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At least 343 records · Page 19

Global Patterns of Lightning Properties Derived by OTD and LIS

The satellite instruments Optical Transient Detector (OTD) and Lightning Imaging Sensor (LIS) provide unique empirical data about the frequency of lightning flashes around the globe (OTD), and the tropics (LIS), which 5 has been used before to compile a well received global climatology of flash rate densities. Here we present a statistical analysis of various additional lightning properties derived from OTD/LIS, i.e. the number of so-called "events" and "groups" per flash, as well as 10 the mean flash duration, footprint and radiance. These normalized quantities, which can be associated with the flash "strength", show consistent spatial patterns; most strikingly, oceanic flashes show higher values than continental flashes for all properties. Over land, regions with high (Eastern US) 15 and low (India) flash strength can be clearly identified. We discuss possible causes and implications of the observed regional differences. Although a direct quantitative interpretation of the investigated flash properties is difficult, the observed spatial patterns provide valuable information for the 20 interpretation and application of climatological flash rates. Due to the systematic regional variations of physical flash characteristics, viewing conditions, and/or measurement sensitivities, parametrisations of lightning NOx based on total flash rate densities alone are probably affected by regional biases.

Beirle, Steffen↗

Joint Assimilation of CO, O3, NO2, SO2, PM, AOD, NH4, PAN, and HNO3 in Support of the Tropospheric Regional Atmospheric Composition and Emissions Reanalysis (2005 - 2024) (TRACER-I)

NASA Ames Research Center is collaborating with the NOAA Chemical Systems Laboratory (NOAA/CSL), the NASA Jet Propulsion Laboratory (JPL), the NASA Goddard Modeling and Assimilation Office, and the National Center for Atmospheric Research to prepare a 20-year Tropospheric Regional Atmospheric Composition and Emissions Reanalysis (2005 – 2024) (TRACER-I) for the continental United States during the summer ozone (O3) and wildfire seasons (April to October). TRACER-I will be a regional complement to JPL’s global Tropospheric Chemistry Reanalyses II and III. We will use WRF-Chem/DART with NOAA/CSL’s WRF-Chem setup at 12 km x 12 km horizontal resolution, 51 vertical levels, and 30 ensemble members. We will assimilate: (i) conventional meteorological observations; (ii) EPA’s Air Quality System in situ measurements of carbon monoxide (CO), O3, nitrogen dioxide (NO2), sulfur dioxide (SO2), particulate matter (PM) with diameters less than 10 µm (PM10), and PM with diameters less than 2.5 µm (PM2.5); and (iii) MOPITT, MODIS, OMI, TROPOMI, GOME-2a, MLS, TES, SCIAMACHY, CrIS, and TEMPO total/partial column and/or profile retrievals of CO, O3, NO2, SO2, aerosol optical depth (AOD), formaldehyde (HCHO), ammonia (NH4), peroxyacetyl nitrate (PAN), and/or nitric acid (HNO3) with 3-hr cycling. We will present an overview of this project, its status, and available results (likely the analysis of sensitivity experiment results from the assimilation/emissions estimation system).

data assimilation↗

Statistical dependence of albedo and cloud cover on sea surface temperature for two tropical marine stratocumulus regions

The relationship between sea surface temperature (SST) and albedo or cloud cover is examined for two tropical regions with high values of cloud radiative forcing and persistent marine stratocumulus (mSc)-one off the west coast of Peru, the other off the west coast of Angola. The data span five years, from December 1984 to November 1989. Albedos are from the Earth Radiation Budget Experiment (ERBE), cloud covers are from the International Satellite Cloud Climatology Project (ISCCP), and SSTS are from the Climate Analysis Center. Negative correlation coefficients between albedo and SST are found to be about -0.8 when the seasonal variation of the entire dataset is analyzed. The interannual variation and the spatial variation of individual months also yields correlation coefficients that are negative. The correlation between cloud cover and SST is found to be similar to but weaker than the correlation between albedo and SST, suggesting a decrease in cloud amount and a decrease in cloud albedo with increasing SST for these regions. The corresponding albedo sensitivity averages -0.018/K with local values reaching -0.04/K. These findings are valid from 19 C to 25 C for the Peru mSc and 22 C to 27 C for the Angola mSc. These temperatures approximately bound the domains over which mSc is the prevalent cloud type within each region. These results imply a potential positive feedback to global warming by marine stratocumulus that ranges from approximately 0.14 W/sq m/K to approximately 1 W/sq m/K, depending on whether or not our results apply to all marine stratocumulus. While these values are uncertain to at least +/- 50%, the sensitivity of albedo to sea surface temperature in the present climate may serve as a useful diagnostic tool in monitoring the performance of global climate models.

