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At least 343 records · Page 19

CAAS-3S Radiation Testing for Y-12 and UPF with Godiva-IV

The Y-12 National Security Complex and the Uranium Processing Facility (UPF) selected the Mirion CAAS-3S as the Criticality Accident Alarm System for UPF and for Y-12 facilities replacing their legacy CAAS as part of efforts to extend the facility lifespans. As part of this process, the CAAS-3S system was exposed to a high radiation dose and dose rate during reactor testing with the Godiva-IV fast burst reactor. The reactor testing was designed around preliminary analyses that determined Y-12 and UPF requirements, and simulations of the radiation field within the reactor facility were used to determine reactor operating parameters, CAAS equipment locations, and the design of a neutron shield wall. This paper presents the design and results of the testing, and discusses how the test results were interpreted by criticality safety engineers at Y-12 and UPF.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Kilopower Reactor Development and Testing

The Kilopower Reactor Using Stirling Technology (KRUSTY) was the first nuclear-powered operation of a truly new fission reactor concept in the US in over 40 years. It provided valuable experience and data, demonstrated the passive reactor operation of the Kilopower reactor class, showed that developing a small reactor is not inherently expensive, and demonstrated a space reactor concept that can be used for near-term space science and exploration. KRUSTY/Kilopower is the first step towards truly astounding space fission capabilities

Gibson, Marc↗

Micro-tensile testing of the bond line in hot isostatic pressed aluminum

Considerable effort is being devoted to development and regulatory qualification of low enriched fuels for research and test reactors by many agencies worldwide. One promising fuel configuration being examined for United States higher power research and test reactors (USHPRRs) are plate-type fuels composed of a metallic uranium-molybdenum foil clad in an aluminum alloy. The two pieces of aluminum alloy cladding are bonded using a hot isostatic pressing method. The mechanical properties of the resulting bond line in the aluminum alloy cladding will vary by the HIP'ing parameters, requiring a need to characterize the bond line. Small scale mechanical testing can provide a path for evaluating the mechanical properties and deformation behavior of the bond line both prior to and following irradiation. Here, in this research, room temperature micro-tensile specimens of non-irradiated and irradiated samples containing an Al alloy (AA 6061) bond line were tested to evaluate its strength and deformation behavior. Observations indicated that the strain rate did not affect the deformation behavior or strength and most of the micro-tensile specimens failed in a ductile mode in grains around the bond line. There was no indication that the microstructural features from the bond line affected the mechanical properties of the micro-tensile specimens. An initial examination was performed on irradiated material but further systematic studies of the effects of irradiation can be performed in the future.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGC-4 Disassembly Report

The Advanced Reactor Terminology Graphite Research and Development program is currently measuring irradiated material property changes in several grades of nuclear graphite to predict behavior and operating performance within the core of these new high temperature reactor designs. The Advanced Graphite Creep (AGC) experiment, consisting of six irradiation capsules, will generate the irradiated graphite performance data for the Very High Temperature Reactor operating conditions. All six capsules in the experiment conducted at Idaho National Laboratory will be irradiated in the Advanced Test Reactor, disassembled in the Hot Fuel Examination Facility, and examined at the Idaho National Laboratory Research Center. This is the disassembly report describing the disassembly, shipment, post irradiation inspection, and storage of the graphite specimens contained within the AGC 4 irradiation test series capsule (the fourth irradiation capsule of the series). AGC 4 was irradiated in the Advanced Test Reactor (ATR) East Flux Trap (EFT) during ATR Cycle 157D, 158A, 162A, 162B, 164A, 164B, 166A, and Cycle 166B. Approximately 3.6 dpa was achieved. Desired experiment temperatures were exceeded by at least 100C during the second Cycle of irradiation due to the insertion of the KJRR experiment. The capsule was removed from the ATR and transferred to the Hot Fuel Examination Facility on May 15, 2020 and eventually unloaded into the Hot Fuel Examination Facility (HFEF) Decon Cell through Penetration 2D on February 26, 2021. It was moved to the HFEF Main Cell Window 3M for disassembly on March 15, 2021. Disassembly and specimen extraction began March 18, 2021, and packaging of the graphite specimens was completed on April 16, 2021. Several anomalies were noted, specifically that the radiological dose rates were nominally an order of magnitude higher than that of the previous AGC experiments. This report summarizes the disassembly of the AGC 4 experiment.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

