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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 343 records · Page 19
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Emulation of Synaptic Plasticity in WO 3 ‐Based Ion‐Gated Transistors

Neuromorphic systems, inspired by the human brain, promise significant advancements in computational efficiency and power consumption by integrating processing and memory functions, thereby addressing the von Neumann bottleneck. This paper explores the synaptic plasticity of a WO3-based ion-gated transistor (IGT) in [EMIM][TFSI] and a 0.1 mol L −1 LiTFSI in [EMIM][TFSI] for neuromorphic computing applications. Cyclic voltammetry (CV), transistor characteristics, and atomic force microscopy (AFM) force–distance (FD) profiling analyses reveal that Li + brings about ion intercalation, together with higher mobility and conductance, and slower response time (τ). WO 3 IGTs exhibit spike amplitude-dependent plasticity (SADP), spike number-dependent plasticity (SNDP), spike duration-dependent plasticity (SDDP), frequency-dependent plasticity (FDP), and paired-pulse facilitation (PPF), which are all crucial for mimicking biological synaptic functions and understanding how to achieve different types of plasticity in the same IGT. The findings underscore the importance of selecting the appropriate ionic medium to optimize the performance of synaptic transistors, enabling the development of neuromorphic systems capable of adaptive learning and real-time processing, which are essential for applications in artificial intelligence (AI).

36 MATERIALS SCIENCE↗
DOE OSTI2016

Bifurcation, chaos, and scan instability in dynamic atomic force microscopy

The dynamical motion at any point on the cantilever of an atomic force microscope can be expressed quite generally as a superposition of simple harmonic oscillators corresponding to the vibrational modes allowed by the cantilever shape. Central to the dynamical equations is the representation of the cantilever-sample interaction force as a polynomial expansion with coefficients that account for the interaction force “stiffness,” the cantilever-to-sample energy transfer, and the displacement amplitude of cantilever oscillation. Renormalization of the cantilever beam model shows that for a given cantilever drive frequency cantilever dynamics can be accurately represented by a single nonlinear mass-spring model with frequency-dependent stiffness and damping coefficients [S. A. Cantrell and J. H. Cantrell, J. Appl. Phys. 110, 094314 (2011)]. Application of the Melnikov method to the renormalized dynamical equation is shown to predict a cascade of period doubling bifurcations with increasing cantilever drive force that terminates in chaos. The threshold value of the drive force necessary to initiate bifurcation is shown to depend strongly on the cantilever setpoint and drive frequency, effective damping coefficient, nonlinearity of the cantilever-sample interaction force, and the displacement amplitude of cantilever oscillation. The model predicts the experimentally observed interruptions of the bifurcation cascade for cantilevers of sufficiently large stiffness. Operational factors leading to the loss of image quality in dynamic atomic force microscopy are addressed, and guidelines for optimizing scan stability are proposed using a quantitative analysis based on system dynamical parameters and choice of feedback loop parameter.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

NO TIME FOR DEAD TIME: TIMING ANALYSIS OF BRIGHT BLACK HOLE BINARIES WITH NuSTAR

Timing of high-count-rate sources with the NuSTAR Small Explorer Mission requires specialized analysis techniques. NuSTAR was primarily designed for spectroscopic observations of sources with relatively low count rates rather than for timing analysis of bright objects. The instrumental dead time per event is relatively long (∼2.5 msec) and varies event-to-event by a few percent. The most obvious effect is a distortion of the white noise level in the power density spectrum (PDS) that cannot be easily modeled with standard techniques due to the variable nature of the dead time. In this paper, we show that it is possible to exploit the presence of two completely independent focal planes and use the cospectrum, the real part of the cross PDS, to obtain a good proxy of the white-noise-subtracted PDS. Thereafter, one can use a Monte Carlo approach to estimate the remaining effects of dead time, namely, a frequency-dependent modulation of the variance and a frequency-independent drop of the sensitivity to variability. In this way, most of the standard timing analysis can be performed, albeit with a sacrifice in signal-to-noise ratio relative to what would be achieved using more standard techniques. We apply this technique to NuSTAR observations of the black hole binaries GX 339–4, Cyg X-1, and GRS 1915+105.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Optical and magneto-optical properties of ferromagnetic monolayer CrBr 3 : A first-principles G W and G W plus Bethe-Salpeter equation study

