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At least 325 records · Page 18

Diagnosing laser-preheated magnetized plasmas relevant to magnetized liner inertial fusion

In this paper, we present a platform on the OMEGA EP Laser Facility that creates and diagnoses the conditions present during the preheat stage of the MAGnetized Liner Inertial Fusion (MagLIF) concept. Experiments were conducted using 9 kJ of 3ω (355 nm) light to heat an underdense deuterium gas (electron density: 2.5 × 10 20 cm -3 = 0.025 of critical density) magnetized with a 10 T axial field. Results show that the deuterium plasma reached a peak electron temperature of 670 ± 140 eV, diagnosed using streaked spectroscopy of an argon dopant. The results demonstrate that plasmas relevant to the preheat stage of MagLIF can be produced at multiple laser facilities, thereby enabling more rapid progress in understanding magnetized preheat. Results are compared with magneto-radiation-hydrodynamics simulations, and plans for future experiments are described.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Characterization of laser-produced carbon plasmas relevant to laboratory astrophysics

Experiments, analytic modeling, and numerical simulations are presented here to characterize carbon plasmas produced by high-intensity (10 9 -10 13 W cm -2 ) lasers relevant to experimental laboratory astrophysics. In the large-scale limit, the results agree well with a self-similar isentropic, adiabatic fluid model. Laser-target simulations, however, show small-scale structure in the velocity distribution of different ion species, which is also seen in experiments. These distributions indicate that most of the plasma energy resides in moderate charge states (C +3 –C +4 ), most of the mass resides in the lowest charge states, and the highest charge states move fastest.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Development of an inertial confinement fusion platform to study charged-particle-producing nuclear reactions relevant to nuclear astrophysics

Here, this paper describes the development of a platform to study astrophysically relevant nuclear reactions using inertial-confinement fusion implosions on the OMEGA and National Ignition Facility laser facilities, with a particular focus on optimizing the implosions to study charged-particle- producing reactions. Primary requirements on the platform are high yield, for high statistics in the fusion product measurements, combined with low areal density, to allow the charged fusion products to escape. This is optimally achieved with direct-drive exploding pusher implosions using thin-glass-shell capsules. Mitigation strategies to eliminate a possible target sheath potential which would accelerate the emitted ions are discussed. The potential impact of kinetic effects on the implosions is also considered. The platform is initially employed to study the complementary T(t,2n)α, T( 3 He,np)α and 3 He( 3 He,2p)α reactions. Proof-of-principle results from the first experiments demonstrating the ability to accurately measure the energy and yields of charged particles are presented. Lessons learned from these experiments will be used in studies of other reactions. Ultimately, the goals are to explore thermonuclear reaction rates and fundamental nuclear physics in stellarlike plasma environments, and to push this new frontier of nuclear astrophysics into unique regimes not reachable through existing platforms, with thermal ion velocity distributions, plasma screening, and low reactant energies.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Positron radiography of ignition-relevant ICF capsules

Laser-generated positrons are evaluated as a probe source to radiograph in-flight ignition-relevant inertial confinement fusion capsules. Current ultraintense laser facilities are capable of producing 2 ×10 12 relativistic positrons in a narrow energy bandwidth and short time duration. Monte Carlo simulations suggest that the unique characteristics of such positrons allow for the reconstruction of both capsule shell radius and areal density between 0.002 and 2g/cm 2 . The energy-downshifted positron spectrum and angular scattering of the source particles are sufficient to constrain the conditions of the capsule between preshot and stagnation. Here, we evaluate the effects of magnetic fields near the capsule surface using analytic estimates where it is shown that this diagnostic can tolerate line integrated field strengths of 100 T mm.

