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At least 343 records · Page 19

Development and testing of neutron cross-section covariance data for Scale 6.2 - 14604

Neutron cross-section covariance data are essential for many sensitivity/uncertainty and uncertainty quantification assessments performed both within the TSUNAMI suite and more broadly throughout the SCALE code system. The release of ENDF/B-VII.1 included a more complete set of neutron cross-section covariance data: these data form the basis for a new cross-section covariance library to be released in SCALE 6.2. A range of testing is conducted to investigate the properties of these covariance data and ensure that the data are reasonable. These tests include examination of the uncertainty in critical experiment benchmark model k{sub eff} values due to nuclear data uncertainties, as well as similarity assessments of irradiated pressurized water reactor (PWR) and boiling water reactor (BWR) fuel with suites of critical experiments. The contents of the new covariance library, the testing performed, and the behavior of the new covariance data are described in this paper. The neutron cross-section covariances can be combined with a sensitivity data file generated using the TSUNAMI suite of codes within SCALE to determine the uncertainty in system k{sub eff} caused by nuclear data uncertainties. The Verified, Archived Library of Inputs and Data (VALID) maintained at Oak Ridge National Laboratory (ORNL) contains over 400 critical experiment benchmark models, and sensitivity data are generated for each of these models. The nuclear data uncertainty in k{sub eff} is generated for each experiment, and the resulting uncertainties are tabulated and compared to the differences in measured and calculated results. The magnitude of the uncertainty for categories of nuclides (such as actinides, fission products, and structural materials) is calculated for irradiated PWR and BWR fuel to quantify the effect of covariance library changes between the SCALE 6.1 and 6.2 libraries. One of the primary applications of sensitivity/uncertainty methods within SCALE is the assessment of similarities between benchmark experiments and safety applications. This is described by a ck value for each experiment with each application. Several studies have analyzed typical ck values for a range of critical experiments compared with hypothetical irradiated fuel applications. The ck value is sensitive to the cross-section covariance data because the contribution of each nuclide is influenced by its uncertainty; large uncertainties indicate more likely bias sources and are thus given more weight. Changes in ck values resulting from different covariance data can be used to examine and assess underlying data changes. These comparisons are performed for PWR and BWR fuel in storage and transportation systems. (authors)

42 ENGINEERING↗

ORNL Neutron Cross-Section Measurements Activities

To support the Nuclear Criticality Safety Program, neutron cross-section measurements have been initiated using GELINA at the European Commission Joint Research Center IRMM. Concerns about data deficiencies in some existing cross-section evaluations from libraries such as ENDF/B, JEFF, or JENDL for nuclear criticality calculations have been the prime motivator for new cross section measurements. Over the past years, many problems with existing nuclear data have been emerging. An example is the use of the evaluated neutron cross-section data for tungsten in nuclear criticality safety calculations, which exhibit discrepancies in benchmark calculations and show the need for reliable covariance data. We recently measured the neutron total and capture cross sections of 182,183,184,186 W, 63,65 Cu, and natural calcium in the neutron energy range from 100 eV to several hundred keV. This will help to improve the representation of the cross sections since most of the available evaluated data rely only on old measurements. Besides, most of the evaluations in the nuclear data libraries are missing high-fidelity covariance data. New covariance data for the libraries can only be created by a reevaluation of the cross-section data; however, sometimes this impossible because the data used in the analysis and evaluations are no longer available. In such cases, this shortfall can be overcome only by new experimental data included in a new evaluation.

97 MATHEMATICS AND COMPUTING↗

An Investigation of MCNP6.1 Beryllium Oxide S(α,β) Cross Sections

In MCNP6.1, materials are constructed by identifying the constituent isotopes (or elements in a few cases) individually. This list selects the corresponding microscopic cross sections calculated from the free-gas model to create the material macroscopic cross sections. The free-gas model and the corresponding material macroscopic cross sections assume that the interactions of atoms do not affect the nuclear cross sections. With certain compounds, the free-gas model cross sections are not sufficient because molecular effects or crystalline structure effects do affect the neutron scattering cross sections at low energies. These effects are included in the MCNP6.1 thermal scattering kernels, or S(α,β) thermal neutron scattering data. To treat a particular isotope (or isotopes) as a molecular compound in the thermal regime, one or more of the available S(α,β) data sets is selected (with the MT card). As MCNP6.1 transports particles, the free-gas model cross sections are used down to the energy where S(α,β) data are available. At that point, the S(α,β) cross sections automatically overrides the free-gas cross sections. Most of the S(α,β) files have a maximum energy of 10 eV. In MCNP6.1, a binary compound may have one or two S(α,β) libraries. Beryllium oxide (BeO) is one of the materials that has two S(α,β) libraries one for the beryllium S(α,β) cross sections (be-o) and one for the oxygen S(α,β) cross sections (o-be). From its moderating properties, it is apparent that the S(α,β) library for the beryllium must be included to accurately model beryllium oxide. The necessity of the S(α,β) library for oxygen is less clear because oxygen is a relatively poor moderator. This paper investigates the effect of using only the be-o S(α,β) library or using both be-o and o-be S(α,β) libraries. The objective is to provide guidance on the use of the beryllium oxide S(α,β) libraries in criticality safety analyses. (authors)