Oreopoulos, Lazaros↗

Critical evaluation of Jet-A spray combustion using propane chemical kinetics in gas turbine combustion simulated by KIVA-2

Jet-A spray combustion has been evaluated in gas turbine combustion with the use of propane chemical kinetics as the first approximation for the chemical reactions. Here, the numerical solutions are obtained by using the KIVA-2 computer code. The KIVA-2 code is the most developed of the available multidimensional combustion computer programs for application of the in-cylinder combustion dynamics of internal combustion engines. The released version of KIVA-2 assumes that 12 chemical species are present; the code uses an Arrhenius kinetic-controlled combustion model governed by a four-step global chemical reaction and six equilibrium reactions. Researchers efforts involve the addition of Jet-A thermophysical properties and the implementation of detailed reaction mechanisms for propane oxidation. Three different detailed reaction mechanism models are considered. The first model consists of 131 reactions and 45 species. This is considered as the full mechanism which is developed through the study of chemical kinetics of propane combustion in an enclosed chamber. The full mechanism is evaluated by comparing calculated ignition delay times with available shock tube data. However, these detailed reactions occupy too much computer memory and CPU time for the computation. Therefore, it only serves as a benchmark case by which to evaluate other simplified models. Two possible simplified models were tested in the existing computer code KIVA-2 for the same conditions as used with the full mechanism. One model is obtained through a sensitivity analysis using LSENS, the general kinetics and sensitivity analysis program code of D. A. Bittker and K. Radhakrishnan. This model consists of 45 chemical reactions and 27 species. The other model is based on the work published by C. K. Westbrook and F. L. Dryer.

Nguyen, H. L.↗

A Method for Assessing the Quality of Model-Based Estimates of Ground Temperature and Atmospheric Moisture Using Satellite Data

A method is developed for validating model-based estimates of atmospheric moisture and ground temperature using satellite data. The approach relates errors in estimates of clear-sky longwave fluxes at the top of the Earth-atmosphere system to errors in geophysical parameters. The fluxes include clear-sky outgoing longwave radiation (CLR) and radiative flux in the window region between 8 and 12 microns (RadWn). The approach capitalizes on the availability of satellite estimates of CLR and RadWn and other auxiliary satellite data, and multiple global four-dimensional data assimilation (4-DDA) products. The basic methodology employs off-line forward radiative transfer calculations to generate synthetic clear-sky longwave fluxes from two different 4-DDA data sets. Simple linear regression is used to relate the clear-sky longwave flux discrepancies to discrepancies in ground temperature ((delta)T(sub g)) and broad-layer integrated atmospheric precipitable water ((delta)pw). The slopes of the regression lines define sensitivity parameters which can be exploited to help interpret mismatches between satellite observations and model-based estimates of clear-sky longwave fluxes. For illustration we analyze the discrepancies in the clear-sky longwave fluxes between an early implementation of the Goddard Earth Observing System Data Assimilation System (GEOS2) and a recent operational version of the European Centre for Medium-Range Weather Forecasts data assimilation system. The analysis of the synthetic clear-sky flux data shows that simple linear regression employing (delta)T(sub g)) and broad layer (delta)pw provides a good approximation to the full radiative transfer calculations, typically explaining more thin 90% of the 6 hourly variance in the flux differences. These simple regression relations can be inverted to "retrieve" the errors in the geophysical parameters, Uncertainties (normalized by standard deviation) in the monthly mean retrieved parameters range from 7% for (delta)T(sub g) to approx. 20% for the lower tropospheric moisture between 500 hPa and surface. The regression relationships developed from the synthetic flux data, together with CLR and RadWn observed with the Clouds and Earth Radiant Energy System instrument, ire used to assess the quality of the GEOS2 T(sub g) and pw. Results showed that the GEOS2 T(sub g) is too cold over land, and pw in upper layers is too high over the tropical oceans and too low in the lower atmosphere.