The discovery of atomically thin two-dimensional (2D) magnetic semiconductors has triggered enormous research interest recently. In this paper, we use first-principles many-body perturbation theory to study a prototypical 2D ferromagnetic semiconductor, monolayer chromium tribromide (CrBr 3 ). With broken time-reversal symmetry, spin-orbit coupling, and excitonic effects included through the full-spinor GW and GW plus Bethe-Salpeter equation (GW-BSE) methods, we compute the frequency-dependent layer polarizability tensor and dielectric function tensor that govern the optical and magneto-optical (MO) properties. In addition, we provide a detailed theoretical formalism for simulating magnetic circular dichroism, MO Kerr effect, and Faraday effect, demonstrating the approach with monolayer CrBr 3 . Due to reduced dielectric screening in 2D and the localized nature of the Cr d orbitals, we find strong self-energy effects on the quasiparticle band structure of monolayer CrBr 3 that give a 3.8 eV indirect bandgap. Also, excitonic effects dominate the low-energy optical and MO responses in monolayer CrBr 3 where a large exciton binding energy of 2.3 eV is found for the lowest bright exciton state with excitation energy at 1.5 eV. We further find that the MO signals demonstrate strong dependence on the excitation frequency and substrate refractive index. Furthermore, our theoretical framework for modeling optical and MO effects could serve as a powerful theoretical tool for future study of optoelectronic and spintronics devices consisting of van der Waals 2D magnets.

36 MATERIALS SCIENCE↗
DOE OSTI2016

A STUDY OF BROADBAND FARADAY ROTATION AND POLARIZATION BEHAVIOR OVER 1.3–10 GHz IN 36 DISCRETE RADIO SOURCES

We present a broadband polarization analysis of 36 discrete polarized radio sources over a very broad, densely sampled frequency band. Our sample was selected on the basis of polarization behavior apparent in narrowband archival data at 1.4 GHz: half the sample shows complicated frequency-dependent polarization behavior (i.e., Faraday complexity) at these frequencies, while half shows comparatively simple behavior (i.e., they appear Faraday simple ). We re-observed the sample using the Australia Telescope Compact Array in full polarization, with 6 GHz of densely sampled frequency coverage spanning 1.3–10 GHz. We have devised a general polarization modeling technique that allows us to identify multiple polarized emission components in a source, and to characterize their properties. We detect Faraday complex behavior in almost every source in our sample. Several sources exhibit particularly remarkable polarization behavior. By comparing our new and archival data, we have identified temporal variability in the broadband integrated polarization spectra of some sources. In a number of cases, the characteristics of the polarized emission components, including the range of Faraday depths over which they emit, their temporal variability, spectral index, and the linear extent of the source, allow us to argue that the spectropolarimetric data encode information about the magneto-ionic environment of active galactic nuclei themselves. Furthermore, the data place direct constraints on the geometry and magneto-ionic structure of this material. We discuss the consequences of restricted frequency bands on the detection and interpretation of polarization structures, and the implications for upcoming spectropolarimetric surveys.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1973

Controlled oscillator system with a time dependent output frequency

A controlled oscillator system is presented for providing an output with a frequency which changes with respect to time and with a phase which is within established phase error limits. The system includes a frequency synthesizer with a symmetrical search oscillator, capable of tuning the output with a range of + or - 100 Hz about any fixed frequency to which the synthesizer is set. For a tuning range of 200 Hz (+ or - 100 Hz) an expanded search oscillator output of a frequency range of 4 MHz (from 1 MHz to 5 MHz) is provided. A counter counts continuously the expanded output cycles and at each of fixed sampling intervals, for every 0.1 second, the count or number accumulated in the counter is read out. The sample number is compared with a theoretical number which should be present in the counter at the particular sampling instant for proper synthesizer's output frequency and phase.

Winkelstein, R. A.↗
NASA NTRS1975

Observations of turbulence in the atmosphere of Venus using Mariner 10 radio occultation measurements

A technique is developed for estimating the outer scale of turbulence in a planetary atmosphere using dual-frequency radio occultation measurements. This technique is based on the frequency dependence of the temporal frequency spectra for the log-amplitude fluctuations and is particularly useful when probing the upper atmosphere where the transverse velocity of the line-of-sight path is decelerating very rapidly. It is applied to the region of strong turbulence located in the vicinity of 60 km on the dayside of the atmosphere of Venus using the Mariner 10 S/X radio occultation measurements. It is found that, contrary to earlier findings from Mariner 5, the outer scale of turbulence is at least 5 km. It appears that the outer scale of turbulence is as large as the vertical extent of the region of strong turbulence. Estimates of the structure constants for refractive index and temperature fluctuations indicate that the turbulence is stronger than that measured near the earth's tropopause.

