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At least 343 records · Page 19

Generalized 3D beam dynamics model for industrial traveling wave linacs design and simulations

Beam dynamics simulations in traveling wave (TW) accelerating structures with significant beam loading is a challenging problem. Some codes are capable of calculating the TW electromagnetic fields, and some can track particles through such fields, but most cannot treat both self-consistently. A few commercial codes can model the physics correctly at the expense of many processor-hour computations to obtain converged self-consistent solutions. However, simple, accurate equations of motion for intensive beam dynamics in TW accelerating structure analysis have been previously obtained by Masunov and subsequently implemented in the Hellweg code, which was developed at the Moscow Engineering-Physics Institute. Hellweg is based on equations that allow fast simulations of beam dynamics while taking into account such effects as beam loading, space charge, and external magnetic fields. In this paper, we describe in detail some recent improvements to the Hellweg physics kernel. We have generalized the Masunov results into a 3D set of equations of motion, which include all spatial components of the radiofrequency (RF) and external magnetic fields. We have also improved the Lapostolle space charge model to the general 3D ellipsoid form for any dimensions’ ratio, consideration for the particles outside the beam core, and the fields from the neighboring bunches that can exist in the real machine. These modifications allow approaching the Hellweg accuracy to the self-consistent commercial codes while keeping the simulation time short, which is essential during the linac design and optimization stage. The implementation of these new capabilities in Hellweg is carefully benchmarked against other codes and analytical calculations. The code is freely available with an open source license.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Crossed beam energy transfer in the presence of laser speckle ponderomotive self-focusing and nonlinear sound waves

Crossed beam energy transfer, CBET, is investigated by taking into account the speckle structure of smoothed laser beams that overlap in a plasma with an inhomogeneous flow profile. Using the two-dimensional simulation code Harmony, it is shown how ponderomotive self-focusing of laser speckles in crossing beams can significantly affect the transfer of energy from one beam to the other. The role of plasma flow in speckle self-focusing is investigated and revisited, in particular its consequences in terms of redirection and increasing angular spread of the laser beams due to beam bending and plasma-induced smoothing, respectively. In close-to-sonic flow, the onset of self-focusing in the beam speckle structure occurs at considerably lower beam intensities than expected for the case without flow. CBET and speckle self-focusing can, hence, occur together when two crossed beams with equal frequency resonantly exchange energy via their ponderomotively driven density perturbations flowing with sound speed. From the simulations, it is found that consequences of ponderomotive self-focusing can be expected above an average intensity threshold scaling as $I_L~ 2 × 10^{14} W cm^{-2}(λ_0/1 μm)^{-2}(T_e/ keV)$, with an impact on the spatial and temporal coherence of the transmitted light. The density perturbations due to the ponderomotive force of the crossing beams can locally be enhanced in self-focusing speckles, partly leading to shock-like structures. These structures eventually increase the effect of plasma-induced smoothing and are at the origin of the stronger angular spread.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Contact discontinuities in a cold collision-free two-beam plasma

The structure of contact discontinuities in a collision-free plasma is examined using a model of a plasma which consists of two oppositely directed cold ion beams and a background of cold massless electrons such that exact charge neutrality is maintained and that the electric field is zero. The basic equations describing self-consistent equilibria are obtained for the more general situation where a net flow across the layer takes place and where the magnetic field has two nonzero tangential components but where the electric field remains zero. These equations are then specialized to the case of no net plasma flow where one of the tangential components is zero, and four different classes of sheets are obtained, all having thickness the order of the ion inertial length. The first class is for layers separating two identical plasma and magnetic field regions, the second is for an infinite array of parallel layers producing an undulated magnetic field, the third is for layers containing trapped ions in closed orbits which separate two vacuum regions with uniform identical magnetic fields, and the fourth is for layers which reflect a single plasma beam, leaving a vacuum with a reversed and compressed tangential field on the other side.