AGC-4 Disassembly Report

The Advanced Reactor Terminology Graphite Research and Development program is currently measuring irradiated material property changes in several grades of nuclear graphite to predict behavior and operating performance within the core of these new high temperature reactor designs. The Advanced Graphite Creep (AGC) experiment, consisting of six irradiation capsules, will generate the irradiated graphite performance data for the Very High Temperature Reactor operating conditions. All six capsules in the experiment conducted at Idaho National Laboratory will be irradiated in the Advanced Test Reactor, disassembled in the Hot Fuel Examination Facility, and examined at the Idaho National Laboratory Research Center. This is the disassembly report describing the disassembly, shipment, post irradiation inspection, and storage of the graphite specimens contained within the AGC 4 irradiation test series capsule (the fourth irradiation capsule of the series). AGC 4 was irradiated in the Advanced Test Reactor (ATR) East Flux Trap (EFT) during ATR Cycle 157D, 158A, 162A, 162B, 164A, 164B, 166A, and Cycle 166B. Approximately 3.6 dpa was achieved. Desired experiment temperatures were exceeded by at least 100C during the second Cycle of irradiation due to the insertion of the KJRR experiment. The capsule was removed from the ATR and transferred to the Hot Fuel Examination Facility on May 15, 2020 and eventually unloaded into the Hot Fuel Examination Facility (HFEF) Decon Cell through Penetration 2D on February 26, 2021. It was moved to the HFEF Main Cell Window 3M for disassembly on March 15, 2021. Disassembly and specimen extraction began March 18, 2021, and packaging of the graphite specimens was completed on April 16, 2021. Several anomalies were noted, specifically that the radiological dose rates were nominally an order of magnitude higher than that of the previous AGC experiments. This report summarizes the disassembly of the AGC 4 experiment.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Catalytic Effects of Silver in Iodine Reactors for Dissolved Used Nuclear Fuel

The dissolution of used nuclear fuel generates a variety of off-gasses including flammable hydrogen and other species that are a concern for environmental release. The H-Canyon facility at the Savannah River Site is currently dissolving aluminum-clad research reactor fuel from material test reactors and the High Flux Isotope Reactor (HFIR) using a mercury-catalyzed nitric acid flowsheet. Savannah River National Laboratory recently developed and deployed a Raman spectrometer to monitor the off-gas stream from the dissolution process. Results from these measurements indicated a lack of the expected hydrogen, nitrous oxide, and nitric oxide in the off-gas stream. It was proposed that the silver on the silver nitrate–coated berl saddles present in the reactors for iodine capture were acting as a catalytic hydrogen recombiner. Nitric oxide is readily oxidized to nitrogen dioxide under normal conditions, but it was unclear what happened to the nitrous oxide. A laboratory-scale iodine reactor was assembled and filled with silver nitrate–coated berl saddles to help ascertain the fate of nitrous oxide and hydrogen. Testing with this laboratory-scale reactor observed the recombination of hydrogen when a simulated dissolver off-gas was passed through the reactor containing silver nitrate–coated berl saddles at the approximate temperatures seen in H-Canyon. However, the nitrous oxide concentration was unchanged, suggesting a more complex process occurring within the off-gas stream before it reaches the iodine reactors at H-Canyon.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

ATF-2 Ramp Conceptual Design Report

The following report documents the conceptual design for the ATF-2 Ramp experiment. The experiment aims to fill the in-pile irradiation testing gap to conduct integral ramp testing, which was created by the closure of R2, Osiris, and Halden test reactors. The concept involves the simultaneous ramping of three fuel pins using a power axial locator mechanism in the Loop-2A testing facility in the center flux trap of the advanced test reactor (ATR). The three fuel pins are ramped in individual coolant channels containing a prototypic PWR environment. Rod failure will be detected using a fuel rod elongation sensor attached to the fuel pin upper end cap. An axial stack of concentric hafnium and zirconium shrouds will be used to shape the flux around the test pins to create different power levels in each pin and to ensure the peak power location of each pin remains in the center of the test rod. Monte Carlo simulations are used to demonstrate the viability of this design concept.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Space station prototype Sabatier reactor design verification testing

A six-man, flight prototype carbon dioxide reduction subsystem for the SSP ETC/LSS (Space Station Prototype Environmental/Thermal Control and Life Support System) was developed and fabricated for the NASA-Johnson Space Center between February 1971 and October 1973. Component design verification testing was conducted on the Sabatier reactor covering design and off-design conditions as part of this development program. The reactor was designed to convert a minimum of 98 per cent hydrogen to water and methane for both six-man and two-man reactant flow conditions. Important design features of the reactor and test conditions are described. Reactor test results are presented that show design goals were achieved and off-design performance was stable.

