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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
NASA NTRS1980

Limits on the possible intrinsic magnetic field of Venus

Magnetic field measurements obtained by the Pioneer Venus orbiter at low altitudes in the solar wind wake region are examined for possible surface-correlated features and any possible intrinsic magnetic moment. The field variations observed in the wake do not resemble those expected for a solar wind interaction with even a weak intrinsic magnetic field. Little orbit-to-orbit persistence of features is found in the magnetic records. The magnetic field measurements in the wake are averaged in 10 deg x 10 deg bins to minimize the effects of external field sources. In these 37 bins, the average fields appear to be randomly oriented and consistent with zero mean in the region mapped. Using these 37 averaged vector fields, a maximum intrinsic magnetic dipole moment is obtained of 4.3 + or - 2.0 x 10 to the 21st G cu cm, approximately an order of magnitude less than previous estimates. It is noted that a more conservative estimate of the probable error of the mean is 5.5 x 10 to the 21st G cu cm. The Pioneer Venus measurements are thus consistent with zero planetary moment. The present measurements are found to be far below estimates made on the basis of angular momentum, the so-called magnetic Bode's law, and far below the dynamo scaling law of Busse.

Russell, C. T.↗
NASA NTRS1972

UK-4 flight spacecraft magnetic tests

Magnetic tests conducted on the UK-4 spacecraft are discussed. The objectives of the test are: (1) to determine the permanent, induced, and stray magnetic moments of the spacecraft, (2) to assess its magnetic stability, (3) to determine the dipole moment produced by energizing the magnetorquer coil, (4) to measure the despin torque due to eddy current and magnetic hysteresis, and (5) to deperm, compensate, and make other adjustments necessary to achieve satisfactory magnetic characteristics for the spacecraft.

Pruett, W. E.↗
DOE OSTI2025

Impact of dynamic Jahn-Teller effect on magnetic excitations, lattice vibration, and thermal conductivity in U 𝑥 ⁢T⁢h 1−𝑥 ⁡O 2 system

Vibrational and magnetic properties of single-crystal uranium-thorium dioxide (U 𝑥 ⁢T⁢h 1−𝑥⁡ O 2 ) with a full range of 0 < 𝑥 < 1 are investigated. Thorium dioxide is a diamagnet whose thermal properties are governed by lattice vibration. The addition of paramagnetic uranium ions leads to the emergence of magnetic effects that alter the thermophysical properties noticeably even at room temperature. The interaction of phonons with magnetic moments of uranium 5⁢𝑓 electrons mediated by magnetoelastic coupling results in an anomalous low-temperature thermal conductivity profile. Analysis of the magnetic susceptibility measurements indicates a departure from the Curie-Weiss relationship characteristic of noninteracting paramagnetic ions, previously associated with the dynamic Jahn-Teller (DJT) effect characterized by coupling between spin and the oxygen sublattice. The T 2⁢g Raman peak position follows a nonlinear trend as a function of uranium concentration and hints that these Raman active optical modes play a role in either DJT or in mediating quadrupole-quadrupole interactions. A first-principle-based thermal transport model is implemented to explain the low-temperature transport measurements, where the anomalous reduction is attributed to phonon-spin resonant scattering. The interplay between spins and phonons is also captured using high-resolution inelastic x-ray scattering (IXS) measurements of phonon linewidths. Our results provide insights into the phonon interactions with the magnetic excitations governing DJT effect and impacting the low-temperature thermal transport processes in this material system. Furthermore, these findings have implications for understanding low-temperature thermal transport and magnetic properties in advanced materials for information processing and energy applications.

36 - MATERIALS SCIENCE↗
DOE OSTI2022

Evidence of dynamical effects and critical field in a cobalt spin crossover complex

The [Co(SQ) 2 (4-CN-py) 2 ] complex exhibits dynamical effects over a wide range of temperature. Additionally, the orbital moment, determined by X-ray magnetic circular dichroism (XMCD) with decreasing applied magnetic field, indicates a nonzero critical field for net alignment of magnetic moments, an effect not seen with the spin moment of [Co(SQ) 2 (4-CN-py) 2 ].

