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All sourcesNASA NTRSDOE OSTI
NASA NTRS1987

Positrons from accelerated particle interactions

Positron production from the decay of radioactive nuclei produced in nuclear interactions of accelerated particles is treated in detail. Laboratory data as well as theoretical considerations are used to construct energy-dependent cross sections for the production of a large number of radioactive positron emitters resulting from proton and alpha-particle interactions with ambient cosmic matter. Using these cross sections, positron production rates are calculated for a variety of energetic particle spectra, assuming solar abundances for both the energetic particles and the ambient medium. These results can be used for the study of astrophysical sites which emit annihilation radiation. In particular, the results have been applied to solar flares, where the observed 0.511 MeV line is shown to be due to positrons resulting from accelerated particle reactions.

Kozlovsky, B.↗
NASA NTRS1988

Circumstellar material in meteorites - Noble gases, carbon and nitrogen

In addition to preserving a record of isotopically distinct reservoirs in the early solar system, some primitive meteorites contain discrete grains of presolar origin. Such grains are distinguished by the isotopically anomalous noble-gas components they contain. One such component consists of monoisotopic Ne-22, produced by decay of radioactive Na-22 with a 2.6 yr half-life. Two xenon components have also been identified: one synthesized apparently in a supernova, the other probably in a red giant star. Most of the grains that carry these noble-gas components are carbonaceous and contain isotopically anomalous C, N, or both. They include diamond and silicon carbide. Two unidentified carriers of isotopically anomalous nitrogen, unaccompanied by noble gases, occur in the brecciated stony iron meteorite, Bencubbin.

Anders, Edward↗
NASA NTRS1993

Thermal history of comets during residence in the Oort cloud - Effect of radiogenic heating in combination with the very low thermal conductivity of amorphous ice

The thermal history of long-period comets initially composed of amorphous ice is studied. It is shown that such comets with a small nucleus thermal conductivity (kappa) experience a runaway increase in the internal temperature during residence in the Oort cloud. The temperature increase is a result of rapid release of the latent heat at crystallization triggered by gradual heating due to decay of radioactive nuclides. The time of the runaway temperature increase is about ten to a hundred million years after the formation of the nucleus depending on the fraction of refractory grains which contain radioactive nuclides. Most of the amorphous ice in the nuclides except just beneath the surface transforms into crystalline ice due to the runaway temperature increase. This implies that the ice in short-period comets is crystalline from the initial time when the long-period comet becomes a short-period one. In comets with large kappa the temperature does not rise much compared to the small kappa case and the initial amorphous ice is preserved. A criterion for the crystallization of the nucleus ice is derived.

Haruyama, Jun'ichi↗
NASA NTRS1997

The source and distribution of Galactic positrons

The oriented scintillation spectrometer experiment (OSSE) observations of the Galactic plane and the Galactic center region were combined with observations acquired with other instruments in order to produce a map of the Galactic 511 keV annihilation radiation. Two mapping techniques were applied to the data: the maximum entropy method, and the basis pursuit inversion method. The resulting maps are qualitatively similar and show evidence for a central bulge and a weak galactic disk component. The weak disk is consistent with that expected from positrons produced by the decay of radioactive Al-26 in the interstellar medium. Both maps suggest an enhanced region of emission near l = -4 deg, b = 7 deg, with a flux of approximately 50 percent of that of the bulge. The existence of this emission appears significant, although the location is not well determined. The source of this enhanced emission is presently unknown.

Purcell, W. R.↗
NASA NTRS1997

Implications of the broad Al-26 1809 keV line observed by GRIS

The astrophysical implications of the large width of the 1809 keV gamma ray line from the decay of radioactive Al-26, recently observed with the gamma ray imaging spectrometer (GRIS), are discussed. While there may be no apparent single mechanism that can explain the observed broadening, high speed dust grains, extremely hot superbubbles and a large, low density gaseous halo were identified in the Galactic center region as the possible origins. The implications of these observations on the hot gas content in the interstellar medium are discussed.

Chen, Wan↗
NASA NTRS1997

Continuum Background in Space-Borne Gamma-Ray Detectors

The background measured with space-borne gamma-ray spectrometers (GRS) in the 100 keV-10 MeV energy region consists of both discrete lines and continuum. The discrete lines originate in the decay of radioactive species. The continuum originates from a number of different processes and can be an important factor in the detection, for example, of weak gamma-ray lines from a planetary surface. Measurements of the gamma-ray background have been made during the cruise portion of a number of planetary missions. The three missions described here are the Apollo 15 and 16 missions each of which carried a 7 cm x 7 cm NaI scintillation detector, the Mars Observer (MO) mission which used a 5.5 cm X 5.5 cm high-purity germanium (HPGe) detector, and the Near Earth Rendezvous Asteroid (NEAR) mission that has a 2.54 cm x 7.6 cm NaI detector. A comparison of the intensity and spectral shape of these background spectra can be useful to help understand how these backgrounds vary with spacecraft size, detector position, and detector size. The use of shields to reduce the background components on these three missions is a test of the effectiveness of different shield designs.

