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At least 343 records · Page 19

Simulation Framework for Regional Geologic CO 2 Storage Along Arches Province of Midwestern United States

This report presents final technical results for the project Simulation Framework for Regional Geologic CO 2 Storage Infrastructure along Arches Province of the Midwest United States . The Arches Simulation project was a three year effort designed to develop a simulation framework for regional geologic carbon dioxide (CO 2 ) storage infrastructure along the Arches Province through development of a geologic model and advanced reservoir simulations of large-scale CO 2 storage. The project included five major technical tasks: (1) compilation of geologic, hydraulic and injection data on Mount Simon, (2) development of model framework and parameters, (3) preliminary variable density flow simulations, (4) multi-phase model runs of regional storage scenarios, and (5) implications for regional storage feasibility. The Arches Province is an informal region in northeastern Indiana, northern Kentucky, western Ohio, and southern Michigan where sedimentary rock formations form broad arch and platform structures. In the province, the Mount Simon sandstone is an appealing deep saline formation for CO 2 storage because of the intersection of reservoir thickness and permeability. Many CO 2 sources are located in proximity to the Arches Province, and the area is adjacent to coal fired power plants along the Ohio River Valley corridor. Geophysical well logs, rock samples, drilling logs, and geotechnical tests were evaluated for a 500,000 km2 study area centered on the Arches Province. Hydraulic parameters and historical operational information was also compiled from Mount Simon wastewater injection wells in the region. This information was integrated into a geocellular model that depicts the parameters and conditions in a numerical array. The geologic and hydraulic data were integrated into a three-dimensional grid of porosity and permeability, which are key parameters regarding fluid flow and pressure buildup due to CO 2 injection. Permeability data were corrected in locations where reservoir tests have been performed in Mount Simon injection wells. The geocellular model was used to develop a series of numerical simulations designed to support CO 2 storage applications in the Arches Province. Variable density fluid flow simulations were initially run to evaluate model sensitivity to input parameters. Two dimensional, multiple-phase simulations were completed to evaluate issues related to arranging injection fields in the study area. A basin-scale, multiple-phase model was developed to evaluate large scale injection effects across the region. Finally, local scale simulations were also completed with more detailed depiction of the Eau Claire formation to investigate to the potential for upward migration of CO 2 . Overall, the technical work on the project concluded that injection large-scale injection may be achieved with proper field design, operation, siting, and monitoring. Records from Mount Simon injection wells were compiled, documenting more than 20 billion gallons of injection into the Mount Simon formation in the Arches Province over the past 40 years, equivalent to approximately 60 million metric tons CO 2 . The multi-state team effort was useful in delineating the geographic variability in the Mount Simon reservoir properties. Simulations better defined potential well fields, well field arrangement, CO 2 pipeline distribution system, and operational parameters for large-scale injection in the Arches Province. Multiphase scoping level simulations suggest that injection fields with arrays of 9 to 50+ wells may be used to accommodate large injection volumes. Individual wells may need to be separated by 3 to 10 km. Injection fields may require spacing of 25 to 40 km to limit pressure and saturation front interference. Basin-scale multiple-phase simulations in STOMP reflect variability in the Mount Simon. While simulations suggest a total injection rate of 100 million metric tons per year (approximately to a 40% reduction of CO 2 emissions from large point sources across the Arches Province) may be feasible, some areas are more suitable due to favorable geology. Sustainable injection rates were higher in areas where there was higher thickness and reservoir permeability. Distribution of injection across well fields is an effective method to reduce pressure and CO 2 saturation front interference.

54 ENVIRONMENTAL SCIENCES↗

Computational Assessment of Naturally Occurring Background Radiation Produced by Extraterrestrial Sources - Paper 43

In recent years there has been increased interest in developing the ability to account for background radiation in real (or near-real) time in support of end-user field experiments or operational search missions. More specifically, the focus has been on creating an array of tools that can provide an estimate of the natural occurring radiation that an experimentalist or search operator can use in the field in real time while making a measurement. Conceptually, these tools would allow the experimentalist or search operator to be able to dynamically account for the background associated with the measurement resulting in significant improvement in the probability of detection and minimization of the false alarm rate. The purpose of this work is to assess the extraterrestrial sources that produce naturally occurring background, the variation of these sources, and the variation in the background due to the sources and the potential measurement environment. This work is part of a larger project that will also assess terrestrial sources of background radiation. The focus of this paper is only the neutron background produced by extraterrestrial sources. The computational assessment will be performed using MCNP6. (authors)

