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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
NASA NTRS1986

Benchmark full configuration-interaction calculations on H2O, F, and

Full configuration-interaction calculations are reported, and compared to other methods, for H2O at its equilibrium geometry and at two geometries with the H-O bonds stretched. Since the percentage of the self-consistent field (SCF) reference in the full configuration-interaction (FCI) wave function decreases greatly with the bond elongation, the accuracy of techniques based on a single reference do not compare well with the FCI results. However, the results from a complete active space SCF/multireference configuration-interaction (CASSCF/MRCI) treatment are in good agreement with the FCI. Correlation effects in F compared to Ne are far more similar than for Fcompared to Ne, despite F- and Ne being isoelectronic. Since the importance of higher than double excitations is more important for F- than F, a very high percentage of the correlation must be obtained to accurately compute the electron affinity. In a CASSCF/MRCI treatment the higher than quadruple excitations contribute 0.02 eV to the electron affinity (EA), even for modest basis sets.

Bauschlicher, C. W., Jr.↗
NASA NTRS1987

Cosmic-ray-produced neon and helium in the summit lavas of Maui

The identification of cosmic-ray-produced Ne-21c in addition to He-3c, components attributed to cosmic ray-induced spallation reactions, are reported in gases extracted by fusion of olivines and clinopyroxenes after vacuum-crushing. The observed (He-3/Ne-21)c ratios and the ratio of Ne-21c in olivine to that in clinopyroxene are consistent with an in situ origin of He-3c and Ne-21c by cosmic-ray spallation reactions. These components could be important for interpreting helium isotopic data in terrestrial reservoirs. Geophysical applications could include determinations of erosion rates and exposure histories of terrestrial rocks.

Marti, K.↗
NASA NTRS1987

Collapse of 9 solar mass stars

General relativistic hydrodynamical calculations of the collapse of O + Ne + Mg cores of a 9 solar mass star are reported. Collapse is induced by rapid electron captures as the O + Ne + Mg is burned to nuclear statistical equilibrium. The high entropy in the core after burning leads to a large abundance of free protons which readily capture electrons. This leads to large neutrino losses and a correspondingly small infalling homologous core. The hydrodynamic shock thus forms at a small mass point. The shock stalls before reaching the edge of the O + Ne + Mg core and thereby fails to produce a successful supernova explosion by the direct mechanism. No enhancement in the shock energy due to nuclear burning is found.

Baron, E.↗
NASA NTRS1988

Spectroscopic observations of the high-ionization planetary nebula NGC 2242 and the H II region K4-45

New optical spectra of two suspected planetary nebulae, K4-45 and NGC 2242, are presented. It is shown that K4-45 (PK 96 + 1) is a reddened H II region with approximately solar abundances, excited by an early B type star. NGC 2242 (PK 170 + 15) is a planetary nebula of exceptionally high ionization, exhibiting He II, and forbidden Ne V, Ar V, Ne III, and O III emission lines. The lack of He I emission and the presence of strong forbidden Ne V and He II emission indicate an optically thin nebula that is ionized by a central star with an effective temperature greater than 100,000 K.

Garnett, Donald R.↗
NASA NTRS1988

Interstellar silicon carbide - How much older than the solar system?

The SiC grains in C2 chondrites have large isotopic anomalies in Si, C, N, Ne, and Xe, and thus are virtually undegraded interstellar matter that survived formation of the solar system. They also contain excess Ne-21, of which only a minor part can have formed during the recent, 1 Myr cosmic-ray exposure of the meteorite. If the excess Ne-21 is cosmogenic, then the presolar exposure age of the SiC is 41 + 20 or - 14 Myr. This age is surprisingly short compared to the predicted lifetime of refractory interstellar grains, 500-1000 Myr. Possible explanations are: (1) the predicted grain lifetime is wrong, (2) the age of SiC has been falsified by neon losses, or (3) the solar system formed in part from atypically young material.

