on 2015 May 15 with the Fermi-Large Area Telescope (LAT). A combined 5 hr VERITAS exposure on May 16 and 18 resulted in a strong 13σ detection with a differential photon spectral index, Γ = 3.8 ± 0.4, and a flux level at 9% of the Crab Nebula above 120 GeV. This also triggered target-of-opportunity observations with Swift, optical photometry, polarimetry, and radio measurements, also presented in this work, in addition to the VERITAS and Fermi-LAT data. A temporal analysis of the gamma-ray flux during this period finds evidence of a shortest variability timescale of τ obs = 6.2 ± 0.9 hr, indicating emission from compact regions within the jet, and the combined gamma-ray spectrum shows no strong evidence of a spectral cutoff. An investigation into correlations between the multiwavelength observations found evidence of optical and gamma-ray correlations, suggesting a single-zone model of emission. Finally, the multiwavelength spectral energy distribution is well described by a simple one-zone leptonic synchrotron self-Compton radiation model.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1978

Flux measurements of CA II H and K emission

A four-channel photon-counting spectrophotometer (designated HKP-2) is described which is designed for measuring stellar chromospheric calcium emission. The HKP-2 is calibrated, and its performance and accuracy evaluated, by observing 63 of Wilson's (1968) program stars on the same nights with both the HKP-2 and a coude scanner designated HKP-1. The results of the observations are discussed in terms of the calibration of mean H-K flux indices, variations in individual stellar fluxes, the flux ratio for H and K, and the instrument color index. It is shown that the HKP-2 provides satisfactory performance in the measurement of stellar chromospheric emission in a manner closely analogous to the method of Wilson and that a single observation yields a color index as well as flux indices for H and K that can be calibrated and transferred unambiguously to Wilson's system of measurement.

Vaughan, A. H.↗

DOE OSTI2025

Progress in the development of an ultrafast pulsed ponderomotive phase plate for cryo-electron tomography

Cryo-electron tomography (cryo-ET) is a powerful modality for resolving cellular structures in their native state. While single-particle cryo-electron microscopy excels in determining protein structures purified from recombinant or endogenous sources due to an abundance of particles, weak contrast issues are accentuated in cryo-ET by low copy numbers in crowded cellular milieux. Continuous laser phase plates offer improved contrast in cryo-ET; however, their implementation demands exceptionally high-peak optical intensities. Instead, a novel experimental approach to enhance contrast in cryo-ET is to manipulate the phase of scattered pulsed electrons using ultrafast pulsed photons. Here, we outline the experimental design of a proof-of-concept electron microscope and demonstrate synchronization between electron packets and laser pulses. Furthermore, we show ultrabright photoemission of electrons from an alloy field emission tip using femtosecond ultraviolet pulses. These experiments pave the way toward exploring the utility of the ponderomotive effect using pulsed radiation to increase phase contrast in cryo-ET of subcellular protein complexes in situ, thus advancing the field of cell biology.

Du, Daniel X. [Columbia Univ., New York, NY (Unite↗

DOE OSTI2021

Electron shelving of a superconducting artificial atom

Interfacing long-lived qubits with propagating photons is a fundamental challenge in quantum technology. Cavity and circuit quantum electrodynamics (cQED) architectures rely on an off-resonant cavity, which blocks the qubit emission and enables a quantum non-demolition (QND) dispersive readout. However, no such buffer mode is necessary for controlling a large class of three-level systems that combine a metastable qubit transition with a bright cycling transition, using the electron shelving effect. Here we demonstrate shelving of a circuit atom, fluxonium, placed inside a microwave waveguide. With no cavity modes in the setup, the qubit coherence time exceeds 50 μs, and the cycling transition’s radiative lifetime is under 100 ns. By detecting a homodyne fluorescence signal from the cycling transition, we implement a QND readout of the qubit and account for readout errors using a minimal optical pumping model. Our result establishes a resource-efficient (cavityless) alternative to cQED for controlling superconducting qubits.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2021

Self-Isolated Raman Lasing with a Chiral Dielectric Metasurface

The light sources that power photonic networks are small and scalable, but they also require the incorporation of optical isolators that allow light to pass in one direction only, protecting the light source from damaging backreflections. Unfortunately, the size and complex integration of optical isolators makes small-scale and densely integrated photonic networks infeasible. Here, we overcome this limitation by designing a single device that operates both as a coherent light source and as its own optical isolator. Our design relies on high-quality-factor dielectric metasurfaces that exhibit intrinsic chirality. By carefully manipulating the geometry of the constituent silicon metaatoms, we design three-dimensionally chiral modes that act as optical spin-dependent filters. Using spin-polarized Raman scattering together with our chiral metacavity, we demonstrate Raman lasing in the forward direction, while the lasing action is suppressed by over an order of magnitude for reflected light. Our high-$\textit{Q}$ chiral metasurface design presents a new approach toward compactly isolating integrated light sources by directly tailoring the emission properties of the light source itself.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2024