42 ENGINEERING↗

Total and partial electron impact ionization cross sections of fusion-relevant diatomic molecules

We discuss calculations of total (and absolute) electron-impact ionization cross sections (EICSs) for the fusion-relevant diatomic molecular species BeH, BeN, BeO, WH, WBe, WN, WO, O 2 , and N 2 by means of the Deutsch-Märk and the binary-encounter-Bethe approaches in the energy range from threshold to 10 keV. In addition, we discuss an empirical scheme to estimate partial cross sections from the total ones based on reaction energetics and empirical threshold laws and explore its accuracy by assessing available experimental data on total and partial EICSs. Lastly, we also observe parameters obtained by fitting the calculated cross sections to an expression commonly used in fusion edge plasma modeling.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

An analytical study of non-resonant transient cross-beam power transfer relevant to recent progress in plasma photonics

Recent experimental and theoretical results have shown that crossing a probe laser in a plasma with a secondary pump can modify the amplitude, phase, and polarization of the probe in a controlled manner. Beyond fundamental physics, these results suggest that a pump-plasma based optical system could be used to amplify and control a laser pulse at high power, where the high fluence precludes using an optical system. This paper attempts to clarify the transient regime of such a pump-probe-plasma system. An analytical solution is derived to the coupled equations in the relevant regime, valid for any frequency detuning, coupling strength, and damping. Asymptotic expressions in the scantly studied off-resonance regime are derived. The time to reach the steady state is found to be roughly independent of the detuning. This time-to-steady-state defines the response time of such a plasma photonics system and can be made potentially much faster than traditional optics by controlling the damping of plasma acoustic waves. Here, we comment on the steady-state assumption typically used to interpret current experiments and design future ones.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Hot-electron generation at direct-drive ignition-relevant plasma conditions at the National Ignition Facility

Laser–plasma interaction instabilities can be detrimental for direct-drive inertial confinement fusion by generating high-energy electrons that preheat the target. Moreover, an experimental platform has been developed and fielded on the National Ignition Facility to investigate hot-electron production from laser–plasma instabilities at direct-drive ignition-relevant conditions. The radiation-hydrodynamic code DRACO has been used to design planar-target experiments that generate plasma and interaction conditions comparable to direct-drive ignition designs: I L ~10 15 W/cm 2 , T e > 3 keV, and density-gradient scale lengths of L n ~ 600 μ m in the quarter-critical density region. The hot-electron properties were inferred by comparing the experimentally observed hard x-ray spectra to Monte Carlo simulations of hard x-ray emission from hot electrons depositing energy in the target. Hot-electron temperatures of ~40 keV to 60 keV and the fraction of laser energy converted to hot electrons of ~0.5% to 5% were inferred in plastic targets for laser intensities at the quarter-critical density surface of (~4 to 14) × 10 14 W/cm 2 . The use of silicon ablators was found to mitigate the hot-electron preheat by increasing the threshold laser intensity for hot-electron generation from ~3.5 × 10 14 W/cm 2 in plastic to ~6 × 10 14 W/cm 2 in silicon. The overall hot-electron production is further reduced in silicon ablators when the intensity threshold is exceeded.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Scaling arguments for a plasma experiment relevant to an interplanetary coronal mass ejection

We present the design of a plasma experiment scaled to be relevant to an interplanetary coronal mass ejection (ICME) traveling from the Sun to the Earth. The experiment would launch a compact torus of plasma (the scaled analog of the coronal mass ejected by the Sun) into a magnetized background plasma (the scaled analog of the interplanetary medium, the diffuse magnetized plasma that fills the Solar System). We present the complete process of scaling the ICME system to a laboratory experiment: beginning with the ICME features that we aim to replicate with a laboratory experiment, explaining how these desired features are translated into specific design constraints, and presenting a set of experimental parameters that meet those constraints. We find that the experiment would be possible with plasma conditions typically achieved in large-scale facilities such as the Big Red Ball at the University of Wisconsin or the LArge Plasma Device at the University of California, Los Angeles.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Laser-plasma instabilities in long scale-length plasmas relevant to shock-ignition