Wu, Man Li C.↗

Multidisciplinary research in the space sciences

Research activities were carried out in the following areas during this reporting period: (1) astrophysics; (2) climate and atmospheric modeling; and (3) climate applications of earth observations & geological studies. An ultra-low-noise 115 GHz receiver based upon a superconducting tunnel diode mixer has been designed and constructed. The first laboratory tests have yielded spectacular results: a single-sideband noise temperature of 75 K considerably more sensitive than any other receiver at this frequency. The receiver will replace that currently in use on the Columbia-GISS CO Sky Survey telescope. The 1.2 meter millimeter-wave telescope at Columbia University has been used to complete two large-scale surveys of molecular matter in the part of the inner galaxy which is visible from the Northern hemisphere (the first galactic quadrant); one of the distant galaxy and one of the solar neighborhood. The research conducted during the past year in the climate and atmospheric modeling programs has been focused on the development of appropriate atmospheric and upper ocean models, and preliminary applications of these models. Principal models are a one-dimensional radiative-convective model, a three-dimensional global climate model, and an upper ocean model. During the past year this project has focused on development of 2-channel satellite analysis methods and radiative transfer studies in support of multichannel analysis techniques.

Broecker, W. S.↗

Joint M3 and Diviner Analysis of the Mineralogy, Glass Composition, and Country Rock Content of Pyroclastic Deposits in Oppenheimer Crater

Here we present our analysis of the near- and mid-infrared spectral properties of pyroclastic deposits within the floor fractured Oppenheimer Crater that are hypothesized to be Vulcanian in origin. These are the first results of our global study of lunar pyroclastic deposits aimed at constraining the range of eruption processes on the Moon. In the near-infrared, we have employed a new method of spectral analysis developed in Horgan et al. (2013) of the 1 m iron absorption band in Chandrayaan-1 Moon Mineralogy Mapper (M3) spectra. By analyzing both the position and shape of the 1 m band we can detect and map the distribution of minerals, glasses, and mixtures of these phases in pyroclastic deposits. We are also using mid-infrared spectra from the Lunar Reconnaissance Orbiter Diviner Lunar Radiometer Experiment to develop ~200 m/pixel Christiansen Feature (CF) maps, which correlate with silica abundance. One of the benefits of using CF maps for analysis of pyroclastic deposits is that they can be used to detect silicic country rock that may have been emplaced by Vulcanian-style eruptions, and are sensitive to iron abundance in glasses, neither of which is possible in the near-infrared. M3 analysis reveals that the primary spectral endmembers are low-calcium pyroxene and iron-bearing glass, with only minor high-calcium pyroxene, and no detectable olivine. The large deposit in the south shows higher and more extensive glass concentrations than the surrounding deposits. We interpret the M3 spectra of the pyroclastic deposits as indicating a mixture of low-calcium pyroxene country rock and juvenile glass, and no significant olivine. Analysis of Diviner CF maps of the Oppenheimer crater floor indicates an average CF value of 8.16, consistent with a mixture of primarily plagioclase and some pyroxene. The average CF values of the pyroclastic deposits range from 8.31 in the SW to 8.24 in the SE. Since CF values within the deposits are as high as 8.49, the lower average CF values of the deposits suggest that each deposit is a mixture of crater floor material and highly mafic juvenile material consistent with either olivine or Fe-bearing pyroclastic glass. Synthesizing our M3 and Diviner results indicates that the crater floor consists of plagioclase with some pyroxene, and the pyroclastic deposits are a mix of this substrate and a glass-rich juvenile material. While we cannot determine the iron content of the glass from M3 spectra alone, the high Diviner CF values suggest that the glass is relatively iron-rich. Indeed, FeO abundances inferred from CF values using the method of Allen et al. (2012) imply that the large southern deposit exhibits a significant enhancement in iron content. This supports our hypothesis that the glass in this deposit is relatively iron-rich.