Larry G. Evans↗
NASA NTRS2004

MGGPOD: a Monte Carlo Suite for Modeling Instrumental Line and Continuum Backgrounds in Gamma-Ray Astronomy

Intense and complex instrumental backgrounds, against which the much smaller signals from celestial sources have to be discerned, are a notorious problem for low and intermediate energy gamma-ray astronomy (approximately 50 keV - 10 MeV). Therefore a detailed qualitative and quantitative understanding of instrumental line and continuum backgrounds is crucial for most stages of gamma-ray astronomy missions, ranging from the design and development of new instrumentation through performance prediction to data reduction. We have developed MGGPOD, a user-friendly suite of Monte Carlo codes built around the widely used GEANT (Version 3.21) package, to simulate ab initio the physical processes relevant for the production of instrumental backgrounds. These include the build-up and delayed decay of radioactive isotopes as well as the prompt de-excitation of excited nuclei, both of which give rise to a plethora of instrumental gamma-ray background lines in addition t o continuum backgrounds. The MGGPOD package and documentation are publicly available for download. We demonstrate the capabilities of the MGGPOD suite by modeling high resolution gamma-ray spectra recorded by the Transient Gamma-Ray Spectrometer (TGRS) on board Wind during 1995. The TGRS is a Ge spectrometer operating in the 40 keV to 8 MeV range. Due to its fine energy resolution, these spectra reveal the complex instrumental background in formidable detail, particularly the many prompt and delayed gamma-ray lines. We evaluate the successes and failures of the MGGPOD package in reproducing TGRS data, and provide identifications for the numerous instrumental lines.

Weidenspointner, G.↗
NASA NTRS2008

Radioisotope Power: A Key Technology for Deep Space Exploration

A Radioisotope Power System (RPS) generates power by converting the heat released from the nuclear decay of radioactive isotopes, such as Plutonium-238 (Pu-238), into electricity. First used in space by the U.S. in 1961, these devices have enabled some of the most challenging and exciting space missions in history, including the Pioneer and Voyager probes to the outer solar system; the Apollo lunar surface experiments; the Viking landers; the Ulysses polar orbital mission about the Sun; the Galileo mission to Jupiter; the Cassini mission orbiting Saturn; and the recently launched New Horizons mission to Pluto. Radioisotopes have also served as a versatile heat source for moderating equipment thermal environments on these and many other missions, including the Mars exploration rovers, Spirit and Opportunity. The key advantage of RPS is its ability to operate continuously, independent of orientation and distance relative to the Sun. Radioisotope systems are long-lived, rugged, compact, highly reliable, and relatively insensitive to radiation and other environmental effects. As such, they are ideally suited for missions involving long-lived, autonomous operations in the extreme conditions of space and other planetary bodies. This paper reviews the history of RPS for the U.S. space program. It also describes current development of a new Stirling cycle-based generator that will greatly expand the application of nuclear-powered missions in the future.

Schmidt, George↗
NASA NTRS2009

Radioisotope Power: A Key Technology for Deep Space Explorations

A Radioisotope Power System (RPS) generates power by converting the heat released from the nuclear decay of radioactive isotopes, such as Plutonium-238 (Pu-238), into electricity. First used in space by the U.S. in 1961, these devices have enabled some of the most challenging and exciting space missions in history, including the Pioneer and Voyager probes to the outer solar system; the Apollo lunar surface experiments; the Viking landers; the Ulysses polar orbital mission about the Sun; the Galileo mission to Jupiter; the Cassini mission orbiting Saturn; and the recently launched New Horizons mission to Pluto. Radioisotopes have also served as a versatile heat source for moderating equipment thermal environments on these and many other missions, including the Mars exploration rovers, Spirit and Opportunity. The key advantage of RPS is its ability to operate continuously, independent of orientation and distance relative to the Sun. Radioisotope systems are long-lived, rugged, compact, highly reliable, and relatively insensitive to radiation and other environmental effects. As such, they are ideally suited for missions involving long-lived, autonomous operations in the extreme conditions of space and other planetary bodies. This paper reviews the history of RPS for the U.S. space program. It also describes current development of a new Stirling cycle-based generator that will greatly expand the application of nuclear-powered missions in the future.

