Use of long-lived radon daughters as indicators of exchange between the free troposphere and the marine boundary layer
Fluxes and exchange coefficients are derived for the transport of Sr-90, Pb-210, Bi-210, and Po-210 between the free troposphere and the marine boundary layer and between the boundary layer and the sea surface. Radionuclide concentrations previously measured near Hawaii are used in the derivations. Values obtained for the free troposphere/boundary layer exchange coefficient (expressed as a piston velocity) were 185, 228 and 203 m/d for Pb-210, Bi-210, and Sr-90, respectively. The magnitude of the local sea-surface source of Po-210 is also determined.