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All sourcesNASA NTRSDOE OSTI
NASA NTRS1988

Infrared measurements in the spring 1987 ozone hole

Solar spectra were recorded from Arrival Heights (McMurdo), Antartica, with a FTIR system during the austral spring of 1987. Spectra were recorded on 22 days from September 13 through October 28. The instrument was setup with 2 detectors for simultaneous operation in 2 wavelength regions. Several stratospheric gases have measurable absorptions in these regions including HCl, HNO3, O3, ClONO2, and NO2. The system is equipped with an automatic solar tracking system and records data on tape cartridges. A portable personal computer allows Fourier transforming and initial processing of some of the data. The HNO3 gas column amount shows large variations, but no apparent correlation with stratospheric temperature. The HCl column shows a steady increase from 0.9 x 10 to the 15th power molecules/sq.cm. on September 13 to 1.5 x 10 to the 15th power on October 6. McMurdo moved out of the polar vortex for a few days, and the HCl column jumped to 2.9 x 10 to the 15th power by October 11. Although McMurdo moved back under the vortex, the HCl continued to increase, reaching 3.4 x 10 to the 15th power at the end of the period.

Murcray, F. J.↗
NASA NTRS1988

Measurements of ozone in the Antarctic region during August and September of 1987

Mixing ratios are presented for ozone in the austral polar atmosphere during Aug. and Sept. of 1987. Since the mid-1970's, there has been a continuing decrease in the total column abundance of ozone over Antarctica during the late winter and early spring. This reduction now amounts to about one-half of the historical October mean. The results presented are derived from an ultraviolet ozone photometer. The ER-2 aircraft carrying 14 instruments participated in a major effort to penetrate the region of depletion. Data were gathered between altitudes of 53 deg and 72 deg S at pressure altitudes up to 21 km in a series of 12 flights. Additional data were obtained between latitudes of 37 deg N and 53 deg S on the 3 flight legs required to reach Punta Arenas from Moffett Field, CA, and on the same return legs to Moffett Field. The observed ozone mixing ratios indicate the effects of chemistry as well as the effects of the stratospheric polar vortex. Examples of the distributions of ozone mixing ratios as a function of altitude, latitude, or a time and the relationships to temperature and other trace gases are presented.

Starr, Walter L.↗
NASA NTRS1988

In situ observations of ClO in the Antarctic: Evidence for chlorine catalyzed destruction of ozone

Results from a series of 12 ER-2 aircraft flights into the Antarctic polar vortex are summarized. These in situ data define the spatial and temporal distribution of ClO as the aircraft flew at an altitude of approx. 18 km from Punta Arenas (54 deg S latitude) to the base of the Palmer Peninsula (72 deg S latitude), executed a rapid descent to approx. 13 km, turned north and climbed bach to approximately 18 km, returning to Punta Arenas. A general pattern in the ClO distribution is reported: mixing ratios of approximately 10 ppt are found at altitude in the vicinity of 55 deg S increasing to 50 ppt at 60 degrees S. In the vicinity of 65 deg S latitude a steep gradient in the ClO mixing ratio is observed. At a fixed potential temperature, the ClO mixing ratio through this sharp transition increases by an order of magnitude within a very few degrees of latitude, thus defining the edge of the chemical containment vessel. From the edge of that containment vessel to the southern extension of the flights, 72 deg S, a dome of slowly increasing ClO best describes the distribution. Conclusion are drawn from the data.

Anderson, J. G.↗
NASA NTRS1988

Southern Hemispheric nitrous oxide measurements obtained during 1987 airborne Antarctic ozone experiment

The chemical lifetime of N2O is about 150 years, which makes it an excellent dynamical tracer of air motion on the time scale of the ozone depletion event. For these reasons it was chosen to help test whether dynamical theories of ozone loss over Antarctica were plausible, particularly the theory that upwelling ozone-poor air from the troposphere was replacing ozone-rich stratospheric air. The N2O measurements were made with the Airborne Tunable Laser Absorption Spectrometer (ATLAS) aboard the NASA ER-2 aircraft. The detection technique involves measuring the diffential absorption of the IR laser radiation as it is rapidly scanned over an N2O absorption feature. For the AAOE mission, the instrument was capable of making measurements with a 1 ppb sensitivity, 1 second response time, over an altitude range of 10 to 20 kilometers. The AAOE mission consisted of a series of 12 flights from Punta Arenas (53S) into the polar vortex (approximately 72S) at which time a vertical profile from 65 to 45 km and back was performed. Comparison of the observed profiles inside the vortex with N2O profiles obtained by balloon flights during the austral summer showed that an overall subsidence had occurred during the winter of about 5 to 6 km. Also, over the course of the mission (mid-August to late September), no trend in the N2O vertical profile, either upward or downward, was discernible, eliminating the possibility that upwelling was the cause of the observed ozone decrease.