Schmidt, George R.↗
NASA NTRS2009

NASA Radioisotope Power System Program - Technology and Flight Systems

NASA sometimes conducts robotic science missions to solar system destinations for which the most appropriate power source is derived from thermal-to-electrical energy conversion of nuclear decay of radioactive isotopes. Typically the use of a radioisotope power system (RPS) has been limited to medium and large-scale missions, with 26 U,S, missions having used radioisotope power since 1961. A research portfolio of ten selected technologies selected in 2003 has progressed to a point of maturity, such that one particular technology may he considered for future mission use: the Advanced Stirling Converter. The Advanced Stirling Radioisotope Generator is a new power system in development based on this Stirling cycle dynamic power conversion technology. This system may be made available for smaller, Discovery-class NASA science missions. To assess possible uses of this new capability, NASA solicited and funded nine study teams to investigate unique opportunities for exploration of potential destinations for small Discovery-class missions. The influence of the results of these studies and the ongoing development of the Advanced Stirling Radioisotope Generator system are discussed in the context of an integrated Radioisotope Power System program. Discussion of other and future technology investments and program opportunities are provided.

Sutliff, Thomas J.↗
NASA NTRS2008

Thermal Expansion Studies of Selected High Temperature Thermoelectric Materials

Radioisotope thermoelectric generators (RTGs) generate electrical power by converting the heat released from the nuclear decay of radioactive isotopes (typically plutonium-238) into electricity using a thermoelectric converter. RTGs have been successfully used to power a number of space missions and have demonstrated their reliability over an extended period of time (tens of years) and are compact, rugged, radiation resistant, scalable, and produce no noise, vibration or torque during operation. System conversion efficiency for state-of-practice RTGs is about 6% and specific power less than or equal to 5.1 W/kg. Higher specific power would result in more on-board power for the same RTG mass, or less RTG mass for the same on-board power. The Jet Propulsion Laboratory has been leading, under the advanced thermoelectric converter (ATEC) project, the development of new high-temperature thermoelectric materials and components for integration into advanced, more efficient RTGs. Thermoelectric materials investigated to date include skutterudites, the Yb14MnSb11 compound, and SiGe alloys. The development of long-lived thermoelectric couples based on some of these materials has been initiated and is assisted by a thermo-mechanical stress analysis to ensure that all stresses under both fabrication and operation conditions will be within yield limits for those materials. Several physical parameters are needed as input to this analysis. Among those parameters, the coefficient of thermal expansion (CTE) is critically important. Thermal expansion coefficient measurements of several thermoelectric materials under consideration for ATEC are described in this paper. The stress response at the interfaces in material stacks subjected to changes in temperature is discussed, drawing on work from the literature and project-specific tools developed here. The degree of CTE mismatch and the associated effect on the formation of stress is highlighted.

silicon germanium↗
NASA NTRS2021

HARM3D+NUC: A New Method for Simulating the Post-merger Phase of Binary Neutron Star Mergers with GRMHD, Tabulated EOS, and Neutrino Leakage

The first binary neutron star merger has already been detected in gravitational waves. The signal was accompanied by an electromagnetic counterpart including a kilonova component powered by the decay of radioactive nuclei, as well as a short γ-ray burst. In order to understand the radioactively powered signal, it is necessary to simulate the outflows and their nucleosynthesis from the post-merger disk. Simulating the disk and predicting the composition of the outflows requires general relativistic magnetohydrodynamical (GRMHD) simulations that include a realistic, finite-temperature equation of state (EOS) and self-consistently calculating the impact of neutrinos. In this work, we detail the implementation of a finite-temperature EOS and the treatment of neutrinos in the GRMHD code HARM3D+NUC, based on HARM3D. We include formal tests of both the finite-temperature EOS and the neutrino-leakage scheme. We further test the code by showing that, given conditions similar to those of published remnant disks following neutron star mergers, it reproduces both recombination of free nucleons to a neutron-rich composition and excitation of a thermal wind.