Woo, R.↗
NASA NTRS1979

Gravity wave propagation in a diffusively separated atmosphere with height-dependent collision frequencies

Numerical calculations of gravity wave propagation through a two-component thermosphere with vertically-varying inter-species collision frequencies are performed using a direct integration method. Reflection of upgoing gravity wave energy into downgoing gravity waves appears to be small though nonnegligible at typical thermospheric periods and wavelengths. Coupling into diffusion waves is completely insignificant in most cases and may be determined in part by the relative abundance of the minor species. Temperature perturbation differences between species can be greater than 10% above 300 km altitude even though coupling into diffusion waves is small. Diffusive dissipation of gravity wave energy can be significant in the lower thermosphere and may be comparable to dissipation by viscosity and heat conduction below about 225 km altitude. Heating by diffusive dissipation may also be comparable to direct heating by solar radiation in the lower thermosphere. As a result of dissipative filtering of long-period and short-wavelength waves and the sensitivity of He-N2 density perturbation phase differences to diffusion, the AE-C satellite wave observations can only be fit by internal gravity waves with periods no greater than about 25 min and horizontal wavelengths no less than about 200 km.

Del Genio, A. D.↗
NASA NTRS1980

Aspect dependence and frequency spectrum of electrical discharges on the P78-2 (SCATHA) satellite

The satellite charging at high altitudes (SCATHA) P78-2 satellite payload includes a charging electrical effects analyzer (CEEA) which measures the characteristics of electrical discharges in both the frequency and time domain. Pulses are detected in response to commands during electron and ion beam operations and during natural discharge events. The pulse analyzer measures the shape of pulses on four sensors and is the primary CEEA diagnostic for the natural discharges. Only five discharges were found in the data at a time when the pulse analyzer was in mode with sufficient time resolution to resolve the frequency components in the waveform.

Koons, H. C.↗
NASA NTRS2004

Remote Measurements of Snowfalls in Wakasa Bay, Japan with Airborne Millimeter- wave Imaging Radiometer and Cloud Radar

In this paper we explore the application of combined millimeter-wave radar and radiometry to remotely measure snowfall. During January-February of 2003, a field campaign was conducted with the NASA P-3 aircraft in Wakasa Bay, Japan for the validation of the AMSRE microwave radiometer on board the Aqua satellite. Among the suite of instruments-on board the P-3 aircraft were the Millimeter-wave Imaging Radiometer (MIR) from the NASA Goddard Space Flight Center and the 94 GHz Airborne Cloud Radar (ACR) which is co-owned and operated by NASA Jet Propulsion Laboratory/University of Massachusetts. MIR is a total power, across-track scanning radiometer that measures radiation at the frequencies of 89, 150, 183.3 +/- 1, 183.3 +/- 3, 183.3 +/-7, 220, and 340 GHz. The MIR has flown many successful missions since its completion in May 1992. ACR is a newer instrument and flew only a few times prior to the Wakasa Bay deployment. These two instruments which are particularly well suited for the detection of snowfall functioned normally during flights over snowfall and excellent data sets were acquired. On January 14, 28, and 29 flights were conducted over snowfall events. The MIR and ACR detected strong signals during periods of snowfall over ocean and land. Results from the analysis of these concurrent data sets show that (1) the scattering of millimeter-wave radiation as detected by the MIR is strongly correlated with ACR radar reflectivity profiles, and (2) the scattering is highly frequency-dependent, the higher the frequency the stronger the scattering. Additionally, the more transparent channels of the MIR (e.g., 89, 150, and 220 GHz) are found to display ambiguous signatures of snowfall because of their exposure to surface features. Thus, the snowfall detection and retrievals of snowfall parameters, such as the ice water path (IWP) and median mass diameter (D(me)) are best conducted at the more opaque channels near 183.3 GHz and 340 GHz. Retrievals of IWP and D(me) using the MIR measurements at 183.3 and 340 GHZ are currently in progress, and the results will be compared with those derived from the ACR reflectivity profiles. Implication from this comparison will be discussed.