Podolske, J. R.↗
NASA NTRS1988

Observations of stratospheric source gas profiles during the Arctic winter

An international campaign was performed at ESRANGE rocket base, near Kiruna, Sweden (68 N) from January 4 to February 15 in order to investigate the Chemistry of Ozone in the Polar Stratosphere (CHEOPS). Within the framework of this campaign two sets of large stratospheric air samples were collected by means of a balloon borne cryogenic air sampler. The two balloons were launched on February 1, and February 10, 1988. At present the samples are analyzed in our laboratory for their contents of several long lived trace gases such as CH4, N2O, H2, CO2, CO and the major halocarbons CH3Cl, CFCl3, CF2Cl2, CCl4, CH3CCl3, and C2F3Cl3. The vertical profiles derived from these samples will be presented and compared with previous observations made in February 1987. The data will be discussed in view of the dynamical evolution of the Arctic polar vortex during this winter.

Schmidt, U.↗
NASA NTRS1988

Antarctic ozone decrease: Possible impact on the seasonal and latitudinal distribution of total ozone as simulated by a 2-D model

Satellite borne instruments, the Total Ozone Mapping Spectrometer (TOMS) and the Solar Backscatter Ultraviolet spectrometer (SBUV), show that total column ozone has decreased by more than 5 percent in the neighborhood of 60 S at all seasons since 1979. This is considerably larger than the decrease calculated by 2-D models which take into account solar flux variation and increases of trace gas concentrations over the same period. The meteorological conditions (warmer temperature and the apparent lack of polar stratospheric clouds) at these latitudes do not seem to favor heterogeneous chemistry as the direct cause for the observed ozone reduction. A mechanism involving the seasonal transport of ozone-poor air mass from within the polar vortex to lower latitudes (the so-called dilution effect) is proposed as a possible explanation for the observed year-round ozone reduction in regions away from the vortex.

Ko, Malcolm K. W.↗
NASA NTRS1989

Barotropic instability of basic states with a realistic jet and a wave

The stability of basic states consisting of a jet similar to the stratospheric polar night jet and a traveling wave with a single zonal wavenumber is examined in a linearized nondivergent barotropic model on a sphere. Basic state waves are chosen to resemble observed traveling and stationary features in the winter stratosphere. Results are presented for disturbance growth rates, propagation characteristics, and energy conversion as a function of the basic state wave amplitude. The effects of small amplitude basic state waves on unstable disturbances arising from a zonally symmetric jet are discussed; results are shown where a small amplitude basic state wave dramatically affects the stability characteristics. Evidence is shown that the presence of a traveling wave may favor the appearance of disturbances that include other zonal wavenumbers which move with the basic state wave; this result is discussed in relation to the origin of observed quasi-nondispersive features in the polar winter stratosphere. Results for a stationary wavenumber 1 basic state wave suggest that a distorted polar vortex may be unstable to disturbances that would lead to further distortion. An unstable disturbance for a basic state with an eastward moving wavenumber 2 has components which resemble, in period and location, traveling waves that are observed in the winter stratosphere.

Manney, Gloria L.↗
NASA NTRS1989

The ultraviolet radiation environment of Antarctica - McMurdo Station during September-October 1987

Daily data from the Nimbus-7 TOMS were combined with a model of atmospheric radiative transfer to compute the time evolution of ultraviolet irradiance, at wavelengths from 290 to 350 nm, incident on McMurdo Station during September-October 1987. Large changes in column ozone occur as the polar vortex moves over the site. This is accompanied by correspondingly large variations in UV radiation at the earth's surface. At a wavelength near 305 nm, the irradiance in early October exceeds values appropriate to an unperturbed ozone layer by a factor of 5-6. As December 21 approaches, the noontime UV irradiance increases, irrespective of changes in ozone.

