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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
NASA NTRS1993

The evolution of strongly modulated, low-frequency, moderate-amplitude wave packets in a dispersive plasma

The evolution of strongly modulated wave packets in a dispersive plasma that propagate parallel to the magnetic field is studied. Modulation effects are shown to reduce significantly (about 30 percent) the rate of spreading from that due to dispersion alone. For fluidlike behavior, nonlinearity has its greatest impact on evolution when the linear sound speed and initial wave packet speeds are well matched, resulting in a strong coupling between the wave magnetic and sonic components. Ion kinetic processes reduce the impact of nonlinearity and cause the rate of spreading to approach that expected from dispersion alone as the ratio of ion and electron temperatures, Ti/Te approaches 4. For Beta equal to or greater than 1 and Ti/Te of about 1, the coupled waveforms correspond qualitatively to kinetic treatments of the derivative nonlinear Schroedinger equation.

Vasquez, Bernard J.↗
DOE OSTI2023

Optical activity of solids from first principles

Within the framework of independent particle approximation, the optical activity tensor of solids is formulated as from different contributions: the magnetic dipole, electric quadrupole, and band dispersion terms. The first two terms have similar counterparts in the theory of finite systems, whereas the last term is unique for crystals. Further, the magnetic dipole and electric quadrupole transition moments are calculated with a sum-over-states formulation. We apply the formulation to calculate and analyze the optical rotation of elemental tellurium and the circular dichroism of the (6,4) carbon nanotube. Decomposed optical activity into different contributions is discussed. The calculated spectra agree well with experiments. As a showcase of achiral crystals, we calculate the optical activity of wurtzite GaN.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Nonlinear Alfvén wave dynamics in plasmas

Nonlinear Alfvén wave dynamics is presented using Lagrangian fluid approach in a compressible collisional magnetized plasma. In the framework of two fluid dynamics, finite electron inertia is shown to serve as a dispersive effect acting against the convective nonlinearity. In a moving frame, the Alfvén wave can, therefore, form an arbitrarily strong amplitude solitary wave structure due to the balance between nonlinearity and dispersion. Weak amplitude Alfvén waves are shown to be governed by a modified KdV equation, which extends for finite dissipation to a mKdV-Burgers equation. These equations have well known solutions. Next, we have analyzed the fourth order nonlinear Alfvén wave system of equations both numerically and by approximation method. The results indicate a collapse of the density and magnetic field irrespective of the presence of dispersion. The wave magnetic field, however, appears to be less singular showing collapse only when the dispersive effects are negligible. These results may contribute to our understanding of the generation of strongly localized magnetic fields (and currents) in plasmas and are expected to be of special importance in the astrophysical context of magnetic star formation.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1979

Magnetic and metallurgical properties of directionally solidified eutectic Bi/MnBi composites - The effects of annealing

Eutectic Bi/MnBi (97.8 a/o Bi) samples have been plane-front directionally solidified. The resultant microstructures consist of elongated, aligned particles of MnBi dispersed in a Bi-matrix. Magnetization as a function of temperature (4.2 to 300 K) and applied field (up to 220 kG) has been used to evaluate solidification parameters and magnetic properties. At room temperature, in addition to the diamagnetic contribution of Bi, one finds a superposition of the ferromagnetic, low temperature (LTP) MnBi phase and paramagnetic phases. At cryogenic temperatures, one of the room temperature paramagnetic phases is ferromagnetic with an intrinsic coercivity of 120 kOe while the other remains paramagnetic for low fields and orders ferromagnetically at high fields in a complicated way. Annealing of as-grown samples was found to produce significant changes in magnetic properties. The origins of the paramagnetic phases and their relation to the mechanisms which control the coercive field of the hard magnetic LTP MnBi phase are discussed.

