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All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Semi-Annual Report for Modular Integrated Gas High Temperature Reactor Development during Performance Period April 2022 - September 2022

Horizontal Compact High Temperature Gas Reactor (HC-HTGR) is being designed by a multidisciplinary team of nuclear, mechanical, and structural engineers under the support of a DOE-NE Advanced Reactor Demonstration Program’s Advanced Reactor Concepts-20 (ARC-20) award. The objective of this ARC-20 project is to deliver a conceptual design for the proposed HC-HTGR in 3 years and support its commercialization as a safe, low-cost HTGR. Argonne National Laboratory (Argonne) is responsible for the design and analysis of the reactor cavity cooling system (RCCS) as a safety system for passive decay heat removal of the reactor concept. Additionally, Argonne is providing analysis of the primary coolant system to ensure temperatures within the core remain below safety margins during steady-state and potential accident scenarios. This second semi-annual report summarized the progress made at Argonne on the two tasks during the second half of FY22. As a part of the RCCS design task, a scoping calculation in estimating HVAC capability for the HC-HTGR reactor building was performed. A water panel modeling study was first performed with the test case, which confirms the capability of the RELAP5-3D modeling approach to explore various design options of the HC-HTGR RCCS under consideration. Then, a reference RELAP5-3D model for the unit geometry of the preliminary design of the HC-HTGR RCCS was developed. A preliminary performance analysis was conducted to evaluate the performances of a single-phase natural circulation and panel conduction in various operating conditions. For the primary coolant system analysis task, preliminary thermal hydraulic analysis of the HC-HTGR core design was performed with a high resolution 1D fluid-3D solid coupled model using the System Analysis Module (SAM) to assess the assembly coolant channel and bypass flow mass flow rate distribution. Some preliminary work on the development of a full core reduced order model was discussed following the assembly level model to predict the core wide coolant flow distribution and to model certain operational and accidental transients.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2019

AGR-5/6/7 Release-to-Birth Ratio Data Analysis for Cycles 162B, 163A, 164A, and 164B

AGR-5/6/7 is the last of a series of Advanced Gas Reactor (AGR) experiments conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory in support of development and qualification of tristructural isotropic (TRISO) low-enriched fuel used in the high-temperature gas cooled reactor (HTGR). Each AGR test consists of multiple independently controlled and monitored capsules containing fuel compacts placed in a graphite cylinder shrouded by a steel shell. These capsules are instrumented with thermocouples (TC) that are embedded in the graphite, thus providing feedback for temperature control. AGR configuration and irradiation conditions are based on prismatic HTGR technology that is distinguished primarily through use of helium coolant, a low-power-density ceramic core capable of withstanding very high temperatures, and TRISO-coated particle fuel. The AGR tests provide valuable irradiation-performance data to support fuel process development, qualify fuel for normal operation and accident conditions, and support development and validation of fuel performance and fission-product transport models and codes. The release-to-birth ratios (R/B) for fission-gas isotopes (i.e., krypton and xenon) are calculated from release rates into the sweep-gas flow, measured by the high-purity germanium detectors used in the AGR Fission Product Monitoring System (FPMS) installed downstream from each irradiated capsule. Birth rates are calculated based on the fission power in the experiment and models of fission-product generation. Thus, the R/B is a measure of the ability of fuel kernel, particle coating layers, and compact matrix to retain fission-gas atoms, preventing their release into the sweep-gas flow, especially in the presence of initially defective particle and/or the event of particle-coating failures that occurred during the irradiation. For fission-gas isotopes, particle failure occurred when all coating layers are fractured that allow gaseous fission atoms to escape from a particle. In this case, the R/B per-exposed-kernel is used to compare fuel performance across experiments.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2014

AGR-2 and AGR-3/4 Release-to-Birth Ratio Data Analysis

A series of Advanced Gas Reactor (AGR) irradiation tests is being conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL) in support of development and qualification of tristructural isotropic (TRISO) low enriched fuel used in the High Temperature Gas-cooled Reactor (HTGR). Each AGR test consists of multiple independently controlled and monitored capsules containing fuel compacts placed in a graphite cylinder shrouded by a steel shell. These capsules are instrumented with thermocouples embedded in the graphite enabling temperature control. AGR configuration and irradiation conditions are based on prismatic HTGR technology that is distinguished primarily through use of helium coolant, a low-power-density ceramic core capable of withstanding very high temperatures, and TRISO coated particle fuel. Thus, these tests provide valuable irradiation performance data to support fuel process development, qualify fuel for normal operating conditions, and support development and validation of fuel performance and fission product transport models and codes.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2015