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Relativistic Three-Dimensional Lippmann-Schwinger Cross Sections for Space Radiation Applications

Radiation transport codes require accurate nuclear cross sections to compute particle fluences inside shielding materials. The Tripathi semi-empirical reaction cross section, which includes over 60 parameters tuned to nucleon-nucleus (NA) and nucleus-nucleus (AA) data, has been used in many of the world’s best-known transport codes. Although this parameterization fits well to reaction cross section data, the predictive capability of any parameterization is questionable when it is used beyond the range of the data to which it was tuned. Using uncertainty analysis, it is shown that a relativistic Three- Dimensional Lippmann-Schwinger (LS3D) equation model based on Multiple Scatter- ing Theory (MST) that uses 5 parameterizations—3 fundamental parameterizations to nucleon-nucleon (NN) data and 2 nuclear charge density parameterizations—predicts NA and AA reaction cross sections as well as the Tripathi cross section parameterization for reactions in which the kinetic energy of the projectile in the laboratory frame (TLab) is greater than 220 MeV/n. The relativistic LS3D model has the additional advantage of being able to predict highly accurate total and elastic cross sections. Consequently, it is recommended that the relativistic LS3D model be used for space radiation applications in which TLab > 220 MeV/n.

C M Werneth↗

MANTA. An Integral Reactor Physics Experiment to Infer the Neutron Capture Cross Sections of Actinides and Fission Products in Fast and Epithermal Spectra

Neutron cross-sections characterize the way neutrons interact with matter. They are essential to most nuclear engineering projects and, even though theoretical progress has been made as far as the predictability of neutron cross-section models, measurements are still indispensable to meet tight design requirements for reduced uncertainties. Within the field of fission reactor technology, one can identify the following specializations that rely on the availability of accurate neutron cross-sections: (1) fission reactor design, (2) nuclear fuel cycles, (3) nuclear safety, (4) nuclear safeguards, (5) reactor monitoring and neutron fluence determination and (6) waste disposal and transmutation. In particular, the assessment of advanced fuel cycles requires an extensive knowledge of transuranics cross sections. Plutonium isotopes, but also americium, curium and up to californium isotope data are required with a small uncertainty in order to optimize significant features of the fuel cycle that have an impact on feasibility studies (e.g. neutron doses at fuel fabrication, decay heat in a repository, etc.). Different techniques are available to determine neutron cross sections experimentally, with the common denominator that a source of neutrons is necessary. It can either come from an accelerator that produces neutrons as a result of interactions between charged particles and a target, or it can come from a nuclear reactor. When the measurements are performed with an accelerator, they are referred to as differential since the analysis of the data provides the cross-sections for different discrete energies, i.e. σ(E i ), and for the diffusion cross sections for different discrete angles. Another approach is to irradiate a very pure sample in a test reactor such as the Advanced Test Reactor (ATR) at INL and, after a given time, determine the amount of the different transmutation products. The precise characterization of the nuclide densities before and after neutron irradiation allows to infer energy-integrated neutron cross sections, i.e. ∫₀ ∞ σ(E)φ(E)dE, where φ(E) is the neutron flux “seen” by the sample. This approach, which is usually defined and led by reactor physicists, is referred to as integral and is the object of this report. These two sources of information, i.e. differential and integral, are complementary and are used by the nuclear physicists in charge of producing the evaluated nuclear data files used by the nuclear community (ENDF, JEFF…). The generation of accurate nuclear data files requires an iterative process involving reactor physicists and nuclear data evaluators. This experimental program has been funded by the ATR National Scientific User Facility (ATR-NSUF) and by the DOE Office of Science in the framework of the Recovery Act. It has been given the name MANTRA for Measurement of Actinides Neutron TRAnsmutation.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Neutrino Cross Section Measurements @ SciBooNE

We report measurements of cross sections of neutrinos of 0.7 GeV average energy scattering off a carbon target cross sections with by the SciBooNE experiment at Fermilab. These measurements are important inputs for current and future accelerator-based neutrino oscillation experiments in the interpretation of neutrino oscillation signals. The measurement of neutrino mixing angle {theta}{sub 13} is one of the most important goals in current neutrino experiments. For the current and next generation of long baseline neutrino oscillation experiments, T2K, NOvA and LBNE, the precise measurement of neutrino-nucleus cross sections in the few GeV energy range is an essential ingredient in the interpretation of neutrino oscillation signals.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Temperature dependency of the photoabsorption cross section for CF2Cl2

The photoabsorption cross section for CF2CL2 is measured at 297 K and 200 K. Cross sections are obtained for the ground and first two vibrationally excited states, allowing for a determination of the photoabsorption as a function of temperature over the range of stratospheric interest.