61 RADIATION PROTECTION AND DOSIMETRY↗

A new look at the position operator in quantum theory

The postulate that coordinate and momentum representations are related to each other by the Fourier transform has been accepted from the beginning of quantum theory by analogy with classical electrodynamics. As a consequence, an inevitable effect in standard theory is the wave packet spreading (WPS) of the photon coordinate wave function in directions perpendicular to the photon momentum. This leads to the following paradoxes: if the major part of photons emitted by stars are in wave packet states (what is the most probable scenario) then we should see not separate stars but only an almost continuous background from all stars; no anisotropy of the CMB radiation should be observable; data on gamma-ray bursts, signals from directional radio antennas (in particular, in experiments on Shapiro delay) and signals from pulsars show no signs of WPS. In addition, a problem arises why there are no signs of WPS for protons in the LHC ring. We argue that the above postulate is based neither on strong theoretical arguments nor on experimental data and propose a new consistent definition of the position operator. Then WPS in directions perpendicular to the particle momentum is absent and the paradoxes are resolved. Different components of the new position operator do not commute with each other and, as a consequence, there is no wave function in coordinate representation. Implications of the results for entanglement, quantum locality and the problem of time in quantum theory are discussed.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Results of an In-Field Validation Exercise in Support of Wide-Area Environmental Sampling

The National Nuclear Security Administration’s (NNSA) Office of Nonproliferation and Arms Control (NA-24) is evaluating Wide-Area Environmental Sampling (WAES) as an additional safeguards verification tool for the International Atomic Energy Agency to detect undeclared nuclear activities. The NNSA is evaluating strategies for conducting a generic WAES campaign, the cost of a WAES campaign, and the effect of technological advancements that have occurred since the last major WAES review in 1999. Until now, the NNSA effort has focused on tabletop exercises (TTXs) in which high-performance computing allows for advanced modeling and simulation efforts to be applied to the WAES question. Although the modeling and simulations used in the TTXs are extremely valuable, field campaigns are still needed to validate the assumptions that underpin the models and the modeling process itself. During a 7 week period beginning in May 2023 and ending in June 2023, which included 4 weeks of active field collections, a multilaboratory team conducted its first in-field validation exercise. Prior to the in-field exercise, abbreviated TTXs were conducted to estimate the performance of all collection systems to be used during the field test. These TTXs guided the selection of materials to be released and the placement of the collection system. Based on these determinations, materials were procured to use in the field test, and an injection/release system was designed, built, and installed at the test facility. Background samples were collected during weeks one and four, and environmental collections against active releases were conducted during weeks two and three. The goals of this validation exercise included a demonstration of (1) the ability to provide controlled releases of particulates of surrogate materials, (2) the fielding and operation of collection systems (including deposition and active air collectors), and (3) the flexibility to revise equipment and campaign plans in the field. This paper presents the results and preliminary conclusions for this initial validation test. Based on these results, subsequent field campaigns are anticipated and will include the addition of other released materials.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Development and testing of a photometric method to identify non-operating solar hot water systems in field settings

This report presents the results of experimental tests of a concept for using infrared (IR) photos to identify non-operational systems based on their glazing temperatures; operating systems have lower glazing temperatures than those in stagnation. In recent years thousands of new solar hot water (SHW) systems have been installed in some utility districts. As these numbers increase, concern is growing about the systems dependability because installation rebates are often based on the assumption that all of the SHW systems will perform flawlessly for a 20-year period. If SHW systems routinely fail prematurely, then the utilities will have overpaid for grid-energy reduction performance that is unrealized. Moreover, utilities are responsible for replacing energy for loads that failed SHW system were supplying. Thus, utilities are seeking data to quantify the reliability of SHW systems. The work described herein is intended to help meet this need. The details of the experiment are presented, including a description of the SHW collectors that were examined, the testbed that was used to control the system and record data, the IR camera that was employed, and the conditions in which testing was completed. The details of the associated analysis are presented, including direct examination of the video records of operational and stagnant collectors, as well as the development of a model to predict glazing temperatures and an analysis of temporal intermittency of the images, both of which are critical to properly adjusting the IR camera for optimal performance. Many IR images and a video are presented to show the contrast between operating and stagnant collectors. The major conclusion is that the technique has potential to be applied by using an aircraft fitted with an IR camera that can fly over an area with installed SHW systems, thus recording the images. Subsequent analysis of the images can determine the operational condition of the fielded collectors. Specific recommendations are presented relative to the application of the technique, including ways to mitigate and manage potential sources of error.