Cusick, R. J.↗

ARCS Replacement at TREAT for TRTR 2020 - Abstract

The Transient REActor Test (TREAT) facility was restarted in 2017 to perform reactor fuels testing under transient conditions, following shutdown in 1994 and 23 years in non-operational standby. TREAT is a transient reactor that, like most pulsing reactors, can create natural shaped power pulses. However, TREAT provides the ability to shape the power pulse and control the energy deposition rate on the test specimens by automatically controlling the amount of reactivity insertion over time. The original automatic reactor control system (ARCS) was created in the 1980s using INTEL 8086 CPU boards and software written in assembly code. The need to maintain the system for the next 40+ years of TREAT life led to the decision to replace ARCS with modern hardware while maintaining the original functionality. After a prototyping effort, the replacement was successfully completed in the first quarter of 2020. The process and results of that effort are reported here.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

AGR 1 and 2 Isotopic Depletion Validation

This presentation includes work performed developing a computational benchmark for the AGR 1 and 2 experiments. These experiments involve irradiation of TRISO particle compact in the Advanced Test Reactor (ATR). Many post-irradiation measurements were made from these experiments, including isotopic concentrations of fission products. The benchmark involves a MCNP-ORIGEN coupled model of the ATR and AGR experiment capsules to calculate a comprehensive inventory of fission product and actinide concentrations in the compacts. This presentation describes the experiments, the measurements obtained, the benchmark model, and results of the model evaluation.

97 - MATHEMATICS AND COMPUTING↗

Demonstration of NEAMS Multiphysics Tools for Fast Reactor Applications

The SHARP toolkit is a high-fidelity reactor simulation tool developed under the U.S. Department of Energy, Office of Nuclear Energy Advanced Modeling and Simulation (NEAMS) Campaign. SHARP toolkit is comprised of the neutronics module PROTEUS thermal hydraulics module Nek5000, and structural mechanics module Diablo. During FY17 and FY18, the PROTEUS and Nek5000 components of SHARP were applied to solve challenging sodium-cooled fast reactor (SFR) problems. In particular, selected hot channel factors (HCF) for a prototype metal-fueled SFR design (the AFR-100) were analyzed in high fidelity, and the “SHARP zooming capability” for SFRs was developed and demonstrated to reduce computational expense for full core problems in cases where detailed data is needed in selected fuel assemblies. After the previous success applying SHARP to challenging SFR problems, the focus in FY19 and FY20 expanded to additional fast reactor applications including lead cooled fast reactors (LFR) and sodium cooled fast reactors (SFR). The specific technical tasks were (1) assessment of hot channel factors for LFR, for which no data currently exists, and (2) demonstration of zooming capability in assemblies of the Versatile Test Reactor (VTR). First-of-a-kind hot channel factor (HCF) estimation for LFR with high fidelity codes (PROTEUS/Nek5000) was successfully demonstrated in this study which began in FY19 and continued in FY20. Selected HCF were computed and compared with SFR data (AFR-100, EBR-II). The findings confirm that different reactor types, design parameters and uncertainties lead to different HCFs. Careful estimation of HCF for a specific design is necessary to obtain appropriate HCFs. In addition to improvement in HCF accuracy, high fidelity tools generate data to help the designer better understand the mechanism of the impact from these uncertainties. For example, the impact of cladding thickness manufacturing tolerance resulted in non-intuitive effects in the corner pins of the LFR assembly. This procedure of computing HCF using high fidelity models shows promise and flexibility for being repeated for any arbitrary reactor of choice. Along with the application on SFR and LFR, the capability of the tools has also been matured to deal with different reactor types and designs. Progress was made towards extending the previously demonstrated SHARP zooming capability to non-fueled SFR assemblies. In particular, in FY19 a gamma transport capability was implemented in both high fidelity PROTEUS solvers in order to accurately account for heat deposition caused by gamma particles, which accounts for ~10% of total core power. Neutronics verification cases were carried out for a candidate Versatile Test Reactor (VTR) design using the new gamma transport capability in PROTEUS. Comparisons were made with continuous energy MCNP calculations and shown to agree well. The models for the full core design with heterogeneous control and fuel assemblies is in progress for PROTEUS-SN and completed with MCNP. The MCNP power distributions were transferred to Nek5000 to perform thermal hydraulic calculations of the control and fuel assembly.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Characterizing the flux effect on the irradiation embrittlement of reactor pressure vessel steels using machine learning