Ming, Tang↗
NASA NTRS1989

Seasonal variability in global sea level observed with Geosat altimetry

Time changes in global mesoscale sea level variances were observed with satellite altimetry between November 1986 and March 1988, showing significant, geographically coherent seasonal patterns. The NE Pacific and NE Atlantic variances show the most reliable patterns, higher than their yearly averages in both the fall and winter. The response to wind forcing appears as the major contributor to the NE Pacific and Atlantic signals; errors in the estimated inverse barometer response due to errors in atmospheric pressure, residual orbit errors, and errors in sea state bias are evaluated and found to be negligible contributors to this particular signal. The equatorial regions also show significant seasonal patterns, but the uncertainties in the wet tropospheric correction prevent definitive conclusions. The western boundary current changes are very large but not statistically significant. Estimates of the regression coefficient between sea level and significant wave height, an estimate of the sea state bias correction, range between 2.3 and 2.9 percent and vary with the type of orbit correction applied.

Zlotnicki, V.↗
NASA NTRS1990

Low Be-10 and Al-26 contents of ureilites - Production at meteoroid surfaces

The Be-10 contents of 22 ureilites and the Al-26 contents of 18 ureilites are reported. When corrected for exposure age, where known, and for composition, the results give production rate, P that are on average 20 percent lower than values typical of other meteorite classes. This depression of production rates, the weak correlations of both P26 and P10 with Ne-22/Ne-21 and the generally high He-3/Ne-21 and Ne-22/Ne-21 ratios in urelities all suggest that many of the samples occupied near-surface locations in their parent meteoroids. A reduced flux of cosmic rays does not by itself explain the elevated Ne-22/Ne-21 ratios and appears inconsistent with a proposed source for ureilites in the inner asteroid belt. Cosmogenic radionuclide data do not support the tentative pairing of ALHA 78019 with ALHa 78262 proposed on the basis of mineralogical similarities. The high Al-26 content of LEW 85440 may be the result of irradiation by solar cosmic rays.

Aylmer, D.↗
NASA NTRS1990

Charge exchange of low-energy ions in thin carbon foils

In order to calibrate a time-of-flight mass spectrometer which is to be flown in the solar wind, the charge exchange properties of low-energy ions in thin carbon foils have been investigated. Incident ions of He, C, N, O, Ne, and Ar with energies in the range 0.5-2 keV/nucleon have been used to measure charge-state distribution, residual energy, and angular distribution after transmission through thin (1-6 microgram/sq cm) carbon foils. Within such foils, an equilibrium between ionization and recombination of the projectile is rapidly established, and, consequently, the charge state of the emerging particle depends essentially on its residual velocity. A comparison of the charge exchange properties of Ne-22 with Ne-20 demonstrates that indeed the velocity (and not the energy) of the emerging particle determines its final charge. A comparison of properties of different elements provides an indication of an electron shell effect. Predictions for the energy loss of ions within the carbon foils made with the TRIM code are in good agreement with the experimental results presented in this paper.

Buergi, Alfred↗
NASA NTRS1990

The molecular spiral arms of NGC 6946

From CO-12(J=1 to 0) observations at 45 seconds resolution Tacconi and Young (1989) have found evidence for enhancements in both the CO emissivity and the massive star formation efficiency (MSFE) on optical spiral arms of the bright spiral galaxy NGC 6946. In the optically luminous and well-defined spiral arm in the NE quadrant, there are enhancements in both the H2 surface density and MSFE relative to the interarm regions. In contrast, a poorly defined arm in the SW shows no arm-interarm contrast in the MSFE. To further investigate the molecular gas content of these two spiral arms, researchers have made CO-12 J=2 to 1 and 3 to 2 observations with the James Clerk Maxwell Telescope. In the J=2 to 1 line, they made observations of the NE and SW spiral arm and interarm regions in 4 x 9 10 seconds spaced grids (36 points per grid). Because of decreased sensitivity in the J=3 to 2 line, they were limited to mapping the two arm regions in 2 x 3 10 seconds spaced grids (6 points per grid). The centers of each of the grids lie 2.4 minutes to the NE and 2.3 minutes to the SW of the nucleus of NGC 6946. With the CO J=2 to 1 data researchers are able to fully resolve the two observed spiral arms in NGC 6946. In both cases the CO emission is largely confined to the optical spiral arm regions with the peak observed T asterisk sub A being up to 4 times higher on the spiral arms than in the interarm regions. Researchers are currently estimating massive star formation efficiencies on and off the spiral arms through direct comparison of the CO maps with an H alpha image. They are also comparing the CO J=2 to 1 data with an HI map made at similar resolution. Thus, they will be able to determine structure in all components of the IS on scales of less than 20 inches.