Kirkland, K. B.↗

State and model error estimation for distributed parameter systems

In-flight estimation of large structure model errors in order to detect inevitable deficiencies in large structure controller/estimator models is discussed. Such an estimation process is particularly applicable in the area of shape control system design required to maintain a prescribed static structural shape and, in addition, suppress dynamic disturbances due to the vehicle vibrational modes. The paper outlines a solution to the problem of static shape estimation where the vehicle shape must be reconstructed from a set of measurements discretely located throughout the structure. The estimation process is based on the principle of least-squares that inherently contains the definition and explicit computation of model error estimates that are optimal in some sense. Consequently, a solution is provided for the problem of estimation of static model errors (e.g., external loads). A generalized formulation applicable to distributed parameters systems is first worked out and then applied to a one-dimensional beam-like structural configuration.

Rodriguez, G.↗

Metal DiSulfide thin films synthesized by pulsed ion beam ablation: Self-assembled structures with improved mechanical properties in humid conditions

Thin films composed of transition metal dichalcogenides such as molybdenum disulfide (MoS 2 ) or tungsten disulfide (WS 2 ) are well known for their solid lubricating behavior in dry environments such as space, but deteriorate rapidly in environments where oxygen is present. There have been many attempts over recent decades to improve MoS 2 lubricating performance in humid environments by addition of metals such as titanium to the film. The additions have come in the form of co-sputtering with the MoS 2 , or formation of nano multilayer coatings. We have previously reported on the synthesis of MoS 2 films by high-power ion beam ablation [Prasad et al, Matls. Lett. 65 (2010) 4–6]. The resulting films are observed to contain spheres of pure Mo of 10–100 nm size evenly dispersed throughout the ~1 μm-thick film, a form of self-assembly not before seen in films produced by sputtering or by pulsed laser deposition (PLD). The remaining Mosingle bondS matrix was observed to crystalize in situ under frictional contact into MoS 2 with the basal planes orienting themselves in the direction of sliding underneath the wear surface. The present study concerns metal additions in the form of alternating layers with MoS 2 deposited in between from an ablation target. The addition of Ti resulted in the extension of good tribological performance to humid air conditions, but the path to good performance appears to be relatively narrow. The same distributed Mo spheres were present in the new film, and similar self-assembled morphologies when V was substituted for the Ti, and when multilayers were formed of WS 2 with Zr additions. Furthermore, it appears that addition of Ti resulted in improvements in mechanical film strength that contributed to the wear ability in humid conditions.

Intense ion beams↗

Growth of PdCoO 2 films with controlled termination by molecular-beam epitaxy and determination of their electronic structure by angle-resolved photoemission spectroscopy

Utilizing the powerful combination of molecular-beam epitaxy (MBE) and angle-resolved photoemission spectroscopy (ARPES), we produce and study the effect of different terminating layers on the electronic structure of the metallic delafossite PdCoO 2 . Attempts to introduce unpaired electrons and synthesize new antiferromagnetic metals akin to the isostructural compound PdCrO 2 have been made by replacing cobalt with iron in PdCoO 2 films grown by MBE. Using ARPES, we observe similar bulk bands in these PdCoO 2 films with Pd-, CoO 2 -, and FeO 2 -termination. Nevertheless, Pd- and CoO 2 -terminated films show a reduced intensity of surface states. Additionally, we are able to epitaxially stabilize PdFe x Co 1– x O 2 films that show an anomaly in the derivative of the electrical resistance with respect to temperature at 20 K, but do not display pronounced magnetic order.