Pirich, R. G.↗
DOE OSTI2012

The Curie temperature distribution of FePt granular magnetic recording media

We present atomistic calculations of the magnetic phase transition behavior in an L1{sub 0} FePt system to study the effect of grain size distribution on the Curie temperature (T{sub c}) dispersion with relevance to heat assisted magnetic recording. Identifying the relation between the size and T{sub c} of a grain by means of finite size scaling analysis of the differentiated magnetization versus T data allows to show that a lognormal size distribution transforms into a lognormal T{sub c} distribution with moments dependent on the critical exponents. We also address the question of the universality class of FePt.

36 MATERIALS SCIENCE↗
DOE OSTI2016

On a theory of surface waves in a smoothly inhomogeneous plasma in an external magnetic field

A theory of surface waves in a magnetoactive plasma with smooth boundaries has been developed. A dispersion equation for surface waves has been derived for a linear law of density change at the plasma boundary. The frequencies of surface waves and their collisionless damping rates have been determined. A generalization to an arbitrary density profile at the plasma boundary is given. The collisions have been taken into account, and the application of the Landau rule in the theory of surface wave damping in a spatially inhomogeneous magnetoactive collisional plasma has been clarified.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Space-charge waves in magnetized and collisional quantum plasma columns confined in carbon nanotubes

We study the dispersion relation of electrostatic waves propagating in a column of quantum magnetized collisional plasma embraced completely by a metallic single-walled carbon nanotubes. The analysis is based on the quantum linearized hydrodynamic formalism of collective excitations within the quasi-static approximation. It is shown when the electronic de Broglie's wavelength of the plasma is comparable in the order of magnitude to the radius of the nanotube, the quantum effects are quite meaningful and our model anticipates one acoustical and two optical space-charge waves which are positioned into three propagating bands. With increasing the nanotube radius, the features of the acoustical branch remain unchanged, yet two distinct optical branches are degenerated and the classical behavior is recovered. This study might provide a platform to create new finite transverse cross section quantum magnetized plasmas and to devise nanometer dusty plasmas based on the metallic carbon nanotubes in the absence of either a drift or a thermal electronic velocity and their existence could be experimentally examined.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2012

Perpendicular propagating modes for weakly magnetized relativistic degenerate plasma

Using the Vlasov-Maxwell system of equations, the dispersion relations for the perpendicular propagating modes (i.e., X-mode, O-mode, and upper hybrid mode) are derived for a weakly magnetized relativistic degenerate electron plasma. By using the density (n{sub 0}=p{sub F}{sup 3}/3{pi}{sup 2} Planck-Constant-Over-Two-Pi {sup 3}) and the magnetic field values for different relativistic degenerate environments, the propagation characteristics (i.e., cutoff points, resonances, dispersions, and band widths in k-space) of these modes are examined. It is observed that the relativistic effects suppress the effect of ambient magnetic field and therefore the cutoff and resonance points shift towards the lower frequency regime resulting in enhancement of the propagation domain. The dispersion relations of these modes for the non-relativistic limit (p{sub F}{sup 2} Much-Less-Than m{sub 0}{sup 2}c{sup 2}) and the ultra-relativistic limit (p{sub F}{sup 2} Much-Greater-Than m{sub 0}{sup 2}c{sup 2}) are also presented.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Whistler wave generation by non-gyrotropic, relativistic, electron beams

Particle-in-cell code, EPOCH, is used for studying features of the wave component evident to propagate backwards from the front of the non-gyrotropic, relativistic beam of electrons injected in the Maxwellian, magnetised background plasma with decreasing density profile. According to recent findings presented in Tsiklauri [Phys. Plasmas 18, 052903 (2011)], Schmitz and Tsiklauri [Phys. Plasmas 20, 062903 (2013)], and Pechhacker and Tsiklauri [Phys. Plasmas 19, 112903 (2012)], in a 1.5-dimensional magnetised plasma system, the non-gyrotropic beam generates freely escaping electromagnetic radiation with properties similar to the Type-III solar radio bursts. In this study, the backwards propagating wave component evident in the perpendicular components of the electromagnetic field in such a system is presented for the first time. Background magnetic field strength in the system is varied in order to prove that the backwards propagating wave's frequency, prescribed by the whistler wave dispersion relation, is proportional to the specified magnetic field. Moreover, the identified whistlers are shown to be generated by the normal Doppler-shifted relativistic resonance. Large fraction of the energy of the perpendicular electromagnetic field components is found to be carried away by the whistler waves, while a small but sufficient fraction is going into L- and R-electromagnetic modes.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Competing magnetic phases and itinerant magnetic frustration in SrCo 2 As 2

