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At least 343 records · Page 19

Ultraconfined terahertz phonon polaritons in hafnium dichalcogenides

The confinement of electromagnetic radiation to subwavelength scales relies on strong light–matter interactions. In the infrared and terahertz spectral ranges, phonon polaritons are commonly employed to achieve deeply subdiffractional light confinement, with such optical modes offering much lower losses in comparison to plasmon polaritons. Among these, hyperbolic phonon polaritons in anisotropic materials offer a promising platform for light confinement. Here we report on ultraconfined phonon polaritons in hafnium-based dichalcogenides with confinement factors exceeding λ 0 /250 in the terahertz spectral range. This extreme light compression within deeply subwavelength thin films is enabled by the large magnitude of the light–matter coupling strength in these compounds and the natural hyperbolicity of HfSe 2 . Our findings emphasize the role of light–matter coupling for polariton confinement, which for phonon polaritons in polar dielectrics is dictated by the transverse–longitudinal optical phonon energy splitting. Our results demonstrate transition-metal dichalcogenides as an enabling platform for terahertz nanophotonic applications.

Kowalski, Ryan A. [Vanderbilt Univ., Nashville, TN↗

Optical amplifiers for coherent lidar

We examine application of optical amplification to coherent lidar for the case of a weak return signal (a number of quanta of the return optical field close to unity). We consider the option that has been explored to date, namely, incorporation of an optical amplifier operated in a linear manner located after reception of the signal and immediately prior to heterodyning and photodetection. We also consider alternative strategies where the coherent interaction, the nonlinear processes, and the amplification are not necessarily constrained to occur in the manner investigated to date. We include the complications that occur because of mechanisms that occur at the level of a few, or one, quantum excitation. Two factors combine in the work to date that limit the value of the approach. These are: (1) the weak signal tends to require operation of the amplifier in the linear regime where the important advantages of nonlinear optical processing are not accessed, (2) the linear optical amplifier has a -3dB noise figure (SN(out)/SN(in)) that necessarily degrades the signal. Some improvement is gained because the gain provided by the optical amplifier can be used to overcome losses in the heterodyned process and photodetection. The result, however, is that introduction of an optical amplifier in a well optimized coherent lidar system results in, at best, a modest improvement in signal to noise. Some improvement may also be realized on incorporating more optical components in a coherent lidar system for purely practical reasons. For example, more compact, lighter weight, components, more robust alignment, or more rapid processing may be gained. We further find that there remain a number of potentially valuable, but unexplored options offered both by the rapidly expanding base of optical technology and the recent investigation of novel nonlinear coherent interference phenomena occurring at the single quantum excitation level. Key findings are: (1) insertion of linear optical amplifiers in well optimized conventional lidar systems offers modest improvements, at best, (2) the practical advantages of optical amplifiers, especially fiber amplifiers, such as ease of alignment, compactness, efficiency, lightweight, etc., warrant further investigation for coherent lidar, (3) the possibility of more fully optical lidar systems should be explored, (4) advantages gained by use of coherent interference of optical fields at the level of one, or a few, signal quanta should be explored, (5) amplification without inversion, population trapping, and use of electromagnetic induced transparency warrant investigation in connection with coherent lidar, (6) these new findings are probably more applicable to earth related NASA work, although applications to deep space should not be excluded, and (7) our own work in the Ultrafast Laboratory at UAH along some of the above lines of investigation, may be useful.