36 MATERIALS SCIENCE↗

Conversion of spectral characteristics of laser radiation in periodic domain structures written by the electron-beam method in planar waveguides formed by Ti diffusion in Y-oriented LiNbO{sub 3}

Periodic domain structures for nonlinear conversion of spectral characteristics of laser radiation in the planar Ti : LiNbO{sub 3} waveguide have been formed by the method of electron-beam writing. Domain gratings with a spatial period of 6.50 μm formed in the Y-cut plate over a wide range of accelerating voltages have been visualised by the method of second harmonic generation microscopy (SHG-microscopy) in transmitting geometry and at waveguide excitation. It is found that the domain structure written at an accelerating voltage of 10 kV in a waveguide with an exponential refractive index profile and an effective thickness of 1.75 μm is characterised by high homogeneity. It is composed of continuous domain rows and provides near-quasi-phase-matching radiation conversion at a wavelength of 1053 nm into the second harmonic for the TE{sub 0} → TE{sub 1} waveguide process. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Investigation of CrMnV and CrMnTiV multi principal element alloys thin films for use as exit windows of electron beam accelerators

Here, this study explores CrMnV and CrMnTiV multi principal element alloy (MPEA) films as candidates for electron beam exit windows in industrial, high-power accelerators. Films were deposited via magnetron sputtering on various substrates and exposed to 66 kGy of 10 MeV e-beam irradiation. Structural and mechanical properties were analyzed using FESEM, XRD, and nanoindentation. CrMnTiV films exhibited superior grain uniformity and hardness, regardless of the substrate type. Compared to bulk materials, both MPEA films demonstrated higher hardness and excellent radiation resistance. These results highlight the potential of MPEA films as durable, radiation-tolerant materials for high-performance accelerator exit window applications.

Electron Beam Irradiation↗

Exact analytical solution of shear-induced flexural vibration of functionally graded piezoelectric beam

The priority of this paper is to obtain the exact analytical solution for free flexural vibration of FGPM beam actuated using the d{sub 15} effect. In piezoelectric actuators, the potential use of d{sub 15} effect has been of particular interest for engineering applications since shear piezoelectric coefficient d15 is much higher than the other piezoelectric coupling constants d{sub 31} and d{sub 33}. The applications of shear actuators are to induce and control the flexural vibrations of beams and plates. In this study, a modified Timoshenko beam theory is used where electric potential is assumed to vary sinusoidaly along the thickness direction. The material properties are assumed to be graded across the thickness in accordance with power law distribution. Hamilton's principle is employed to obtain the equations of motion along with the associated boundary conditions for FGPM beams. Exact analytical solution is derived thus obtained equations of motion. Results for clamped-clamped and clamped-free boundary conditions are presented. The presented result and method shell serve as benchmark for comparing the results obtained from the other approximate methods.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Investigation of the Structural Stability of Ion-Implanted Gd 2 Ti 2-x Sn x O 7 Pyrochlore-Type Oxides by Glancing Angle X-ray Absorption Spectroscopy

Rare-earth titanate and stannate pyrochlore-type oxides have been investigated in the past for the sequestration of nuclear waste elements because of their resistance to radiation-induced structural damage. In order to enhance this property, it is necessary to understand the effect of radioactive decay of the incorporated actinide elements on the local chemical environment. In this study, Gd 2 Ti 2–x Sn x O 7 materials have been implanted with Au– ions to simulate radiation-induced structural damage. Glancing angle X-ray absorption near-edge spectroscopy (GA-XANES), glancing angle X-ray absorption fine structure (GA-EXAFS) analysis, and powder X-ray diffraction have been used to investigate changes in the local coordination environment of the metal atoms in the damaged surface layer. Examination of GA-XANES/EXAFS spectra from the implanted Gd 2 Ti 2–x Sn x O 7 materials collected at various glancing angles allowed for an investigation of how the local coordination environment around the absorbing atoms changed at different depths in the damaged surface layer. This study has shown the usefulness of GA-XANES to the examination of ion-implanted materials and has suggested that Gd 2 Ti 2–x Sn x O 7 becomes more susceptible to ion-beam-induced structural damage with increasing Sn concentration.

