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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 325 records · Page 18
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Anomalous interfacial dynamics of single proton charges in binary aqueous solutions

Our understanding of the dynamics of charge transfer between solid surfaces and liquid electrolytes has been hampered by the difficulties in obtaining interface, charge, and solvent-specific information at both high spatial and temporal resolution. Here, we measure at the single charge scale the dynamics of protons at the interface between an hBN crystal and binary mixtures of water and organic amphiphilic solvents (alcohols and acetone), evidencing a marked influence of solvation on interfacial dynamics. Applying single-molecule localization microscopy to emissive crystal defects, we observe correlated activation between adjacent ionizable surface defects, mediated by the transport of single excess protons along the solid/liquid interface. Solvent content has a nontrivial effect on interfacial dynamics, leading at intermediate water fraction to an increased surface diffusivity, as well as an increased affinity of the proton charges to the solid surface. Our measurements evidence the notable role of solvation on interfacial proton charge transport.

36 MATERIALS SCIENCE↗
NASA NTRS2002

Broadband Observations and Modeling of the Shell-Type Supernova Remnant G347.3-0.5

The supernova remnant G347.3-0.5 emits a featureless power law in X-rays, thought to indicate shock acceleration of electrons to high energies. We here produce a broadband spectrum of the bright northwest limb of this source by combining radio observations from the Australia Telescope Compact Array (ATCA), X-ray observations from the Advanced Satellite for Cosmology and Astrophysics (ASCA), and TeV gamma-ray observations from the CANGAROO imaging Cerenkov telescope. We assume that this emission is produced by an electron population generated by diffusive shock acceleration at the remnant forward shock. The nonlinear aspects of the particle acceleration force a connection between the widely different wavelength bands and between the electrons and the unseen ions, presumably accelerated simultaneously with the electrons. This allows us to infer the relativistic proton spectrum and estimate ambient parameters such as the supernova explosion energy, magnetic field, matter density in the emission region, and efficiency of the shock acceleration process. We find convincing evidence that the shock acceleration is efficient, placing greater than 25% of the shock kinetic energy flux into relativistic ions. Despite this high efficiency, the maximum electron and proton energies, while depending somewhat on assumptions for the compression of the magnetic field in the shock, are well below the observed 'knee' at 10(exp 15) eV in the Galactic cosmic-ray spectrum.

Ellison, Donald C.↗
NASA NTRS2014

First Hard X-Ray Detection of the Non-Thermal Emission Around the Arches Cluster: Morphology and Spectral Studies With NuSTAR

The Arches cluster is a young, densely packed massive star cluster in our Galaxy that shows a high level of star formation activity. The nature of the extended non-thermal X-ray emission around the cluster remains unclear. The observed bright Fe K(alpha) line emission at 6.4 keV from material that is neutral or in a low ionization state can be produced either by X-ray photoionization or by cosmic-ray particle bombardment or both. In this paper, we report on the first detection of the extended emission around the Arches cluster above 10 keV with the NuSTAR mission, and present results on its morphology and spectrum. The spatial distribution of the hard X-ray emission is found to be consistent with the broad region around the cluster where the 6.4 keV line is observed. The interpretation of the hard X-ray emission within the context of the X-ray reflection model puts a strong constraint on the luminosity of the possible illuminating hard X-ray source. The properties of the observed emission are also in broad agreement with the low-energy cosmic-ray proton excitation scenario. Key words: cosmic rays - Galaxy: center - ISM: general - X-rays: individual (Arches cluster)

Arches cluster↗
DOE OSTI2024

Electron tail suppression and effective collisionality due to synchrotron emission and absorption in mildly relativistic plasmas

Synchrotron radiation losses are a significant cause of concern for high-temperature aneutronic fusion reactions such as proton–Boron 11. The fact that radiation losses occur primarily in the high-energy tail, where the radiation itself has a substantial impact on the electron distribution, necessitates a self-consistent approach to modeling the diffusion and drag induced by synchrotron absorption and emission. Furthermore, an accurate model must account for the fact that the radiation emission spectrum is momentum-dependent, and the plasma opacity is frequency-dependent. Here, we present a simple Fokker–Planck operator, built on a newly solved-for blackbody synchrotron diffusion operator, which captures all relevant features of the synchrotron radiation. Focusing on magnetic mirror fusion plasmas, we show that significant suppression of the electron distribution occurs for relativistic values of the perpendicular electron momentum, which therefore emit much less radiation than predicted under the assumption of a Maxwell–Jüttner distribution.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2024

Early-time γ -ray constraints on cosmic-ray acceleration in the core-collapse SN 2023ixf with the Fermi Large Area Telescope