Fork, Richard↗

Optical transparency of LiF (100) shock compressed to ∼360 GPa

High-purity [100] lithium fluoride (LiF) is the most widely used optical window in dynamic compression experiments due to its wide bandgap and well-characterized mechanical response. Recent plate-impact experiments established the [100] LiF Hugoniot to ∼230 GPa and demonstrated shock-induced melting onset at 182 GPa with complete melting by 195 GPa; theoretical models predict LiF optical transparency to nearly 900 GPa. To experimentally examine the optical transparency of [100] LiF at higher pressures and in the liquid state, laser-driven shock experiments were performed at peak stresses ranging from 223 to 363 GPa. Optical response was examined by measuring the particle velocity histories at the Kapton/LiF interface using laser interferometry at 532 and 1550 nm wavelengths; in-material particle velocities were obtained using established refractive-index corrections. Continuous photonic Doppler velocimetry fringes were observed across the entire stress range, demonstrating that LiF remains transparent to 1550 nm light throughout the multi-megabar regime investigated. At 532 nm, fringe visibility depended on the reflector coating: aluminum mirrors provided signals to ∼235 GPa, while gold mirrors extended this limit to 270.5 GPa, indicating that the shorter-wavelength response is likely sensitive to experimental configuration rather than to the loss of LiF transparency. Continued optical transparency to at least 360 GPa indicates that shock-melted LiF does not display bandgap closure over the stress range explored. Furthermore, these results provide direct experimental constraints on the high-pressure optical response and establish LiF (100) as a robust optical window material for laser-driven dynamic compression experiments approaching 400 GPa.

Renganathan, P. [Argonne National Laboratory (ANL)↗

Ultrafast carrier dynamics in terahertz photoconductors and photomixers: beyond short-carrier-lifetime semiconductors

Abstract Efficient terahertz generation and detection are a key prerequisite for high performance terahertz systems. Major advancements in realizing efficient terahertz emitters and detectors were enabled through photonics-driven semiconductor devices, thanks to the extremely wide bandwidth available at optical frequencies. Through the efficient generation and ultrafast transport of charge carriers within a photo-absorbing semiconductor material, terahertz frequency components are created from the mixing products of the optical frequency components that drive the terahertz device – a process usually referred to as photomixing. The created terahertz frequency components, which are in the physical form of oscillating carrier concentrations, can feed a terahertz antenna and get radiated in case of a terahertz emitter, or mix with an incoming terahertz wave to down-convert to DC or to a low frequency photocurrent in case of a terahertz detector. Realizing terahertz photoconductors typically relies on short-carrier-lifetime semiconductors as the photo-absorbing material, where photocarriers are quickly trapped within one picosecond or less after generation, leading to ultrafast carrier dynamics that facilitates high-frequency device operation. However, while enabling broadband operation, a sub-picosecond lifetime of the photocarriers results in a substantial loss of photoconductive gain and optical responsivity. In addition, growth of short-carrier-lifetime semiconductors in many cases relies on the use of rare elements and non-standard processes with limited accessibility. Therefore, there is a strong motivation to explore and develop alternative techniques for realizing terahertz photomixers that do not rely on these defect-introduced short-carrier-lifetime semiconductors. This review will provide an overview of several promising approaches to realize terahertz emitters and detectors without short-carrier-lifetime semiconductors. These novel approaches utilize p-i-n diode junctions, plasmonic nanostructures, ultrafast spintronics, and low-dimensional materials to offer ultrafast carrier response. These innovative directions have great potentials for extending the applicability and accessibility of the terahertz spectrum for a wide range of applications.

36 MATERIALS SCIENCE↗

A Featureless Infrared Transmission Spectrum for the Super-puff Planet Kepler-79d

Extremely low-density planets (“super-puffs”) are a small but intriguing subset of the transiting planet population. With masses in the super-Earth range (1 − 10 M{sub ⊕}) and radii akin to those of giant planets (> 4 R{sub ⊕}), their large envelopes may have been accreted beyond the water snow line and many appear to be susceptible to catastrophic mass loss. Both the presence of water and the importance of mass loss can be explored using transmission spectroscopy. Here, we present new Hubble space telescope WFC3 spectroscopy and updated Kepler transit depth measurements for the super-puff Kepler-79d. We do not detect any molecular absorption features in the 1.1 − 1.7 μm WFC3 bandpass, and the combined Kepler and WFC3 data are consistent with a flat-line model, indicating the presence of aerosols in the atmosphere. We compare the shape of Kepler-79d’s transmission spectrum to predictions from a microphysical haze model that incorporates an outward particle flux due to ongoing mass loss. We find that photochemical hazes offer an attractive explanation for the observed properties of super-puffs like Kepler-79d, as they simultaneously render the near-infrared spectrum featureless and reduce the inferred envelope mass-loss rate by moving the measured radius (optical depth unity surface during transit) to lower pressures. We revisit the broader question of mass-loss rates for super-puffs and find that the age estimates and mass-loss rates for the majority of super-puffs can be reconciled if hazes move the photosphere from the typically assumed pressure of ∼10 mbar to ∼10 μbar.

