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At least 343 records · Page 19

A decay database of coincident γ–γ and γ–X -ray branching ratios for in-field spectroscopy applications

Current fieldable spectroscopy techniques often use single detector systems heavily impacted by interferences from intense background radiation fields. These effects result in low-confidence measurements that can lead to misinterpretation of the collected spectrum. To help improve interpretation of the fission products and short-lived radionuclides produced in a composite sample, a coincidence-database is being developed in support of a robust portable and X-ray coincidence detector system concurrently under development at the Pacific Northwest National Laboratory for in-field deployment. Hitherto, no database exists containing coincident γ–γ and γ–X-ray branching-ratio intensities on an absolute scale that will greatly enhance isotopic identification for in-field applications. As part of this project, software has been developed to parse all radioactive-decay data sets from the Evaluated Nuclear Structure Data File (ENSDF) archive to enable translation into a more useful JavaScript Object Notation (JSON) formats that more readily supports query-based data manipulation. The coincident database described in this work is the first of its kind and contains coincidence γ–γ and γ–X-ray intensities and their corresponding uncertainties, together with auxiliary metadata associated with each decay data set. The new JSON format provides a convenient and portable means of data storage that can be imported into analysis frameworks with relatively low overhead allowing for meaningful comparison with measured data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Quantum driven dissipative parametric oscillator in a blackbody radiation field

We consider the general open system problem of a charged quantum oscillator confined in a harmonic trap, whose frequency can be arbitrarily modulated in time, that interacts with both an incoherent quantized (blackbody) radiation field and with an arbitrary coherent laser field. We assume that the oscillator is initially in thermodynamic equilibrium with its environment, a non-factorized initial density matrix of the system and the environment, and that at t = 0 the modulation of the frequency, the coupling to the incoherent and the coherent radiation are switched on. The subsequent dynamics, induced by the presence of the blackbody radiation, the laser field, and the frequency modulation, is studied in the framework of the influence functional approach. This approach allows incorporating, in analytic closed formulae, the non-Markovian character of the oscillator-environment interaction at any temperature as well the non-Markovian character of the blackbody radiation and its zero-point fluctuations. Expressions for the time evolution of the covariance matrix elements of the quantum fluctuations and the reduced density-operator are obtained.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Alpha channeling with high-field launch of lower hybrid waves

Although lower hybrid waves are effective at driving currents in present-day tokamaks, they are expected to interact strongly with high-energy particles in extrapolating to reactors. In the presence of a radial alpha particle birth gradient, this interaction can take the form of wave amplification rather than damping. While it is known that this amplification more easily occurs when launching from the tokamak high-field side, the extent of this amplification has not been made quantitative. Here, by tracing rays launched from the high-field-side of a tokamak, the required radial gradients to achieve amplification are calculated for a temperature and density regime consistent with a hot-ion-mode fusion reactor. These simulations, while valid only in the linear regime of wave amplification, nonetheless illustrate the possibilities for wave amplification using high-field launch of the lower hybrid wave.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Molecular dynamics simulations of cholesterol-rich membranes using a coarse-grained force field for cyclic alkanes

The architecture of a biological membrane hinges upon the fundamental fact that its properties are determined by more than the sum of its individual components. Studies on model membranes have shown the need to characterize in molecular detail how properties such as thickness, fluidity, and macroscopic bending rigidity are regulated by the interactions between individual molecules in a non-trivial fashion. Simulation-based approaches are invaluable to this purpose but are typically limited to short sampling times and model systems that are often smaller than the required properties. To alleviate both limitations, the use of coarse-grained (CG) models is nowadays an established computational strategy. We here present a new CG force field for cholesterol, which was developed by using measured properties of small molecules, and can be used in combination with our previously developed force field for phospholipids. The new model performs with precision comparable to atomistic force fields in predicting the properties of cholesterol-rich phospholipid bilayers, including area per lipid, bilayer thickness, tail order parameter, increase in bending rigidity, and propensity to form liquid-ordered domains in ternary mixtures. We suggest the use of this model to quantify the impact of cholesterol on macroscopic properties and on microscopic phenomena involving localization and trafficking of lipids and proteins on cellular membranes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Coupled laboratory and field investigations resolve microbial interactions that underpin persistence in hydraulically fractured shales