Aluri, Esther Rani↗

Heavy ion linear accelerator for radiation damage studies of materials

A new eXtreme MATerial (XMAT) research facility is being proposed at Argonne National Laboratory to enable rapid in situ mesoscale bulk analysis of ion radiation damage in advanced materials and nuclear fuels. This facility combines a new heavy-ion accelerator with the existing high-energy X-ray analysis capability of the Argonne Advanced Photon Source. The heavy-ion accelerator and target complex will enable experimenters to emulate the environment of a nuclear reactor making possible the study of fission fragment damage in materials. Material scientists will be able to use the measured material parameters to validate computer simulation codes and extrapolate the response of the material in a nuclear reactor environment. Utilizing a new heavy-ion accelerator will provide the appropriate energies and intensities to study these effects with beam intensities which allow experiments to run over hours or days instead of years. The XMAT facility will use a CW heavy-ion accelerator capable of providing beams of any stable isotope with adjustable energy up to 1.2 MeV/u for 238 U 50+ and 1.7 MeV for protons. This energy is crucial to the design since it well mimics fission fragments that provide the major portion of the damage in nuclear fuels. The energy also allows damage to be created far from the surface of the material allowing bulk radiation damage effects to be investigated. Furthermore, the XMAT ion linac includes an electron cyclotron resonance ion source, a normal-conducting radio-frequency quadrupole and four normal-conducting multi-gap quarter-wave resonators operating at 60.625 MHz. This paper presents the 3D multi-physics design and analysis of the accelerating structures and beam dynamics studies of the linac.

47 OTHER INSTRUMENTATION↗

Beam-swinging facilities for the Goonhilly satellite-communication aerial

The mode of satellite tracking adopted at the Goonhilly earth station is to steer the aerial primarily by means of predicted data computed from the satellite orbital parameters and to superimpose, during the passage of the satellite, corrections to remove any prediction errors or aberrations due the transmission path. Predictions have proved to be highly accurate for satellites having a high mass to projected area ratio orbiting at altitudes at which air drag is very small; hence the corrections are small and infrequent.

COMMUNICATIONS SATELLITE↗

Al and Ge simultaneous oxidation using neutral beam post-oxidation for formation of gate stack structures

To obtain a high-quality Germanium (Ge) metal–oxide–semiconductor structure, a Ge gate stacked structure was fabricated using neutral beam post-oxidation. After deposition of a 1-nm-thick Al metal film on a Ge substrate, simultaneous oxidation of Al and Ge was carried out at 300 °C, and a Ge oxide film with 29% GeO{sub 2} content was obtained by controlling the acceleration bias power of the neutral oxygen beam. In addition, the fabricated AlO{sub x}/GeO{sub x}/Ge structure achieved a low interface state density of less than 1 × 10{sup 11 }cm{sup −2 }eV{sup −1} near the midgap.

36 MATERIALS SCIENCE↗

Gas Electric Discharge with a Developed Streamer Structure in a Quasi-Optical Microwave Beam

Experiments on initiating an electrical discharge with a developed streamer structure in atmospheric pressure air are described. The discharge was initiated in a quasi-optical linearly polarized microwave beam with a subcritical field. Air breakdown was initiated by an electromagnetic vibrator placed in free space, on the surface of a dielectric plate, and on the outer or inner surface of a quartz tube. From experimental data, the velocity of the discharge front propagation toward the wavevector of the electromagnetic wave has been estimated.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Terahertz Chiral Metamaterials Enabling Broadband Polarization Conversion Using Polarization Guiding Effect

Polarization control plays a vital role in terahertz (THz) photonics, enabling a wide range of applications from imaging and spectroscopy to sensing and wireless communication. However, conventional polarization control methods at THz frequencies are limited by narrow operational bandwidths and excessive absorption losses. In this work, we present a broadband THz polarization control based on the polarization guiding effect. We design and fabricate a THz polarization rotator capable of rotating incident linear polarization by 90°. The device consists of 24 twistingly stacked silicon–air metagrating layers that introduce a large degree of form birefringence, with each metagrating layer being 280 µm thick and sequentially twisted by 3.75°. Numerical simulations using the Berreman 4 × 4 method predict broadband operation of the device. Experimental validation using THz time-domain spectroscopy confirms efficient and broadband 90° polarization rotation from 0.2 to 1.25 THz. Based on this concept, we further propose THz Q-plates for the generation of broadband structured vector beams with radial and azimuthal polarization states. This work offers a scalable, material-agnostic platform for advanced THz polarization manipulation and vector beam engineering, opening new pathways for next-generation THz photonic devices.