79 ASTRONOMY AND ASTROPHYSICS↗

Peculiarities of adaptive phase correction of optical wave distortions under conditions of ‘strong’ intensity fluctuations

The reason for the loss of efficiency of adaptive phase correction in the propagation of optical waves in a turbulent atmosphere under conditions of ‘strong’ intensity fluctuations is experimentally explained for the first time. Based on the data from experiments conducted on both horizontal and vertical atmospheric paths, we have found that intensity fluctuations begin to significantly affect phase measurements when the coherence radius of the optical wave becomes less than the radius of the first Fresnel zone. Under these conditions, the main meter of adaptive optics systems, i. e. the Hartmann sensor, no longer provides correct measurements of the phase distribution in the presence of deep amplitude modulation. Based on the study of the behaviour of the mode components of the phase fluctuations reconstructed from the results of measurements in various operating regimes, we have found that, first of all, the amplitudes of the lowest modes of phase fluctuation expansion (tilts, defocusing, and astigmatism) are distorted, which, as the analysis shows, is very different from the regime of weak fluctuations. (atmospheric optics)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Optical Design and Characterization of 40-GHz Detector and Module for the BICEP Array

Families of cosmic inflation models predict a primordial gravitational-wave background that imprints B-mode polarization pattern in the cosmic microwave background (CMB). High-sensitivity instruments with wide frequency coverage and well-controlled systematic errors are needed to constrain the faint B-mode amplitude. We have developed antenna-coupled transition edge sensor arrays for high-sensitivity polarized CMB observations over a wide range of millimeter-wave bands. BICEP array, the latest phase of the BICEP/Keck experiment series, is a multi-receiver experiment designed to search for inflationary B-mode polarization to a precision σ(r) between 0.002 and 0.004 after 3 full years of observations, depending on foreground complexity and the degree of lensing removal. We describe the electromagnetic design and measured performance of BICEP array’s low-frequency 40-GHz detector, their packaging in focal plane modules, and optical characterization including efficiency and beam matching between polarization pairs. We summarize the design and simulated optical performance, including an approach to improve the optical efficiency due to mismatch losses. Here, we report the measured beam maps for a new broadband corrugation design to minimize beam differential ellipticity between polarization pairs caused by interactions with the module housing frame, which helps minimize polarized beam mismatch that converts CMB temperature to polarization (T→P) anisotropy in CMB maps.

47 OTHER INSTRUMENTATION↗

Superradiance and Exciton Delocalization in Perovskite Quantum Dot Superlattices

Achieving superradiance in solids is challenging due to fast dephasing processes from inherent disorder and thermal fluctuations. Perovskite quantum dots (QDs) are an exciting class of exciton emitters with large oscillator strength and high quantum efficiency, making them promising for solid-state superradiance. However, a thorough under-standing of the competition between coherence and dephasing from phonon scattering and energetic disorder is currently unavailable. Here, we present an investigation of exciton coherence in perovskite QD solids using temperature-dependent photoluminescence line width and lifetime measurements. Our results demonstrate that excitons are coherently delocalized over 3 QDs at 11 K in superlattices leading to superradiant emission. Scattering from optical phonons leads to the loss of coherence and exciton localization to a single QD at temperatures above 100 K. Further, at low temperatures, static disorder and defects limit exciton coherence. These results highlight the promise and challenge in achieving coherence in perovskite QD solids.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