Hydraulic fracturing is one of the industrial processes behind the surging natural gas output in the United States. This technology inadvertently creates an engineered microbial ecosystem thousands of meters below Earth’s surface. Here, we used laboratory reactors to perform manipulations of persisting shale microbial communities that are currently not feasible in field scenarios. Metaproteomic and metabolite findings from the laboratory were then corroborated using regression based modeling performed on metagenomic and metabolite data from more than 40 produced fluids from five hydraulically fractured shale wells. Collectively, our findings show that Halanaerobium, Geotoga, and Methanohalophilius strain abundances predict a significant fraction of nitrogen and carbon metabolites in the field. Our laboratory findings also exposed cryptic predatory, cooperative, and competitive interactions that impact microorganisms across fractured shales. Scaling these results from the laboratory to the field identified mechanisms underpinning biogeochemical reactions, yielding knowledge that can be harnessed to potentially increase energy yields and inform management practices in hydraulically fractured shales.

hydraulic fracturing, metaproteomics, methanogenes↗

MID-INFRARED SELECTION OF ACTIVE GALACTIC NUCLEI WITH THE WIDE-FIELD INFRARED SURVEY EXPLORER. II. PROPERTIES OF WISE-SELECTED ACTIVE GALACTIC NUCLEI IN THE NDWFS BOOeTES FIELD

Stern et al. presented a study of Wide-field Infrared Survey Explorer (WISE) selection of active galactic nuclei (AGNs) in the 2 deg{sup 2} COSMOS field, finding that a simple criterion W1-W2 {>=} 0.8 provides a highly reliable and complete AGN sample for W2 < 15.05, where the W1 and W2 passbands are centered at 3.4 {mu}m and 4.6 {mu}m, respectively. Here we extend this study using the larger 9 deg{sup 2} NOAO Deep Wide-Field Survey Booetes field which also has considerably deeper WISE observations than the COSMOS field, and find that this simple color cut significantly loses reliability at fainter fluxes. We define a modified selection criterion combining the W1-W2 color and the W2 magnitude to provide highly reliable or highly complete AGN samples for fainter WISE sources. In particular, we define a color-magnitude cut that finds 130 {+-} 4 deg{sup -2} AGN candidates for W2 < 17.11 with 90% reliability. Using the extensive UV through mid-IR broadband photometry available in this field, we study the spectral energy distributions of WISE AGN candidates. We find that, as expected, the WISE AGN selection can identify highly obscured AGNs, but that it is biased toward objects where the AGN dominates the bolometric luminosity output. We study the distribution of reddening in the AGN sample and discuss a formalism to account for sample incompleteness based on the step-wise maximum-likelihood method of Efstathiou et al. The resulting dust obscuration distributions depend strongly on AGN luminosity, consistent with the trend expected for a receding torus. At L{sub AGN} {approx} 3 Multiplication-Sign 10{sup 44} erg s{sup -1}, 29% {+-} 7% of AGNs are observed as Type 1, while at {approx}4 Multiplication-Sign 10{sup 45} erg s{sup -1} the fraction is 64% {+-} 13%. The distribution of obscuration values suggests that dust in the torus is present as both a diffuse medium and in optically thick clouds.