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Localized spin-orbit polaron in magnetic Weyl semimetal Co 3 Sn 2 S 2

The kagome lattice Co 3 Sn 2 S 2 exhibits the quintessential topological phenomena of a magnetic Weyl semimetal such as the chiral anomaly and Fermi-arc surface states. Probing its magnetic properties is crucial for understanding this correlated topological state. Here, using spin-polarized scanning tunneling microscopy/spectroscopy (STM/S) and non-contact atomic force microscopy (nc-AFM) combined with first-principle calculations, we report the discovery of localized spin-orbit polarons (SOPs) with three-fold rotation symmetry nucleated around single S-vacancies in Co 3 Sn 2 S 2. The SOPs carry a magnetic moment and a large diamagnetic orbital magnetization of a possible topological origin associated relating to the diamagnetic circulating current around the S-vacancy. Appreciable magneto-elastic coupling of the SOP is detected by nc-AFM and STM. Our findings suggest that the SOPs can enhance magnetism and more robust time-reversal-symmetry-breaking topological phenomena. Controlled engineering of the SOPs may pave the way toward practical applications in functional quantum devices.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Electronic and vibrational properties of bulk Cr 2 Ge 2 Te 6 from first-principles calculations

Here we use density functional theory based ab initio calculations to investigate the structural, vibrational, magnetic, and electronic properties of the layered ferromagnet Cr 2 Ge 2 Te 6 (CGT) that has attracted attention for potential spintronic applications. We optimize the structure for a fixed c/a ratio. Our results are in excellent agreement with experimental data on structure, phonons, and electronic properties. The use of van der Waals interactions and relativistic spin-orbit coupling yields accurate lattice constants and interlayer distances. Simultaneously, the adopted theoretical methods lead to a rigorous description of the vibrational normal modes, as well as the valence bands, that are in excellent agreement with Raman spectroscopy and angle-resolved photoemission spectroscopy spectra, respectively. The magnetic moment is slightly overestimated, and the magnetic anisotropy has the correct sign but is greater in magnitude than that in experiment. We find that inclusion of the on-site Coulomb repulsion on Cr−3d orbitals worsens agreement with experiment, in contrast to previous studies. Our results provide a path toward ab initio analysis of magnetic heterostructures based on CGT.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Global polarization of Λ and $\overline{Λ}$ hyperons in Au + Au collisions at $\sqrt{s_{NN}}$ = 19.6 and 27 GeV

In relativistic heavy-ion collisions, a global spin polarization, 𝑃 H , of Λ and $\overline{Λ}$ hyperons along the direction of the system angular momentum was discovered and measured across a broad range of collision energies and demonstrated a trend of increasing 𝑃 H with decreasing $\sqrt{s_{NN}}$. A splitting between Λ and $\overline{Λ}$ polarization may be possible due to their different magnetic moments in a late-stage magnetic field sustained by the quark-gluon plasma which is formed in the collision. The results presented in this study find no significant splitting at the collision energies of $\sqrt{s_{NN}}$ = 19.6 and 27 GeV in the BNL Relativistic Heavy Ion Collisions Beam Energy Scan Phase II using the STAR detector, with an upper limit of 𝑃 $\overline{Λ}$ – 𝑃 Λ < 0.24% and 𝑃 $\overline{Λ}$ – 𝑃 Λ < 0.35%, respectively, at a 95% confidence level. We derive an upper limit on the naive extraction of the late-stage magnetic field of 𝐵 < 9.4 × 10 12 T and 𝐵 < 1.4 × 10 13 T at $\sqrt{s_{NN}}$ = 19.6 and 27 GeV, respectively, although more thorough derivations are needed. Differential measurements of 𝑃 H were performed with respect to collision centrality, transverse momentum, and rapidity. With our current acceptance of |𝑦| < 1 and uncertainties, we observe no dependence on transverse momentum and rapidity in this analysis. Furthermore, these results challenge multiple existing model calculations following a variety of different assumptions which have each predicted a strong dependence on rapidity in this collision-energy range.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Tunable magnetic excitations in the honeycomb antiferromagnet (Co,Ni)⁢TiO3

The solid solution of the honeycomb antiferromagnet (AFM) Co0.5⁢Ni0.5⁢TiO3 (CNTO) was synthesized by mixing a 1:1 molar ratio of CoTiO3 (CTO) and NiTiO3 (NTO). Powder neutron scattering was used to determine the structure and magnetic spectrum, where the nuclear and magnetic structures resemble those of the end members. The Néel temperature (T𝑁 = 27 ± 1 K), the ordered magnetic moment (M = 2.29 ± 0.03 𝜇𝐵 per magnetic ion), and lattice parameters are intermediate between those of the two. From inelastic neutron scattering, it is observed that the magnon density of states (MDOS) extends up to 13 meV, and the interaction can be described by an XXZ-type magnetic Hamiltonian. Above 15 meV, spin-orbit excitons (SOEs) are observed similarly to those in CTO, but with modified spin-orbit crystal-field splitting because of the substitution of Ni at Co sites, and the disorder induced by the Ni substitution modifies the spin-orbit crystal field. Thus, the magnetic dynamics of the CNTO cannot be described as a simple average of the two parent compounds.