36 MATERIALS SCIENCE↗

Effect of X-ray beam on the molecular–topological structure of the surface of kynar® polyvinylidene fluoride resin

Thermomechanical analysis of poly(vinylidene fluoride) (PVDF) film shows that, unlike the completely amorphous structure of the native polymer, after irradiation with X-rays, the weight fraction of the crystalline modification in the polymer is 0.5. The initial PVDF film had a linear thermal expansion coefficient of α 1 = 11.33х10 5 K -1 and a glass transition temperature of T g =256 K. An efficient conversion of the amorphous structures of the polymer pseudo-network into crystalline networks occurs under X-ray irradiation. The irradiated polymer exhibits amorphous ( T g =239 K) and crystalline topological blocks ( T m =385 K). The presence of polyenyl and alkyl radicals is found in the electron paramagnetic resonance (EPR) spectra of the irradiated polymer. Lines with a splitting of 3.3 m T can be observed at the edges of the EPR spectra, consistent with radical centers like -CF 2 -C • H-CF 2 - . At high doses of radiolysis, polyenyl radicals are the main observed radicals. The macromolecular chains contain all three (α, β, γ) morphologies of the polymer. The Raman spectra show that X-ray irradiation can lead to carbonization and the formation of unsaturated bonds. Electronic structure calculations were used to aid in the analysis of the observed spectra.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

In-line three-dimensional holography of nanocrystalline objects at atomic resolution

We report that resolution and sensitivity of the latest generation aberration-corrected transmission electron microscopes allow the vast majority of single atoms to be imaged with sub-Ångstrom resolution and their locations determined in an image plane with a precision that exceeds the 1.9-pm wavelength of 300 kV electrons. Such unprecedented performance allows expansion of electron microscopic investigations with atomic resolution into the third dimension. Here we show a general tomographic method to recover the three-dimensional shape of a crystalline particle from high-resolution images of a single projection without the need for sample rotation. The method is compatible with low dose rate electron microscopy, which improves on signal quality, while minimizing electron beam-induced structure modifications even for small particles or surfaces. Lastly, we apply it to germanium, gold and magnesium oxide particles, and achieve a depth resolution of 1–2 Å, which is smaller than inter-atomic distances.

36 MATERIALS SCIENCE↗

Broadband polarization conversion with anisotropic plasmonic metasurfaces

Metasurfaces offer exciting opportunities that enable precise control of light propagation, optical intensity, phase and polarization. Plasmonic metasurface based quarter-wave plates have been recently studied to realize the conversion between linear polarization and circular polarization. However, it is still quite challenging to directly measure the birefringent phase retardation introduced by metasurface wave plates with a reliable technique. Here, we report a high-performance broadband metasurface quarter-wave plate made of anisotropic T-shaped plasmonic antennas in near-infrared wavelength range, where the achromatic nearly 90° transmitted phase retardation through the metasurface is precisely characterized with an optical vortex based interferometric approach. Based on the measured transmission amplitude and phase of two orthogonal linear polarization components, nearly unit degree of linear polarization is extracted from the Stokes parameters, indicating excellent broadband polarization conversion between linearly and circularly polarized light through the metasurface. Our results will be an important step forward in the advancement of integrated metasurface devices for polarization conversion and beam manipulation, structured light control, as well as new spectroscopic and interferometric techniques for metasurface characterization.

Science & Technology - Other Topics↗