Thermal Predictions of the AGR-3/4 Experiment With Time-Varying Gas Gaps

In this paper, a thermal analysis was performed for the Advanced Gas Reactor test experiment (AGR-3/4) with time-varying gas gaps. The experiment was irradiated at the Advanced Test Reactor (ATR) at the Idaho National Laboratory (INL). Several fuel irradiation experiments are planned for the AGR Fuel Development and Qualification Program that supports the development of the Very-High-Temperature Gas-Cooled Reactor (VHTR) under the Next-Generation Nuclear Plant (NGNP) project. AGR-3/4 combines two tests in a series of planned AGR experiments to test tristructural-isotropic (TRISO)-coated, low-enriched uranium oxy-carbide fuel. Forty-eight TRISO-fueled compacts were inserted into 12 separate capsules for the experiment (four compacts per capsule). The purpose of this analysis was to calculate the temperatures of each compact and graphite layer to obtain daily average temperatures using time (fast neutron fluence)-varying gas gaps and to compare with experimentally measured thermocouple data. A finite-element heat transfer model was created for each capsule using the commercial code ABAQUS. Finally, model results are compared to thermocouple data taken during the experiment.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2014

AGR-2 safety test predictions using the PARFUME code

This report documents calculations performed to predict failure probability of TRISO-coated fuel particles and diffusion of fission products through these particles during safety tests following the second irradiation test of the Advanced Gas Reactor program (AGR-2). The calculations include the modeling of the AGR-2 irradiation that occurred from June 2010 to October 2013 in the Advanced Test Reactor (ATR) and the modeling of a safety testing phase to support safety tests planned at Oak Ridge National Laboratory and at Idaho National Laboratory (INL) for a selection of AGR-2 compacts. The heat-up of AGR-2 compacts is a critical component of the AGR-2 fuel performance evaluation, and its objectives are to identify the effect of accident test temperature, burnup, and irradiation temperature on the performance of the fuel at elevated temperature. Safety testing of compacts will be followed by detailed examinations of the fuel particles to further evaluate fission product retention and behavior of the kernel and coatings. The modeling was performed using the particle fuel model computer code PARFUME developed at INL. PARFUME is an advanced gas-cooled reactor fuel performance modeling and analysis code (Miller 2009). It has been developed as an integrated mechanistic code that evaluates the thermal, mechanical, and physico-chemical behavior of fuel particles during irradiation to determine the failure probability of a population of fuel particles given the particle-to-particle statistical variations in physical dimensions and material properties that arise from the fuel fabrication process, accounting for all viable mechanisms that can lead to particle failure. The code also determines the diffusion of fission products from the fuel through the particle coating layers, and through the fuel matrix to the coolant boundary. The subsequent release of fission products is calculated at the compact level (release of fission products from the compact). PARFUME calculates the release fraction as the ratio of the number of atoms released from the compact to the amount produced in the compact fuel kernels and through uranium contamination. These safety test predictions aim at giving guidance for the upcoming safety tests to be conducted at ORNL and INL. The AGR-2 compacts modeled in this study belong to the four U.S. capsules of the AGR-2 irradiation test train. For each capsule, the compacts with the lowest and highest burnups were selected to provide a prediction envelope. The objective of this document is to present results of calculations and analyses made by PARFUME on these selected AGR-2 compacts. These results include: • Fuel failure probability • Palladium penetration • Fractional release of fission products Details associated with completion of these calculations are provided in the remainder of this document: the AGR-2 Safety Testing plan is briefly introduced in Section 2, PARFUME modeling is outlined in Section 3, results are described in Section 4, conclusions are given in Section 5, and references are listed in Section 6.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2022

Delivery of Dynamic Thermal Energy Storage Models and Advanced Reactor Concept Models to the HYBRID Repository