Bennett, Kristen A.↗

Assessing Global Surface Water Inundation Dynamics Using Combined Satellite Information from SMAP, AMSR2 and Landsat

A method to assess global land surface water (fw) inundation dynamics was developed by exploiting the enhanced fw sensitivity of L-band (1.4 GHz) passive microwave observations from the Soil Moisture Active Passive (SMAP) mission. The L-band fw (fw(sub LBand)) retrievals were derived using SMAP H-polarization brightness temperature (Tb) observations and predefined L-band reference microwave emissivities for water and land endmembers. Potential soil moisture and vegetation contributions to the microwave signal were represented from overlapping higher frequency (Tb) observations from AMSR2. The resulting (fw(sub LBand)) global record has high temporal sampling (1-3 days) and 36-km spatial resolution. The (fw(sub LBand)) annual averages corresponded favourably (R=0.84, p<0.001) with a 250-m resolution static global water map (MOD44W) aggregated at the same spatial scale, while capturing significant inundation variations worldwide. The monthly (fw(sub LBand)) averages also showed seasonal inundation changes consistent with river discharge records within six major US river basins. An uncertainty analysis indicated generally reliable (fw(sub LBand)) performance for major land cover areas and under low to moderate vegetation cover, but with lower accuracy for detecting water bodies covered by dense vegetation. Finer resolution (30-m) (fw(sub LBand)) results were obtained for three sub-regions in North America using an empirical downscaling approach and ancillary global Water Occurrence Dataset (WOD) derived from the historical Landsat record. The resulting 30-m (fw(sub LBand)) retrievals showed favourable spatial accuracy for water (70.71%) and land (98.99%) classifications and seasonal wet and dry periods when compared to independent water maps derived from Landsat-8 imagery. The new (fw(sub LBand)) algorithms and continuing SMAP and AMSR2 operations provide for near real-time, multi-scale monitoring of global surface water inundation dynamics and potential flood risk.

WOD↗

Validation of Carbon Trace Gas Profile Retrievals from the NOAA-Unique Combined Atmospheric Processing System for the Cross-Track Infrared Sounder

This paper provides an overview of the validation of National Oceanic and Atmospheric Administration (NOAA) operational retrievals of atmospheric carbon trace gas profiles, specifically carbon monoxide (CO), methane (CH4) and carbon dioxide (CO2), from the NOAA-Unique Combined Atmospheric Processing System (NUCAPS), a NOAA enterprise algorithm that retrieves atmospheric profile environmental data records (EDRs) under global non-precipitating (clear to partly cloudy) conditions. Vertical information about atmospheric trace gases is obtained from the Cross-track Infrared Sounder (CrIS), an infrared Fourier transform spectrometer that measures high resolution Earth radiance spectra from NOAA operational low earth orbit (LEO) satellites, including the Suomi National Polar-orbiting Partnership (SNPP) and follow-on Joint Polar Satellite System (JPSS) series beginning with NOAA-20. The NUCAPS CO, CH4, and CO2 profile EDRs are rigorously validated in this paper using well-established independent truth datasets, namely total column data from ground-based Total Carbon Column Observing Network (TCCON) sites, and in situ vertical profile data obtained from aircraft and balloon platforms via the NASA Atmospheric Tomography (ATom) mission and NOAA AirCore sampler, respectively. Statistical analyses using these datasets demonstrate that the NUCAPS carbon gas profile EDRs generally meet JPSS Level 1 global performance requirements, with the absolute accuracy and precision of CO 5% and 15%, respectively, in layers where CrIS has vertical sensitivity; CH4 and CO2 product accuracies are both found to be within ±1%, with precisions of ≈1.5% and ⪅0.5%, respectively, throughout the tropospheric column.

satellite cal/val; error analysis; greenhouse gase↗

How emissions uncertainty influences the distribution and radiative impacts of smoke from fires in North America