New particle pusher with hadronic interactions for modeling multimessenger emission from compact objects

We propose novel numerical schemes based on the Boris method in curved spacetime, incorporating both hadronic and radiative interactions for the first time. Once the proton has lost significant energy due to radiative and hadronic losses, and its gyroradius has decreased below typical scales on which the electromagnetic field varies, we apply a guiding center approximation (GCA). We fundamentally simulate collision processes either with a Monte-Carlo method or, where applicable, as a continuous energy loss, contingent on the local optical depth. To test our algorithm for the first time combining the effects of electromagnetic, gravitational, and radiation fields including hadronic interactions, we simulate highly relativistic protons traveling through various electromagnetic fields and proton backgrounds. We provide unit tests in various spatially dependent electromagnetic and gravitational fields and background photon and proton distributions, comparing the trajectory against analytic results. We propose that our method can be used to analyze hadronic interactions in black hole accretion disks, jets, and coronae to study the neutrino abundance from active galactic nuclei.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Development of Solar Cells with Trapezoidal Grid Fingers

In concentrator solar cells, traditional metallic contacts cover a substantial portion of the device area, resulting in reflected light that diminishes the amount of current collected. In this paper, we developed trapezoidal front grid fingers to decrease the optical shadowing and the resulting loss of the device short-circuit current. By using a negative photoresist, a thick metal layer can be deposited by metal evaporation. The formation of an organic and metallic reflective deposit under the negative sloped photoresist is observed, though. By removing this deposit, a similar short-circuit current to typical Ni/Au contacts deposited by electrodeposition is obtained. Even though the Ti/Al grid fingers have larger width, they have the same effective shadowing due to the trapezoidal shape. At high concentration, a higher efficiency is obtained as well due to a high fill factor and improved open circuit voltage.

14 SOLAR ENERGY↗

Good plasmons in a bad metal

Correlated metals may exhibit unusually high resistivity that increases linearly in temperature, breaking through the Mott-Ioffe-Regel bound, above which coherent quasiparticles are destroyed. The fate of collective charge excitations, or plasmons, in these systems is a subject of debate. Several studies have suggested that plasmons are overdamped, whereas other studies have detected propagating plasmons. Here, in this work, we present direct nano-optical images of low-loss hyperbolic plasmon polaritons (HPPs) in the correlated van der Waals metal MoOCl 2 . HPPs are plasmon-photon modes that waveguide through extremely anisotropic media and are remarkably long-lived in MoOCl 2 . Photoemission data presented here reveal a highly anisotropic Fermi surface, reconstructed and made partly incoherent, likely through electronic interactions as explained by many-body theory. HPPs remain long-lived despite this, revealing previously unseen imprints of many-body effects on plasmonic collective modes.

36 MATERIALS SCIENCE↗

Microwave emission from stars.

An attempt is made to summarize the observations of masered emission from stars and to outline some basic conclusions that can be drawn from the data. The association of masered microwave emission with well studied objects like stars makes it possible to use the information gathered by conventional optical observations to attack the general masering problem and, conversely, the radio observations may be used to obtain information about a star not readily accessible optically, such as the mass loss rate or the physical conditions in a circumstellar shell.

Schwartz, P. R.↗

A new concept for solar pumped lasers

A new approach is proposed in which an intermediate body heated by sunlight is used as the pumping source for IR systems, i.e., concentration solar radiation is absorbed and reradiated via an intermediate blackbody. This body is heated by focused sunlight to a high temperature and its heat losses are engineered to be small. The cooled laser tube (or tubes) is placed within the cavity and is pumped by it. The advantage is that the radiation spectrum is like a blackbody at the intermediate temperature and the laser medium selectively absorbs this light. Focusing requirements, heat losses, and absorption bandwidths of laser media are examined, along with energy balance and potential efficiency. The results indicate that for lasers pumped through an IR absorption spectrum, the use of an intermediate blackbody offers substantial and important advantages. The loss in radiative intensity for optical pumping by a lower-temperature body is partly compensated by the increased solid angle of exposure to the radiative environment.