Tacconi, L. J.↗
NASA NTRS1992

The interstellar gas experiment: Analysis in progress

The interstellar gas experiment (IGE) exposed thin metallic foils in order to collect neutral interstellar particles which penetrate the solar system due to their motion relative to the sun. These atoms were entrapped in the collecting foils along with precipitating magnetospheric ions and with ambient atmospheric atoms. For the entire duration of the LDEF mission, seven of the foils collected particles arriving from seven different directions as seen from the spacecraft. In the mass spectrometric analysis of the trapped noble gas component, we detected the He-3, He-4, Ne-20, and Ne-22 isotopes. In order to infer the isotopic ratios in the interstellar medium from the measured concentrations found in the foil piece, several lines of investigation had to be initiated. The flux of incident noble gas atoms from the ambient atmosphere was estimated by detailed calculations. The contributions proved to be negligible, supporting the experimental evidence. Foil and machine backgrounds for the four isotopes which were measured had to be assessed individually. While this was easy for He-4, spurious foil background of He-3 had to be monitored carefully by analyzing unflown foil pieces. Trapped Ne concentrations are not far above the background. During the flight, a stuck electrical relay precluded the foil-trays from sequencing as designed. Therefore, we could not use the seasonal variation of the direction of the incoming interstellar atoms to make the distinction between interstellar and magnetospheric components of the trapped particles. Instead, we had to try the method of stepwise heating to extract the interstellar component at lower temperatures than we use to extract the magnetospheric component (the interstellars hit the foil with lower energies than most of the magnetospherics). New limiting values for the isotopic composition of the interstellar medium, unavailable yet from any other method of measurement, are emerging from this analysis.

Buehler, F.↗
NASA NTRS1991

Composition of solar flare noble gases preserved in meteorite parent body regolith

Isotopic composition of solar-flare (SF) Ne was determined in acid-etched pyroxene mineral separates from the Kapoeta meteorite, a brecciated meteorite known to contain implanted solar gases. The results yield the SF Ne-20/Ne-22 ratio of 11.6 +/-0.2, confirming previous determinations of this SF ratio in lunar and meteoritic samples. The same SF Ne composition was also obtained by applying an ordinate intercept technique to the same data set. The ordinate intercept technique was then applied to the Ar and He data. The results are SF Ar-36/Ar-38 = 4.9 +/-0.1 and SF He-4/He-3 = 3800 +/-200. These values are significantly different from the solar-wind (SW) Ar and He values. It is estimated that the concentration of the SF component in Kapoeta pyroxenes is about 20 percent that of the SW component, orders of magnitude higher than expected from SW and SF proton flux measurements.

Rao, M. N.↗
NASA NTRS1991

Element abundances in solar (He-3) rich events

The results of a survey of over 228 (He-3)-rich events, with He-3/H-4 of more than 0.1, observed by the ISEE-3 spacecraft from 1978 August through 1991 April. In these events the elements above C are enhanced relative to the corresponding abundances in the corona and the degree of enhancement increases with Z or A. The flare-to-flare variations in abundances are different in character from those seen in large proton events. For example, using Fe/C as a parameter to describe these variations, the slope of the least-squares fits to ln(X/C) vs ln(Fe/C), where X is the intensity of N, O, Ne, Mg, Si, or S. Slopes of these abundance-correlation lines are much steeper for the (He-3)-rich events than for a sample of 36 large proton events, especially for Ne and heavier ions. The event-to-event variations for the (He-3)-rich events distinguish 3 groups of elements, He-O, Ne-S, and Fe. The abundances of all of the species within each group seem to vary in unison.

