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At least 343 records · Page 19

All sources NASA NTRS DOE OSTI

DOE OSTI2021

Ultrafast time-resolved x-ray absorption spectroscopy of ionized urea and its dimer through ab initio nonadiabatic dynamics

Investigating the early dynamics of chemical systems following ionization is essential for our understanding of radiation damage. However, experimental as well as theoretical investigations are very challenging due to the complex nature of these processes. Time-resolved x-ray absorption spectroscopy on a femtosecond timescale, in combination with appropriate simulations, is able to provide crucial insights into the ultrafast processes that occur upon ionization due to its element-specific probing nature. In this theoretical study, we investigate the ultrafast dynamics of valence-ionized states of urea and its dimer employing Tully's fewest switches surface hopping approach using Koopmans' theorem to describe the ionized system. We demonstrate that following valence ionization through a pump pulse, the time-resolved x-ray absorption spectra at the carbon, nitrogen, and oxygen K-edges reveal rich insights into the dynamics. Excited states of the ionized system give rise to time-delayed blueshifts in the x-ray absorption spectra as a result of electronic relaxation dynamics through nonadiabatic transitions. Moreover, our statistical analysis reveals specific structural dynamics in the molecule that induce time-dependent changes in the spectra. For the urea monomer, we elucidate the possibility to trace effects of specific molecular vibrations in the time-resolved x-ray absorption spectra. For the urea dimer, where ionization triggers a proton transfer reaction, we show how the x-ray absorption spectra can reveal specific details on the progress of proton transfer.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2020

Soft-Switching Solid-State Transformer With Reduced Conduction Loss

Solid-state transformers (SSTs) are a promising solution photovoltaic (PV), wind, traction, data center, battery energy storage system (BESS), and fast charging electric vehicle (EV) applications. The traditional SSTs are typically three-stage, i.e., hard-switching cascaded multilevel rectifiers and inverters with dual active bridge (DAB) converters, which leads to bulky passives, low efficiency, and high electromagnetic interference (EMI). This article proposes a new soft-switching solid-state transformer (S4T). The S4T has full-range zero-voltage switching (ZVS), electrolytic capacitor-less dc link, and controlled dv/dt, which reduces EMI. The S4T comprises two reverse-blocking current-source inverter (CSI) bridges, auxiliary branches for ZVS, and transformer magnetizing inductor as a reduced dc link with 60% ripple. Compared with the prior S4T, an effective change on the leakage inductance diode is made to reduce the number of the devices on the main power path by 20% for significant conduction loss saving and retain the same functionality of damping the resonance between the leakage and resonant capacitors and recycling trapped leakage energy. The conduction loss saving is crucial, being the dominating loss mechanism in SSTs. Importantly, the proposed single-stage SST not only holds the potential for high power density and high efficiency but also has full functionality, e.g., multiport dc loads integration, voltage regulation, and reactive power compensation, unlike the traditional single-stage matrix SST. The S4T can achieve single-stage isolated bidirectional dc–dc, ac–dc, dc–ac, or ac–ac conversion. It can also be configured input-series output-parallel (ISOP) in a modular way for medium-voltage (MV) grids. Hence, the S4T is a promising candidate for the SST. The full functionality, e.g., voltage buck–boost, multiport, etc., and the universality of the S4T for the dc–dc, dc–ac, and ac–ac conversion are verified through the simulations and experiments of two-port and three-port MV prototypes based on 3.3 kV SiC MOSFETs in dc–dc, dc–ac, and ac–ac modes at 2 kV.