Whereas magnetic frustration is usually associated with local-moment magnets in special geometric arrangements, here we show that SrCo 2 As 2 is a candidate for frustrated itinerant magnetism. Using inelastic neutron scattering (INS), we determine that antiferromagnetic (AF) spin fluctuations develop in the square Co layers of SrCo 2 As 2 below T ≈ 100 K centered at the stripe-type AF propagation vector of ($\frac{1}{2}$, $\frac{1}{2}$), and that their development is concomitant with a suppression of the uniform magnetic susceptibility determined via magnetization measurements. We interpret this switch in spectral weight as signaling a temperature-induced crossover from an instability towards FM ordering to an instability towards stripe-type AF ordering on cooling, and show findings from Monte-Carlo simulations for a J 1 -J 2 Heisenberg model that illustrate how the crossover develops as a function of the frustration ratio –J 1 /(2J 2 ). By putting our INS data on an absolute scale, we quantitatively compare them and our magnetization data to exact-diagonalization calculations for the J 1 -J 2 model [N. Shannon et al., Eur. Phys. J. B 38, 599 (2004)], and show that the calculations predict a lower level of magnetic frustration than indicated by experiment. We trace this discrepancy to the large energy scale of the fluctuations (J avg ≳ 75 meV), which, in addition to the steep dispersion, is more characteristic of itinerant magnetism.

36 MATERIALS SCIENCE↗
DOE OSTI2019

Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet

Topological matter is known to exhibit unconventional surface states and anomalous transport owing to unusual bulk electronic topology. In this study, we use photoemission spectroscopy and quantum transport to elucidate the topology of the room temperature magnet Co 2 MnGa. We observe sharp bulk Weyl fermion line dispersions indicative of nontrivial topological invariants present in the magnetic phase. On the surface of the magnet, we observe electronic wave functions that take the form of drumheads, enabling us to directly visualize the crucial components of the bulk-boundary topological correspondence. By considering the Berry curvature field associated with the observed topological Weyl fermion lines, we quantitatively account for the giant anomalous Hall response observed in this magnet. Our experimental results suggest a rich interplay of strongly interacting electrons and topology in quantum matter.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Ligand Binding Enhances Millisecond Conformational Exchange in Xylanase B2 from Streptomyces lividans

Xylanases catalyze the hydrolysis of xylan, an abundant carbon and energy source with important commercial ramifications. Despite tremendous efforts devoted to the catalytic improvement of xylanases, success remains limited because of our relatively poor understanding of their molecular properties. Previous reports suggested the potential role of atomic-scale residue dynamics in modulating the catalytic activity of GH11 xylanases; however, dynamics in these studies was probed on time scales orders of magnitude faster than the catalytic time frame. Here, we used nuclear magnetic resonance titration and relaxation dispersion experiments ( 15 N-CPMG) in combination with X-ray crystallography and computational simulations to probe conformational motions occurring on the catalytically relevant millisecond time frame in xylanase B2 (XlnB2) and its catalytically impaired mutant E87A from Streptomyces lividans 66. Our results show distinct dynamical properties for the apo and ligand-bound states of the enzymes. The apo form of XlnB2 experiences conformational exchange for residues in the fingers and palm regions of the catalytic cleft, while the catalytically impaired E87A variant displays millisecond dynamics only in the fingers, demonstrating the long-range effect of the mutation on flexibility. Ligand binding induces enhanced conformational exchange of residues interacting with the ligand in the fingers and thumb loop regions, emphasizing the potential role of residue motions in the fingers and thumb loop regions for recognition, positioning, processivity, and/or stabilization of ligands in XlnB2. To the best of our knowledge, this work represents the first experimental characterization of millisecond dynamics in a GH11 xylanase family member. Furthermore, these results offer new insights into the potential role of conformational exchange in GH11 enzymes, providing essential dynamic information to help improve protein engineering and design applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2014