Christiansen, W. H.↗

Photocell heat engine solar power systems

A combined photocell heat engine concept is proposed for high efficiency solar energy conversion in space. In this concept the short wavelength portion of the solar spectrum is split by a dichroic filter and sent to a bank of photocells. The long wave-length remainder of the spectrum is used by the heat engine. This technique allows the photocells to operate with the minimum amount of waste heat, increasing their efficiency and reducing the amount of cooling required. The heat engine operates by direct absorption in a working fluid containing broadband absorber molecules or particulates. A window in the heat engine admits the long wave-lengths from the solar spectrum. The window may also reflect a portion of the internal gaseous reradiation spectrum (e.g., a heat mirror) to help reduce radiation losses. Flow-induced thermal gradients may also reduce reradiation losses in the case of optically thick working fluids. The efficiencies computed for the photocell heat engine solar energy converter can be as high as 42 percent.

Taussig, R. T.↗

Studies of single-mode injection lasers and of quaternary materials. Volume 2: Measurement of electro-optic effects in InGaAsP junction waveguides

Both the linear electro-optic (Pockel's) effect and electroabsorption (Franz-Keldysh effect) in waveguiding junctions of InGaAsP were measured. The electro-optic coefficient is found to be 0.1-0.14x10 to the -12 power m/V at lambda = 1.54 - 1.65 micrometers. Possibly this is the first reported measurement of the electro-optic coefficient for InGaAsP. The value found for the electroabsorption is on the order of 7x10 to the -4 power cm to the -1 power/(V/cm) or approximately 100 cm/1 for fields of 200,000 V/cm at lambda 1.3 micrometers. All measurements were made on a quaternary film with a bandgap wavelength of 1.23 micrometers. Because of the rapid commercial introduction of quaternary lasers, LEDs, and detectors to take advantage of large optical fiber bandwidths and low losses in the 1.2- to 1.7- micrometer region, these measurements are significant in providing some of the basic physical constants needed to design modulators and switches capable of operating at microwave frequencies in this wavelength region.

Hammer, J. M.↗

The 20 GHz proof-of-concept test model results for a multiple scan beam dual reflector antenna

A full scale 20 GHz antenna model was designed, fabricated and tested. The model is intended to test the low sidelobe beam scanning capability of a new class of an offset dual reflector and feed array configuration. The offset main reflector and subreflector surfaces are custom shaped by a computer synthesis procedure. The derived optics result in beam scan loss under 1 db over the + or - 12.3 beamwidths by + or - 5.8 beamwidths scan volume while maintaining low sidelobes. It is found that the measured and computed patterns are in good agreement.

Roberts, T.↗

Crystallization of heavy metal fluoride glasses

The kinetics of crystallization of a number of fluorozirconate glasses were studied using isothermal and dynamic differential scanning calorimetry and X-ray diffraction. The addition of the fluorides LiF, NaF, AlF3, LaF3 to a base glass composition of ZrF4-BaF2 reduced the tendency to crystallize, probably by modifying the viscosity-temperature relation. ZrF4-BaF2-LaF3-AlF3-NaF glass was the most stable against devitrification and perhaps is the best composition for optical fibers with low scattering loss. Some glasses first crystallize out into metastable beta-BaZr2F10 and beta-BaZrF6 phases, which transform into the most stable alpha-phases when heated to higher temperatures. The size of the crystallites was estimated to be about 600 A from X-ray diffraction.

Bansal, Narottam P.↗

Property changes induced by the space environment in polymeric materials on LDEF

Property changes that occurred in four groups of polymer-based materials in the Long Duration Exposure Facility (LDEF) due to exposure to the outer space environment for 5.8 yrs are examined. Evaluations of contamination and mass loss are presented along with optical, thermal, and electrical analyses and mechanical property evaluations for TFE Teflon, the fluorinated material Halar, the silicone-based material RTV 511, and PEEK resin.

Whitaker, Ann F.↗