Context. While supernova remnants (SNRs) have been considered the most relevant Galactic cosmic ray (CR) accelerators for decades, core-collapse supernovae (CCSNe) could accelerate particles during the earliest stages of their evolution and hence contribute to the CR energy budget in the Galaxy. Some SNRs have indeed been associated with TeV γ -rays, yet proton acceleration efficiency during the early stages of an SN expansion remains mostly unconstrained. Aims. The multi-wavelength observation of SN 2023ixf, a Type II supernova (SN) in the nearby galaxy M 101 (at a distance of 6.85 Mpc), opens the possibility to constrain CR acceleration within a few days after the collapse of the red super-giant stellar progenitor. With this work, we intend to provide a phenomenological, quasi-model-independent constraint on the CR acceleration efficiency during this event at photon energies above 100 MeV. Methods. We performed a maximum-likelihood analysis of γ -ray data from the Fermi Large Area Telescope up to one month after the SN explosion. We searched for high-energy, non-thermal emission from its expanding shock, and estimated the underlying hadronic CR energy reservoir assuming a power-law proton distribution consistent with standard diffusive shock acceleration. Results. We do not find significant γ -ray emission from SN 2023ixf. Nonetheless, our non-detection provides the first limit on the energy transferred to the population of hadronic CRs during the very early expansion of a CCSN. Conclusions. Under reasonable assumptions, our limits would imply a maximum efficiency on the CR acceleration of as low as 1%, which is inconsistent with the common estimate of 10% in generic SNe. However, this result is highly dependent on the assumed geometry of the circumstellar medium, and could be relaxed back to 10% by challenging spherical symmetry. Consequently, a more sophisticated, inhomogeneous characterisation of the shock and the progenitor’s environment is required before establishing whether or not Type II SNe are indeed efficient CR accelerators at early times.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Point defects in Ga 2 O 3

In the field of high-power electronics, gallium oxide (Ga 2 O 3 ) is attracting attention due to its wide band gap and ability to be doped n-type. Point defects, including vacancies, impurities, and dopants, play important roles in optimizing device performance. This tutorial discusses the fundamental properties of point defects in monoclinic β-Ga 2 O 3 and the methods employed to study them. Oxygen vacancies are deep donors that do not cause n-type conductivity but may compensate acceptors. Gallium vacancies are deep acceptors that can be partially passivated by hydrogen. Substitutional magnesium is a promising acceptor that produces semi-insulating material and also forms a complex with hydrogen. Calcium and iron also have deep acceptor levels. Iridium deep donors are introduced into crystals grown from a melt in an Ir crucible. Here, other defects are introduced by irradiation with energetic particles such as neutrons or protons. In addition to altering the electronic properties, defects give rise to UV/visible emission bands in photoluminescence and cathodoluminescence spectra.

36 MATERIALS SCIENCE↗
NASA NTRS1976

Proton aurora on Io

The Jovian satellite Io should exhibit substantial auroral activity due to interactions of the satellite's atmosphere with Jovian magnetospheric particles. Plasma sheaths that may form around the satellite will cause substantial proton aurorae on the Jupiter-facing hemisphere and electron aurorae on the outward-facing hemisphere. A sample calculation indicates that Doppler-shifted radiation from high-velocity hydrogen atoms (proton aurora) will be observable from a spacecraft in the vicinity of Jupiter. Emission near Lyman-alpha may be present at a level as much as 100 times that of the solar background reflected from Io's surface.

Pilcher, C. B.↗
NASA NTRS1976

Proton aurora on Io

The Jovian satellite Io should exhibit substantial auroral activity due to interactions of the satellite's atmosphere with Jovian magnetospheric particles. Plasma sheaths that may form around the satellite will cause substantial proton aurora on the Jupiter-facing hemisphere and electron aurora on the outward-facing hemisphere. A sample calculation indicates that Doppler-shifted radiation from high-velocity hydrogen atoms (proton aurora) will be observable from a spacecraft in the vicinity of Jupiter. Emission near Lyman-alpha may be present at a level as much as 100 times that of the solar background reflected from Io's surface.

Pilcher, C. B.↗
NASA NTRS1982

On the interaction of auroral protons with the earth's atmosphere

The interaction of energetic auroral protons with the atmosphere is investigated. The results of a random number algorithm that describes the proton-hydrogen interconversion reactions as the beam loses energy are adopted to construct an energy deposition curve applicable over a wide range of initial proton energies. Ionization rates and production rates of ejected electrons are computed and emission rates of hydrogen Balmer alpha and beta lines are evaluated using recently available low energy cross-sections.