Boitnott, C. A.↗

Differential and integral cross sections in OH(X) + Xe collisions

Differential cross sections (DCSs) for inelastic collisions of OH(X) with Xe have been measured at a collision energy of 483 cm{sup −1}. The hydroxyl (OH) radicals were initially prepared in the X{sup 2}Π{sub 3/2} (v = 0, j = 1.5, f) level using the hexapole electric field selection method. Products were detected state-selectively by [2 + 1] resonance-enhanced multiphoton ionization of OH, combined with velocity-map imaging. Integral cross sections in OH(X) + Xe at a collision energy of 490 cm{sup −1} were also measured by laser-induced fluorescence. The results are compared with exact close-coupling quantum mechanical scattering calculations on the only available ab initio potential energy surface (PES). The agreement between experimental and theoretical results is generally very satisfactory. This highlights the ability of such measurements to test the available PES for such a benchmark open-shell system. The agreement between experiment and theory for DCSs is less satisfactory at low scattering angles, and possible reasons for this disagreement are discussed. Finally, theoretical calculations of OH(X) + He DCSs have been obtained at various collision energies and are compared with those of OH(X) + Xe. The role of the reduced mass in the DCSs and partial cross sections is also examined.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Reduce-Order Modeling of Multigroup Neutron Cross Sections for High-Temperature Gas-cooled Reactors

Deterministic neutronics calculations rely on multigroup neutron cross section libraries, which usually consists of a database of tabulated values, used to calculate the cross sections through multivariate linear interpolation. However, interpolation of the multidimensional cross section data becomes memory inefficient and time consuming as the number of tabulations increases, significantly slowing down the neutronics calculation, especially in the case of micro cross section libraries where every isotope (on the order of hundreds) has its own set of specific reactions and cross sections. To address this challenge, this work constructs efficient and robust reduced-order models (ROMs) of the multi-group cross sections to support the Griffin simulation of high-temperature gas-cooled reactors (HTGRs). The first part of the study investigates the linearity of the multi-group cross section data across isotopes, reaction types and energy groups on pre-generated datasets for the purpose of dimensionality reduction. Secondly, a down-selection of ROM techniques is presented on representative classical machine learning (ML) techniques, including variants of linear regression, kernel-based methods, tree-based algorithms, and artificial neural networks. The selection criteria jointly consider the memory efficiency, predictive accuracy, prediction speed, and scalability in comparison to the multidimensional interpolation. Among all the ML techniques, deep neural networks (DNNs) have proven to be the best selection with sufficient accuracy, high robustness, good memory efficiency, great scalability, and superior flexibility. DNNs for have been trained for all isotopes in this work and systematic Griffin testing is ongoing at this moment to ensure the feasibility of this ROM technique for cross section predictions.

42 - ENGINEERING↗

Prospects for Precision Neutrino Cross Section Measurements

The need for precision cross section measurements is more urgent now than ever before, given the central role neutrino oscillation measurements play in the field of particle physics. The definition of precision is something worth considering, however. In order to build the best model for an oscillation experiment, cross section measurements should span a broad range of energies, neutrino interaction channels, and target nuclei. Precision might better be defined not in the final uncertainty associated with any one measurement but rather with the breadth of measurements that are available to constrain models. Current experience shows that models are better constrained by 10 measurements across different processes and energies with 10% uncertainties than by one measurement of one process on one nucleus with a 1% uncertainty. This article describes the current status of and future prospects for the field of precision cross section measurements considering the metric of how many processes, energies, and nuclei have been studied.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Absolute cross sections for electronic excitation of pyrimidine by electron impact

We measured differential cross sections for electron-impact electronic excitation of pyrimidine, both as a function of electron energy up to 18 eV, and of scattering angle up to 180°. The emphasis of the present work is on recording detailed excitation functions revealing resonances in the excitation process. The differential cross sections were summed to obtain integral cross sections. These are compared to results of R-matrix calculations, which successfully reproduce both the magnitude of the cross section and the major resonant features. Comparison of the experiment to the calculated contributions of different symmetries to the integral cross section permitted assignment of several features to specific core-excited resonances. Comparison of the resonant structure of pyrimidine with that of benzene revealed pronounced similarities and thus a dominant role of π–π{sup ∗} excited states and resonances. Electron energy loss spectra were measured as a preparation for the cross section measurements and vibrational structure was observed for some of the triplet states. A detailed analysis of the electronic excited states of pyrimidine is also presented.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Fragmentation cross sections of O-16 between 0.9 and 200 GeV/nucleon

Inclusive cross sections for high energy interactions at 0.9, 2.3, 3.6, and 13.5 GeV/nucleon of O-16 with C, CR-39 (C12H18O7), CH2, Al, Cu, Ag, and Pb targets were measured. The total charge-changing cross sections and partial charge-changing cross sections for the production of fragments with charge Z = 6 and Z = 7 are compared to previous experiments at 60 and 200 GeV/nucleon. The contributions of Coulomb dissociation to the total cross sections are calculated. Using factorization rules the partial electromagnetic cross sections are separated from the nuclear components. Energy dependence of both components are investigated and discussed.