This publication details newly created energy storage and reactor models developed within the HYBRID modeling repository as part of the Department of Energy Office of Nuclear Energy (DOE-NE) Integrated Energy Systems (IES) program, led by Idaho National Laboratory (INL). Model development to-date includes creation of dynamic systems-level models of a pebble bed high temperature gas reactor (HTGR), sodium fast reactor (SFR), compressed air energy storage (CAES), liquid air energy storage (LAES) and Modelica standard library based two-tank sensible heat storage (SHS) in the IES-based HYBRID repository. Models are developed using the latest publicly available data and incorporate the possibility of control strategy inclusion for use with the existing IES modeling, analysis, and optimization toolset. Simulations showcase the abilities of each technology to flexibly operate in ways consistent with IES operation expectations. When these models are available, they can be utilized within different integrated energy park concepts to understand optimal system operation, control, and dispatching. Moreover, given the generic nature of the models, industrial partner technologies can be quickly added to the repository using the existing models as a basis. Additional dynamic models for thermal energy storage concepts can be developed and added to the HYBRID repository as needed. Also detailed in this report are future development goals for the HYBRID repository including adding suites of steady-state models, economic costing information, and reduced-order models. By adding these models in addition to the physical transient models currently existing within HYBRID, HYBRID will be a fully integrable tool for FORCE users.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗
DOE OSTI2023

Toward local core outlet temperature monitoring in gas-cooled nuclear reactors using distributed fiber-optic temperature sensors

Gas-cooled nuclear reactors operate at temperatures up to 950 °C with significant spatial variations in power generation and coolant flow through hundreds of parallel flow channels, resulting in complex mixing at the core outlet. The high temperatures and complex mixing can damage downstream components, challenge reactor calorimetry for power determination, and result in significant conservatism in calculated peak fuel temperatures, which ultimately limits the total power output. Directly measuring each gas stream individually is unrealistic using single point thermocouples, requiring more robust sensing techniques. Fiber-optic sensors are resilient to high temperatures (up to 1,000 °C) and radiation damage. Moreover, distributed measurements can be made along the length of one fiber, making them potential candidates for monitoring local core outlet temperatures to improve core calorimetry and identify hot channels. Here, to the authors’ knowledge, this manuscript is the first to report spatially distributed fiber optic temperature measurements to quantify mixing at the outlet of a relevant orifice plate under prototypic temperature and flow regimes to assess the feasibility of using fiber-optic sensors for distributed measurements of coolant temperature in gas-cooled reactors. A single optical fiber captured dynamic changes in local temperatures, whereas the mixed outlet temperature exhibited a muted response and could not identify which channels were responsible for the change in the mixed outlet temperature. The discussion focuses on potential challenges for deploying distributed optical fibers in gas-cooled reactors, including the effects of vibrations, radiation-induced signal attenuation and drift, and routing of the fiber while minimizing flow obstructions.

42 ENGINEERING↗
DOE OSTI2018

AGR-5/6/7 Irradiation Experiment Test Plan

This document presents the test plan for the AGR-5/6/7 irradiation experiment, the combined fifth, sixth, and seventh irradiations of the United States Department of Energy Advanced Gas Reactor (AGR) Fuel Development and Qualification Program. The combined irradiation tests will consist of fuel qualification tests (AGR-5/6) and a margin test (AGR-7) for the industrially produced uranium oxycarbide (UCO) tristructural isotropic (TRISO) coated particle fuel developed by the AGR Program. The objective of the AGR-5/6/7 irradiation experiment is to establish the performance of UCO TRISO fuel fabricated using engineering-scale equipment in a production environment under and beyond normal operating conditions. Specifically, the goals of the AGR 5/6/7 irradiation experiment are: 1. Irradiate reference design fuel containing low-enriched UCO TRISO fuel particles to support fuel qualification. 2. Establish the operating margins for the fuel beyond normal operating conditions. 3. Provide irradiated fuel performance data and irradiated fuel samples for post-irradiation examination and safety testing. 4. Support the refinement of fuel performance and fission product transport models with online, post-irradiation examination and safety test data. In order to achieve the test objectives, the AGR-5/6/7 experiment will be irradiated in the northeast flux trap position of the Advanced Test Reactor at Idaho National Laboratory. The larger diameter of the northeast flux trap provides greater flexibility for test train design, significantly enhancing the capability for the combined irradiations. The test train contains five separate and independently controlled and monitored capsules. The middle capsule contains the AGR 7 margin test fuel. The two bottom and two top capsules contain the AGR 5/6 fuel. Each capsule contains a variable number of fuel compacts filled with UCO TRISO particles.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2020