Fires and the aerosols that they emit impact air quality, health, and climate, but the abundance and properties of carbonaceous aerosol (both black carbon and organic carbon) from biomass burning (BB) remain uncertain and poorly constrained. We aim to explore the uncertainties associated with fire emissions and their air quality and radiative impacts from underlying dry matter consumed and emissions factors. To investigate this, we compare model simulations from a global chemical transport model, GEOS-Chem, driven by a variety of fire emission inventories with surface and airborne observations of black carbon (BC) and organic aerosol (OA) concentrations and satellite-derived aerosol optical depth (AOD). We focus on two fire-detection-based and/or burned-area-based (FD-BA) inventories using burned area and active fire counts, respectively, i.e., the Global Fire Emissions Database version 4 (GFED4s) with small fires and the Fire INventory from NCAR version 1.5 (FINN1.5), and two fire radiative power (FRP)-based approaches, i.e., the Quick Fire Emission Dataset version 2.4 (QFED2.4) and the Global Fire Assimilation System version 1.2 (GFAS1.2). We show that, across the inventories, emissions of BB aerosol (BBA) differ by a factor of 4 to 7 over North America and that dry matter differences, not emissions factors, drive this spread. We find that simulations driven by QFED2.4 generally overestimate BC and, to a lesser extent, OA concentrations observations from two fire-influenced aircraft campaigns in North America (ARCTAS and DC3) and from the Interagency Monitoring of Protected Visual Environments (IMPROVE) network, while simulations driven by FINN1.5 substantially underestimate concentrations. The GFED4s and GFAS1.2-driven simulations provide the best agreement with OA and BC mass concentrations at the surface (IMPROVE), BC observed aloft (DC3 and ARCTAS), and AOD observed by MODIS over North America. We also show that a sensitivity simulation including an enhanced source of secondary organic aerosol (SOA) from fires, based on the NOAA Fire Lab 2016 experiments, produces substantial additional OA; however, the spread in the primary emissions estimates implies that this magnitude of SOA can be neither confirmed nor ruled out when comparing the simulations against the observations explored here. Given the substantial uncertainty in fire emissions, as represented by these four emission inventories, we find a sizeable range in 2012 annual BBA PM2.5 population-weighted exposure over Canada and the contiguous US (0.5 to 1.6 µg/cu. m). We also show that the range in the estimated global direct radiative effect of carbonaceous aerosol from fires (−0.11 to −0.048 W/sq. m) is large and comparable to the direct radiative forcing of OA (−0.09 W/sq. m) estimated in the Fifth Assessment Report (AR5) of the Intergovernmental Panel on Climate Change (IPCC). Our analysis suggests that fire emissions uncertainty challenges our ability to accurately characterize the impact of smoke on air quality and climate.

North America↗

Astronaut Photography of Coral Reefs

Astronaut photographs of tropical coastal areas may contain information on submerged features, including coral reefs, up to depths of about 15 m in clear waters. Previous research efforts have shown that astronaut photographs can aid in estimating coral reef locations and extent on national, regional and global scales, and allow characterization of major geomorphological rim and lagoon features (Andrefouet et al. 2000, in preparation). They can be combined with traditional satellite data to help distinguish between clouds and lagoon features such as pinnacles (Andrefouet and Robinson, in review). Furthermore, astronaut photographs may provide reef scientists and managers with information on the location and extent of river plumes and sediment run off, or facilitate identification of land cover types, including mangroves (Webb et al., in press). Photographs included in the section were selected based on several criteria. The primary consideration of the editors was that the photographs represent a worldwide distribution of coral reefs, have extremely low visual interference by cloud cover, and display a spatial scale reasonable for examining reef-related features. Once photographs were selected, they were digitized from 2nd generation copies. The color and contrast were hand corrected to an approximation of natural color (required to account for spectral differences between photographs due to the color sensitivities of films used, and differences in sun angle and exposure of the photographs). None of the photographs shown here have been georeferenced to correct them to a map projection and scale. Any distortions in features due to slightly oblique look angles when the photographs were taken through spacecraft windows remain. When feasible, near vertical photographs have been rotated so that north is toward the top. An approximate scale bar and north arrow have added using distinctive features on each photograph with reference to a 1:1,000,000 scale navigation chart. Astronaut photographs provide a unique source of moderate resolution reef remote sensing data because of their global coverage and (immediate) availability in the public domain. The database of photographs can be searched an browsed online and high-resolution digital copies of photographs in this atlas can be accessed via the Website of Earth Science and Image Analysis at NASA's Johnson Space Center:

Robinson, Julie A.↗

BOREAS (Boreal Ecosystem-Atmosphere Study): Global change and biosphere-atmosphere interactions in the boreal forest

The Boreal Ecosystems Atmosphere Study (BOREAS) is a cooperative field and analysis project involving elements of land surface climatology, tropospheric chemistry, and terrestrial ecology. The goal of the study is to understand the interactions between the boreal forest biome and the atmosphere in order to clarify their roles in global change. The study will be centered on two 20 by 20 km sites within the North American boreal forest region, located near the northern and southern limits of the biome. Studies based at these sites will be used to explore the roles of various environmental factors in controlling the extent and character of the biome. The sites will be the subject of surface, airborne, and satellite based observations which aim to improve understanding of the biological and physical processes and states which govern the exchanges of energy, water, carbon, and trace gases between boreal forest ecosystems and the atmosphere. Particular reference will be made to those processes and states that may be sensitive to global change. The study also aims to develop the use of remote sensing techniques to transfer understanding of the above process from local scales out to regional scales. The BOREAS project is being planned for 1992-1996, with a major field effort in 1994.