79 ASTRONOMY AND ASTROPHYSICS↗

AMUSE-Field. II. Nucleation of early-type galaxies in the field versus cluster environment

The optical light profiles of nearby early-type galaxies are known to exhibit a smooth transition from nuclear light deficits to nuclear light excesses with decreasing galaxy mass, with as much as 80% of the galaxies with stellar masses below 10{sup 10} M {sub ☉} hosting a massive nuclear star cluster (NSC). At the same time, while all massive galaxies are thought to harbor nuclear supermassive black holes (SMBHs), observational evidence for SMBHs is slim at the low end of the mass function. Here, we explore the environmental dependence of the nucleation fraction by comparing two homogeneous samples of nearby field versus cluster early-type galaxies with uniform Hubble Space Telescope (HST) coverage. Existing Chandra X-ray Telescope data for both samples yield complementary information on low-level accretion onto nuclear SMBHs. Specifically, we report on dual-band (F475W and F850LP) Advanced Camera for Surveys (ACS) imaging data for 28 out of the 103 field early-type galaxies that compose the AMUSE-Field Chandra survey, and compare our results against the companion HST and Chandra surveys for a sample of 100 Virgo Cluster early-types (ACS Virgo Cluster and AMUSE-Virgo surveys, respectively). We model the two-dimensional light profiles of the field targets to identify and characterize NSCs, and find a field nucleation fraction of 26%{sub −11%}{sup +17%} (at the 1σ level), consistent with the measured Virgo nucleation fraction across a comparable mass distribution (30%{sub −12%}{sup +17%}). Coupled with the Chandra result that SMBH activity is higher for the field, our findings indicate that, since the last epoch of star formation, the funneling of gas to the nuclear regions has been inhibited more effectively for Virgo galaxies, arguably via ram pressure stripping.

79 ASTRONOMY AND ASTROPHYSICS↗

Field-free molecular orientation by a multicolor laser field

We theoretically study the field-free molecular orientation by a multicolor laser field with a superposition of the fundamental wave and its harmonics. It is shown that the molecular orientation will be up to a maximum value pumped by the four-color laser field at the same laser intensity, and the molecular orientation direction and its degree can be controlled by varying the carrier-envelope phase of the four-color laser field. It is also indicated that the molecular orientation induced by a four-color laser field can be tremendously enhanced by applying another in-phase or out-phase four-color laser field at the beginning of the rotational wave-packet rephasing or the end of the rotational wave-packet dephasing.

74 ATOMIC AND MOLECULAR PHYSICS↗

Anisotropic upper critical field of pristine and proton-irradiated single crystals of the magnetically ordered superconductor RbEuFe{sub 4}As{sub 4

We present a study of the upper critical field H-c2 of pristine and proton-irradiated RbEuFe4As4 crystals in pulsed magnetic fields of up to 65 T. The data for H-c2 reveal pronounced downwards curvature, particularly for the in-plane field orientation, and a superconducting anisotropy that decreases with decreasing temperature. These features are indicative of Pauli paramagnetic limiting. For the interpretation of these data, we use a model of a clean single-band superconductor with an open Fermi surface in the shape of a warped cylinder, which takes into account Zeeman spin splitting. Fits to the data reveal that the in-plane upper critical field is Pauli paramagnetic limited, while the out-of-plane upper critical field is orbitally limited and that the orbital and paramagnetic fields have opposite anisotropies. A consequence of this particular combination is the unusual inversion of the anisotropy H-c2(ab) < H-c2(c) of the irradiated sample at temperatures below 10 K. The fits also yield an in-plane Maki parameter alpha(110)(M) approximate to 2.6 exceeding the critical value for the formation of the Fulde-Ferrell-Larkin-Ovchinnikov state. Nevertheless, the current measurements did not reveal direct evidence for the occurrence of this state.

Smylie, M. P.↗

Ultrafast terahertz-field-driven ionic response in ferroelectric BaTiO 3

The dynamical processes associated with electric field manipulation of the polarization in a ferroelectric remain largely unknown but fundamentally determine the speed and functionality of ferroelectric materials and devices. Here in this paper we apply subpicosecond duration, single-cycle terahertz pulses as an ultrafast electric field bias to prototypical BaTiO 3 ferroelectric thin films with the atomic-scale response probed by femtosecond x-ray-scattering techniques. We show that electric fields applied perpendicular to the ferroelectric polarization drive large-amplitude displacements of the titanium atoms along the ferroelectric polarization axis, comparable to that of the built-in displacements associated with the intrinsic polarization and incoherent across unit cells. This effect is associated with a dynamic rotation of the ferroelectric polarization switching on and then off on picosecond time scales. These transient polarization modulations are followed by long-lived vibrational heating effects driven by resonant excitation of the ferroelectric soft mode, as reflected in changes in the c-axis tetragonality. The ultrafast structural characterization described here enables a direct comparison with first-principles-based molecular-dynamics simulations, with good agreement obtained.