High quality Y-type hexaferrite thick films for microwave applications by an economical and environmentally benign crystal growth technique

Thick barium hexaferrite Ba{sub 2}Zn{sub 2}Fe{sub 12}O{sub 22} (i.e., Zn{sub 2}Y) films having thicknesses of ∼100 μm were epitaxially grown on MgO (111) substrates using an environmentally benign ferrite-salt mixture by vaporizing the salt. X-ray diffraction pole figure analyses showed (00l) crystallographic alignment with little in plane dispersion confirming epitaxial growth. Saturation magnetization, 4πM{sub s}, was measured for as-grown films to be 2.51 ± 0.1 kG with an out of plane magnetic anisotropy field H{sub A} of 8.9 ± 0.1 kOe. Ferromagnetic resonance linewidth, as the peak-to-peak power absorption derivative at 9.6 GHz, was measured to be 62 Oe. These properties demonstrate a rapid, convenient, cost-effective, and nontoxic method of growing high quality thick crystalline ferrite films which could be used widely for microwave device applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2014

Templated fabrication and characterization of SiO{sub 2} nanotube covered Fe nanowires

In this study, Fe nanowires coated with SiO{sub 2} nanotubes have been synthesized by electrodeposition method using anodic alumina oxide template. Before growing Fe nanowires, 6–8 nm thick SiO{sub 2} nanotubes are grown inside the template using a “surface sol-gel” technique. The nanotube structures were characterized by field emission scanning electron microscopy and energy dispersive x-ray spectroscopy. Magnetic properties of the SiO{sub 2} insulated Fe nanowires inside the membrane are characterized by superconducting quantum interference device. Coercivities of around 120 Oe with field parallel to the nanowire axis and 240 Oe with field perpendicular the nanowire axis are observed at room temperature. These values are comparable to Fe nanowires without insulating layer in membrane. The magnetic hysteresis loop suggests that the SiO{sub 2} insulated nanowires have uniaxial magnetic anisotropy with the easy axis magnetization direction along the nanowire arrays due to their large shape anisotropy.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2016

Comment on “Surface electromagnetic wave equations in a warm magnetized quantum plasma” [Phys. Plasmas 21, 072114 (2014)]

In a recent article [C. Li et al., Phys. Plasmas 21, 072114 (2014)], Li et al. studied the propagation of surface waves on a magnetized quantum plasma half-space in the Voigt configuration (in this case, the magnetic field is parallel to the surface but is perpendicular to the direction of propagation). Here, we present a fresh look at the problem and obtain a new form of dispersion relation of surface waves of the system. We find that our new dispersion relation does not agree with the result obtained by Li et al.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Robust superconductivity and the suppression of charge-density wave in the quasi-skutterudites Ca 3 ( Ir 1 – x Rh x ) 4 Sn 13 single crystals at ambient pressure