Cylindricity Sensitivity Thermal Model of the AGR-5/6/7 Experiment in the Advanced Test Reactor

The AGR-5/6/7 experiment is currently being irradiated in the Advanced Test Reactor (ATR) at the Idaho National Laboratory and is approximately 70% complete. Several fuel and material irradiation experiments have been planned for the U.S. Department of Energy Advanced Gas Reactor Fuel Development and Qualification Program, which supports the development and qualification of tristructural isotropic (TRISO) coated particle fuel for use in high-temperature gas-cooled reactors. The goals of these experiments are to provide irradiation performance data to support fuel process development, qualify fuel for normal operating conditions, support development of fuel performance models and codes, and provide irradiated fuel and materials for post-irradiation examination and safety testing. Originally planned and named as separate fuel experiments, but subsequently combined into a single test train, AGR-5/6/7 is testing low-enriched uranium oxycarbide TRISO fuel. The AGR-5/6/7 test train has 5 capsules with thermocouples and independent gas control mixtures. Unique to this paper is a sensitivity study concerning the cylindricity of the graphite holders containing the fuel compacts and their eccentricity in relation to the stainless-steel capsule walls. Each capsule has small nubs on the outside used for centering the graphite holder inside the stainless-steel capsule with a small gas gap used to control temperature. Due to machining tolerances of these nubs and vibration wearing the nubs down when the experiment is running in the reactor, the possibility exists that the holder may move around radially. Each capsule is equipped with several thermocouples placed at various radii and depths within each graphite holder. This paper will show the sensitivity of offsetting the graphite holder for various radii in 45-degree increments around the circle with the objective of minimizing the difference between the measured thermocouples and the modeled thermocouple temperatures. Separate gas mixtures of helium/neon are introduced into this gas gap between the holder and capsule wall and changed as necessary to maintain the desired thermocouple temperatures to keep the fuel compacts at constant temperature as the nuclear reactor conditions change. The goal of the sensitivity study is to find a radius and an angle to offset the holder from perfectly centered for each of the five capsules separately. The complex thermal model includes fission heating, gamma heating, radiation heat transfer, and heat transfer via conduction and radiation across the control gaps. Subroutines linked to the thermal model offer an easy method to offset the graphite holder from the capsule walls without remeshing the entire model.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2018

Effect of Neutron Irradiation Damage on Fission Product Transport in the SiC Layer of TRISO Fuel Particles (HTR2018)

Abstract – Metallic fission products are found to transport through the SiC layer of the tristructural isotropic (TRISO) fuel particle and various studies has been undertaken to understand the transport behavior. It has been recently discovered that the precipitation of intragranular palladium containing fission products in SiC layer of neutron-irradiated TRISO fuel particles occurs via a novel dual-step nucleation mechanism. Direct observations of Pd silicide imprinting into morphological templates of a-SiC precipitates in neutron irradiated SiC layer of TRISO fuel will be discussed with examples from selected particles from both the Advanced Gas Reactor (AGR)-1 (fabricated laboratory-scale at Oak Ridge National Laboratory) and AGR-2 (fabricated at pilot scale by an industrial vendor) experiments. As neutron irradiation damage structures are expected to accelerate the intragranular diffusion kinetics of fission products, their size, shape, density and distribution patterns across the radial thickness of the SiC layer can be directly correlated with the nature of intragranular transport pathways of fission products. In this work, the distinction of neutron irradiation damage structures as a function of fuel type, burnup level and fabrication histories of TRISO coated particles from the AGR-1 and AGR-2 experiments has been studied. The five particles investigated, three AGR-1 and two AGR-2 particles, represent irradiation histories of four fuel types with burnup levels varying from 12.55 to 17.4 % fissions per initial metal atom.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2019