15 GEOTHERMAL ENERGY↗

Phase space theory of Bose-Einstein condensates and time-dependent modes

A phase space theory approach for treating dynamical behaviour of Bose-Einstein condensates applicable to situations such as interferometry with BEC in time-dependent double well potentials is presented. Time-dependent mode functions are used, chosen so that one, two, Horizontal-Ellipsis highly occupied modes describe well the physics of interacting condensate bosons in time dependent potentials at well below the transition temperature. Time dependent mode annihilation, creation operators are represented by time dependent phase variables, but time independent total field annihilation, creation operators are represented by time independent field functions. Two situations are treated, one (mode theory) is where specific mode annihilation, creation operators and their related phase variables and distribution functions are dealt with, the other (field theory) is where only field creation, annihilation operators and their related field functions and distribution functionals are involved. The field theory treatment is more suitable when large boson numbers are involved. The paper focuses on the hybrid approach, where the modes are divided up between condensate (highly occupied) modes and non-condensate (sparsely occupied) modes. It is found that there are extra terms in the Ito stochastic equations both for the stochastic phases and stochastic fields, involving coupling coefficients defined via overlap integrals between mode functions and their time derivatives. For the hybrid approach both the Fokker-Planck and functional Fokker-Planck equations differ from those derived via the correspondence rules, the drift vectors are unchanged but the diffusion matrices contain additional terms involving the coupling coefficients. Results are also presented for the combined approach where all the modes are treated as one set. Here both the Fokker-Planck and functional Fokker-Planck equations are exactly the same as those derived via the correspondence rules. However, although the Ito stochastic field equations are also unchanged, the Ito equations for the stochastic phases contain an extra classical term involving the coupling coefficients. - Highlights: Black-Right-Pointing-Pointer Wigner, P+ representations used for condensate and non-condensate bosons, respectively. Black-Right-Pointing-Pointer Time dependence of modes leads to novel Fokker-Planck and Ito equations. Black-Right-Pointing-Pointer Field theory and separate mode treatments.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Dirac matrices for Chern-Simons gravity

A genuine gauge theory for the Poincare, de Sitter or anti-de Sitter algebras can be constructed in (2n- 1)-dimensional spacetime by means of the Chern-Simons form, yielding a gravitational theory that differs from General Relativity but shares many of its properties, such as second order field equations for the metric. The particular form of the Lagrangian is determined by a rank n, symmetric tensor invariant under the relevant algebra. In practice, the calculation of this invariant tensor can be reduced to the computation of the trace of the symmetrized product of n Dirac Gamma matrices {Gamma}{sub ab} in 2n-dimensional spacetime. While straightforward in principle, this calculation can become extremely cumbersome in practice. For large enough n, existing computer algebra packages take an inordinate long time to produce the answer or plainly fail having used up all available memory. In this talk we show that the general formula for the trace of the symmetrized product of 2n Gamma matrices {Gamma}{sub ab} can be written as a certain sum over the integer partitions s of n, with every term being multiplied by a numerical cofficient {alpha}{sub s}. We then give a general algorithm that computes the {alpha}-coefficients as the solution of a linear system of equations generated by evaluating the general formula for different sets of tensors B{sup ab} with random numerical entries. A recurrence relation between different coefficients is shown to hold and is used in a second, 'minimal' algorithm to greatly speed up the computations. Runtime of the minimal algorithm stays below 1 min on a typical desktop computer for up to n = 25, which easily covers all foreseeable applications of the trace formula.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Matching the quark model to the 1/N{sub c} expansion

We compute the coefficients of the effective mass operator of the 1/N{sub c} expansion for negative parity L = 1 excited baryons using the Isgur-Karl model in order to compare the general approach, where the coefficients are obtained by fitting to data, with a specific constituent quark model calculation. We discuss the physics behind the fitted coefficients for the scalar part of the most general two-body quark-quark interaction. We find that both pion exchange and gluon exchange lead to the dominance of the same operator at the level of the effective mass operator, which is also observed from data.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Methylammonium Lead Tribromide Single Crystal Detectors towards Robust Gamma-Ray Photon Sensing

In recent years, hybrid perovskite single crystalline solid-state detectors have shown promise in γ-ray spectroscopy. Here, the γ-ray photon induced electrical pulses are investigated, which are produced by perovskite solid-state detectors made with the commonly used methylammonium lead tribromide crystals with chlorine incorporation. Under low electric field detector operation, slow pulses generated by γ-rays with average rise times of 65 µs are observed, which decreases to 20 µs when a higher electrical field of 500 V cm -1 is applied. However, the baseline becomes noisy quickly, which prevents collection of clean pulses for spectra construction. Further, by systematically measuring the temperature dependence and current–voltage characteristics, such instability is attributed to the local ion migration under electrical field creating a fluctuating dark noise, which presents a major challenge in perovskite γ-ray detector technologies. It is demonstrated that cycling the bias between positive and negative polarity can stabilize the detector, allowing for longer periods of pulse accumulation for generating energy resolved spectra with resolutions of ≈35% at 59.6 keV and ≈25% at 662 keV at room temperature. The study indicates that the main limiting factors of perovskite-based γ-ray detectors are slow rise times and bias instability. Finally, these challenges must be properly addressed to achieve reproducible, high-resolution γ-ray detection.