We present 2D particle-in-cell simulations of laser-plasma instabilities (LPI) performed using conditions relevant to experiments on the OMEGA and NIF laser facilities. The laser intensity used is 2×10 15 W cm -2 , which allows comparison with previous experiments and simulations investigating shock ignition, though this is a relatively low intensity for the scheme. We find that the large convective gain of the instabilities leads to dynamics that are largely controlled by pump depletion and to scattering or absorption by LPIs predominantly occurring away from the quarter-critical density. The two-plasmon decay (TPD) instability is dominant for OMEGA-type conditions and remains important at the NIF-scale. In both cases, most absorption from TPD occurs near its Landau cutoff density, and we examine its nonlinear dynamics in this region, focusing on the ion-acoustic waves responsible for saturation. For NIF-type conditions, stimulated Raman scattering (SRS) and stimulated Brillouin scattering divert significant fractions of laser energy, and we find that SRS backscatter can occur with high gain at low densities due to kinetic effects. An in-depth analysis of hot-electron production is performed to identify the main sources and their characteristic electron temperature. For both simulations presented, the overall hot-electron temperature lies between 30 and 35 keV. This is relatively low and will likely increase shock pressure; however, the distributions also contain a significant number of high-energy (E k >100 keV) electrons that would likely cause unacceptable preheat. We, therefore, suggest some strategies that may be utilized to minimize this high-energy component. I. INTROD

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The effect of laser entrance hole foil thickness on MagLIF-relevant laser preheat

The magnetized liner inertial fusion (MagLIF) scheme relies on coupling laser energy into an underdense fuel raising the fuel adiabat at the start of the implosion. To deposit energy into the fuel, the laser must first penetrate a laser entrance hole (LEH) foil which can be a significant energy sink and introduce mix. In this paper, we report on experiments investigating laser energy coupling into MagLIF-relevant gas cell targets with LEH foil thicknesses varying from 0.5 μm to 3 μm. Two-dimensional (2D) axisymmetric simulations match the experimental results well for 0.5 μm and 1 μm thick LEH foils but exhibit whole-beam self-focusing and excessive penetration of the laser into the gas for 2 μm and 3 μm thick LEH foils. Additionally, better agreement for the 2 μm-thick foil is found when using a different thermal conductivity model in 2D simulations, while only 3D Cartesian simulations come close to matching the 3 μm-thick foil experiments. The study suggests that simulations may over-predict the tendency for the laser to self-focus during MagLIF preheat when thicker LEH foils are used. This effect is pronounced with 2D simulations where the azimuthally symmetric density channel effectively self-focuses the rays that are forced to traverse the center of the plasma. The extra degree of freedom in 3D simulations significantly reduces this effect. The experiments and simulations also suggest that, in this study, the amount of energy coupled into the gas is highly correlated with the laser propagation length regardless of the LEH foil thickness.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Cross-beam energy transfer in conditions relevant to direct-drive implosions on OMEGA

In cross-beam energy transfer (CBET), the interference of two laser beams ponderomotively drives an ion-acoustic wave that coherently scatters light from one beam into the other. This redirection of laser beam energy can severely inhibit the performance of direct-drive inertial confinement fusion (ICF) implosions. To assess the role of nonlinear and kinetic processes in direct-drive-relevant CBET, the energy transfer between two laser beams in the plasma conditions of an ICF implosion at the OMEGA laser facility was modeled using particle-in-cell simulations. For typical laser beam intensities, the simulations are in excellent agreement with linear kinetic theory, indicating that nonlinear processes do not play a role in direct-drive implosions. At higher intensities, CBET can be modified by pump depletion, backward stimulated Raman scattering, or ion trapping, depending on the plasma density.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Nonlocal effects on thermal transport in hydrodynamic simulations of unmagnetized MagLIF-relevant gaspipes on NIF

We present simulations of heat flow relevant to gaspipe experiments on the National Ignition Facility to investigate kinetic effects on transport phenomena. D 2 and neopentane (C 5 H 12 ) filled targets are used to study the laser preheat stage of a MagLIF scheme where an axial magnetic field is sometimes applied to the target. Simulations were done with the radiation-MHD code HYDRA with a collision-dominated fluid model and the SNB nonlocal electron thermal conduction model. Using the SNB model to evolve the electron temperature increased the heat front propagation of neopentane gas targets compared to a local model by limiting radial heat flow. This increases electron temperature near the axis, which decreases laser absorption. We find that the effect of heat flow models on temperature profiles and laser propagation is modest. Beyond the SNB model, we utilize HYDRA to initialize plasma conditions for the Vlasov–Fokker–Planck K2 code. We run K2 until a quasi-steady state is reached and examine the impact of kinetic effects on heat transport. Although axial heat flow is well predicted by fluid models, the fluid model consistently overpredicts radial heat flow up to 150% in regions with the largest temperature gradient of D 2 filled gaspipes. On the other hand, the SNB nonlocal electron conduction model is found to be adequate for capturing kinetic heat flow in gaspipes.