36 MATERIALS SCIENCE↗

Magnetic field induced evolution of intertwined orders in the Kitaev magnet β – Li 2 IrO 3

Recent scattering experiments in the 3D Kitaev magnet β–Li 2 IrO 3 have shown that a relatively weak magnetic field along the crystallographic b axis drives the system from its incommensurate counter-rotating order to a correlated magnet, with a significant uniform ‘zigzag’ component superimposing the magnetization along the field. Here it is shown that the zigzag order is not emerging from its linear coupling to the field (via a staggered, off-diagonal element of the g tensor) but from its intertwining with the incommensurate order and the longitudinal magnetization. The emerging picture explains all qualitative experimental findings at zero and finite fields, including the rapid decline of the incommensurate order with field and the so-called intensity sum rule. The latter are shown to be independent signatures of the smallness of the Heisenberg exchange J, compared to the Kitaev coupling K and the off-diagonal anisotropy Γ. Remarkably, in the regime of interest, the field H* at which the incommensurate component vanishes, depends essentially only on J, which allows us to extract an estimate of J≃4 K from reported measurements of H*. Lastly, we also comment on recent experiments in pressurized β–Li 2 IrO 3 and conclude that J decreases with pressure.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Effects of retarded electrical fields on observables sensitive to the high-density behavior of the nuclear symmetry energy in heavy-ion collisions at intermediate energies

Within the isospin- and momentum-dependent transport model IBUU11, we examine here the relativistic retardation effects of electrical fields on the π - / π + ratio and neutron-proton differential transverse flow in heavy-ion collisions at intermediate energies. Compared to the static Coulomb fields, the retarded electric fields of fast-moving charges are known to be anisotropic and the associated relativistic corrections can be significant. They are found to increase the number of energetic protons in the participant region at the maximum compression by as much as 25% but that of energetic neutrons by less than 10% in 197 Au + 197 Au reactions at a beam energy of 400 MeV/nucleon. Consequently, more π + and relatively fewer π - mesons are produced, leading to an appreciable reduction of the π - / π + ratio compared to calculations with the static Coulomb fields. Also, the neutron-proton differential transverse flow, as another sensitive probe of high-density symmetry energy, is also decreased appreciably due to the stronger retarded electrical fields in directions perpendicular to the velocities of fast-moving charges compared to calculations using the isotropic static electrical fields. Moreover, the retardation effects on these observables are found to be approximately independent of the reaction impact parameter.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Strong Local-Field Effect on the Dynamics of a Dilute Atomic Gas Irradiated by Two Counterpropagating Optical Fields: Beyond Standard Optical Lattices

We study a recent experiment [K. Li et al., Phys. Rev. Lett. 101, 250401 (2008)] on diffracting a Bose-Einstein condensate by two counterpropagating optical fields. Including the local-field effect, we explain the asymmetric momentum distribution and self-imaging of the Bose-Einstein condensate self-consistently. Moreover, we find that the two counterpropagating optical fields could not produce a perfect optical lattice, which is actually deformed by the local-field effect. Our work implies that the local-field effect could be essential for getting a better quantitative analysis of other optical lattice experiments. In particular, the intensity imbalance of the two optical fields could act as a new means to tailor both cold atom dynamics and light propagation.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Evaluation and Field Assessment of Bifacial Photovoltaic Module Power Rating Methodologies