Rathnayaka, Srimal [University of Virginia, Charlo↗
DOE OSTI2022

Oxygen Deficiency and Migration-Mediated Electric Polarization in Magnetic Fe,Co-Substituted SrTiO3−δ

We use density functional theory (DFT) calculations to show that oxygen vacancies (vO) and mobility induce noncentrosymmetric polar structures in SrTi1−x−yFexCoyO3−δ (STFC, x=y=0.125) with δ={0.125,0.25}, enhance the saturation magnetization, and give rise to large changes in the electric polarization |ΔP|. We present an intuitive set of rules to describe the properties of STFC, which are based on the interplay between (Co/Fe)-vO defects, magnetic cation coordination, and topological vacancy disorder. STFC structures consist of layered crystals with sheets of linearly organized O4,5,6-coordinated Fe–Co pairs, sandwiched with layers of O5-coordinated Ti. (Co/Fe)-vO defects are the source of crystal distortions, cation off-centering and bending of the oxygen octahedra which, considering the charge redistribution mediated by vO and the cations’ electronegativity and valence states, triggers an effective electric polarization. Oxygen migration for δ=0.125 leads to |ΔP|>∼10 µC/cm2 due to quantum-of-polarization differences between δ=0.125 structures. Increasing the oxygen deficiency to δ=0.25 yields |ΔP|, the O migration of which resolved polarization for δ=0.25 is >∼3 µC/cm2. Magnetism is dominated by the Fe,Co spin states for δ=0.125, and there is a contribution from Ti magnetic moments (∼1 μB) for δ=0.25. Magnetic and electric order parameters change for variations of δ or oxygen migration for a given oxygen deficiency. Our results capture characteristics observed in the end members of the series SrTi(Co,Fe)O3, and suggest the existence of a broader set of rules for oxygen-deficient multiferroic oxides.

36 MATERIALS SCIENCE↗
NASA NTRS1978

Spin-related magnetism of interstellar grains

The magnetic dipole moments and internal magnetic fields due to the spin of electrically charged elongated nonmagnetic interstellar grains in kinetic equilibrium with their surroundings are computed for the grain-size range from 0.01 to 1.0 micron. It is shown that the induced magnetic moments and internal magnetic fields of charged spinning nonmagnetic grains of arbitrary composition and prolate spheroidal shape can be appreciable, possibly even exceeding 0.01 emu/cu cm for 0.01-micron grains. The results indicate that virtually all grains smaller than 0.1 micron in mean diameter, and all elongated grains smaller than about 1 micron in length, are immersed in local magnetic fields due to spin that are much larger than the ambient galactic field. Some implications of this effect are discussed in relation to the polarization of starlight by aligned dust grains and the primordial remanent magnetization found in primitive carbonaceous chondrites.

Srnka, L. J.↗
NASA NTRS1993

Strong-field cyclotron scattering. I - Scattering amplitudes and natural line width

The introduction of resonance line width into the QED cyclotron scattering amplitudes is considered. It is shown that the width arises from loop corrections to the electron propagator, which also bring about shifts in the Landau energy levels. A formalism is developed that allows the dressed electron propagator to be derived. It is shown that the states of Herold et al. (1982) and of Sokolov and Ternov (1968), which diagonalize the component of the magnetic moment operator parallel to the external magnetic field, are appropriate for calculation of the scattering amplitudes, whereas the states of Johnson and Lippmann (1949) are not. In addition, it is shown that the Breit-Wigner broadening approximation E tends to E - i(Gamma)/2 is consistent with the perturbation-theoretic order of the calculation, if the former basis states are chosen, but not the latter.

Graziani, Carlo↗
NASA NTRS1994

Kinetic and thermodynamic properties of a convecting plasma in a two-dimensional dipole field