Reames, D. V.↗
NASA NTRS1993

Classical novae - Contributions to the interstellar medium

Theoretical results predicting yields of various isotopes in nova outbursts are reviewed. Emphasis is placed on the stardust and gas-phase chemical anomalies that may be contributed to the Galactic ISM by classic novae. It is concluded that most of the heavy isotope anomalies are produced by about 25 percent of novae that occur in systems containing massive O-Ne-Mg white dwarfs. The dust-production scenario for novae is summarized, and it is argued that explosions on O-Ne-Mg white dwarfs may lead to the formation of dust grains that carry the Ne-E and Mg-26 anomalies. Quantitative constraints are placed on the degree to which classical novae participate in the production of chemical anomalies, both in the primitive solar system and on a Galactic scale.

Gehrz, Robert D.↗
NASA NTRS1993

Yana ring structure, North-Eastern Siberia: A possible counterpart of coronae on Venus

An arch of Verkhoyansky Range in NE Siberia, Russia is considered as W and S parts of the rim of the large ring structure, referred hereafter as Yana Ring Structure (YRS). It has general appearance similar to coronae on Venus and could be considered as the terrestrial counter part of coronae. The structure is located between 63 and 70 deg N, 125 and 140 deg E. The outer diameter of YRS (between the rim feet) is 680-700 km. The rim crest diameter is 500-520 km. The inner diameters (between the inner feet of the rim) is 320-350 km. The rim of YRS consist of the following topographic features: W segment is Orulgan Range (N part of Verkhoyansky Range), SW and S segments consist of S part of Verkhoyansky Range, SE segment is Elginskoye Ploskogorye (Tableland), E segment is Chersky Range (its part W of Indigirka River), NE segment is Selennyakhsky Range, and NW segment is Kular Range. Inside this ring of mountains Yanskoye Ploskogorye (Tableland) is located. The circular outlines of YRS are marked with the large river valleys located outside: Lena River (lower of Aldan River mouth) is located W from YRS, Aldan River (lower of Amga River mouth) is from S, Indigirka River (between 64 and 67 deg N lat) is from E, and Selennyakh River (the part running N to S) is from NE. The ring patterns inside the mountaineous rim of YRS are marked with the tributaries of Yana River. The largest ring here, 300 km in diameter, consists of Bytangay (with Bellyakh) River at W, Nelgese and Derbeke Rivers at S/SE, and Tuostakh River at E. The typical altitudes of YRS mountain rim are 1000-2000 m. The maximal ones are: 2400 m in W part of the rim, 2300 m in S, 1600 m in SE, 2200-2500 m in E, and 1300-1500 m in N. The central part of YRS have typical altitudes of 400-600 m. There are lowlands with altitudes 50-200 m to the S, W, N, and NW outside YRS Oymyakonskoye Nagorye (Highland) is located SE of YRS at 500-1500 m altitudes. It should be recognized from this description YRS have a general appearance of circular highland with its central plateau located 1000-2000 m lower than surrounding mountain rim, but 300-400 m higher than plains of lowlands located outside the rim. Such topographic patterns are typical for coronae on Venus. The diameter of YRS is equal to the largest coronae on Venus. There are only 3 or 4 structures of such or larger size on the whole Venus. This calls to compare morphology and geologic evolution of YRS with morphology and models of coronae evolutions especially the largest ones, to search the similarities and/or differences in geologic histories of the structures on the Earth and Venus.

Burba, G. A.↗
NASA NTRS1993

Exposure ages of carbonaceous chondrites, 1

The recent exposure histories of carbonaceous chondrites have been investigated using cosmogenic radionuclides. Our results may indicate a clustering of exposure ages of C1 and C2 chondrites into two peaks, 0.2 My and 0.6 My, perhaps implying two collisional events of Earth-crossing parent bodies. Among carbonaceous chondrites are some having short exposure ages which Mazor et al. hypothesized cluster into a small number of families. This hypothesis is based on spallogenic Ne-21 exposure ages, which in some instances are difficult to determine owing to the large amounts of trapped noble gases in carbonaceous chondrites. Also, since Ne-21 is stable, it integrates a sample's entire exposure history, so meteorites with complex exposure histories are difficult to understand using exclusively Ne-21. Cosmogenic radionuclides provide an alternative means of determining the recent cosmic ray exposure duration. To test the hypothesis of Mazor et al. we have begun a systematic investigation of exposure histories of Antarctic and non-Antarctic carbonaceous chondrites especially C2s.