47 OTHER INSTRUMENTATION↗

A relativistic self-consistent model for studying enhancement of space charge limited field emission due to counter-streaming ions

Recently, field emission has attracted increasing attention despite the practical limitation that field emitters operate below the Child-Langmuir space charge limit. By introducing counter-streaming ion flow to neutralize the electron charge density, the space charge limited field emission (SCLFE) current can be dramatically enhanced. In this work, we have developed a relativistic self-consistent model for studying the enhancement of SCLFE by a counter-streaming ion current. The maximum enhancement is found when the ion effect is saturated, as shown analytically. The solutions in non-relativistic, intermediate, and ultra-relativistic regimes are obtained and verified with 1-D particle-in-cell simulations. This self-consistent model is general and can also serve as a benchmark or comparison for verification of simulation codes, as well as extension to higher dimensions.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Time-Dependent Boundary Modeling to Inform Design of SPARC Diagnostic and Actuators

The purpose of this work was to inform the design of diagnostic and actuator systems for a new experimental facility for Commonwealth Fusion Systems (CFS), called SPARC [Creely2020], using time-dependent plasma boundary simulations with the Scrape Off Layer Plasma Simulator (SOLPS) code [Wiesen2015]. The SPARC tokamak is a device that aims to demonstrate fusion energy production and high-field plasma operating scenarios. The developed technologies will be incorporated into a net-electricity pilot that will demonstrate approximately 200MW of electric power. A major difference from other private industry fusion companies is the use of a standard aspect ratio, but at a high magnetic field strength, which provides a well-established physics basis and a modest extrapolation to reactor operation. Time-dependent simulations were used to inform the design of main-chamber plasma facing components, which are protected by feedback control of the heat and particle loads during high power operation. The simulations provide the timescales and magnitudes of plasma and neutral particle response useful for determining the position and operation of diagnostics and actuators that will enable control. The plasma response and phase-space diagrams also provide input into advanced model-based control schemes, which are envisioned for later SPARC operation. Model-based control can reduce the risk of component failure, which would require expensive in-situ repairs and the associated delays, by predicting the system response to actuators over a short time-horizon.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

State-operator correspondence in celestial conformal field theory

The bulk-to-boundary dictionary for 4D celestial holography is given a new entry defining 2D boundary states living on oriented circles on the celestial sphere. The states are constructed using the 2D CFT state-operator correspondence from operator insertions corresponding to either incoming or outgoing particles which cross the celestial sphere inside the circle. The BPZ construction is applied to give an inner product on such states whose associated bulk adjoints are shown to involve a shadow transform. Scattering amplitudes are then given by BPZ inner products between states living on the same circle but with opposite orientations. 2D boundary states are found to encode the same information as their 4D bulk counterparts, but organized in a radically different manner.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Gauge-invariant observables, gravitational dressings, and holography in AdS

This paper explores construction of gauge (diffeomorphism)-invariant observables in anti de Sitter (AdS) space and the related question of how to find a "holographic map" providing a quantum equivalence to a boundary theory. Observables are constructed perturbatively to leading order in the gravitational coupling by gravitationally dressing local field theory operators in order to solve the gravitational constraints. Many such dressings are allowed and two are explicitly examined, corresponding to a gravitational line and to a Coulomb field; these also reveal an apparent role for more general boundary conditions than considered previously. The observables obey a nonlocal algebra, and we derive explicit expressions for the boundary generators of the SO(D-1,2) AdS isometries that act on them. We examine arguments that gravity {\it explains} holography through the role of such a boundary Hamiltonian. Our leading-order gravitational construction reveals some questions regarding how these arguments work, and indeed construction of such a holographic map appears to require solution of the non-perturbative generalization of the bulk constraint equations.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

A Laguerre expansion method for the field particle portion in the linearized Coulomb collision operator