1-sun power ratings for bifacial modules are currently undefined. This is partly because there is no standard definition of rear irradiance given 1000 Wm-2 on the front. Using field measurements and simulations, we evaluate multiple deployment scenarios for bifacial modules and provide details on the amount of irradiance that could be expected. A simplified case that represents a single module deployed under conditions consistent with existing 1-sun irradiance standards leads to a bifacial reference condition of 1000 Wm-2 Gfront and 130-140 Wm-2 Grear. For fielded systems of bifacial modules, Grear magnitude and spatial uniformity will be affected by self-shade from adjacent modules, varied ground cover, and ground-clearance height. A standard measurement procedure for bifacial modules is also currently undefined. A proposed international standard is under development, which provides the motivation for this work. Here, we compare outdoor field measurements of bifacial modules with irradiance on both sides with proposed indoor test methods where irradiance is only applied to one side at a time. The indoor method has multiple advantages, including controlled and repeatable irradiance and thermal environment, along with allowing the use of conventional single-sided flash test equipment. The comparison results are promising, showing that the indoor and outdoor methods agree within 1%-2% for multiple rear-irradiance conditions and bifacial module types.

14 SOLAR ENERGY↗

SU-E-T-432: Field Size Influence On the Electron and Photon Spectra Within Small MV Field Detectors

Purpose: To investigate the influence of photon field size on the electron and photon fluence spectra in the active volume of small field detectors. Methods: The PENELOPE MC system based usercode PenEasy was used to calculate the material influence on the spectra by scoring the differential fluence in inserts of silicon, carbon, phosphorus and aluminium having 3 mm diameter and height. The spectra were then calculated inside the active volume of eleven detectors (ion chambers and solid-state detectors) whose geometry was simulated with great detail. The inserts/detectors were placed at 10 cm depth in a 30 cm x 30 cm x 30 cm water phantom and irradiated with 2.5 MeV photons and Varian Clinac 6 MV beams of small, medium and large size. Results: For all configurations, photon spectra in the scoring volume were similar to that in a small water volume except for additional characteristic x-ray peaks resulting from the material itself and from the materials surrounding the detectors (i.e. high-Z shielding the silicon). Electron fluence calculated in the inserts were up to 60% larger than in water; the difference increased with material density and decreasing field size. MC-calculated doses were compared to analytically determined collision kerma and restricted cema (cut-off=15keV). For the inserts, with large and medium fields K-col agreed with MC-dose, but K-col overestimated the dose for small fields due to lack of lateral CPE. For the detectors, up to 15% differences between K-col and the MC-dose were found. For all configurations the C-delta and MC-dose agreed within ±2%. Conclusion: The most relevant findings were that shielding affects substantially the photon spectra and material conditions the electron spectra, their field size dependence varying with the geometry configuration. These affect the values of factors entering into relative dosimetry.

60 APPLIED LIFE SCIENCES↗

Radiation dose and cancer risk to out-of-field and partially in-field organs from radiotherapy for symptomatic vertebral hemangiomas

Purpose: Vertebral hemangiomas (VHs) are the most common benign tumors of the spine that may cause bone resorption. Megavoltage irradiation is usually the treatment of choice for the management of symptomatic VHs. The current study was conducted to estimate the risk for carcinogenesis from radiotherapy of this benign disease on the basis of the calculated radiation doses to healthy organs. Methods: The Monte Carlo N-particle transport code was employed to simulate the irradiation with 6 MV x-rays of a VH presented in the cervical, upper thoracic, lower thoracic, and lumbar spine. The average radiation dose (D{sub av}) received by each critical organ located outside the primarily irradiated area was calculated. Three-dimensional treatment plans were also generated for the VHs occurring at the four different sites of the spinal cord based on patients’ computed tomography data. The organ equivalent dose (OED) to each radiosensitive structure, which was partly encompassed by the applied treatment fields, was calculated with the aid of differential dose–volume histograms. The D{sub av} and the OED values were combined with a linear-no-threshold model and a nonlinear mechanistic model, respectively, to estimate the organ-, age-, and gender-specific lifetime attributable risks (LARs) for cancer development. The estimated risks were compared with the respective nominal lifetime intrinsic risks (LIRs) for the unexposed population. Results: For a standard target dose of 34 Gy, the OED varied from 0.39–5.15 Gy by the organ of interest and the irradiation site. The D{sub av} range for the out-of-field organs was 4.9 × 10{sup −4} to 0.56 Gy. The LAR for the appearance of malignancies in the partially in-field organs after radiotherapy of male and female patients was (0.08%–1.8%) and (0.09%–1.9%), respectively. These risk values were 1.5–15.5 times lower when compared to the respective LIRs. The lifetime probability for out-of-field cancer induction in irradiated males and females was (2.5 × 10{sup −4} to 7.7 × 10{sup −2})% and (1.4 × 10{sup −4} to 2.6 × 10{sup −1})%, respectively. The above risks were one to four orders of magnitude lower than the LIRs. Conclusions: The probability for the development of out-of-field malignancies due to radiotherapy for VHs is trivial with respect to the nominal risk for unexposed population. The respective cancer risks to partially in-field organs are smaller than the nominal probabilities but they should not be considered as inconsiderable. These risks may be taken into account during the follow-up of patients treated for a symptomatic VH.