Rees, M. H.↗
NASA NTRS1984

Development of a radiation-hard photomultiplier tube

In a radiation-hard photomultiplier tube (PMT) such as has been developed for stabilization of the Galileo spacecraft as it goes through the Jovian high energy radiation belts, the primary effects of high energy electron and proton radiation that must be resisted are the production of fluorescence and Cerenkov emission. The present PMT envelope is ceramic rather than glass, and employs a special, electron-focusing design which will collect, accelerate and amplify electrons only from desired photocathode areas. Tests in a Co-60 radiation facility have shown that the radiation-hard PMT produces less than 2.5 percent of the radiation noise of a standard PMT.

Birnbaum, M. M.↗
NASA NTRS1985

The propagation of solar flare particles in a turbulent coronal loop

Energetic solar flare particles, both electrons and protons, must survive the turbulent environment of a flaring loop and propogate to the lower corona or chromosphere in order to produce hard X-ray and gamma ray bursts. This plasma turbulence, often observed in soft X-ray line widths to be in excess of 100 km/s, is presumably capable of efficiently scattering the fast flare particles. This prevents to some degree the free streaming of accelerated particles and depending on the amplitude of the turbulence, restricts the particles to diffusive propagation along the length of the loop to the target chromosphere. In addition this turbulence is capable of performing additional acceleration of the fast particles by the second order Fermi mechanism. For compact flares with rise times 10s, the acceleration effect is small and the propagation of the particles is governed by spatial diffusion and energy loss in the ambient medium. The solution of the time dependent diffusion equation with velocity dependent diffusion and energy loss coefficients yields for the case of nonrelativistic protons particle precipitation rates which are necessary for calculating thick target gamma ray emission and also yields the total thin target emissivity.

Ryan, J. M.↗
NASA NTRS1984

Synoptic observations of coronal transients and their interplanetary consequences

Conclusions reached to date after 5 yr of pooled, extensive monitoring of the solar coronal mass ejection (CME) at the Hawaiian High Altitude Observatory, Skylab and with the SMM are reported. Additional white light data have been gathered with the OSO-7 and P78-1 spacecraft. CME provides 5 percent of the solar wind mass flux and was the dominant driving force in interplanetary shocks in the last solar maximum phase. Both bubble and cloud shapes have been observed in CME events, which are nearly ubiquitous in proton events. Each of the CME shapes possesses distinctive dynamical characteristics. Finally, steady emissions of soft X-rays have been identified as precursors to CMEs, which display some latitudinal confinement.

Michels, D. J.↗
NASA NTRS1986

Variability of Lyman-alpha and the ultraviolet continuum of 3C 446

IUE observations have been conducted over the 1230-3175 A range for the violently variable quasar 3C 446, beginning in June 1980, at intervals of 1.2, 2.2, 0.5, and 0.4 yr. Strong absorption of the continuum was found below 1830 A, probably corresponding to a Lyman edge at z of 1.00 + or - 0.01. The absence of Mg II 2798 A absorption implies that the column density is in the lower end of the range, unless the gas is metal-poor. The Lyman-alpha emission line was detected in five spectra; relative to the number of ionizing protons, the line strengths are the same as in normal quasars, and line equivalent widths are small due to the continuum's rise redward of 912 A, which is much steeper than in normal quasars. The Lyman-alpha line and the nearby continuum vary so as to maintain constant equivalent width.

Bregman, J. N.↗
NASA NTRS1997

Multi-Wavelength Observations of 3C 273 in 1993-1995

We present the results of the multi-wavelength campaigns on 3C 273 in 1993-1995. During the observations in late 1993 this quasar showed an increase of its flux for energies >= 100 MeV from about 2.1 x 10(exp -7) photons/sq cm.s to approximately 5.6 x 10(exp -7) photons/sq cm.s during a radio outburst at 14.5, 22 and 37 GHz. However, no one-to-one correlation of the gamma-ray radiation with any frequency could be found. The photon spectral index of the high energy spectrum changed from GAMMA(sub gamma) = (3.20 +/- 0.54) to GAMMA(sub gamma) = (2.20 +/- 0.22) in the sense that the spectrum flattened when the gamma-ray flux increased. Fits of the three most prominent models (synchrotron self-Comptonization, external inverse Comptonization and the proton initiated cascade model) for the explanation of the high gamma-ray emission of active galactic nuclei were performed to the multi-wavelength spectrum of 3C 273 . All three models are able to represent the basic features of the multi-wavelength spectrum. Although there are some differences the data are still not decisive enough to discriminate between the models.

vonMontigny, C.↗
NASA NTRS2001

Dayside Aurora Dynamics

Images from the FUV (Far UltraViolet) instrument on board the IMAGE spacecraft will be presented to demonstrate the auroral dynamics in the dayside auroral zone and the polar cap region. optical emissions detected by three different detectors of FUV come from precipitations of energetic protons, electrons, and both species, respectively. In general, auroral activities in these regions responded very well to variations in the boundary conditions either external or internal to the magnetosphere, i.e., in the solar wind or the magnetotail. As a result, auroral images from FUV provide an excellent tool to investigate particle acceleration and transport processes within the geospace, such as shock acceleration, substorm injections, etc. we will interpret the observed auroral images using various models, discuss difference and similarity in the auroral activity from several typical cases, and assess conditions optimal to each type of auroral activity.