Wang, J. R.↗
DOE OSTI2019

Effect of Zn Concentration on the Structure, Morphology, and Magnetic Behavior of Ni{sub 1 − x}Zn{sub x}Fe{sub 2}O{sub 4} Ferrofluid

In this work, we investigated the effect of doping zinc ions onto nickel ferrite upon the structure, morphology, and magnetic properties of Ni{sub 1 − x}Zn{sub x}Fe{sub 2}O{sub 4} ferrite nanoparticles (x = 0, 0.25, and 0.75) prepared via co-precipitation method. X-ray diffraction analysis showed the presence of the most intense peak corresponding to the (311) crystallographic orientation of NiFe{sub 2}O{sub 4} cubic spinel phase, and the crystallite size obtained from Scherrer formula increased from 6.8 to 11.2 nm when the Zn concentration increases from x = 0 to x = 0.75. Fourier transform infrared spectroscopy analysis confirmed the presence of a prominent band associated to the vibrations of metal ions, as a feature of spinel ferrite phase formation, observing that their band positions were very sensitive to Zn doping concentration. Transmission electron microscopy studies allowed to determinate that for all Zn concentrations, the particle sizes are around 15 nm. The magnetic properties were studied by using the vibrating sample magnetometer at room temperature. The results reveal superparamagnetic behavior determined by the shape of the hysteresis loop, presenting decreased coercive magnetic field and increased saturation magnetization, with increased zinc concentration. Additionally, from field cooling and zero field cooling curves, we can observe the typical behavior of the blocking process assembly of superparamagnetic nanoparticles. Alternate current susceptibility measurements show that the blocking temperature is frequency dependent and shifts toward higher temperatures by increasing the frequency, a characteristic of superparamagnetic, and glassy systems. Furthermore, τ{sub 0}, related to the jump attempt frequency of the magnetic moment of the nanoparticle between the opposite directions of the magnetization easy axis, is in the range of 2 × 10{sup −10} and 7 × 10{sup −13} s for the three different Zn concentrations, which agrees with characteristic of non-interacting superparamagnetic systems.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Structural and magnetic properties of Ni-doped SnO{sub 2}

Samples of Ni doped SnO{sub 2} nanocrystalline were successfully prepared by chemical co-precipitation method. X-ray diffraction pattern infers that Sn{sub 1-x}Ni{sub x}O{sub 2} (x=0.00, 0.10, 0.15 and 0.20) samples are in single phase with tetragonal structure (P4{sub 2}/mnm). Raman spectroscopy reveals the observed phonon modes of SnO{sub 2} are at about 387-397, and 559 - 572 cm{sup −1}. For Sn{sub 0.9}Ni{sub 0.1}O{sub 2}, these peaks are shifted to higher wave numbers, while to that for Sn{sub 0.85}Ni{sub 0.15}O{sub 2} and Sn{sub 0.8}Ni{sub 0.2}O{sub 2}, peaks are shifted to the lower wave numbers. The frequency dependent dielectric constant decreases with the increase in the frequency and becomes constant at high frequencies for all compositions of Ni substituted SnO{sub 2}. The magnetization curve confirms the paramagnetic nature of all Ni doped SnO{sub 2} samples.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Theoretical study of symmetry of flux onto a capsule

An analytic model to describe the flux asymmetry onto a capsule based on the viewfactor approximation is developed and verified with numerical simulations. By using a nested spheres technique to represent the various sources of flux asymmetry, the model can treat spherically and cylindrically symmetric hohlraums, e.g., cylinder, elliptic, and rugby. This approach includes the more realistic case of frequency-dependent flux asymmetry compared with the more standard frequency-integrated or single-frequency approaches [D. W. Phillion and S. M. Pollaine, Phys. Plasmas 1, 2963 (1994)]. Correspondingly, the approach can be used to assess x-ray preheat asymmetry generated from localized laser absorption in the high-Z hohlraum wall. For spherical hohlraums with 4, 6, or 8 laser entrance holes (LEHs), an optimal configuration of LEHs, laser spot placement, and angle-of-incidence of the single-ringed laser beams is defined. An analogy between minimizing the flux asymmetry onto a capsule and the Thomson problem of point charge placement on a sphere for minimized energy is shown.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2014