14 SOLAR ENERGY↗

DOE OSTI2025

Job Scheduler-Driven Power Gateway for High Performance Computing

Power gateways in the form of a microgrid can incorporate multiple distributed energy resources (DER) in either grid forming or grid following mode and support high performance computing (HPC) power profiles including the large load-follow requirements observed in multi-user HPC systems. The microgrid’s flexibility to operate in either grid forming or grid following mode and to actively switch between these modes enables baseline power from multiple non-baseline DER while maintaining high power quality metrics for the HPC system. But this enormous flexibility in demand response and time of use shifting is generally programmed independently of any integration with an HPC job scheduler which can better inform the load shaping by the microgrid. While there are many existing approaches where the HPC job scheduler takes in information from the grid to make queue scheduling decisions, this work takes the opposite view and explores a scheduler where the jobs in the queue can directly impact the settings of the grid. Several HPC scheduler strategies are tested where the jobs in the queue directly impact the settings of a microgrid designed for HPC operation which is driving a datacenter with three classes of HPC architectures. The scheduler operation is shown using a microgrid with 64 kW of solar capacity and 320 kWh of battery over a period of 21 days operating with significant low-follow swings, a throttled grid, cloudy conditions, switching between grid following and grid forming modes, and a wide range of battery states-of-charge all while maintaining high quality power metrics. The scheduler provides a mechanism for the job queue to directly impact a power gateway like a microgrid and to improve HPC power outcomes such as maximizing renewable energy usage

microgrid↗

DOE OSTI2023

Interoperability between Three-Phase and Single-Phase WPT Systems

This paper presents an analysis and optimal position alignments of the transmitting and receiving couplers for achieving interoperability between a three-phase and a single-phase inductive wireless power transfer (WPT) system. In addition, single-phase operation modes for the six-switch three-phase inverter are identified for maximal power transfer from the three-phase transmitter pad to the single-phase receiver pad. Simulation results are included to show the power transfer capability between a 50 kW three-phase and an 11 kW double-D or circular single-phase WPT system at various alignment positions of the couplers.

Su, Gui-Jia↗

DOE OSTI2021

Design of a Robust Memristive Spiking Neuromorphic System with Unsupervised Learning in Hardware

Spiking neural networks (SNN) offer a power efficient, biologically plausible learning paradigm by encoding information into spikes. The discovery of the memristor has accelerated the progress of spiking neuromorphic systems, as the intrinsic plasticity of the device makes it an ideal candidate to mimic a biological synapse. Despite providing a nanoscale form factor, non-volatility, and low-power operation, memristors suffer from device-level non-idealities, which impact system-level performance. To address these issues, this article presents a memristive crossbar-based neuromorphic system using unsupervised learning with twin-memristor synapses, fully digital pulse width modulated spike-timing-dependent plasticity, and homeostasis neurons. Additionally, the implemented single-layer SNN was applied to a pattern-recognition task of classifying handwritten-digits. The performance of the system was analyzed by varying design parameters such as number of training epochs, neurons, and capacitors. Furthermore, the impact of memristor device non-idealities, such as device-switching mismatch, aging, failure, and process variations, were investigated and the resilience of the proposed system was demonstrated.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2024

A Deep Learning Approach for In-Network Synchrophasor Missing Data Recovery Using Programmable Network Switches

Phasor measurement unit (PMU) networks deliver accurate and timely measurements, which is essential for managing today’s electric power systems. To ensure data quality and enhance the cyber-resilience of PMU networks against malicious attacks and data errors, this study presents an online PMU missing data recovery scheme by leveraging P4 programmable switches. The data plane incorporates a customized PMU protocol parser that abstracts the necessary payload data for recovery. Recovery processes are executed in the control plane using a pre-trained machine learning model. Both traditional and advanced ML models, such as transformer and TimeGPT, are explicitly employed for data prediction. This approach ensures rapid and precise data recovery. Performance evaluations focus on recovery speed and accuracy, using a real dataset from a campus microgrid. With 20% missing PMU data, the mean absolute percentage error for voltage magnitude is 0.0384%, and the phase angle error discrepancy is approximately 0.4064%.