Nishiizumi, K.↗
NASA NTRS1993

A long-term change of the AR/KR/XE fractionation in the solar corpuscular radiation

Solar noble gases in an ilmenite separate from breccia 79035 (antiquity greater than 1 Ga) were analyzed by closed system stepped etching (CSSE). All five gases show the familiar two-component structure: first solar-wind (SW) gases are released, followed by gases from solar energetic particles (SEP). Element patterns in 79035 are similar to those of 71501 ilmenite. SW-He-Ne were partly lost, but SEP-He-Ne-Ar are retained (nearly) unfractionated. Constant Ar/Kr/Xe ratios indicate that ilmenites contain an unfractionated sample of the heavy SW-SEP noble gases. Ar/Kr/Xe ratios in the solar corpuscular radiation are, however, different from 'solar system' values, whereby the Kr/Xe difference in 79035 is about twice as large as in 71501. We propose that Xe is less fractionated than Kr and Ar, though its first ionization potential (FIP) is higher than the 'cutoff' at approximately 11.5 eV, above which all elements in SEP are usually assumed to be depleted by a roughly constant factor. SW-Ne may be isotopically slightly heavier in the ancient SW trapped by 79035, as proposed earlier. In this work we extend our previous CSSE studies of solar noble gases including Kr and Xe to a lunar sample irradiated at least 1 Ga ago (breccia 79035, ilmenite separate, 42-64 microns). This sample was particularly gently etched in the first steps. Surprisingly, the first three steps, each releasing less than or equal to 0.5% of the total 36-Ar, showed an SEP-like trapped component plus relatively large concentrations of cosmogenic gases. Steps 4ff contain much less cosmogenic and more solar gas with a SW-like isotope pattern. Thus, a very minor easily etchable phase that has completely lost its SW-gases must be responsible for steps 1-3. We will not discuss these steps here and refer to the actual step 4 as the 'initial' etching step.

Wieler, R.↗
NASA NTRS1993

New evidence for geomagnetically trapped anomalous cosmic rays

We report new observations of 15 MeV/nuc or greater trapped heavy ions with Z equal to or greater than 2, made on the polar-orbiting SAMPEX spacecraft in late 1992 and early 1993. A trapped population that includes He, N, O, and Ne is found to be located at L = 2. We conclude that the observed N, O, and Ne ions are 'anomalous' cosmic rays, trapped by the mechanism proposed by Blake and Friesen (1977). While it is not expected that this mechanism would also trap anomalous He, the characteristics of the trapped He population are generally consistent with those of N, O, and Ne.

Cummings, J. R.↗
NASA NTRS1994

Investigation of a laboratory candidate for the carrier of the 4430 A diffuse interstellar band

The 4430 A diffuse interstellar band (DIB) is unique among DIB's in that as one of the strong bands, it is the bluest strong band with no others observed at shorter wavelengths. This position at the edge of the DIF 'forrest' suggests it may be the easiest to replicate in the laboratory. In earlier experiments (Wdowiak 1980) an interesting candidate using a gas discharge followed by cryogenic matrix isolation was produced, and this report details its further investigation. This absorption feature, produced when 1 part CH4 in 200 parts Ar is discharged and frozen out approximately 10 K, is at a wavelength of 4500 A in the argon matrix. Our recent experiments strongly indicate it is due to a carbon-based reactive species that is stable against mercury vapor UV radiation, and not likely to be from a contaminant. The effect of matrix shift can be estimated by considering the blueward shift between Ar and Ne matrices in the cases of the pyrene and C60 cations. This suggests that a shift from 4500 A for an Af matrix to the vicinity of 4300 A for a Ne matrix and the gas phase is not unreasonable. A liquid He cooled Ne matrix isolation experiment was prepared to determine the wavelength of the feature in that matrix. Replacing CH4 with C2H2 results in an equivalent absorption due to C3, greatly diminished absorptions from C2 and Ch, and no observable feature at 4500 A. To date our experiments indicate CH4 is a favored precursor for production of the reactive carrier of the 4500 A feature. Perhaps C2H2 is not suitable because of its tendency to polymerize easily in the discharge.

Wdowiak, Thomas J.↗