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At least 343 records · Page 19

Constrained Bayesian Optimization of Criticality Experiments at LLNL [Slides]

The design of criticality experiments is typically an iterative process that employs a Monte Carlo transport code. The goal is to find a design that optimizes some variable, like the sensitivity of a response to a cross section, while simultaneously ensuring criticality. The high fidelity of the Monte Carlo code is a great asset, but it makes exploring the design space computationally expensive. Herein, we present how a constrained Bayesian optimization algorithm can be used to efficiently design a criticality experiment. It uses Gaussian processes as a surrogate model to probe the design space and to reduce the number of code executions that are needed to find the optimum. We demonstrate constrained Bayesian optimization with a Pu-239/polyethylene solution system and a TEX experiment that is designed for critical ity safety validation of a nuclear waste model at the Hanford Site. For both systems, a global optimum was found within 75 Monte Carlo simulations.

42 ENGINEERING↗

Constrained Bayesian Optimization of Criticality Experiments [Slides]

The design of criticality experiments is typically an iterative process that employs a Monte Carlo transport code. The goal is to find a design that optimizes some variable, like the sensitivity of a response to a cross section, while simultaneously ensuring criticality. The high fidelity of the Monte Carlo code is a great asset, but it makes exploring the design space computationally expensive. Herein, we present how a constrained Bayesian optimization algorithm can be used to efficiently design a criticality experiment. It uses Gaussian processes as a surrogate model to probe the design space and to reduce the number of code executions that are needed to find the optimum. We demonstrate constrained Bayesian optimization with a Pu-239/polyethylene solution system and a TEX experiment that is designed for criticality safety validation of a nuclear waste model at the Hanford Site. For both systems, a global optimum was found within 75 Monte Carlo simulations.

42 ENGINEERING↗

Neutronics Analysis of Cold Critical KRUSTY Experiments using MCNP and Serpent

Kilowatt Reactor Using Stirling Technology (KRUSTY) is a prototype designed as a proof of concept for NASA’s Kilo power program, which was funded in order to create a small reactor for various space applications such as providing power for a colony on Mars or the moon and eventually as a possible option for powering rockets on deep space missions. KRUSTY was tested at the National Criticality Experiments Research Center (NCERC) located at the Nevada National Security Site (NNSS) from November 2017, through March 2018. The experimental campaign was conducted in four phases: com ponent critical experiments, cold critical experiments, warm critical runs, and high temperature demonstration. The component critical and cold critical experiments were used to determine the worth of the beryllium oxide (BeO) reflector rings and the boron carbide (B4C) control rod disks under different conditions. These conditions were altered by the addition and subtraction of other components in the assembly. The component critical phase was performed at atmospheric pressure and had four solid support rods spanning the center core; whereas the cold critical phase had the center core placed in a vacuum chamber and eight sodium-filled heat pipes spanning the center core region. This summary discusses the static neutronic analysis completed on the cold critical phase of the campaign using MCNP ® and Serpent. These two codes were used to assess any potential differences or biases in the simulation results. Understanding these potential biases is a key step toward the final goal of being able to fully analyze the transient experiments performed during phases 3 and 4 of the campaign.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

The Jupiter High-240 Experiment

The Jupiter High-240 experiment was performed in May of 2019 by researchers from Los Alamos National Laboratory (LANL) at the National Criticality Experiments Research Center (NCERC) in the Device Assembly Facility (DAF) located at the Nevada National Security Site (NNSS). This experiment has previously been mentioned briefly in prior publication related to a collaborative effort with the Japan Atomic Energy Agency (JAEA) to assess lead void coefficients of reactivity in uranium- and plutonium-fueled systems with lead. This series of experiments supports JAEA’s research into the development of an accelerator driven transmutation system for spent nuclear fuel. The Jupiter High-240 experiment built upon the previous Jupiter experiment by incorporating plutonium fuel plates with higher 240 Pu content. Efforts to formally benchmark the original Jupiter experiment have continued for inclusion in the benchmark handbook of the International Criticality Safety Benchmark Evaluation Project (ICSBEP). Whereas there is much similarity between the two Jupiter experiments, there is a desire to also evaluate and benchmark this second experiment to further contribute towards the availability of lead-sensitive benchmarks. The components utilized in these two experiments have also been used to perform other subcritical and Rossi-α measurements.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Chlorine Worth Study in Support of PF-4 Operations [Slides]

Aqueous Chloride Operations at PF-4 are important because they recover Pu from other processes, reduce waste sent to WIPP, and increase throughput for Am production. Aqueous Chloride Operations have very conservative mass limits (~520 grams Pu) and significant amounts of Chlorine but calculations not crediting Cl-35 neutron absorption accounting for Cl-35 absorption leads to higher mass limits. Can experiments be designed/conducted to provide technical justification to NCS in order to increase mass limits?