Lubin, Dan↗
NASA NTRS1989

Balloon-borne measurements of aerosol, condensation nuclei, and cloud particles in the stratosphere at McMurdo Station, Antarctica, during the spring of 1987

Measurements of the vertical profile of particles with condensation nuclei counters and eight channel aerosol detectors at McMurdo Station, Antarctica, in 1987 verified observations made in 1986 concerning the absence of upwelling in the polar vortex and the presence of a condensation nuclei layer in conjunction with the ozone hole region. New observations of a bimodal aerosol size distribution, consisting of a large-particle mode mixed in with the small-particle sulfate mode, at temperatures below -79 C are consistent with the presence of nitric acid-water particles at low concentrations. Higher concentrations of large particles were observed in association with nacreous clouds. An unusual particle layer which contained enhanced concentrations of both the small-particle (sulfate) mode and the large-particle (nitric acid) mode was detected at temperatures below -85 C, suggesting simultaneous nucleation and growth phenomena. The vortex condensation nuclei layer was observed to form at the same time as the ozone hole, indicating that formation of the layer is triggered by photochemical processes and may be important in controlling ozone depletion above 22 km.

Hofmann, D. J.↗
NASA NTRS1989

Airborne measurements of stratospheric constituents over Antarctica in the austral spring 1987. I - Method and ozone observations

A Fourier transform spectrometer was flown aboard a DC-8 on 10 flights over Antarctica during August and September, 1987, as part of the Airborne Antarctic Ozone Experiment (AAOE). Observing the sun at infrared wavelengths, it was possible to determine the integrated column amount above the flight altitude for ozone and a number of other chemical species that are believed to be important in the perturbed chemistry of the 'ozone hole'. The paper describes the method, the observations, the data analysis procedure, and the ozone results. During the observation period, ozone developed a steep gradient near the edge of the polar vortex; deep within the vortex, the average ozone column decreased by about 1.6 percent per day during September.

Mankin, William G.↗
NASA NTRS1989

Antarctic ozone hole - Possible implications for ozone trends in the Southern Hemisphere

Satellite-borne instruments (the Total Ozone Mapping Spectrometer and the Solar Backscattered Ultraviolet Instrument) show that, compared to 1979, total column ozone has a year-round decrease of more than 5 percent in the neighborhood of 60 deg S. The meteorological conditions (warmer temperatures, the absence of polar stratospheric clouds) at these latitudes do not seem to favor heterogeneous chemistry as the direct cause for the observed year-round ozone reduction. A mechanism involving the seasonal transport of ozone-poor air from within the polar vortex to lower latitudes (the so-called 'dilution effect') is proposed as a possible explanation for the observed year-round ozone reduction in subpolar regions. A two-dimensional model with an imposed springtime Antarctic ozone depletion is used to study the post-ozone hole impact on the spatial and temporal distributions of column ozone at latitudes north of 60 deg S. It is found that the time constant associated with the dilution effect in the latitude region 40-60 deg S is about 1 year, long enough to contribute to the observed year-round decrease of total ozone in that region.

Sze, N. D.↗
NASA NTRS1989

Temperature and horizontal wind measurements on the ER-2 aircraft during the 1987 Airborne Antarctic Ozone Experiment

The accuracy of temperature, pressure, potential temperature, and horizontal wind measurements is discussed in connection with the use of Meteorological Measurement System data in the AAOE. The vertical distribution of temperature measurements and latitudinal variations of the zonal wind for 12 flights over Antarctica during the 1987 AAOE campaign are summarized. Model atmospheres from 0 to 32 km at 70 deg and 55 deg S for the August-September period are constructed. Above the 420 K isentropic surface, the polar vortex remains strong throughout August and September of 1987.

Chan, K. R.↗
NASA NTRS1989

Meteorological atlas of the Northern Hemisphere lower stratosphere for January and February 1989 during the Airborne Arctic Stratospheric Expedition

Northern Hemisphere meteorological data for the months of January and February 1989 in the lower stratosphere are shown. National Meteorological Center (NMC) data, and Total Ozone Mapping Spectrometer (TOMS) data are used to display polar stereographic projections of 100-mb temperatures, 50-mb temperatures, 50-mb geopotential heights, total ozone, and Ertel's potential vorticity (Epv) on both 400 K and 460 K isentropic surfaces. In addition, latitude/height cross sections at 10 E of balanced wind isotachs, wind vectors, potential temperature, and temperature are also shown. Horizontal traces of NASA ER-2 and DC-8 flight tracks are also included. Vertical profiles of NMC temperatures following flight paths of both aircraft are shown. In addition, vertical profiles of wind speed are contoured following the ER-2 for estimating the lateral penetration into the polar vortex, while vertical profiles of Ertel's potential vorticity are included for estimating the vertical penetration of the DC-8 into the stratosphere.