Phasor Measurement Unit, Machine Learning, Program↗

DOE OSTI2022

Automating Component-Level Stress Measurements for Inverter Reliability Estimation

In the near future, grid operators are expected to regularly use advanced distributed energy resource (DER) functions, defined in IEEE 1547-2018, to perform a range of grid-support operations. Many of these functions adjust the active and reactive power of the device through commanded or autonomous operating modes which induce new stresses on the power electronics components. In this work, an experimental and theoretical framework is introduced which couples laboratory-measured component stress with advanced inverter functionality and derives a reduction in useful lifetime based on an applicable reliability model. Multiple DER devices were instrumented to calculate the additional component stress under multiple reactive power setpoints to estimate associated DER lifetime reductions. A clear increase in switch loss was demonstrated as a function of irradiance level and power factor. This is replicated in the system-level efficiency measurements, although magnitudes were different—suggesting other loss mechanisms exist. Using an approximate Arrhenius thermal model for the switches, the experimental data indicate a lifetime reduction of 1.5% when operating the inverter at 0.85 PF—compared to unity PF—assuming the DER failure mechanism thermally driven within the H-bridge. If other failure mechanisms are discovered for a set of power electronics devices, this testing and calculation framework can easily be tailored to those failure mechanisms.

Flicker, Jack (ORCID:0000000212232154)↗

DOE OSTI2020

A Novel AC to AC Wireless Power Transfer System for EV Charging Applications

In this paper, a novel ac to ac wireless power transfer (WPT) system is introduced for electric vehicle (EV) charging applications to reduce cost and design complexity. The presented wireless power transfer concept achieves unity power factor (UPF) on the grid-side by using a hybrid frequency ac / ac converter without an additional converter stage and closed loop control compared to the conventional systems. Due to inherent merit of the proposed ac / ac converter, ac input with 60 Hz grid frequency can be directly transferred to the load by superimposing with high frequency switching signal through the wireless coils. To validate the theoretical analysis of the proposed WPT system, the experimental results of the proposed converter are provided for 650 W output power by using 6 inches air gap between the couplers with the input of 110 VRMS ac source. The system overall efficiency is measured 89 % achieving 0.99 power factor (PF) and 1.5 % current total harmonic distortion (THD).

Asa, Erdem↗

DOE OSTI2024

1 kV 150 A Bidirectional Isolated DC/DC Converter With Full Range ZVS For Charger Application

This paper focusses on the development of a bidirectional DC/DC converter based on dual active bridge (DAB) converter for 1 kV class fast charger applications. A novel modulation technique is proposed to achieve zero voltage switching across the entire operating range of a vehicle battery system. The topology includes a tap changer to support multiple class of vehicles. The full range ZVS operation will allow high efficiency operation even at light load, reduced dv/dt to improve transformer insulation lifetime and mitigate EMI impact. A 1 kV class, 150 A prototype was developed to validate the proposed concepts.

Kandula, Prasad↗

DOE OSTI2020

A new approach to removing H atoms in hydrogen depassivation lithography

Hydrogen deppasivation lithography (HDL) carried out by a scanning tunneling microscope (STM) is used to make patterns of Si dimers on a hydrogen passivated silicon surface. In this paper we discuss a new STM mode of operation that is highly suitable for removing single H atoms from the surface. This is made possible by changes we have made to the STM feedback control system that allows the STM to remove hydrogen atoms without switching the operational mode from imaging to lithography. Employing this method can potentially reduce the chance of tip-sample crash and increase the lithography precision.

Moheimani, S. O. Reza↗

DOE OSTI2020

Matrix converter operation in current control mode with regulation of output voltage vector

A matrix converter system having a current control mode operation is provided. The matrix converter system includes a matrix converter that includes a plurality of switches. A unity current reference vector having an amplitude of one is determined that defines an angle and frequency of an output current vector as a function of a reference phase angle, which is a function of the output current vector and an output voltage vector representing feedback signals of a multiphase signal output to a load. The unity current reference vector is used to control the matrix converter, to cause the output current vector to be aligned with the unity current reference vector. A unity voltage reference vector having an amplitude of one is provided that defines a reference angle and frequency as a function of a zero phase angle. The output voltage vector and the unity voltage reference vector are aligned to determine the reference phase angle as an angle between the aligned output voltage vector and the output current vector.