2019 ARCHIMEDES LDRD project↗

IER305: Molybdenum Sleeve Experiments in the Sandia Critical Experiments Facility [Slides]

This presentation is on the Molybdenum (Mo) sleeve experiments at the Sandia Critical Experiments Facility. The Institut de Radioprotection et de Sûreté Nucléaire (IRSN) performed the preliminary design of the experiment. IRSN performed the final nuclear design of the experiment. Sandia performed the detailed design of the experiment to make it work in the critical assembly and Sandia also oversaw the fabrication and installation of the hardware. The slides include cutaway and overall views and a look into the results.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Generating Models of the Flattop Critical Assembly for Benchmark Experiments with Python

Los Alamos National Laboratory has been performing nuclear criticality experiments since 1946 at the Pajarito site, starting the Los Alamos Critical Experiments Facility in 1948. A transition period occurred between 2004 and 2011 as operations moved to the National Criticality Experiments Research Center (NCERC), where criticality experiments are now performed. Criticality experiments are essential for determination and verification of nuclear data used in calculations and modeling—such as radiation transport codes—throughout the industry, enhancing nuclear criticality safety. In addition to nuclear data validation and benchmarking, the remotely operated critical assemblies at NCERC are used for a variety of experiments and training classes supporting criticality safety.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

The First ICNC February 10-12, 1981 [Slides]

The first meeting that became the International Conference on Nuclear Criticality—ICNC—was held at the Los Alamos National Laboratory in February 1981. This presentation includes information on that meeting, including several experiments performed around that time period.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

MULTIPHYSICS-MODELING OF FIRE-INDUCED URANIUM AEROSOL FORMATION – A-POSTERIORI BENCHMARKING OF EXPERIMENTS

The formulation and solution of a model that properly described the temperature profiles of uranium in fire conditions was prepared, verified and validated, to support a-posteriori benchmarking of historical experiments. Data from the multi-physics model combined with data regression from the experiments provides a useful tool for exploring sources of potential bias in historical experiments. The approaches used are augmented by visual observations and photographic evidence allowing for correlations between various phenomena, independent of whether or not that specific phenomena are part of the validated model. In this manner, the validated model is a tool for a-posteriori benchmarking, and not a model designed to replicate the experimental output exactly for any specific experiment. For experiments like the Clark (2015) experiments, this integrated model (including chemistry) demonstrated that the largest bias was associated in the metallurgy of the coupons. The model developed does serve as a basis for defending which of the historical alloys tested are the most appropriate for any other alloy being considered (e.g., one that has not yet been tested). The model identifies key reactions that impact uranium chemistry and can significantly bias experimental results. Through use of the model and energy balances, data from historical experiments by Elder and Tinkle (1980) were regressed and benchmarked. This study identifies that all uranium alloys are not equal and that there are distinct differences between the dominant alloys representing distinct metallurgical phases.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Sensitivity Coefficients Calculated for the Prompt Neutron Decay Constant At or Near Delayed Critical

The derivation of a non-invasive prompt neutron decay constant sensitivity coefficient is provided in this work. The computation of the sensitivity coefficient derived in this work does not require modification of Monte Carlo source code and is based on capabilities available in Monte Carlo N-Particle R© Code Version 6.2. The prompt neutron decay constant sensitivity coefficients are calculated for 44-group and 252-group energy structures for specific nuclide-reaction pairs in the Jezebel benchmark experiment. The nuclide-reaction pairs investigated in this work include Pu- 239(n,f), Pu-240(n,f), and Pu-241(n,f). Physical explanations of the sensitivity profiles exhibited by the 252-group energy structure are investigated for the prompt neutron multiplication factor, mean neutron lifetime, and prompt neutron decay constant. The prompt neutron decay constant sensitivity coefficients calculated for the 44-group and 252-group energy structure of Pu-239(n,f) are compared. Lastly, the 44-group energy structure sensitivity coefficients calculated are used for nuclear-data induced uncertainty quantification of the neutron multiplication factor. This work shows that a reduction in the nuclear data-induced uncertainty of the neutron multiplication factor is possible for all nuclide-reaction pairs investigated when prompt neutron decay constant sensitivity coefficients are utilized. This is important for new critical experiment design optimization studies of measurement configurations. This work provides a basis for more detailed sensitivity analysis and uncertainty quantification of nuclide, reaction, and energy-specific cross section data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Using Prompt Neutron Decay Constant Measurements to Obtain Additional Kinetics Information