Sellers, Piers J.↗

GEOS Constituent Data Assimilation Beyond Aura MLS: Assimilating NASA SAGE III/ISS Profiles of Stratospheric Water Vapor

Ozone and water vapor in the lower stratosphere are important trace gases for atmospheric chemistry and radiative budget. The Stratospheric Aerosol and Gas Experiment (SAGE) missions have been crucial in monitoring the stratospheric ozone loss and the subsequent recovery as well as the trends in water vapor linked to surface temperature trends. The SAGE III instrument aboard the International Space Station (ISS) continues the SAGE mission record, with high vertical resolution profiles of ozone and water vapor available since mid 2017. The NASA GEOS Earth system model has the new capability to assimilate multi-constituents from ground and space-based instruments using the GEOS Constituent Data Assimilation System (CoDAS). The recently released MERRA-2 Stratospheric Composition Reanalysis with Aura MLS (M2-SCREAM) assimilates version 4.2 MLS ozone, water vapor and other chemically-reactive species with the NASA GEOS model coupled to a stratospheric-only chemistry mechanism and transport constrained to the MERRA-2 reanalysis. While the number of solar occultation observations a day from SAGE III/ISS is about 1% of the total number of profiles observed globally by MLS, the chemical timescales of ozone and water vapor in the lower stratosphere are long enough that the SAGE III/ISS data may provide a useful constraint on the assimilated product. Using the same GEOS CoDAS configuration as M2-SCREAM, we will present a series of experiments to investigate if water vapor trends are consistent with the assimilation of SAGE observations with and without Aura retrievals, and to determine if the assimilation of SAGE observations produces a steady product for trend analysis, especially as the end of the Aura mission nears. In our experiments, assimilating only SAGE III/ISS water vapor profiles results in water vapor fields more consistent with experiments that assimilate MLS v5; however, in the polar regions SAGE III/ISS observations are not available and the modelled values are unconstrained. We are encouraged by the positive benefit assimilating the less frequent SAGE III/ISS observations has on stratospheric composition. Sensitivity experiments such as these will allow us to assess the added value of SAGE data for continued monitoring of the stratospheric composition for climate and ozone recovery assessments.

K Emma Knowland↗

Use of Radon for Evaluation of Atmospheric Transport Models: Sensitivity to Emissions

This paper presents comparative analyses of atmospheric radon (Rn) distributions simulated using different emission scenarios and the observations. Results indicate that the model generally reproduces observed distributions of Rn but there are some biases in the model related to differences in large-scale and convective transport. Simulations presented here use an off-line three-dimensional chemical transport model driven by assimilated winds and two scenarios of Rn fluxes (atom/cm s) from ice-free land surfaces: (A) globally uniform flux of 1.0, and (B) uniform flux of 1.0 between 60 deg. S and 30 deg. N followed by a sharp linear decrease to 0.2 at 70 deg. N. We considered an additional scenario (C) where Rn emissions for case A were uniformly reduced by 28%. Results show that case A overpredicts observed Rn distributions in both hemispheres. Simulated northern hemispheric (NH) Rn distributions from cases B and C compare better with the observations, but are not discernible from each other. In the southern hemisphere, surface Rn distributions from case C compare better with the observations. We performed a synoptic scale source-receptor analysis for surface Rn to locate regions with ratios B/A and B/C less than 0.5. Considering an uncertainty in regional Rn emissions of a factor of two, our analysis indicates that additional measurements of surface Rn particularly during April-October and north of 50 deg. N over the Pacific as well as Atlantic regions would make it possible to determine if the proposed latitude gradient in Rn emissions is superior to a uniform flux scenario.