In-service exposure to high-energy neutrons embrittles reactor pressure vessel (RPV) steels. An increase in the yield stress (Δσ y ) results in a corresponding increase in the brittle to ductile transition temperature (ΔT c ). Most existing models underpredict ΔT c at higher fluence following accelerated irradiations in test reactors. High fluence, up to 10 20 n/cm 2 in some cases, will be reached over extended RPV vessel operation of 80 years, or more, at low service flux. Embrittlement has been extensively studied in accelerated, higher flux test reaction irradiations. However, the use of test reactor data naturally raises the question of flux effects. Here, this study used a machine learning approach trained on a set of hardening data, covering a wide range of flux, fluence, and steel compositions to determine the interactive effects of both irradiation and material variables on Δσ y . The analysis included machine learning-based cross-plots of the variable dependence of Δσ y for six core steels (i.e., CM6, LC, LD, LG, LH, and LI), with controlled differences in their Cu and Ni contents. A primary objective is to evaluate an effective to actual fluence (Φt e /Φt) ratio, as a function of flux, fluence, and steel composition. This is information critical to properly use intermediate flux-high fluence data in calibrating a low flux-high fluence embrittlement model. The predicted Φt e /Φt is reasonably consistent with estimates previously derived from a physics-based solute recombination trap model.

36 MATERIALS SCIENCE↗

Reactor Simulator Testing Overview

Test Objectives Summary: a) Verify operation of the core simulator, the instrumentation & control system, and the ground support gas and vacuum test equipment. b) Examine cooling & heat regeneration performance of the cold trap purification. c) Test the ALIP pump at voltages beyond 120V to see if the targeted mass flow rate of 1.75 kg/s can be obtained in the RxSim. Testing Highlights: a) Gas and vacuum ground support test equipment performed effectively for operations (NaK fill, loop pressurization, and NaK drain). b) Instrumentation & Control system effectively controlled loop temperature and flow rates or pump voltage to targeted settings and ramped within prescribed constraints. It effectively interacted with reactor simulator control model and defaulted back to temperature control mode if the transient fluctuations didn't dampen. c) Cold trap design was able to obtain the targeted cold temperature of 480 K. An outlet temperature of 636 K was obtained which was lower than the predicted 750 K but 156 K higher than the minimum temperature indicating the design provided some heat regeneration. d) ALIP produce a maximum flow rate of 1.53 kg/s at 800 K when operated at 150 V and 53 Hz.

Schoenfeld, Michael P.↗

Experimental results of conductive inserts to reduce nuclear fuel temperature during nuclear volumetric heating

Advanced fuel designs that incorporate thinner fuel UO2 pellets interspaced by high thermal conductivity inserts have been proposed, with the primary goals of reducing peak centerline temperatures and temperature gradients across fuel pellets and enhancing heat transfer from the fuel to the coolant. An initial series of experiments has been performed on this design, including laboratory experiments and a series of experiments using the Idaho National Laboratory (INL) Transient Reactor Test (TREAT) Facility, the latter of which compared thermal gradient driven fracture of standard pellet designs with that in the proposed advanced fuel design. Although reducing fracture is not the primary objective of the new fuel design, the lower thermal gradients are expected to reduce fracture, so it can serve as an indicator of the thermal behavior of this fuel in the reactor. The in-reactor tests were conducted at multiple linear heat generation rates and confirm the expected result that fracture in both the standard and advanced fuel pellets occurs during the first ramp to power in standard light-water reactor conditions. Post-irradiation examination of the experiment material was performed and included quantification of the extent of fracture in the fuel pellets. It was found that the advanced-design pellets reduce the extent of fracture in a statistically significant way. This confirms the expected behavior predicted by two-dimensional axisymmetric models of this experiment. Here in this study is an important first experimental confirmation of the efficacy of the proposed inserts for achieving their desired effect on the thermal behavior of the fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Cracking in first ramp to power of standard versus high thermal conductivity UO2 pellets via internal nuclear heating

Advanced fuel designs that incorporate thinner fuel UO2 pellets interspaced by high thermal conductivity inserts have been proposed, with the primary goals of reducing peak centerline temperatures and temperature gradients across fuel pellets and enhancing heat transfer from the fuel to the coolant. An initial series of experiments has been performed on this design, including laboratory experiments and a series of experiments using the Idaho National Laboratory (INL) Transient Reactor Test (TREAT) Facility, the latter of which compared thermal gradient driven fracture of standard pellet designs with that in the proposed advanced fuel design. Although reducing fracture is not the primary objective of the new fuel design, the lower thermal gradients are expected to reduce fracture, so it can serve as an indicator of the thermal behavior of this fuel in the reactor. The in-reactor tests were conducted at multiple linear heat generation rates and confirm the expected result that fracture in both the standard and advanced fuel pellets occurs during the first ramp to power in standard light-water reactor conditions. Post-irradiation examination of the experiment material was performed and included quantification of the extent of fracture in the fuel pellets. It was found that the advanced-design pellets reduce the extent of fracture in a statistically significant way. This confirms the expected behavior predicted by two-dimensional axisymmetric models of this experiment. This study is an important first experimental confirmation of the efficacy of the proposed inserts for achieving their desired effect on the thermal behavior of the fuel.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Irradiation Experiments and Thermal Analysis for Reactor System Design and Analysis at INL