42 ENGINEERING↗

DOE OSTI2023

Fluid level and conductivity sensor for high temperature applications

A fluid level and conductivity sensor having a sensing probe with four electrodes disposed therein particularly suited for high temperature applications. A distal end of the second and third electrodes are positioned a distance from the sensing end that is greater than distal ends of the first and fourth electrodes. The sensor includes an electronics system having a signal relay system for receiving signals from each of the electrodes and switching between different measurement modes by determining a resistance between selected pairs of electrodes based on instructions from the microcontroller. The measurement modes include a conductivity measurement mode in which a resistance between the first and fourth electrodes is determined, and a fluid level measurement mode in which a resistance between the first and third electrodes is determined and compared to a resistance between the second and third electrodes.

Holland, Justin M.↗

DOE OSTI2022

Model predictive control for matrix converter operating in current control mode with load current estimation

A matrix converter system operating in current control mode is provided. The matrix converter includes a switching matrix coupled between a low voltage side and a high voltage side, wherein the matrix converter is coupled at its low voltage side to a generator for receiving an input power including an input current and transforming the input power into an output power at its high voltage side, wherein a load is coupled to the high voltage side. The control system includes a load observer and a model predictive controller (MPC). The load observer is configured to estimate a load current that flows to the load from the high voltage side of the matrix converter as a function of a switching state of the switching matrix, an output voltage output at the high voltage side of the matrix converter, and the input current. The MPC is configured to select the switching state of the switching matrix to meet one or more control objectives defined by minimization of a multi-objective function that tracks the output voltage and the input current using the estimated load current.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2024

Voltage Optimization

Voltage optimization refers to a volt-var optimization technique which was originally designed to minimize energy consumption and improve end-use efficiency on the distribution system. This reduces source voltage at a substation, which lowers generation demand, reduces system losses, and improves system stability. This has been the conventional implementation of voltage optimization: focusing on regulation of voltages throughout the distribution system via coordinated adjustments of load tap changers, line-voltage regulators, switched shunt compensation, and the targeted placement of new shunt compensation. These methods have received increased focus following a growth in distributed-energy resources (DERs) interconnecting at the distribution level, given their developing capability to participate in voltage regulation. This is paired with the intermittency challenges they pose, load imbalances, and voltage fluctuations. Voltage optimization has long been an area of extensive research within the distribution system, with various strategies and philosophies demonstrating a range of effects. The conventional focus on the distribution system owes to the typical operation of transmission systems, which assumes firm local resources and flows strictly from generation resources to loads. The strategies employed in distribution have also been optimized for this typically radial configuration and operation of the distribution system.

24 - POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2021

Polarization-Insensitive Medium-Switchable Holographic Metasurfaces

The adoption of metasurfaces has led to revolutionary advances in holography due to improved compactness, integrability, and performance. Switchable meta-holograms projecting different replay field images in a controllable manner are highly desirable. Still, existing technologies generally rely on the use of polarized light and additional optics to facilitate switching. Consequently, the potential benefits afforded through the use of metasurfaces are limited both by the system complexity and a fixed relationship between the optical input and output. In this manuscript, we demonstrate polarization-insensitive metasurfaces encoding arbitrary and independent holograms, which can be switched between by changing the refractive index of the infiltration medium while maintaining identical illumination conditions. Finally, by sidestepping the requirements for high-performance light sources, switching optics, or delicate alignment, this approach points toward ultracompact and cost-effective switchable meta-holograms for various practical applications, such as holographic image projection, eye-perceptible sensors, optical information storage, processing, and security.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Safety Basis Compliant Flexible Operations [Capstone Project]