60 APPLIED LIFE SCIENCES↗

SU-F-T-387: A Novel Optimization Technique for Field in Field (FIF) Chestwall Radiation Therapy Using a Single Plan to Improve Delivery Safety and Treatment Planning Efficiency

Purpose: A novel optimization technique was developed for field-in-field (FIF) chestwall radiotherapy using bolus every other day. The dosimetry was compared to currently used optimization. Methods: The prior five patients treated at our clinic to the chestwall and supraclavicular nodes with a mono-isocentric four-field arrangement were selected for this study. The prescription was 5040 cGy in 28 fractions, 5 mm bolus every other day on the tangent fields, 6 and/or 10 MV x-rays, and multileaf collimation.Novelly, tangents FIF segments were forward planned optimized based on the composite bolus and non-bolus dose distribution simultaneously. The prescription was spilt into 14 fractions for both bolus and non-bolus tangents. The same segments and monitor units were used for the bolus and non-bolus treatment. The plan was optimized until the desired coverage was achieved, minimized 105% hotspots, and a maximum dose of less than 108%. Each tangential field had less than 5 segments.Comparison plans were generated using FIF optimization with the same dosimetric goals, but using only the non-bolus calculation for FIF optimization. The non-bolus fields were then copied and bolus was applied. The same segments and monitor units were used for the bolus and non-bolus segments. Results: The prescription coverage of the chestwall, as defined by RTOG guidelines, was on average 51.8% for the plans that optimized bolus and non-bolus treatments simultaneous (SB) and 43.8% for the plans optimized to the non-bolus treatments (NB). Chestwall coverage of 90% prescription averaged to 80.4% for SB and 79.6% for NB plans. The volume receiving 105% of the prescription was 1.9% for SB and 0.8% for NB plans on average. Conclusion: Simultaneously optimizing for bolus and non-bolus treatments noticeably improves prescription coverage of the chestwall while maintaining similar hotspots and 90% prescription coverage in comparison to optimizing only to non-bolus treatments.

60 APPLIED LIFE SCIENCES↗

Role of nonlinear refraction in the generation of terahertz field pulses by light fields

The generation of microwave (terahertz) pulses without any envelope in a four-level quasi-resonant medium is considered. Two intense quasi-monochromatic laser fields lead to a partial upper-level population. Microwave field pulses cause the transition between these levels. For appropriately chosen scales, the evolution of the fields is shown to be described by the pseudo-spin evolution equations in a microwave field with the inclusion of nonlinear refraction caused by an adiabatic upper-level population. The evolution of terahertz field pulses is described outside the scope of the slow-envelope approximation. When a number of standard approximations are taken into account, this system of equations is shown to be equivalent to an integrable version of the generalized reduced Maxwell-Bloch equations or to the generalized three-wave mixing equations. The soliton solution found by the inverse scattering transform method is used as an example to show that nonlinear refraction leads to a strong compression of the microwave (terahertz) field soliton.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