Ariadna Murguia-Berthier↗
NASA NTRSDate not supplied

Phosphate (U-Th)/He Thermochronology of Apollo 14 Melt Breccia 14311

Our ability to confidently characterize the impact history of the inner solar system is limited by discrepancies in radiometric dates and age interpretations for lunar rocks, impact melts, and recovered meteorites. It is therefore important to explore different thermally sensitive radiometric systems to unravel the timing and extent of the long term impact flux. Low-temperature thermochronology of lunar samples has the potential to provide more complementary geochronological datasets and further test dynamical models related to the evolution of the inner solar system (e.g., [1]). (U-Th)/He dating is based on the production of 4He atoms by radioactive alpha decay of U and Th (and to a lesser extent, Sm) in a crystal and the thermally activated volumetric diffusion of those 4He nuclides. At high temperatures, the crystal is an open system from which 4He can escape; at lower temperatures, 4He may be retained. This retention temperature depends on factors such as crystal structure and volume fraction of radiation damage in the crystal (e.g., [2, 3]), but is significantly lower for phosphate minerals compared to the diffusion of the radiogenic daughter products in other widely used chronometric systems (e.g., ~75°C in terrestrial apatite (U-Th)/He vs. ~500°C in apatite U-Th-Pb vs. ~900°C in zircon U-Th-Pb chronometry). Phosphate (U-Th)/He dating has been used to decipher peak temperatures and cooling rates related to terrestrial impact events (e.g., [4]). Pairing a low-temperature thermochronometer with higher-temperature approaches (i.e., a combined 207Pb-206Pb and (U-Th)/He approach), can therefore resolve multiple impact ages within a given sample or even grain. However, despite its potential, phosphate (U-Th)/He dating has not been reported on any lunar samples. Here we present the first lunar phosphate (U-Th)/He thermochronology on an Apollo 14 impact melt-breccia.

C A Diaz↗
DOE OSTI2023

PARTITIONING AND TRANSMUTATION OF USED NUCLEAR FUEL IN SUPPORT OF GEOLOGICAL WASTE DISPOSAL

Nuclear energy is a low-carbon technology that generates bulk baseload electricity and supports long-lasting eco-friendly sustainability goals. However, it still faces challenges, such as the securing and managing of long-lived nuclear actinides and fission products—most notably the used fuel, which is considered high-level waste (HLW). Direct geological waste disposal would be the most economical option for HLW but requires highly qualified sites whose geophysical behavior will remain stable for 10,000 years. Partitioning and transmutation (P&T) of used fuel reduces radioactivity and decay heat generation, enabling efficient geological waste disposal. P&T research and development, along with the prospects of P&T techniques such as wet/dry separation and accelerator-driven systems, were reviewed to identify critical needs that must be met to foster their successful implementation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2023

PARTITIONING AND TRANSMUTATION OF USED NUCLEAR FUEL IN SUPPORT OF GEOLOGICAL WASTE DISPOSAL

Nuclear energy is a low-carbon technology that generates bulk baseload electricity and supports long-lasting eco-friendly sustainability goals. However, it still faces challenges, such as the securing and managing of long-lived nuclear actinides and fission products—most notably the used fuel, which is considered high-level waste (HLW). Direct geological waste disposal would be the most economical option for HLW but requires highly qualified sites whose geophysical behavior will remain stable for 10,000 years. Partitioning and transmutation (P&T) of used fuel reduces radioactivity and decay heat generation, enabling efficient geological waste disposal. P&T research and development, along with the prospects of P&T techniques such as wet/dry separation and accelerator-driven systems, were reviewed to identify critical needs that must be met to foster their successful implementation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2020

Testing claims of the GW170817 binary neutron star inspiral affecting β-decay rates

On August 17, 2017, the first gravitational wave signal from a binary neutron star inspiral (GW170817) was detected by Advanced LIGO and Advanced VIRGO. Here we present radioactive β-decay rates of three independent sources 44 Ti, 60 Co and 137 Cs, monitored during the same period by a precision experiment designed to investigate the decay of long-lived radioactive sources. We do not find any significant correlations between decay rates in a 5 h time interval following the GW170817 observation. This contradicts a previous claim published in this journal of an observed 2.5σ Pearson Correlation between fluctuations in the number of observed decays from two β-decaying isotopes ( 32 Si and 36 Cl) in the same time interval. By correcting for the choice of an arbitrary time interval, we find no evidence of a correlation above 1.5σ confidence. In addition, we argue that such analyses on correlations in arbitrary time intervals should always correct for the so-called Look-Elsewhere effect by quoting the global significance.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

RA Decay

The concept of the software is for a user to input the desired decay period and initial isotopic distribution and radioactivity, and RA-Decay will return the new isotopic distribution and radioactivity including the progeny ingrowth.

Todd, Don↗
DOE OSTI2021

A novel experimental system for the KDK measurement of the 40 K decay scheme relevant for rare event searches

Potassium-40 ( 40 K) is a long-lived, naturally occurring radioactive isotope. The decay products are prominent backgrounds for many rare event searches, including those involving NaI-based scintillators. 40 K also plays a role in geochronological dating techniques. The branching ratio of the electron capture directly to the ground state of argon-40 has never been measured, which can cause difficulty in interpretingcertain results or can lead to lack of precision depending on the field and analysis technique. Additionally, the KDK (Potassium (K) Decay (DK)) collaboration is measuring this decay. A composite method has a silicon drift detector with an enriched, thermally deposited 40 K source inside the Modular Total Absorption Spectrometer. This setup has been characterized in terms of energy calibration, gamma tagging efficiency, live time and false negatives and positives. A complementary, homogeneous, method is also discussed; it employs a KSr 2 I 5 :Eu scintillator as source and detector.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