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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

A probabilistic inverse prediction method for predicting plutonium processing conditions

In the past decade, nuclear chemists and physicists have been conducting studies to investigate the signatures associated with the production of special nuclear material (SNM). In particular, these studies aim to determine how various processing parameters impact the physical, chemical, and morphological properties of the resulting special nuclear material. By better understanding how these properties relate to the processing parameters, scientists can better contribute to nuclear forensics investigations by quantifying their results and ultimately shortening the forensic timeline. This paper aims to statistically analyze and quantify the relationships that exist between the processing conditions used in these experiments and the various properties of the nuclear end-product by invoking inverse methods. In particular, these methods make use of Bayesian Adaptive Spline Surface models in conjunction with Bayesian model calibration techniques to probabilistically determine processing conditions as an inverse function of morphological characteristics. Not only does the model presented in this paper allow for providing point estimates of a sample of special nuclear material, but it also incorporates uncertainty into these predictions. This model proves sufficient for predicting processing conditions within a standard deviation of the observed processing conditions, on average, provides a solid foundation for future work in predicting processing conditions of particles of special nuclear material using only their observed morphological characteristics, and is generalizable to the field of chemometrics for applicability across different materials.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2022

Origin of Plutonium-244 in the Early Solar System

We investigate the origin in the early Solar System of the short-lived radionuclide 244 Pu (with a half life of 80 Myr) produced by the rapid (r) neutron-capture process. We consider two large sets of r-process nucleosynthesis models and analyse if the origin of 244 Pu in the ESS is consistent with that of the other r and slow (s) neutron-capture process radioactive nuclei. Uncertainties on the r-process models come from both the nuclear physics input and the astrophysical site. The former strongly affects the ratios of isotopes of close mass ( 129 I/ 127 I, 244 Pu/ 238 U, and 247 Pu/ 235 U). The 129 I/ 247 Cm ratio, instead, which involves isotopes of a very different mass, is much more variable than those listed above and is more affected by the physics of the astrophysical site. We consider possible scenarios for the evolution of the abundances of these radioactive nuclei in the galactic interstellar medium and verify under which scenarios and conditions solutions can be found for the origin of 244 Pu that are consistent with the origin of the other isotopes. Solutions are generally found for all the possible different regimes controlled by the interval (δ) between additions from the source to the parcel of interstellar medium gas that ended up in the Solar System, relative to decay timescales. If r-process ejecta in interstellar medium are mixed within a relatively small area (leading to a long δ), we derive that the last event that explains the 129 I and 247 Cm abundances in the early Solar System can also account for the abundance of 244 Pu. Due to its longer half life, however, 244 Pu may have originated from a few events instead of one only. If r-process ejecta in interstellar medium are mixed within a relatively large area (leading to a short δ), we derive that the time elapsed from the formation of the molecular cloud to the formation of the Sun was 9-16 Myr.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS2021

Microsphere Plutonium-238 Oxide Fuel to Revolutionize New Radioisotope Power Systems and Heat Sources for Planetary Exploration

Microsphere 238PuO2 fuels have potential to provide performance and safety enhancements for future radioisotope heat and power systems (RPS) as well as enable more flexible and compact RPS designs. Improvements in RPS specific power and more flexible geometries were recently investigated by JPL and PNNL as part of a study on cryobot devices for exploring Ocean Worlds. Missions to penetrate ice and explore oceans, such as on Europa, will require RPS with high specific power within the vehicle to provide both heat and power. Such missions will be mass-constrained, and the energy required to penetrate the ice is highly dependent on cryobot size. Therefore, compact RPS geometries are needed to maximize heat and power while minimizing 238Pu inventory. Microsphere-based heat sources are an attractive way to obtain flexible geometries and high volumetric power loadings because they can fill a region of any size and shape provided fuel temperatures are kept below a threshold and launch/re-entry safety are not compromised. The sol-gel technique to produce 238PuO2 microsphere particles for heat sources has the benefit of preventing dust generation, as opposed to the current 238PuO2 powder/pellet processing method, reducing hazards in the fuel fabrication line. Microspheres can also be individually coated to enhance thermal conductivity, and/or reduce the likelihood of 238PuO2 fuel dispersal in an accident. Although PNNL has produced 238PuO2 microspheres using the sol-gel method, the application of coatings and their integrity over time has yet to be investigated. Continued R&D could demonstrate the feasibility of advanced, microspherebased heat sources and provide baseline data for planning future missions requiring new RPS with different heat source configurations.

Fleurial, Jean-Pierre↗