Hirzebruch, S. E.↗

Design and Construction of a High-Resolution Hodoscope for the GlueX Experiment with High-Statistics Analysis of the p0, ¿, and ¿1 Photoproduction Cross Sections from the RadPhi Experiment

Differential cross sections for forward-angle photoproduction of p0, ¿, and ¿ 1 pseudoscalar mesons were measured using data from the RadPhi experiment conducted in Hall B at Jef ferson Lab. RadPhi utilized a tagged bremsstrahlung photon beam incident on a stationary 9Be target, with a detector system configured to trigger on a recoil proton in coincidence with multiple neutral showers in the calorimeter. Events were reconstructed and subjected to kinematic constraints, with background suppressed via sideband subtraction guided by Monte Carlo modeling of background contributions. Cross sections were extracted over the photon energy range 4.4– 5.4 GeV and binned in invariant momentum transfer t, providing measurements from one of the first high-statistics experiments of forward ¿ and ¿1 pro duction from a nuclear target at these energies. Acceptance corrections were applied using a detailed GEANT-based simulation of the detector geometry and response. The resulting cross sections are consistent with 2020 CLAS results, when scaled by the number of protons in beryllium, and show broad agreement with other data and theoretical models. In parallel, a high-resolution photon tagger detector, the Tagger Microscope (TAGM), was designed, constructed, and commissioned for the GlueX experiment in Hall D at Jefferson Lab. The TAGM was developed to provide high-rate tagging capability in the coherent bremsstrahlung peak by detecting post-bremsstrahlung electrons across a one GeV range along the focal plane of the tagging spectrometer. The detector consists of a 5ˆ102 array of 2ˆ2 mm2 square BCF-20 plastic scintillating fibers thermally fused to BCF-98 light guide fibers optically coupled to silicon photomultipliers. These fibers are mounted in a precision machined framework enabling fine positional adjustments to maintain precise alignment with post-bremsstrahlung electron trajectories, while ensuring mechanical rigidity, thermal stability, optical isolation, minimal inactive area, and radiation shielding for electronics. The construction effort involved extensive testing of fiber quality, light transmission, thermal fusing, radiation hardness, and defect analysis using SEM and EDX techniques. Following its installation and commissioning, the TAGM became a critical component of the GlueX beamline, enabling high-rate tagging essential for studies of hybrid mesons and gluonic ex citations.

McIntyre, James [Univ. of Connecticut, Storrs, CT ↗

Photoneutron cross sections for Au

Photoneutron cross sections were measured for Au in the entire energy range of the ({gamma},n) channel based on a direct neutron-counting technique with quasimonochromatic {gamma} rays produced in inverse Compton-scattering of laser photons with relativistic electrons. We present results of the measurement in comparison with the past data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Kernel reconstruction methods for Doppler broadening — Temperature interpolation by linear combination of reference cross sections at optimally chosen temperatures

This paper establishes a new family of methods to perform temperature interpolation of nuclear interactions cross sections, reaction rates, or cross sections times the energy. One of these quantities at temperature T is approximated as a linear combination of quantities at reference temperatures (T j ). The problem is formalized in a cross section independent fashion by considering the kernels of the different operators that convert cross section related quantities from a temperature T 0 to a higher temperature T — namely the Doppler broadening operation. Doppler broadening interpolation of nuclear cross sections is thus here performed by reconstructing the kernel of the operation at a given temperature T by means of linear combination of kernels at reference temperatures (T j ). The choice of the L 2 metric yields optimal linear interpolation coefficients in the form of the solutions of a linear algebraic system inversion. The optimization of the choice of reference temperatures (T j ) is then undertaken so as to best reconstruct, in the L∞ sense, the kernels over a given temperature range [T min ,T max ]. The performance of these kernel reconstruction methods is then assessed in light of previous temperature interpolation methods by testing them upon isotope 238 U. Temperature-optimized free Doppler kernel reconstruction significantly outperforms all previous interpolation-based methods, achieving 0.1% relative error on temperature interpolation of 238 U total cross section over the temperature range [300 K,3000 K] with only 9 reference temperatures.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