Newman, Paul A.↗
NASA NTRS1989

A shallow water model of the winter stratosphere

The shallow water equations are used to investigate the interaction of planetary wave-breaking with a 'diabatic' forcing. The numerical integrations demonstrate the formation of a sharp gradient in potential vorticity at the edge of the polar vortex, despite 'diabatic relaxation' toward a smooth gradient. Successive cycles of Rossby wave-breaking accentuate the distinction between the vortex and the surf-zone. Persistent easterly acceleration in the tropics eventually produces a flow regime of little relevance to the atmosphere. For the period when the flow has some qualitative resemblance to the middle stratosphere diffusion coefficients are calculated from the meridional fluxes of potential vorticity and of passive tracers. It is found that the unique dynamical nature of potential vorticity among tracers is not reflected in its diffusion coefficient.

Juckes, Martin↗
NASA NTRS1989

Airborne measurements of stratospheric constituents over Antarctica in the austral spring, 1987. II - Halogen and nitrogen trace gases

The IR absorption spectra of the polar stratosphere, recorded by a Fourier transform spectrometer aboard the NASA DC-8 aircraft during the Airborne Antarctic Ozone Experiment, were used to derive vertical column amounts above flight altitude of HCl, HF, NO, NO2, ClONO2, and HNO3 in the region of disturbed ozone chemistry during September 1987. Significant reductions in the amounts of HCl, NO, NO2, and HNO3 were observed within the confines of the polar vortex, compared with amounts outside the vortex. When compared with the springtime observations by the same instrument in the Northern Hemisphere, the HCl and NO2 species displayed the most dramatic depletions. The results obtained are generally in agreement with the earlier ground measurements conducted at the McMurdo Station.

Coffey, M. T.↗
NASA NTRS1989

In situ observations of ClO in the Antarctic - ER-2 aircraft results from 54 deg S to 72 deg S latitude

The spatial and temporal distributions of ClO in the latitude belt from 54 to 72 deg S during the later stages of austral winter were obtained from measurements aboard the ER-2 aircraft flying at the altitude of about 18 km into the Antarctic polar vortex. Mixing ratios of about 10 parts per trillion by volume (pptv) were found in the vicinity of 55 deg S, increasing to 50 pptv at 60 deg S. A steep gradient of the ClO mixing ratio occurred in the vicinity of 65 deg S, where, at a fixed potential temperature, the value of the ClO mixing ratio increased by an order of magnitude within a very few degrees of latitude, defining the edge of the 'chemically perturbed region' (CPR). At the southern extension of the flight track, peak mixing ratios increased sharply from 800 pptv on August 23 to 1100 pptv in early September, and then increased more slowly to 1200 pptv on September 22. This corresponds to enhancements 500 times the typical mid-latitude values.

Brune, W. H.↗
NASA NTRS1989

Stratospheric nitrous oxide distribution in the Southern Hemisphere

Nitrous oxide measurements were made in the Southern Hemisphere as part of the Airborne Antarctic Ozone Experiment in late winter and early spring 1987, covering the altitude range 14-21 km. This paper reports on N2O measurements made by the airborne tunable laser absorption spectrometer, which was flown onboard the NASA ER-2 aircraft. Average vertical N2O profiles at latitudes 72 deg S, 54 deg S, and 42 deg S are presented and compared, when possible, with equivalent summer profiles. Latitudinal gradients of N2O on isentropic surfaces are presented and discussed in terms of their implications about the inhibition of horizontal mixing near the polar vortex. Finally, a large-scale distribution of N2O for the region 72 deg S to 42 deg S latitude is presented.

Podolske, J. R.↗
NASA NTRS1990

The role of chlorine chemistry in Antarctic ozone loss - Implications of new kinetic data

New kinetic data yielding a slower formation rate and larger absorption cross sections of Cl2O2 are incorporated into a photochemical model to reassess the role of chlorine chemistry in accounting for the ozone reductions derived from TOMS observations in different regions of the Antarctic polar vortex during 1987. The model is further constrained by existing measurements from the Airborne Antarctic Ozone Experiment and the National Ozone Expedition II. Calculated concentrations of ClO based on the new kinetic data increase by almost a factor of two between the collar and core regions of the vortex during the second half of September. The calculated ozone reductions in the vortex core appear to be consistent with the TOMS observations in spite of the slower rate for the self-reaction of ClO.

Rodriguez, Jose M.↗