The spherical coordinates expressions of the Rosenbluth potentials are applied to the field particle portion in the linearized Coulomb collision operator. The Sonine (generalized Laguerre) polynomial expansion formulas for this operator allowing general field particles' velocity distributions are derived. An important application area of these formulas is the study of flows of thermalized particles in NBI-heated or burning plasmas since the energy space structure of the fast ions' slowing down velocity distribution cannot be expressed by usual orthogonal polynomial expansions, and since the Galilean invariant property and the momentum conservation of the collision must be distinguished there.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

End-User Perspectives on Using Quantitative Real-Time PCR and Genomic Sequencing in the Field

Quantitative real-time PCR and genomic sequencing have become mainstays for performing molecular detection of biological threat agents in the field. There are notional assessments of the benefits, disadvantages, and challenges that each of these technologies offers according to findings in the literature. However, direct comparison between these two technologies in the context of field-forward operations is lacking. Most market surveys, whether published in print form or provided online, are directed to product manufacturers who can address their respective specifications and operations. One method for comparing these technologies is surveying end-users who are best suited for discussing operational capabilities, as they have hands-on experience with state-of-the-art molecular detection platforms and protocols. These end-users include operators in military defense and first response, as well as various research scientists in the public sector such as government and service laboratories, private sector, and civil society such as academia and nonprofit organizations performing method development and executing these protocols in the field. Our objective was to initiate a survey specific to end-users and their feedback. We developed a questionnaire that asked respondents to (1) determine what technologies they currently use, (2) identify the settings where the technologies are used, whether lab-based or field-forward, and (3) rate the technologies according to a set list of criteria. Of particular interest are assessments of sensitivity, specificity, reproducibility, scalability, portability, and discovery power. This article summarizes the findings from the end-user perspective, highlighting technical and operational challenges.

59 BASIC BIOLOGICAL SCIENCES↗

Stability and Performance of an Undersea Kite Operating in a Turbulent Flow Field

In this paper, we examine the effects of flow disturbances resulting from turbulence on the dynamic behavior of an underwater energy-harvesting kite system that executes periodic figure-8 flight. Due to the periodic nature of the kite’s operation, we begin by assessing orbital stability using the Floquet analysis and stroboscopic intersection analysis of a Poincaré section, with the former analysis performed on a simplified “unifoil” model and the latter performed on a six-degree-of-freedom (6-DOF)/flexible tether model. With periodic stability established, a frequency-domain analysis based on a linearization about the kite’s path is used to predict the quality of flight path tracking as a function of the turbulence frequency. To validate the accuracy of these simulation-based predictions under flow disturbances, we compare the predictions of the kite’s behavior against the results of small-scale tow testing experiments performed in a controlled pool environment.

13 HYDRO ENERGY↗

Tunable band gap in few-layer graphene by surface adsorption

There is a tunable band gap in ABC-stacked few-layer graphene (FLG) via applying a vertical electric field, but the operation of FLG-based field effect transistor (FET) requires two gates to create a band gap and tune channel’s conductance individually. Using first principle calculations, we propose an alternative scheme to open a band gap in ABC-stacked FLG namely via single-side adsorption. The band gap is generally proportional to the charge transfer density. The capability to open a band gap of metal adsorption decreases in this order: K/Al . Cu/Ag/Au . Pt. Moreover, we find that even the band gap of ABA-stacked FLG can be opened if the bond symmetry is broken. Finally, a single-gated FET based on Cu-adsorbed ABC-stacked trilayer graphene is simulated. A clear transmission gap is observed, which is comparable with the band gap. This renders metal-adsorbed FLG a promising channel in a single-gated FET device.

ELECTRONIC PROPERTIES AND MATERIALS↗

Near-field scanning magneto-optical spectroscopy of Wigner molecules

We study the emission spectra of single self-organized InP/GaInP QDs (size 100-220 nm) using high-spatial-resolution, low-temperature (5 K) near-field scanning optical microscope (NSOM) operating at magnetic field strength B=0-10 T. The dots contain up to twenty electrons and represent natural Wigner molecules (WM). We observed vibronic-type shake-up structure in single electron QDs manifesting formation of two electron (2e) WM in photo-excited state. We found that relative intensities of the shake-up components described well by vibronic Frank-Condon factors giving for dots having parabolic confinement energy ħω{sub 0}=1.2-4 meV molecule bond lengths 40-140 nm. We used measurements of magnetic-field-induced shifts to distinguish emission of 2e-WM and singly charged exciton (trion). We also observed magnetic-field-induced molecular-droplet transition for two electron dot, emitting through doubly charge exciton (tetron) at zero magnetic field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