AGR-5/6/7 Fuel Fabrication Report

The Idaho National Laboratory (INL) Advanced Reactor Technologies (ART) program, under contract with the U.S. Department of Energy-Office of Nuclear Energy (DOE-NE), manages the Advanced Gas Reactor (AGR) Fuel Development and Qualification program (referred to as AGR Fuel program hereafter) in pursuing qualification of tristructural isotropic (TRISO) coated-particle fuel for use in high-temperature gas-cooled reactors (HTGRs). The AGR Fuel program was established to provide a fuel-qualification data set in support of the licensing and operation of an HTGR. BWX Technologies Nuclear Operations Group (BWXT-NOG) was subcontracted to fabricate the fuel for the AGR program.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2026

BISON analyses of TRISO fuel performance, its dependence on time-at-temperature, and possible implications for fuel design and qualification

The Advanced Gas Reactor Fuel Development and Qualification (AGR) program has established a substantial technical foundation to support private entry into the U.S. high-temperature gas-cooled reactor market. However, emerging tristructural isotropic (TRISO)-fueled reactor applications include small modular reactors and microreactors with longer fuel residence times, which may expose fuels to higher time-at-temperature (TAT) values than were explored by the AGR program. Increased TAT could affect diffusive and thermomechanical behaviors such as Pd penetration, fission gas release, creep, and fission product transport. In this work, we applied multiscale best-estimate BISON fuel performance modeling to assess these effects within a representative design space based on the AGR-5/6/7 experiment and analyzed trends in predicted particle and compact fuel performance metrics with possible implications for near-term fuel design and qualification. BISON unambiguously predicted that TRISO fuel performance is sensitive to TAT. Increasing TAT was not predicted to increase the magnitude of failure-inducing tangential stresses in particle coating layers. Predictions obtained using a mechanistic model for Pd penetration indicated that penetration depth does not depend strongly on TAT. While these observations suggest that AGR testing provides a conservative upper bound for the steady-state operation of TRISO particles at lower powers and higher residence times, BISON also predicted that the release of poorly retained Ag would increase with TAT. Because these analyses applied models to extrapolate beyond the available experimental data, the authors recommend performing targeted experiments to confirm these predictions. Nevertheless, these predictions may provide reactor developers with enough confidence to make near-term design decisions associated with the potential fuel performance trade-offs of increasing TAT.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2014

Determination of the Quantity of I-135 Released from the AGR Experiment Series

A series of three Advanced Gas Reactor (AGR) experiments have been conducted in the Advanced Test Reactor (ATR) at Idaho National Laboratory (INL). From 2006 through 2014, these experiments supported the development and qualification of the new U.S. tri structural isotropic (TRISO) particle fuel for Very High Temperature Reactors (VHTR). Each AGR experiment consisted of multiple fueled capsules, each plumbed for independent temperature control using a mix of helium and neon gases. The gas leaving a capsule was routed to individual Fission Product Monitor (FPM) detectors. For intact fuel particles, the TRISO particle coatings provide a substantial barrier to fission product release. However, particles with failed coatings, whether because of a minute percentage of initially defective particles, those which fail during irradiation, or those designed to fail (DTF) particles, can release fission products to the flowing gas stream. Because reactive fission product elements like iodine and cesium quickly deposit on cooler capsule components and piping structures as the effluent gas leaves the reactor core, only the noble fission gas isotopes of Kr and Xe tend to reach FPM detectors. The FPM system utilizes High Purity Germanium (HPGe) detectors coupled with a thallium activated sodium iodide NaI(Tl) scintillator. The germanium detector provides individual isotopic information, while the NaI(Tl) scintillator is used as a gross count rate meter. During irradiation, the 135mXe concentration reaching the FPM detectors is from both direct fission and by decay of the accumulated 135I. About ~2.5 hours after irradiation (ten 15.3 minute 135mXe half lives) the directly produced 135mXe has decayed and only the longer lived 135I remains as a source. Decay systematics dictate that 135mXe will be in secular equilibrium with its 135I parent, such that it’s production rate very nearly equals the decay rate of the parent, and its concentration in the flowing gas stream will appear to decay with the parent half life. This equilibrium condition enables the determination of the amount of 135I released from the fuel particles by measurement of the 135mXe at the FPM following reactor shutdown. In this paper, the 135I released will be reported and compared to similar releases for noble gases as well as the unexpected finding of 131I deposition from intentional impure gas injection into capsule 11 of experiment AGR 3/4.