Stochastic many-body perturbation theory for anharmonic molecular vibrations

A new quantum Monte Carlo (QMC) method for anharmonic vibrational zero-point energies and transition frequencies is developed, which combines the diagrammatic vibrational many-body perturbation theory based on the Dyson equation with Monte Carlo integration. The infinite sums of the diagrammatic and thus size-consistent first- and second-order anharmonic corrections to the energy and self-energy are expressed as sums of a few m- or 2m-dimensional integrals of wave functions and a potential energy surface (PES) (m is the vibrational degrees of freedom). Each of these integrals is computed as the integrand (including the value of the PES) divided by the value of a judiciously chosen weight function evaluated on demand at geometries distributed randomly but according to the weight function via the Metropolis algorithm. In this way, the method completely avoids cumbersome evaluation and storage of high-order force constants necessary in the original formulation of the vibrational perturbation theory; it furthermore allows even higher-order force constants essentially up to an infinite order to be taken into account in a scalable, memory-efficient algorithm. The diagrammatic contributions to the frequency-dependent self-energies that are stochastically evaluated at discrete frequencies can be reliably interpolated, allowing the self-consistent solutions to the Dyson equation to be obtained. This method, therefore, can compute directly and stochastically the transition frequencies of fundamentals and overtones as well as their relative intensities as pole strengths, without fixed-node errors that plague some QMC. It is shown that, for an identical PES, the new method reproduces the correct deterministic values of the energies and frequencies within a few cm{sup −1} and pole strengths within a few thousandths. With the values of a PES evaluated on the fly at random geometries, the new method captures a noticeably greater proportion of anharmonic effects.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

New edge magnetoplasmon interference like photovoltage oscillations and their amplitude enhancement in the presence of an antidot lattice

We present new photovoltage oscillation in a pure two dimensional electron gas (2DEG) and in the presence of circular or semicircular antidot lattices. Results were interpreted as EMPs-like photovoltage oscillations. We observed and explained the photovoltage oscillation amplitude enhancement in the presence of an antidot lattice with regard to the pure 2DEG. The microwave frequency excitation range is 139 – 350 GHz. The cyclotron and magnetoplasmon resonances take place in the magnetic field range 0.4 – 0.8 T. This original experimental condition allows edge magnetoplasmons EMPs interference like observation at low magnetic field, typically B < B{sub c} where B{sub c} is the magnetic field at which the cyclotron resonance takes place. The different oscillation periods observed and their microwave frequency dependence were discussed. For 139 and 158 GHz microwave excitation frequencies, a unique EMPs-like interference period was found in the presence of antidots whereas two periods were extracted for 295 or 350 GHz. An explanation of this effect is given taking account of strong electron interaction with antidot at low magnetic field. Indeed, electrons involved in EMPs like phenomenon interact strongly with antidots when electron cyclotron orbits are larger than or comparable to the antidot diameter.

36 MATERIALS SCIENCE↗
DOE OSTI2015

Electronic and optical properties of titanium nitride bulk and surfaces from first principles calculations

Prediction of the frequency-dependent dielectric function of thin films poses computational challenges, and at the same time experimental characterization by spectroscopic ellipsometry remains difficult to interpret because of changes in stoichiometry and surface morphology, temperature, thickness of the film, or substrate. In this work, we report calculations for titanium nitride (TiN), a promising material for plasmonic applications because of less loss and other practical advantages compared to noble metals. We investigated structural, electronic, and optical properties of stoichiometric bulk TiN, as well as of the TiN(100), TiN(110), and TiN(111) outermost surfaces. Density functional theory (DFT) and many-body GW methods (Green's (G) function-based approximation with screened Coulomb interaction (W)) were used, ranging from G{sub 0}W{sub 0}, GW{sub 0} to partially self-consistent sc-GW{sub 0}, as well as the GW-BSE (Bethe-Salpeter equation) and time-dependent DFT (TDDFT) methods for prediction of the optical properties. Structural parameters and the band structure for bulk TiN were shown to be consistent with previous work. Calculated dielectric functions, plasma frequencies, reflectivity, and the electron energy loss spectrum demonstrated consistency with experiment at the GW{sub 0}-BSE level. Deviations from experimental data are expected due to varying experimental conditions. Comparison of our results to spectroscopic ellipsometry data for realistic nanostructures has shown that although TDDFT may provide a computationally feasible level of theory in evaluation of the dielectric function, application is subject to validation with GW-BSE calculations.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2016

Temperature-sensitive photoluminescent CdSe-ZnS polymer composite film for lock-in photothermal characterization

The temperature dependence of the fluorescence spectrum of CdSe−ZnS core–shell quantum dots embedded in a polystyrene matrix is characterized between 30 °C and 60 °C. The spectrally integrated photoluminescence intensity is found to linearly decrease with −1.3%/ °C. This feature is exploited in a dual coating-substrate-configuration, consisting of a layer of this nanocomposite material, acting as a temperature sensor with optical readout, on top of an optically absorbing and opaque layer, acting as a photothermal excitation source, and covering a substrate material or structure of interest. From the frequency dependence of the optically detected photothermal signal in the frequency range between 5 Hz and 150 Hz, different thermal parameters of the constituent layers are determined. The fitted values of thermal properties of the different layers, determined in different scenarios in terms of the used a priori information about the layers, are found to be internally consistent, and consistent with literature values.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