Single crystals of the quasi-skutterudite compounds Ca 3 (Ir 1-x Rh x ) 4 Sn 13 (3–4–13) were synthesized by flux growth and characterized by x-ray diffraction, energy dispersive x-ray spectroscopy, magnetization, resistivity, and radio frequency magnetic susceptibility techniques. The coexistence and competition between the charge density wave (CDW) and superconductivity was studied by varying the Rh/Ir ratio. The superconducting transition temperature, T c , varies from 7 K in pure Ir (x = 0) to 8.3 K in pure Rh (x = 1). Temperature-dependent electrical resistivity reveals monotonic suppression of the CDW transition temperature, T CDW (x). The CDW starts in pure Ir, x = 0, at T CDW ≈ 40 K and extrapolates roughly linearly to zero at x c ≈ 0.53–0.58 under the superconducting dome. Magnetization and transport measurements show a significant influence of CDW on superconducting and normal states. Meissner expulsion is substantially reduced in the CDW region, indicating competition between the CDW and superconductivity. The low-temperature resistivity is higher in the CDW part of the phase diagram, consistent with the reduced density of states due to CDW gapping. Its temperature dependence just above T c shows signs of non-Fermi liquid behavior in a cone-like composition pattern. We conclude that the Ca 3 (Ir 1-x Rh x ) 4 Sn 13 alloy is a good candidate for a composition-driven quantum critical point at ambient pressure.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Magnon damping in the zigzag phase of the Kitaev-Heisenberg- Γ model on a honeycomb lattice

We calculate dispersions and damping of the magnetic excitations in the model that is relevant to a description of the magnetic properties of iridium oxides α-Li 2 IrO 3 and Na 2 IrO 3 , and Ru-based materials such as α-RuCl 3 . Focusing on the parameter regime with the zigzag spin pattern in the ground state that is consistent with experiments, we are able to obtain explicit analytical expressions for magnon energies and eigenstates and go beyond the standard linear spin-wave theory approximation by calculating magnon damping and demonstrating its role in the dynamical structure factor. Here, we show that the magnon damping effects in both Born and self-consistent approximations are very significant, underscoring the importance of nonlinear magnon coupling in interpreting broad features in the neutron-scattering spectra.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2020

Ferromagnetic cluster-glass phase in Ca(Co 1-x Ir x ) 2-y As 2 crystals

In this study, single crystals of Ca(Co 1-x Ir x ) 2-y As 2 with 0≤x≤0.35 and 0.10≤y≤0.14 have been grown using the self-flux technique and characterized by single-crystal x-ray diffraction (XRD), energy-dispersive x-ray spectroscopy, magnetization M, and magnetic susceptibility χ measurements versus temperature T, magnetic field H, and time t, and heat-capacity C p (H,T) measurements. The XRD refinements reveal that all the Ir-substituted crystals crystallize in a collapsed-tetragonal structure as does the parent CaCo 2-y As 2 compound. A small 3.3% Ir substitution for Co in CaCo 1.86 As 2 drastically lowers the A-type antiferromagnetic (AFM) transition temperature T N from 52 to 23 K with a significant enhancement of the Sommerfeld electronic heat-capacity coefficient. The A-type AFM structure consists of ab-plane layers of spins ferromagnetically aligned along the c axis with AFM alignment of the spins in adjacent layers along this axis. The positive Weiss temperatures obtained from Curie-Weiss fits to the χ(T>T N ) data indicate that the dominant magnetic interactions are ferromagnetic (FM) for all x. A magnetic phase boundary is inferred to be present between x=0.14 and x=0.17 from a discontinuity in the x dependencies of the effective moment and Weiss temperature in the Curie-Weiss fits. FM fluctuations that strongly increase with increasing x are also revealed from the χ(T) data. Furthermore, the magnetic ground state for x≥0.17 is a spin glass as indicated by hysteresis in χ(T) between field-cooled and zero-field-cooled measurements and from the relaxation of M in a small field that exhibits a stretched-exponential time dependence. The spin glass has a small FM component to the ordering and is hence inferred to be comprised of small FM clusters. The competing AFM and FM interactions along with crystallographic disorder associated with Ir substitution are inferred to be responsible for the development of a FM cluster-glass phase. A logarithmic T dependence of Cp at low T for x=0.14 is consistent with the presence of significant FM quantum fluctuations. This composition is near the T=0 boundary at x≈0.16 between the A-type AFM phase containing ferromagnetically-aligned layers of spins and the FM cluster-glass phase.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