Free-electron crystals for enhanced X-ray radiation

Abstract Bremsstrahlung—the spontaneous emission of broadband radiation from free electrons that are deflected by atomic nuclei—contributes to the majority of X-rays emitted from X-ray tubes and used in applications ranging from medical imaging to semiconductor chip inspection. Here, we show that the bremsstrahlung intensity can be enhanced significantly—by more than three orders of magnitude—through shaping the electron wavefunction to periodically overlap with atoms in crystalline materials. Furthermore, we show how to shape the bremsstrahlung X-ray emission pattern into arbitrary angular emission profiles for purposes such as unidirectionality and multi-directionality. Importantly, we find that these enhancements and shaped emission profiles cannot be attributed solely to the spatial overlap between the electron probability distribution and the atomic centers, as predicted by the paraxial and non-recoil theory for free electron light emission. Our work highlights an unprecedented regime of free electron light emission where electron waveshaping provides multi-dimensional control over practical radiation processes like bremsstrahlung. Our results pave the way towards greater versatility in table-top X-ray sources and improved fundamental understanding of quantum electron-light interactions.

47 OTHER INSTRUMENTATION↗

DOE OSTI2021

Investigation of the competition between Tl + and Ce 3+ scintillation in Tl2LiYCl6:Ce, an elpasolite scintillator

Li-containing elpasolite scintillators are currently investigated for their ability to detect both thermal neutrons and gamma photons with a single inorganic crystal. The scintillation is typically triggered by using an activator such as Ce. However, when Tl, also a luminescent ion, is present in the matrix, competition between the two centers Tl and Ce can occur. In this study, we are using Ce doped Tl 2 LiYCl 6 to investigate this competition. To this end, the Ce (which substitutes Y) concentration is varied from 0 to 1 in the Tl 2 LiY 1-x CexCl 6 composition. In the low concentration range in which Ce remains a dopant, the photo- and radioluminescence spectra show that the scintillation of Tl 2 LiYCl 6 :Ce is mostly dominated by recombination on intrinsic luminescent centers. For cerium concentrations higher than x = 0.02, very different emissions can be easily distinguished from the photo- and radioluminescence of undoped and low Ce doped Tl 2 LiYCl 6 crystals. These emissions are attributed to the formation of a second phase Tl 2 CeCl 5 , identified by X-ray diffraction. We conclude that the intrinsic luminescence related to Tl dominates the scintillation in the range of concentration for which Ce does substitute on the Y-site.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

NASA NTRS1987

Analytic and numerical calculations of quantum synchrotron spectra from relativistic electron distributions

Calculations are performed numerically and analytically of synchrotron spectra for thermal and power-law electron distributions using the single-particle synchrotron power spectrum derived from quantum electrodynamics. It is found that the photon energy at which quantum effects appear is proportional to temperature and independent of field strength for thermal spectra; quantum effects introduce an exponential roll-off away from the classical spectra. For power law spectra, the photon energy at which quantum effects appear is inversely proportional to the magnetic field strength; quantum effects produce a steeper power law than is found classically. The results are compared with spectra derived from the classical power spectrum with an energy cutoff ensuring conservation of energy. It is found that an energy cutoff is generally an inadequate approximation of quantum effects for low photon energies and for thermal spectra, but gives reasonable results for high-energy emission from power-law electron distributions.

Brainerd, J. J.↗

NASA NTRS1995

Surface temperature of a magnetized neutron star and interpretation of the ROSAT data. 1: Dipole fields

We model the temperature distribution at the surface of a magnetized neutron star and study the effects on the observed X-ray spectra and light curves. Generalrelativistic effects, i.e., redshift and lensing, are fully taken into account. Atmospheric effects on the emitted spectral flux are not included: we consider only blackbody emission at the local effective temperature. In this first paper we restrict ourselves to dipole fields. General features are studied and compared with the ROSAT data from the pulsars 0833 - 45 (Vela), 0656 + 14, 0630 + 178 (Geminga), and 1055 - 52, the four cases for which there is strong evidence that thermal radiation from the stellar surface is detected. The composite spectra we obtain are not very different from a blackbody spectrum at the star's effective temperature. We conclude that, as far as blackbody spectra are considered, temperature estimates using single-temperature models give results practically identical to our composite models. The change of the (composite blackbody) spectrum with the star's rotational phase is also not very large and may be unobservable inmost cases. Gravitational lensing strongly suppresses the light curve pulsations. If a dipole field is assumed, pulsed fractions comparable to the observed ones can be obtained only with stellar radii larger than those which are predicted by current models of neutron star struture, or with low stellar masses. Moreover, the shapes of the theoretical light curves with dipole fields do not correspond to the observations. The use of magnetic spectra may raise the pulsed fraction sufficiently but will certainly make the discrepancy with the light curve shapes worse: dipole fields are not sufficient to interpret the data. Many neutron star models with a meson condensate or hypersons predict very small radii, and hence very strong lensing, which will require highly nondipolar fields to be able to reproduce the observed pulsed fractions, if possible at all: this may be a new tool to constrain the size of neutron stars. The pulsed fractions obtained in all our models increase with photon energy: the strong decrease observed in Geminga at energies 0.3-0.5 keV is definitely a genuine effect of the magnetic field on the spectrum in contradistinction to the magnetic effects on the surface temperature considered her. Thus, a detailed analysis of thermal emission from the four pulsars we consider will require both complex surface field configurations and the inclusion of magnetic effects in the atmosphere (i.e., on the emitted spectrum).

Page, Dany↗