Compliant nuclear operations must be weighed against the radiological risk to the worker, public, and the environment. This project set out to look at one facility at Los Alamos National Laboratory (LANL or the Laboratory) and compare the risk with the operational restrictions associated with the Technical Safety Requirements (TSRs). The hope was to identify controls that could be reduced or simplified while maintaining compliance with 10 CFR 830, Nuclear Safety Management. This would result in increasing facility operational flexibility and efficiency. Controls were identified to be simplified or eliminated based on risk. This identification was initially envisioned from the perspective of reanalysis of the accident and hazard analysis consequences. Additionally, it was envisioned that fire testing could show that the consequences of a fire are not as dramatic as analyzed. Specific facility controls were identified that cause operational inefficiencies. Based on data collection, two controls were identified for further evaluation. The first control was combustible loading within the waste storage buildings, and the second control is related to the seismic power cutoff switch. In evaluating the combustible loading control, the thought is that the fire suppression system (FSS) provides adequate protection and the combustible loading controls do not need elevation to a TSR control. The FSS, along with the Fire Protection Program, would provide protection to prevent a fire from impacting large amounts of stored waste material. The seismic switch was more of a challenge. When reviewing the facility operation, it was determined that the facility does not operate anywhere near the established material-at-risk (MAR – radioactive material) limits. By adjusting these limits, a reduced consequence could be achieved and hence, a significant risk reduction achieved. A new operating mode would be used to achieve this reduction. A reduced MAR limit was successfully used as a test case for snow removal during this project. This project expands on that trial case as related to combustible loading and the seismic power cutoff switch TSRs. This will increase the efficiency of operations with reduced TSR controls while reducing overall facility risk. This is a win-win situation for Triad National Security, LLC (Triad) and the U.S. Department of Energy (DOE). Due to schedule and budgetary constraints, not all envisioned work scope was accomplished. However, it is maintained in this report for future efforts.

61 RADIATION PROTECTION AND DOSIMETRY↗

DOE OSTI2022

Scalable Al 2 O 3 –TiO 2 Conductive Oxide Interfaces as Defect Reservoirs for Resistive Switching Devices

Abstract Resistive switching devices herald a transformative technology for memory and computation, offering considerable advantages in performance and energy efficiency. Here, a simple and scalable material system of conductive oxide interfaces is employed, and their unique properties are leveraged for a new type of resistive switching device. An Al 2 O 3 –TiO 2 ‐based valence‐change resistive switching device, where the conductive oxide interface serves both as the bottom electrode and as a reservoir of defects for switching, is demonstrated. The amorphous–polycrystalline Al 2 O 3 –TiO 2 conductive interface is obtained following the technological path of simplifying the fabrication of the 2D electron gases (2DEGs), making them scalable for practical mass integration. Physical analysis of the device chemistry and microstructure with comprehensive electrical analysis of its switching behavior and performance is combined. The origin of the resistive switching is pinpointed to the conductive oxide interface, which serves both as the bottom electrode and as a reservoir of oxygen vacancies. The latter plays a key role in valence‐change resistive switching devices. The new device, based on scalable and complementary metal–oxide–semiconductor (CMOS)‐technology‐compatible fabrication processes, opens new design spaces toward increased tunability and simplification of the device selection challenge.

36 MATERIALS SCIENCE↗

DOE OSTI2026

Switching speed limits in electrically driven VO 2 structural Mott–Peierls transition

Mott materials are archetypal quantum systems actively explored as next-generation electronic and photonic platforms, with potential applications spanning non-Von Neumann computing, robotics, energy storage, and microwave technologies. Among these, vanadium dioxide (VO 2 ) has emerged as one of the most intensively studied compounds, owing to its sharp, near-room-temperature insulator-to-metal phase transition. VO 2 also serves as a benchmark system for testing cutting-edge theories and experimental techniques. Here, we directly visualize the electrically driven transition dynamics in VO 2 using a microwave-driven, frequency-tunable pulsed transmission electron microscope that combines nanometer spatial and picosecond temporal resolution. Under high-frequency (MHz–GHz) excitation, we capture the ultrafast nucleation, propagation, and dissolution of metallic domains within an operating device over millions of reversible cycles. We observe the ultrafast formation of consistent metallic nuclei beneath the electrodes, followed by the propagation of a structural phase front at 4.54 nm/ns. Our experiments show that phonon-mediated structural recovery ultimately limits reversible switching of VO 2 at GHz frequencies, and that a tunable regime for reversible operation spans from kHz to GHz through device engineering. Beyond VO 2 , our approach provides a powerful framework for probing non-equilibrium structural transformations in correlated and functional materials under realistic electrical stimuli.

36 MATERIALS SCIENCE↗