Charged particle guiding center motion is considered in the magnetic field of a two-dimensional ('line') dipole on which is superimposed a small, static, perpendicular electric field. The parallel equation of motion is that of a simple harmonic oscillator for cos theta, the cosine of magnetic colatitude theta. Equations for the perpendicular electric and magnetic drifts are derived as well as their bounce-averaged forms. The latter are solved to yield a bounce-averaged guiding center trajectory, which is the same as that obtained from conversation of magnetic moment mu, longitudinal invariant J, and total (kinetic plus electrostatic) energy K. The algebraic simplicity of the trajectory equations is also manifest in the forms of the invariants. An interesting result is that guiding centers drift in such a way that they preserve the values of their equatorial pitch angles and (equivalently) mirror latitudes. The most general Maxwellian form of the equilibrium one-particle distribution function f is constructed from the invariants, and spatially varying density and pressure moments, parallel and perpendicular to the magnetic field, are identified. Much of the paper deals with the more restricted problem in which f is specified as a bi-Maxwellian over a straight line of finite length in the equatorial plane of the dipole and perpendicular to field lines. This might be thought of as specifying a cross-tail ion injection source; our formalism then describes the subsequent spatial development. The distribution away from the source is a scaled bi-Maxwellian but one that is cut off at large and small kinetic energies, which depend on position. Density and pressure components are reduced from the values they would have if the total content of individual flux tubes convected intact. The equatorial and meridional variations of density and pressure components are examined and compared systematically for the isotropic and highly anisotropic situations. There appears to be little qualitative difference due to anisotropy. An anisotropy measure is defined, and its spatial variation determined as a signature of possible MHD instability. Extreme values are found, larger than at the source, but the plasma beta in such regions is probably so low as to render the effect inconsequential energetically. Finally, the possible consequence of 'nonadia- batic' pressure profiles on electrostatic interchanges is considered, and a boundary delineating stabilizing and destabilizing regions determined.

Huang, T. S.↗
DOE OSTI2021

Epitaxy, exfoliation, and strain-induced magnetism in rippled Heusler membranes

Single-crystalline membranes of functional materials enable the tuning of properties via extreme strain states; however, conventional routes for producing membranes require the use of sacrificial layers and chemical etchants, which can both damage the membrane and limit the ability to make them ultrathin. Here we demonstrate the epitaxial growth of the cubic Heusler compound GdPtSb on graphene-terminated Al 2 O 3 substrates. Despite the presence of the graphene interlayer, the Heusler films have epitaxial registry to the underlying sapphire, as revealed by x-ray diffraction, reflection high energy electron diffraction, and transmission electron microscopy. The weak Van der Waals interactions of graphene enable mechanical exfoliation to yield free-standing GdPtSb membranes, which form ripples when transferred to a flexible polymer handle. Whereas unstrained GdPtSb is antiferromagnetic, measurements on rippled membranes show a spontaneous magnetic moment at room temperature, with a saturation magnetization of 5.2 bohr magneton per Gd. First-principles calculations show that the coupling to homogeneous strain is too small to induce ferromagnetism, suggesting a dominant role for strain gradients. Our membranes provide a novel platform for tuning the magnetic properties of intermetallic compounds via strain (piezomagnetism and magnetostriction) and strain gradients (flexomagnetism).

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Tuning interfacial Dzyaloshinskii-Moriya interactions in thin amorphous ferrimagnetic alloys

Skyrmions can be stabilized in magnetic systems with broken inversion symmetry and chiral interactions, such as Dzyaloshinskii-Moriya interactions (DMI). Further, compensation of magnetic moments in ferrimagnetic materials can significantly reduce magnetic dipolar interactions, which tend to favor large skyrmions. Tuning DMI is essential to control skyrmion properties, with symmetry breaking at interfaces offering the greatest flexibility. However, in contrast to the ferromagnet case, few studies have investigated interfacial DMI in ferrimagnets. Here we present a systematic study of DMI in ferrimagnetic CoGd films by Brillouin light scattering. We demonstrate the ability to control DMI by the CoGd cap layer composition, the stack symmetry and the ferrimagnetic layer thickness. The DMI thickness dependence confirms its interfacial nature. In addition, magnetic force microscopy reveals the ability to tune DMI in a range that stabilizes sub-100 nm skyrmions at room temperature in zero field. Our work opens new paths for controlling interfacial DMI in ferrimagnets to nucleate and manipulate skyrmions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Effect of lattice strain on magnetism in epitaxial YCrO 3 films

The influence of lattice strain on magnetism is studied for perovskite rare-earth chromite, YCrO 3 (YCO) thin films. A combined theoretical and experimental approach is used to demonstrate the correlation between lattice-strain and magnetic properties of YCO films. The first-principles calculations reveal that the local Cr magnetic moments and the out-of-plane magnetization linearly increase with changing the in-plane lattice strain from compressive to tensile. The experimental results agree with the theory findings showing a strong dependence of magnetization on epitaxial strain in YCO films. These results unveil the lattice-strain-controlled functionalities on perovskite rare-earth chromites and related material systems.

36 MATERIALS SCIENCE↗