Prompt neutron decay constant measurements are typically used to infer the prompt neutron lifetime in a chain-reacting system, but these measurements include much more information about the kinetics of the system. This work focuses specifically on the Rossi-α method of measuring the prompt neutron decay constant. The Rossi-α system of equations consists of five unknown parameters. With five unknowns and three equations, the system of equations solved by the Rossi-α measurement is under-determined. It has been postulated that a well posed problem can be formulated using independent measurement configurations on a single system. The external source strength, the effective delayed neutron fractions, and Diven’s parameter do not typically change for different configurations of a single experiment. If good detector geometry is chosen, the detector efficiency does not change for multiple measurements of a single experiment using Rossi-α measurements. By making these assumptions, there are only two unique variables. This knowledge can be used to solve for most of the unique parameters using two independent, unique Rossi-α measurements.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Completion of IER 305: Molybdenum Sleeve Experiments and Preparations for Performing IER 441: Epithermal Tantalum Experiments [Slides]

This presentation includes a look into Sandia critical experiments including the 7uPCX, BUCCX, and assembly design. This presentation touches on the completion of IER 305 with CED-3b, CED-4a, and CED-4b. Finally, there are preparations to perform IER 441 including new hardware, critical configurations, and next steps.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Preliminary Benchmark Uncertainties for Deimos, a HALEU-Fueled and Graphite-Moderated Advanced Reactor Testbed

Many advanced reactor concepts will make use of various uranium fuels with levels of enrichment higher than previously seen in current light water reactors. In particular, High-Assay Low Enriched Uranium (HALEU), that is uranium enriched to 235 U ≈ 20 w/o%, is planned to be used in over ten new reactor concepts. HALEU is attractive for advanced reactors as it enables longer intervals between refueling. Unfortunately, little to no experience with HALEU is available in experimental literature raising concerns for not only licensing advanced re actors but also fabrication and transportation of HALEU fuels. This is where Deimos, a Los Alamos National Laboratory internal project, comes in. Deimos is a new critical experiment scheduled for FY24 at the National Criticality Experiments Research Center (NCERC). Deimos is a graphite moderated, graphite and beryllium reflected critical experiment making use of HALEU TRi-structural ISOtropic (TRISO) fuel from the Compact Nuclear Power System (CNPS). This transaction entails a brief description of efforts to benchmark Deimos for inclusion into the International Criticality Safety

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

IER 501: Pulsed Neutron Die-Away Experiments at LLNL [Slides]

Pulsed neutron die away experiments occur as follows: (1) a pulse of neutrons is injected into a target material via a D-T neutron generator, (2) neutrons thermalize, (3) neutrons spatially equilibrate, and (4) exponential decay is measured in fundamental mode.

43 PARTICLE ACCELERATORS↗

Horizontal Split Table Conceptual Design for Validation of Nuclear Data used in Advanced Reactors [Slides]

This presentation discusses a methodology that was developed to create conceptual designs of benchmark critical experiments for advanced reactors and nuclear data testing. A first concept that was explored was a pebble-bed high-temperature gas cooled reactor, based on the HTR-10 reactor. The very high correlation is a proof of concept that the design is similar to the application, and performing such critical experiments would help nuclear data testing and validation. Other concepts could be explored if needed, such as a molten-salt reactor, a sodium-cooled fast reactor, or heat pipe reactors/microreactor.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

The Prompt Fission Uranium Neutron Spectrum (PFUNS) Experiment: Critical Configurations and Irradiations

The objective of the Prompt Fission Uranium Neutron Spectrum (PFUNS) experiment is to reduce the uncertainty of the Prompt Fission Neutron Spectrum (PFNS) of 235 U above 8 MeV. The experiment was performed at the DOE National Criticality Experiments Research Center (NCERC) at the Nevada National Security Site. To meet the experiment objective, activation foils were placed in a central void region of a critical configuration consisting of concentric highly enriched uranium (HEU) metal hemishells. The set of activation foils were chosen based on threshold reactions to neutron energies across the fission spectrum, but especially those in the high energy tail of the fission spectrum. PFUNS was performed on the Planet critical assembly machine at NCERC and uses the Rocky Flats (RF) HEU hemishells. PFUNS has similarities to the Measurement of Uranium Subcritical and Critical (MUSiC) experiment conducted at NCERC in 2021, which also used RF hemishells, but contains a large central cavity to allow for a sample plate to be inserted. This large void means that much more HEU is needed to achieve a critical configuration (108 kg for PFUNS versus 59 kg for MUSiC). This work describes the 2024 experiment execution of four critical configurations and two irradiations for the PFUNS project.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Preliminary Design of a New Pulsed-Neutron Die-Away Experimental Testbed for Thermal Scattering Law Benchmarks (PNDA) (IER-501 CED-1)

This report presents the preliminary design (CED-1) of IER-501, a new testbed for pulsed-neutron die-away (PNDA) experiments at Lawrence Livermore National Laboratory (LLNL). The PNDA experiments will be high-quality benchmarks that serve to optimize and validate thermal scattering laws (TSLs), which are high-priority nuclear data for the Department of Energy’s Criticality Safety Program (NCSP). PNDA experiments can be used to generate nuclear data validation benchmarks quickly and cheaply, as they do not require fissile material or a nuclear facility to conduct them.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