Gupta, Mohan L.↗

GEOS Constituent Data Assimilation Beyond Aura MLS: Assimilating NASA SAGE III/ISS Profiles of Stratospheric Water Vapor and Ozone

Ozone and water vapor in the lower stratosphere are important trace gases for atmospheric chemistry and radiative budget. The Stratospheric Aerosol and Gas Experiment (SAGE) missions have been crucial in monitoring the stratospheric ozone loss and the subsequent recovery as well as the trends in water vapor linked to surface temperature trends. The SAGE III instrument aboard the International Space Station (ISS) continues the SAGE mission record, with high vertical resolution profiles of ozone and water vapor available since mid 2017. The NASA GEOS Earth system model has the new capability to assimilate multi-constituents from ground and space-based instruments using the GEOS Constituent Data Assimilation System (CoDAS). The recently released MERRA-2 Stratospheric Composition Reanalysis with Aura MLS (M2-SCREAM) assimilates version 4.2 MLS ozone, water vapor and other chemically-reactive species with the NASA GEOS model coupled to a stratospheric-only chemistry mechanism and transport constrained to the MERRA-2 reanalysis. While the number of solar occultation observations a day from SAGE III/ISS is about 1% of the total number of profiles observed globally by MLS, the chemical timescales of ozone and water vapor in the lower stratosphere are long enough that the SAGE III/ISS data may provide a useful constraint on the assimilated product. Using the same GEOS CoDAS configuration as M2-SCREAM, we will present a series of experiments to investigate if ozone and water vapor trends are consistent with the assimilation of SAGE observations with and without Aura retrievals, and to determine if the assimilation of SAGE observations produces a steady product for trend analysis, especially as the end of the Aura mission nears. In our experiments, assimilating only SAGE III/ISS water vapor profiles results in water vapor fields more consistent with experiments that assimilate MLS v5; however, in the polar regions SAGE III/ISS observations are not available and the values are unconstrained. We are encouraged by the positive benefit assimilating the less frequent SAGE III/ISS observations has on stratospheric composition. Sensitivity experiments such as these will allow us to assess the added value of SAGE data for continued monitoring of the stratospheric composition for climate and ozone recovery assessments.

SAGE↗

Re-Evaluation of Low Cloud Amount Relationships With Lower-Tropospheric Stability and Estimated Inversion Strength

Lower-tropospheric stability (LTS) and estimated inversion strength (EIS) have a widely accepted relationship with low cloud amount and are key observational foundations for understanding and modeling low-level stratiform clouds. Using the updated surface-based and satellite cloud data, we find that low cloud amount is not as strongly correlated with LTS, and not as sensitive to LTS, as established in the past. EIS does not provide a stronger correlation with low cloud amount than LTS over all eight regions (including the midlatitudes). Further analyzing the relationships between LTS and EIS with different types of low clouds, we find that there is a strong correlation of LTS and EIS with stratocumulus only. This explains the weaker correlation of low cloud fraction (including cumulus, stratocumulus, and stratus) to both LTS and EIS. These results also suggest the need to re-evaluate these relationships in Earth system models. Plain Language Summary: Low-level clouds play an important role in the global radiation budget. Low cloud amount has two established linear relationships with lower-tropospheric stability (LTS) and estimated inversion strength (ETS). These two relationships are re-evaluated here using three separate observational cloud and two reanalysis datasets for three distinct but overlapping time periods. The analysis shows that the strength of the LTS and ETS relationships with low cloud amount varies, depending on the cloud data used. They have a strong relationship with stratocumulus cloud amount only.

Lauren Cutler↗

Optimized Profile Retrievals of Aerosol Microphysical Properties from Simulated Spaceborne Multiwavelength Lidar