Idaho National Laboratory (INL) is the nation's lead nuclear laboratory working to enhance reactor systems' safety, security, economics, and efficiency. Research and development (R&D) programs at INL support the current fleet of nuclear reactors for safer operation and newer reactors technology design, development, demonstration, and deployment. A major focus of INL's mission is the reactor system design and analysis supported by the irradiation experiments and thermal analysis of advanced and current-generation nuclear fuels and materials. The irradiation experiments and thermal analysis provide a deeper understanding of basic radiation damage processes that can determine the basis for performance improvements and verification of modeling assumptions. These experiments and analyses include experiment management: design, fabrication, characterization, irradiation, and post-irradiation examination. This research involves thermal, neutronic, and material investigation using the INL's Advanced Test Reactor (ATR) and Transient Reactor Test (TREAT) facilities. The results from these experiments and analysis are required to develop the regulatory basis for deploying new or modified fuels and materials. This seminar talk will also provide a general overview of the INL's research facilities, ongoing research programs, core capabilities, and opportunities for students and faculties.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Modeling and Analysis of the Transport and Disposal of Beryllium Moderator Blocks and Greater than Class C (GTCC) Waste

Radioactive waste in the United states is categorized based on its source, radioactivity, and security risk. The categorization method employed by the Nuclear Regulatory Committee (NRC) for low-level radioactive waste is not currently applied to any waste generated by the Department of Energy (DOE) or disposed of in DOE facilities. As a result, there is a large volume of DOE-generated waste with characteristics similar to the NRC’s “Greater than Class C” (GTCC) waste category which presently do not have a path for long-term disposal. Much of this waste cannot undergo the standard commercial disposition process due to it being categorized as Transuranic (TRU) waste under DOE guidelines, due to elevated concentrations of key fission products. Possible solutions to this dilemma are explored in the Environmental Impact Statement for the “Disposal of Greater-Than-Class-C Low Level Radioactive Wave” (EIS-0375). This paper analyzes several EIS possible paths for disposal for this “orphaned” waste. One example that highlights this categorization issue is the spent beryllium cladding that has been extracted from the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) throughout its operational lifetime. These beryllium blocks surround the reactor’s main chambers and components and serve as neutron moderators. This paper will use this particular waste form to analyze the economic and technological viability of transporting and storing this material under the storage and transportation criteria of the Waste isolation Pilot Plant (WIPP), which was deemed the most feasible disposition path according to the EIS. The example of this waste form used in this paper that highlights this categorization issue is the spent beryllium cladding extracted from Idaho National Laboratory’s (INL) Advanced Test Reactor (ATR). These beryllium blocks surround the reactor’s components and serve as neutron moderators, and thus have accumulated high concentration of high-activity transuranic isotopes. This paper analyzed the viability of transporting and storing this material under the storage and transportation criteria of the five primary disposition paths covered in EIS-0375. An array of calculations was carried out to assess the viability of the various disposition paths for the beryllium shipments as well as other waste shipments that fall within the GTCC category. Modeling with MCNP 6.2 was conducted to determine whether the beryllium blocks could be safely stored and transported within a 72-B cask; the standard shipping container for remote-handled, transuranic waste, while also meeting regulatory limits at various disposition paths. A cost analysis of the transportation and long-term disposal paths mentioned in the EIS was also carried out using available data and information from similar waste shipments. Lastly, a geochemical analysis of the various geological repository discussed in the EIS was also carried out using the Geochemists Workbench Release 14. Long-term disposal of the beryllium blocks at the Waste Isolation Pilot Plant (WIPP) proved to be the most cost-effective long-term disposition option of the ones considered in the EIS. A dose rate calculation at both contact and remote-handling distances indicate that the analyzed beryllium shipments should not exceed the exposure limits at any of the considered locations. Greater-than-class-C waste has been left in a regulatory state of limbo for years, resulting in backlogs of inventory across several research sites in the United States. Due to its high activity and presence of transuranic isotopes, it is imperative to ensure that it remains inaccessible and sequestered both in its short-term interim as well as a long-term geologic time scale. The information and assessments done in the paper could potentially serve as a reference for any future shipments of this waste form at the WIPP facility as well as other disposition paths that may be considered in the future.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