Lau, Ryan Y. [Univ. of Colorado, Boulder, CO (Unit↗

Robustness of inertial fusion energy relevant implosions to low-mode asymmetries

Inertial confinement fusion implosions for power production need to be robust. Degradation sources need to be understood and considered for an economic power plant. In this work, the impact of low-mode asymmetries on yield is studied using 2D radiation hydrodynamics simulations for inertial fusion energy relevant implosions. First, a high-gain indirectly driven capsule design is developed. This design is subsequently degraded with low-mode drive asymmetries. The results show that yield is constant with increasing amounts of asymmetry until a cliff is reached where the yield quickly drops below ignition. Robustness arises because the degraded hotspot still has enough time to get to ignition before capsule decompression. This robustness occurs even though the asymmetry couples less energy to the hotspot and causes decompression to occur sooner. The robustness is linked to the generalized Lawson parameter, χ⁠. The value of χ steadily decreases with increasing asymmetry. Once χ is close to one, the hotspot is no longer able to ignite before the capsule decompresses. A simple piston model is used to predict where the robustness cliff is for any design. The trade-off between yield and robustness is also demonstrated.

Physics - Plasma physics↗

Atomic-resolution structure of a disease-relevant Aβ(1–42) amyloid fibril

Amyloid-β (Aβ) is present in humans as a 39- to 42-amino acid residue metabolic product of the amyloid precursor protein. Although the two predominant forms, Aβ(1–40) and Aβ(1–42), differ in only two residues, they display different biophysical, biological, and clinical behavior. Aβ(1–42) is the more neurotoxic species, aggregates much faster, and dominates in senile plaque of Alzheimer’s disease (AD) patients. Although small Aβ oligomers are believed to be the neurotoxic species, Aβ amyloid fibrils are, because of their presence in plaques, a pathological hallmark of AD and appear to play an important role in disease progression through cell-to-cell transmissibility. Here, we solved the 3D structure of a disease-relevant Aβ(1–42) fibril polymorph, combining data from solid-state NMR spectroscopy and mass-per-length measurements from EM. The 3D structure is composed of two molecules per fibril layer, with residues 15–42 forming a double-horseshoe–like cross–β-sheet entity with maximally buried hydrophobic side chains. Lastly, residues 1–14 are partially ordered and in a β-strand conformation, but do not display unambiguous distance restraints to the remainder of the core structure.

59 BASIC BIOLOGICAL SCIENCES↗

The contribution of black carbon to global ice nucleating particle concentrations relevant to mixed-phase clouds

Significance The Earth’s climate is affected by the radiative properties of clouds. In clouds containing both supercooled water droplets and ice particles (mixed-phase clouds), cloud lifetime and albedo are affected by the presence of ice nucleating particles (INP). After decades of research, the importance of black carbon (BC) as an INP remains unresolved. In this work, we determined the contribution of BC to INP concentrations ([INP]) from real-world wildfires and prescribed burns. We found that BC does not contribute significantly to [INP] in near-field biomass burning plumes. These results were applied as parameterizations to global climate model output. Combined with previous work on diesel-engine exhaust, we find that BC does not contribute significantly to global [INP] relevant to mixed-phase clouds.