Spann, James F.↗
NASA NTRS2004

High Temperature Polymers for use in Fuel Cells

NASA Glenn Research Center (GRC) is currently working on polymers for fuel cell and lithium battery applications. The desire for more efficient, higher power density, and a lower environmental impact power sources has led to interest in proton exchanges membrane fuels cells (PEMFC) and lithium batteries. A PEMFC has many advantages as a power source. The fuel cell uses oxygen and hydrogen as reactants. The resulting products are electricity, heat, and water. The PEMFC consists of electrodes with a catalyst, and an electrolyte. The electrolyte is an ion-conducting polymer that transports protons from the anode to the cathode. Typically, a PEMFC is operated at a temperature of about 80 C. There is intense interest in developing a fuel cell membrane that can operate at higher temperatures in the range of 80 C- 120 C. Operating the he1 cell at higher temperatures increases the kinetics of the fuel cell reaction as well as decreasing the susceptibility of the catalyst to be poisoned by impurities. Currently, Nafion made by Dupont is the most widely used polymer membrane in PEMFC. Nafion does not function well above 80 C due to a significant decrease in the conductivity of the membrane from a loss of hydration. In addition to the loss of conductivity at high temperatures, the long term stability and relatively high cost of Nafion have stimulated many researches to find a substitute for Nafion. Lithium ion batteries are popular for use in portable electronic devices, such as laptop computers and mobile phones. The high power density of lithium batteries makes them ideal for the high power demand of today s advanced electronics. NASA is developing a solid polymer electrolyte that can be used for lithium batteries. Solid polymer electrolytes have many advantages over the current gel or liquid based systems that are used currently. Among these advantages are the potential for increased power density and design flexibility. Automobiles, computers, and cell phones require highly efficient power density for lowering emissions and meeting increasing consumer demands. Many of the solutions can be provided by proton exchange membrane fuel cells and lithium batteries. NASA Glenn Research Center has recognized this need, and is presently engaged in a solution. The goals for the summer include mastering synthesis techniques, understanding the reactions occurring during the synthesis, and characterizing the resulting polymer membranes using NMR, DSC, and TGA for the PEMFC and lithium batteries.

Peplowski, Katherine M.↗
DOE OSTI2020

Resolution of a discrepancy in the γ-ray emission probability from the β decay of 137 Ce g

We have deduced the emission probability of the 447-keV γ ray from the ε + β + decay of Ce g 137 (9.0 h) relative to that of the 254-keV γ ray from the Ce m 137 (34.4 h) decay in transient equilibrium. The time-dependent factor in transient equilibrium was applied following the Bateman equation for a radioactive decay chain. The isotope was produced via the La 139 ( p , 3 n ) Ce m , g 137 reaction by bombarding nat La with a proton beam from the 88-in. cyclotron at Lawrence Berkeley National Laboratory. γ -ray intensities were measured using an HPGe detector. The emission probability for the 447-keV γ ray deduced in this work is 1.21(3) (that is 1.21 ± 0.03) per hundred parent decays, which differs significantly from an earlier published value of 2.24(10). We identify the source of this discrepancy to be an incorrect use of the time-dependent factor. Additionally, we have deduced the emission probability of the 504-keV γ ray from the decay of Y g 85 (2.68 h) relative to that of the 232-keV γ ray from the Sr m 85 (1.127 h) decay in transient equilibrium. The isotope was produced via the Sr 86 ( p , 2 n ) Y g 85 reaction by bombarding SrCO 3 86 with a proton beam at the same facility. Overall, the study confirms the assumption of the time-dependent correction for recommending the emission probability of the 504-keV γ ray in the literature. Our work highlights the importance of explicit description by authors of any time-dependent correction they have made when reporting γ -ray intensities for nuclides in transient equilibrium. The need and significance of accurate and precise decay data of Ce g 137 and Y g 85 in basic science and medicine is briefly outlined.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Regulation of Absorption and Emission in a Protein/Fluorophore Complex

Human cellular retinol binding protein II (hCRBPII) was used as a protein engineering platform to rationally regulate absorptive and emissive properties of a covalently bound fluorogenic dye. We demonstrate the binding of a thio-dapoxyl analog via formation of a protonated imine between an active site lysine residue and the chromophore’s aldehyde. Rational manipulation of the electrostatics of the binding pocket results in a 204 nm shift in absorption and a 131 nm shift in emission. The protein is readily expressed in mammalian systems and binds with exogenously delivered fluorophore as demonstrated by live-cell imaging experiments.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