AGR↗
DOE OSTI2019

Thermal Model Details and Description of the AGR-5/6/7 Experiment

The AGR-5/6/7 experiment is currently being irradiated in the Advanced Test Reactor (ATR) at the Idaho National Laboratory and is approximately 25% complete. Several fuel and material irradiation experiments have been planned for the U.S. Department of Energy Advanced Gas Reactor Fuel Development and Qualification Program, which supports the development and qualification of tristructural isotropic (TRISO) coated particle fuel for use in high-temperature gas-cooled reactors. The goals of these experiments are to provide irradiation performance data to support fuel process development, qualify fuel for normal operating conditions, support development of fuel performance models and codes, and provide irradiated fuel and materials for post-irradiation examination and safety testing. Originally planned and named as separate fuel experiments, but subsequently combined into a single test train, AGR-5/6/7 will test low-enriched uranium oxycarbide (UCO – a heterogeneous mixture of uranium oxide and uranium carbide) TRISO fuel. The AGR-5/6 portion of the experiment will provide data to support qualification of the selected reference fuel design, while the AGR-7 portion will serve as a margin test, irradiating the fuel beyond normal operating conditions.

42 ENGINEERING↗
DOE OSTI2018

Special Purpose Application Reactors: Systems Integration Decision Support

Microreactors, also known as very-Small Modular Reactors (vSMRs) or Special Purpose Reactors (SPRs), are being considered for use in unique applications where other methods of megawatt level energy production are uneconomical or unavailable. For the purposes of this report, a microreactor is defined as meeting the following criteria: • Factory manufacturable • Easily transportable by truck, plane, train, and/or ship • Produce no more than 20 megawatt thermal (MWth) energy, in order to qualify as Hazard Category 2 under 10CFR830 • Maintains neutronic simplicity, allowing semi- or fully-autonomous operation In the United States (U.S.), there are two general types of microreactors under development: high-temperature gas reactors (HTGRs) and heat pipe reactors. These two reactor types may, due to their differences in working fluid temperatures, be more effectively suited to different use cases. Additionally, they will require different interfacing components depending on their intended use. This report identifies a broad range of use cases for micro-reactors. Additionally, multiple reactor technologies are examined with an emphasis on the reactor sub-systems and interconnections. Using this information, a decision framework is developed to guide future efforts.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2018

Fuel – clad chemical interaction evaluation of the TREAT reactor conceptual low-enriched-uranium fuel element

The Transient Reactor Test (TREAT) facility resides at the Materials and Fuels Complex (MFC) at Idaho National Laboratory (INL). The TREAT reactor is currently undergoing design and engineering studies for its conversion from a high enriched uranium (HEU) to a low-enriched uranium (LEU) core. The conceptual design of the LEU fuel element identified two main design differences compared with the HEU fuel element; namely, it will contain four times more fissionable material in its graphite matrix and distinct nuclear-grade Zirconium alloy, as Zircaloy-3 was used in the HEU fuel assembly and is not commercially available currently. These design changes may impact the magnitude of chemical interaction between fuel and cladding materials during physical contact under expected TREAT operation conditions and, therefore, was evaluated through a combination of experimental testing and thermodynamic modeling in order to determine implications for the fuel assembly. In this study, two potential cladding material types, Zircaloy-4 or Zr-1Nb alloys, were evaluated, and it was found for both material types that the extent of interaction and specific chemical reactions are minimal and no detrimental effect on the overall cladding properties is observed. Here, the resulting interaction layer of 3-6 µm was measured after a 2-week exposure at 820°C. The thermodynamic analysis was extended to temperatures beyond the TREAT reactor operation and accident conditions in order to give some insight that may be of interest for other reactor systems as the High Temperature Gas Reactors (operation above 1,000°C) and for Nuclear Reactor Severe Accident phenomenology study where the UO 2 fuel could reach temperatures over 2,800°C and melt.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