This work is an expanded study of one previously published onretrievals of aerosol microphysical properties from space-borne multiwavelengthlidarmeasurements. The earlier studiesand this one weredone in the framework of the NASA Aerosol-Clouds-Ecosystems (now the Aerosol Clouds Convection and Precipitation) NASA mission. The focus here is on the capabilities of a simulated spacebornemultiwavelengthlidar system for retrieving aerosol complex refractive index (m = mr+ imi) and spectral single scattering albedo (SSA(λ)), although other bulk parameters such as effective (reff) radius and particle volume (V) and surface (S) concentrations are also studied. The novelty presented here is the use of recently published, case dependent optimized-constraints on the microphysical retrievals using three backscattering coefficients (β) at 355, 532 and 1064 nm and two extinction coefficients (α) at 355 and 532 nm, typically known as the stand-alone 3β+2α lidar inversion. Case-dependent optimized-constraints (CDOC) limit the ranges of refractive index, both real (mr) and imaginary (mi) parts, and of radii that are permitted in the retrievals. Such constraints are selected directly from the 3β+2α41measurements through an analysis of the relationship between spectral dependence of aerosol extinction-to-backscatter ratios (LR) and the Ångström exponent of extinction. The analyses presented here for different sets ofsize distributions and refractive indices reveal that the direct determination of CDOCareonly feasible for cases where the uncertaintiesin the input optical data areless than 15 %.Forthe same simulated spacebornesystem and yield than in Whiteman et al., (2018), we demonstrated that the use of CDOC as essential for the retrievals of refractive index and also largely improved retrieval of bulk parameters. A discussion of the global representativeness of CDOC is presented using simulated lidar data from a 24-hour satellite track using GEOS model output to initialize the lidar simulator.We found that CDOCare representative of many aerosol mixtures in spite of some outliers (e.g. highly hydrated particles) associatedwith the assumptions of bimodal size distributions and of the same refractive index for fine and coarse modes. Moreover, sensitivity tests performed using synthetic data reveal that retrievals of imaginary refractive index (mi) and SSA are extremely sensitive to β(355).

NASA Aerosol-Clouds-Ecosystems↗

The Geoscience Laser Altimeter System (GLAS) for the ICESAT Mission

The Laser In space Technology Experiment, Shuttle Laser Altimeter and the Mars Observer Laser Altimeter have demonstrated accurate measurements of atmospheric backscatter and Surface heights from space. The recent MOLA measurements of the Mars surface have 40 cm vertical resolution and have reduced the global uncertainty in Mars topography from a few km to about 5 m. The Geoscience Laser Altimeter System (GLAS) is a next generation lidar for Earth orbit being developed as part of NASA's Icesat Mission. The GLAS design combines a 10 cm precision surface lidar with a sensitive dual wavelength cloud and aerosol lidar. GLAS will precisely measure the heights of the Earth's polar ice sheets, establish a grid of accurate height profiles of the Earth's land topography, and profile the vertical backscatter of clouds and aerosols on a global scale. GLAS is being developed to fly on a small dedicated spacecraft in a polar orbit with a 590 630 km altitude at inclination of 94 degrees. GLAS is scheduled to launch in the summer 2001 and to operate continuously for a minimum of 3 years with a goal of 5 years. The primary mission for GLAS is to measure the seasonal and annual changes in the heights of the Greenland and Antarctic ice sheets. GLAS will continuously measure the vertical distance from orbit to the Earth's surface with 1064 nm pulses from a ND:YAG laser at a 40 Hz rate. Each 5 nsec wide laser pulse is used to produce a single range measurement, and the laser spots have 66 m diameter and about 170 m center-center spacings. When over land GLAS will profile the heights of the topography and vegetation. The GLAS receiver uses a 1 m diameter telescope and a Si APD detector. The detector signal is sampled by an all digital receiver which records each surface echo waveform with I nsec resolution and a stored echo record lengths of either 200, 400, or 600 samples. Analysis of the echo waveforms within the instrument permits discrimination between cloud and surface echoes. Ground based echo analysis permits precise ranging, determining the roughness or slopes of the surface as well as the vertical distributions of vegetation illuminated by the laser. Accurate knowledge of the laser beam's pointing angle is needed to prevent height biases when over sloped surfaces. For surfaces with 2 deg. slopes, knowledge of pointing angle of the beam's centroid to about 8 urad is needed to achieve 10 cm height accuracy. GLAS uses a stellar reference system (SRS) to determine the pointing angle of each laser firing relative to inertial space. The SRS uses a high precision star camera oriented toward local zenith and a gyroscope to determine the inertial orientation of the SRS optical bench. The far field pattern of each laser is measured pulse relative to the star camera with a laser reference system (LRS). Optically measuring each laser far field pattern relative to the orientation of the star camera and gyroscope permits the precise pointing angle of each laser pulse to be determined. GLAS will also determine the vertical distributions of clouds and aerosols by measuring the vertical profile of laser energy backscattered by the atmosphere at both 1064 and 532 nm. The 1064 nm measurements use the Si APD detector and profile the height and vertical structure of thicker clouds. The measurements at 532 nm use new highly sensitive photon counting, detectors, and measure the height distributions of very thin Clouds and aerosol layers. With averaging these can be used to determine the height of the planetary boundary layer. The instrument design and expected performance will be discussed.

Abshire, James B.↗