54 ENVIRONMENTAL SCIENCES↗

GAS-PHASE REACTIONS OF POLYCYCLIC AROMATIC HYDROCARBON ANIONS WITH MOLECULES OF INTERSTELLAR RELEVANCE

We have studied reactions of small dehydrogenated polycyclic aromatic hydrocarbon anions with neutral species of interstellar relevance. Reaction rate constants are measured at 300 K for the reactions of phenide (C{sub 6}H{sup -}{sub 5}), naphthalenide (C{sub 10}H{sup -}{sub 7}), and anthracenide (C{sub 14}H{sup -}{sub 9}) with atomic H, H{sub 2}, and D{sub 2} using a flowing afterglow-selected ion flow tube instrument. Reaction rate constants of phenide with neutral molecules (CO, O{sub 2}, CO{sub 2}, N{sub 2}O, C{sub 2}H{sub 2}, CH{sub 3}OH, CH{sub 3}CN, (CH{sub 3}){sub 2}CO, CH{sub 3}CHO, CH{sub 3}Cl, and (CH{sub 3}CH{sub 2}){sub 2}O) are also measured under the same conditions. Experimental measurements are accompanied by ab initio calculations to provide insight into reaction pathways and enthalpies. Our measured reaction rate constants should prove useful in the modeling of astrophysical environments, particularly when applied to dense regions of the interstellar and circumstellar medium.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

ON THE RELEVANCE OF POLYYNYL-SUBSTITUTED POLYCYCLIC AROMATIC HYDROCARBONS TO ASTROPHYSICS

We report on the absorption spectra of the polycyclic aromatic hydrocarbon (PAH) molecules anthracene, phenanthrene, and pyrene carrying either an ethynyl (-C{sub 2}H) or a butadiynyl (-C{sub 4}H) group. Measurements were carried out in the mid-infrared at room temperature on grains embedded in CsI pellets and in the near-ultraviolet at cryogenic temperature on molecules isolated in Ne matrices. The infrared measurements show that interstellar populations of polyynyl-substituted PAHs would give rise to collective features in the same way as non-substituted PAHs give rise to the aromatic infrared bands. The main features characteristic of the substituted molecules correspond to the acetylenic CH stretching mode near 3.05 {mu}m and to the almost isoenergetic acetylenic CCH in- and out-of-plane bending modes near 15.9 {mu}m. Sub-populations defined by the length of the polyynyl side group cause collective features which correspond to the various acetylenic CC stretching modes. The ultraviolet spectra reveal that the addition of an ethynyl group to a non-substituted PAH molecule results in all of its electronic transitions being redshifted. Due to fast internal energy conversion, the bands at shorter wavelengths are significantly broadened. Those at longer wavelengths are only barely affected in this respect. As a consequence, their relative peak absorption increases. The substitution with the longer butadiynyl chain causes the same effects with a larger magnitude, resulting in the spectra showing a prominent if not dominating {pi}-{pi}* transition at long wavelengths. After discussing the relevance of polyynyl-substituted PAHs to astrophysics, we conclude that this class of highly conjugated, unsaturated molecules represents valid candidates for the carriers of the diffuse interstellar bands.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

NEAR-INFRARED BAND STRENGTHS OF MOLECULES DILUTED IN N{sub 2} AND H{sub 2}O ICE MIXTURES RELEVANT TO INTERSTELLAR AND PLANETARY ICES

The relative abundances of ices in astrophysical environments rely on accurate laboratory measurements of physical parameters, such as band strengths (or absorption intensities), determined for the molecules of interest in relevant mixtures. In an extension of our previous study on pure-ice samples, here we focus on the near-infrared absorption features of molecules in mixtures with the dominant components of interstellar and planetary ices, H{sub 2}O and N{sub 2}. We present experimentally measured near-infrared spectral information (peak positions, widths, and band strengths) for both H{sub 2}O- and N{sub 2}-dominated mixtures of CO (carbon monoxide), CO{sub 2} (carbon dioxide), CH{sub 4} (methane), and NH{sub 3} (ammonia). Band strengths were determined during sample deposition by correlating the growth of near-infrared features (10,000-4000 cm{sup -1}, 1-2.5 {mu}m) with better-known mid-infrared features (4000-400 cm{sup -1}, 2.5-25 {mu}m) at longer wavelengths.

79 ASTRONOMY AND ASTROPHYSICS↗